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Dielectric and magnetic anomalies and spin frustration in hexagonal RMnO3 (R=Y, Yb, and Lu)

作     者:T. Katsufuji S. Mori M. Masaki Y. Moritomo N. Yamamoto H. Takagi 

作者机构:Department of Advanced Materials Science and Department of Applied Chemistry University of Tokyo Tokyo 113-8656 Japan Core Research for Evolutional Science and Technology (CREST) Japan Science and Technology Corporation Japan Department of Physics Tokyo Institute of Technology Tokyo 152-8551 Japan CIRSE and Department of Crystalline Materials Science Nagoya University Nagoya 464-8601 Japan 

出 版 物:《Physical Review B》 (Phys. Rev. B Condens. Matter Mater. Phys.)

年 卷 期:2001年第64卷第10期

页      面:104419-104419页

核心收录:

学科分类:0808[工学-电气工程] 0809[工学-电子科学与技术(可授工学、理学学位)] 07[理学] 0805[工学-材料科学与工程(可授工学、理学学位)] 0702[理学-物理学] 

摘      要:Single crystals of hexagonal RMnO3 (R=Y, Yb, and Lu), where Mn ions form the triangular lattice, were investigated, focusing on their dielectric/magnetic anomalies as well as geometrical spin frustration. It is found that the ratio of a Weiss temperature to TN is ∼10 in RMnO3, indicating the dominant role of strong geometrical frustration. The effect of geometrical frustration also appears in specific heat, which shows a presence of a substantial amount of residual magnetic contribution below TN, indicating that a part of the spins are still fluctuating at T≪TN. It is also found that the dielectric anomaly at TN is strongly anisotropic, suggesting a unique correlation between magnetism and dielectric properties in these compounds.

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