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Laser‑Induced and MOF‑Derived Metal Oxide/Carbon Composite for Synergistically Improved Ethanol Sensing at Room temperature

作     者:Hyeongtae Lim Hyeokjin Kwon Hongki Kang Jae Eun Jang Hyuk‑Jun Kwon Hyeongtae Lim;Hyeokjin Kwon;Hongki Kang;Jae Eun Jang;Hyuk-Jun Kwon

作者机构:Department of Electrical Engineering and Computer ScienceDGISTDaegu 42988South Korea Convergence Research Advanced Centre for OlfactionDGISTDaegu 42988South Korea 

出 版 物:《Nano-Micro Letters》 (纳微快报(英文版))

年 卷 期:2024年第16卷第6期

页      面:210-220页

核心收录:

学科分类:081702[工学-化学工艺] 080202[工学-机械电子工程] 08[工学] 0817[工学-化学工程与技术] 0805[工学-材料科学与工程(可授工学、理学学位)] 080502[工学-材料学] 0802[工学-机械工程] 

基  金:supported by the National Research Foundation of Korea(NRF)grants funded by the Ministry of Science and ICT(MSIT)(RS-2023-00251283,and 2022M3D1A2083618) by the Ministry of Education(2020R1A6A1A03040516) 

主  题:Metal-organic frameworks Metal oxide Carbon composite Laser Gas sensor 

摘      要:Advancements in sensor technology have significantly enhanced atmospheric ***,metal oxide and carbon(MO_(x)/C)hybrids have gained attention for their exceptional sensitivity and room-temperature sensing ***,previous methods of synthesizing MO_(x)/C composites suffer from problems,including inhomogeneity,aggregation,and challenges in ***,we introduce a refined method that employs a metal–organic framework(MOF)as a precursor combined with direct laser *** inherent structure of MOFs ensures a uniform distribution of metal ions and organic linkers,yielding homogeneous MO_(x)/C *** laser processing facilitates precise micropatterning(2μm,comparable to typical photolithography)of the MO_(x)/C *** optimized MOF-derived MO_(x)/C sensor rapidly detected ethanol gas even at room temperature(105 and 18 s for response and recovery,respectively),with a broad range of sensing performance from 170 to 3,400 ppm and a high response value of up to 3,500%.Additionally,this sensor exhibited enhanced stability and thermal resilience compared to previous MOF-based *** research opens up promising avenues for practical applications in MOF-derived sensing devices.

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