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Manipulating Vertical Phase Separation Enables Pseudoplanar Heterojunction Organic Solar Cells Over 19% Efficiency via Ternary Polymerization

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ADVANCED MATERIALS 2024年第5期36卷 2308909-2308909页

作者： He, Dan Zhou, Jixiang Zhu, Yufan Li, Yawen Wang, Ke Li, Jie Zhang, Jianqi Li, Bao lin, Yuze He, Yuehui Wang, Chunru Zhao, fuwen Cent South Univ State Key Lab Powder Met Changsha 410083 Peoples R China Chinese Acad Sci Beijing Natl Lab Mol Sci CAS Key Lab Organ Solids Inst Chem Beijing 100190 Peoples R China Chinese Acad Sci Inst Chem Lab Mol Nanostruct & Nanotechnol Beijing 100190 Peoples R China Univ Chinese Acad Sci Beijing 100190 Peoples R China CAS Ctr Excellence Nanosci Natl Ctr Nanosci & Technol CAS Key Lab Nanosyst & Hierarch Fabricat Beijing 100190 Peoples R China Henan Normal Univ Sch Chem & Chem Engn Xinxiang 453007 Peoples R China

Controlling vertical phase separation of the active layer to enable efficient exciton dissociation and charge carrier transport is crucial to boost power conversion efficiencies (PCEs) of pseudoplanar heterojunction (PPHJ) organic solar cells (OSCs). However, how to optimize the vertical phase separation of PPHJ OSCs via molecule design is rarely reported yet. Herein, ternary polymerization strategy is employed to develop a series of polymer donors, DL1-DL4, and regulate their solubility, molecular aggregation, molecular orientation, and miscibility, thus efficiently manipulating vertical phase separation in PPHJ OSCs. Among them, DL1 not only has enhanced solubility, inhibited molecular aggregation and partial edge-on orientation to facilitate acceptor molecules, Y6, to permeate into polymer layer and increase donor/acceptor interfaces, but also sustains high crystallinity and appropriate miscibility with Y6 to acquire ordered molecular packing, thus achieving optimized vertical phase separation to well juggle exciton dissociation and charge transport in PPHJ devices. Therefore, DL1/Y6 based PPHJ OSCs gain the best exciton dissociation probability, highest charge carrier mobilities and weakest charge recombination, and thus afford an impressive PCE of 19.10%, which is the record value for terpolymer donors. It demonstrates that ternary polymerization is an efficient method to optimize vertical phase separation in PPHJ OSCs for high PCEs. Ternary polymerization strategy is employed to manipulate the vertical phase separation in pseudoplanar heterojunction (PPHJ) organic solar cells (OSCs). The terpolymer DL1, with enhanced solubility, partial edge-on orientation, and high crystallinity, endows DL1/Y6 PPHJ blend film with the optimized vertical phase separation. Therefore, DL1/Y6 based PPHJ OSCs afford an impressive PCE of 19.10%, which is the record for terpolymer ***

关键词： layer-by-layer techniques organic solar cells terpolymers vertical phase separation

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Highly efficient fused ring electron acceptors based on a new undecacyclic core

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MATERIALS CHEMISTRY FRONTIERS 2021年第4期5卷 2001-2006页

作者： Zhao, fuwen He, Dan Xin, Jingming Zhang, Huotian Zhou, Jixiang lin, Baojun He, Yongju Li, Jiang Ma, Wei Li, Bao Gao, Feng Li, Yongfang Wang, Chunru Cent South Univ State Key Lab Powder Met Changsha 410083 Peoples R China Chinese Acad Sci Inst Chem Beijing 100190 Peoples R China Linkoping Univ Dept Phys Chem & Biol IFM SE-58183 Linkoping Sweden Xi An Jiao Tong Univ State Key Lab Mech Behav Mat Xian 710049 Peoples R China Henan Normal Univ Sch Chem & Chem Engn Xinxiang 453007 Henan Peoples R China

Two FREAs, IUIC-O and IUIC-T, based on an undecacyclic core were developed. IUIC-T having a higher extinction coefficient affords aligned energy levels with PBDB-T, finer nanoscale morphology and more orderly molecular stacking, thus achieving more efficient exciton dissociation and charge transport. Therefore, the PBDB-T:IUIC-T based OSC gains a higher PCE of 13.05%.

