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Stable nanobubbles on ordered water monolayer near ionic model surfaces

作     者:Luyao Huang Cheng Ling Limin Zhou Wenlong Liang Yujie Huang Lijuan Zhang Phornphimon Maitarad Dengsong Zhang Chunlei Wang 黄璐瑶;凌澄;周利民;梁文龙;黄雨婕;张立娟;Phornphimon Maitarad;张登松;王春雷

作者机构:Research Center of Nano Science and TechnologyDepartment of ChemistryCollege of SciencesShanghai UniversityShanghai 200444China International Joint Laboratory of Catalytic ChemistryCollege of SciencesShanghai UniversityShanghai 200444China Shanghai Institute of Applied PhysicsChinese Academy of SciencesShanghai 201800China University of Chinese Academy of SciencesBeijing 100049China Shanghai Synchrotron Radiation FacilityShanghai Advanced Research InstituteChinese Academy of SciencesShanghai 201204China 

出 版 物:《Chinese Physics B》 (中国物理B(英文版))

年 卷 期:2025年第34卷第1期

页      面:143-148页

核心收录:

学科分类:081704[工学-应用化学] 07[理学] 070304[理学-物理化学(含∶化学物理)] 08[工学] 0817[工学-化学工程与技术] 0703[理学-化学] 

基  金:supported by the National Natural Science Foundation of China(Grant Nos.12022508,12074394,and 22125604) Shanghai Supercomputer Center of China Shanghai Snowlake Technology Co.Ltd 

主  题:nanobubbles molecular dynamic simulation ordered water monolayer hydrogen bond network 

摘      要:The stable nanobubbles adhered to mineral surfaces may facilitate their efficient separation via flotation in the mining ***,the state of nanobubbles on mineral solid surfaces is still *** this study,molecular dynamics(MD)simulations are employed to examine mineral-like model surfaces with varying degrees of hydrophobicity,modulated by surface charges,to elucidate the adsorption behavior of nanobubbles at the *** findings not only contribute to the fundamental understanding of nanobubbles but also have potential applications in the mining *** observed that as the surface charge increases,the contact angle of the nanobubbles increases accordingly with shape transformation from a pancake-like gas film to a cap-like shape,and ultimately forming a stable nanobubble upon an ordered water *** the solid–water interactions are weak with a small partial charge,the hydrophobic gas(N_(2))molecules accumulate near the solid ***,we have found,for the first time,that gas molecules assemble a nanobubble on the water monolayer adjacent to the solid surfaces with large partial *** phenomena are attributed to the formation of a hydrophobic water monolayer with a hydrogen bond network structure near the surface.

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