Nanostructures and catalytic atoms engineering of tellurium-based materials and their roles in electrochemical energy conversion

作     者：Tiantian Li Yuting Deng Xiao Rong Chao He Mi Zhou Yuanjiao Tang Hongju Zhou Chong Cheng Changsheng Zhao 

作者机构：State Key Laboratory of Polymer Materials EngineeringCollege of Polymer Science and EngineeringSichuan UniversityChengduChina Department of NephrologyDepartment of UltrasoundWest China HospitalSichuan UniversityChengduChina Department of PhysicsChemistry and PharmacyDanish Institute for Advanced Study(DIAS)University of Southern DenmarkOdenseDenmark Med-X Center for MaterialsSichuan UniversityChengduChina College of Chemical EngineeringSichuan UniversityChengduChina 

出 版 物：《SmartMat》 (智能材料（英文）)

年 卷 期：2023年第4卷第1期

页      面：72-105页

核心收录：

学科分类：081705[工学-工业催化] 08[工学] 0817[工学-化学工程与技术] 080502[工学-材料学] 0805[工学-材料科学与工程（可授工学、理学学位）] 

基　　金：Science and Technology Project of Sichuan Province,Grant/Award Numbers:2022YFH0042,2022YFH0088,2022YFH0111,2022YFH0112 National Natural Science Foundation of China,Grant/Award Numbers:82001829,52161145402,52173133 State Key Laboratory of Polymer Materials Engineering,Grant/Award Number:sklpme2021-4-02 Fundamental Research Funds for the Central Universities 

主　　题：electrocatalytic applications energy conversion nanocatalysts and nanostructures Te-based materials transition metal tellurides 

摘      要：With the dramatic developments of renewable and environmental-friendly electrochemical energy conversion systems,there is an urgent need to fabricate durable and efficient electrocatalysts to address the limitation of high overpotentials exceeding thermodynamic requirements to facilitate practical ***,tellurium-based nanomaterials(Te NMs)with unique chemical,electronic,and topological properties,including Te-derived nanostructures and transition metal tellurides(TMTs),have emerged as one of the most promising electrocatalytic *** the absence of comprehensive and guiding reviews,this review comprehensively summarizes the main advances in designing emerging Te NMs for ***,the engineering strategies and principles of Te NMs to enhance their electrocatalytic activity and stability from the nanostructures to the catalytic atoms are discussed in detail,especially on the chemical/physical/multiplex templating strategies,heteroatom doping,vacancy/defect engineering,phase engineering,and the corresponding mechanisms and structure-performance ***,typical applications of Te NMs in electrocatalysis are also discussed in ***,the existing key issues and main challenges of Te NMs for electrocatalysis are highlighted,and the development trend of Te NMs as electrocatalysts is *** review provides new concepts to guide future directions for developing Te NMs-based electrocatalysts,thereby promoting their future wide applications in electrochemical energy systems.