Experimental analysis on calcination and carbonation process in calcium looping for CO_(2) capture: study case of cement plants in Indonesia

作     者：Triya Setia Febriatna Prihadi Setyo Darmanto Firman Bagja Juangsa 

作者机构：Master Program of Mechanical EngineeringFaculty of Mechanical and Aerospace EngineeringInstitut Teknologi BandungBandungIndonesia Faculty of Mechanical and Aerospace EngineeringInstitut Teknologi BandungBandungIndonesia Research Center for New and Renewable EnergyInstitut Teknologi BandungBandungIndonesia 

出 版 物：《Clean Energy》 (清洁能源（英文）)

年 卷 期：2023年第7卷第2期

页      面：313-327页

核心收录：

学科分类：083002[工学-环境工程] 0830[工学-环境科学与工程（可授工学、理学、农学学位）] 08[工学] 

基　　金：supported by Research and Community Service Program(P2MI)ITB 

主　　题：CO_(2)emissions cement industry carbon capture calcium looping calcination carbonation 

摘      要：Carbon dioxide(CO_(2))is the main contributor to greenhouse gases that affect global *** industrial sector is the third largest producer of CO_(2) and the cement industry is one of the industries that consistently produces the most significant CO_(2) *** cement industry produces 5-8% of global CO_(2) *** methods for reducing specific CO_(2) emissions have been reported in the cement industry,including calcium looping,which uses the reversible reaction between calcination[calcium carbonate(CaCO_(3))decomposition]and carbonation[CO_(2) capture by calcium oxide(CaO)].This work investigates calcium looping employing limestone obtained directly from several cement factories in Indonesia to observe the carbon-absorption characteristics of limestone from different mining *** experiment was carried out using a tube furnace equipped with a controlled atmospheric condition that functions as a calciner and a carbonator.X-ray diffraction and scanning electron microscopy with energy-dispersive x-ray spec-troscopy characterization were conducted to analyse the changes in the experimental *** results demonstrated that the reactor configuration was capable of performing the calcination process,which converted CaCO_(3) to calcium hydroxide[Ca(OH)_(2)],as well as the carbonation process,which captured carbon and converted it back to CaCO_(3).Parametric analysis was performed on both reactions,including pressure,temperature,duration,particle size and reaction *** results show that the limestone obtained from all sites can be used as the sorbents for the calcium-looping process with an average reactivity of 59.01%.Limestone from cement plants in various parts of Indonesia has the potential to be used as carbon sorbents in calcium-looping *** a similar CO_(2) concentration as the flue gas of 16.67%,the experimental results show that Bayah limestone has the maximum reactivity,as shown by the highest carbon-content a