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Suppressing Exciton-Vibration Coupling to Prolong Exciton Lifetime of Nonfullerene Acceptors Enables High-Efficiency Organic Solar Cells

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ENERGY REPORTS 2024年第8期11卷 e202316227-e202316227页

作者： Zhu, Yufan He, Dan Wang, Chong Han, Xiao Liu, Zesheng Wang, Ke Zhang, Jianqi Shen, Xingxing Li, Jie lin, Yuze Wang, Chunru He, Yuehui Zhao, fuwen Cent South Univ State Key Lab Powder Met Changsha 410083 Peoples R China Cent South Univ Coll Chem & Chem Engn Changsha 410083 Peoples R China Univ Chinese Acad Sci Beijing 100190 Peoples R China Chinese Acad Sci Beijing Natl Lab Mol Sci CAS Key Lab Organ Solids Beijing 100190 Peoples R China Chinese Acad Sci Lab Mol Nanostruct & Nanotechnol Inst Chem Beijing 100190 Peoples R China

The limited exciton lifetime (tau, generally < 1 ns) leads to short exciton diffusion length (L-D) of organic semiconductors, which is the bottleneck issue impeding the further improvement of power conversion efficiencies (PCEs) for organic solar cells (OSCs). However, efficient strategies to prolong intrinsic tau are rare and vague. Herein, we propose a facile method to efficiently reduce vibrational frequency of molecular skeleton and suppress exciton-vibration coupling to decrease non-radiative decay rate and thus prolong tau via deuterating nonfullerene acceptors. The tau remarkably increases from 0.90 ns (non-deuterated L8-BO) to 1.35 ns (deuterated L8-BO-D), which is the record for organic photovoltaic materials. Besides, the inhibited molecular vibration improves molecular planarity of L8-BO-D for enhanced exciton diffusion coefficient. Consequently, the L-D increases from 7.9 nm (L8-BO) to 10.7 nm (L8-BO-D). The prolonged L-D of L8-BO-D enables PM6: L8-BO-D-based bulk heterojunction OSCs to acquire higher PCEs of 18.5% with more efficient exciton dissociation and weaker charge carrier recombination than PM6: L8-BO-based counterparts. Moreover, benefiting from the prolonged L-D, D18/L8-BO-D-based pseudo-planar heterojunction OSCs achieve an impressive PCE of 19.3%, which is among the highest values. This work provides an efficient strategy to increase the tau and thus L-D of organic semiconductors, boosting PCEs of OSCs.

关键词： Deuteration Exciton Diffusion Length Exciton Lifetime Exciton-Vibration Coupling Organic Solar Cells

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Integrative study to determine the anti-tumor role and mechanism of Chouchunpi San in colorectal cancer

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Pharmacological Research - Modern Chinese Medicine 2024年 13卷

作者： Shi, Nuolin Li, Mingjie Li, Xuehui Hou, Xinxin Wang, Mingzhu Ni, Zhongya lin, Shan Hu, Liang Yuan, fuwen School of Integrative Medicine Shanghai University of Traditional Chinese Medicine Cailun Rd #1200 Shanghai 201203 China Shanghai TCM-Integrated Hospital Shanghai University of Traditional Chinese Medicine Jingan Zhijiang Middle Rd #274 Shanghai 200082 China Yueyang Hospital of Integrated Traditional Chinese and Western Medicine Shanghai University of Traditional Chinese Medicine Shanghai 200437 China Jsinnopharm Shanghai 201203 China

Introduction: The herbal formula Chouchunpi San (CCPS) is a traditional formula that has been widely used and proven effective in various clinical cancer treatments. However, the mechanism of its anticancer effect remains unclear. This study aims to determine the anti-tumor effect of CCPS on colorectal cancer (CRC) in vivo and in vitro and to explore the underlying molecular mechanisms. Methods: Cell counting kit-8 assays, colony-forming assays, and flow cytometry for cell cycle and apoptosis assays were employed to determine the anti-tumor roles of CCPS. Liquid chromatography-mass spectrometry (LC-MS), network pharmacology, molecular docking, analysis of real-world clinical datasets of CRC, and western blotting were conducted to explore the molecular mechanism of CCPS on CRC. CRC xenografted mouse model, western blotting, and public CRC data analysis were conducted to evaluate the anti-tumor efficacy and mechanisms of CCPS on CRC. Results: CCPS suppresses the growth of CRC cells and increases the number of apoptotic cells dose-dependently. CCPS targets and significantly downregulates RPA1 and enhances the phosphorylation of its downstream effectors, ATR and CHK1, which are critical for CRC progression. Additionally, CCPS shows a comparable anti-tumor effect in CRC xenografted mouse models compared to Capecitabine, a chemotherapy drug commonly used in clinics. Discussion: Our findings demonstrate the potential use of CCPS in cancer treatment by suppressing cancer cell growth and modulating the RPA1/ATR/CHK1 signaling pathway in CRC. Further investigations on the application of CCPS in cancer therapies could be extended to evaluate the potential in vivo toxicity and adverse events, as well as the synergistic effect of CCPS in combination with other chemotherapeutic agents. © 2024 The Author(s)

关键词： Ailanthone ATR/CHK1 signaling Chouchunpi San Colorectal cancer RPA1

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Toxicological assessment and underlying mechanisms of tetrabromobisphenol A exposure on the soil nematode Caenorhabditis elegans

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CHEMOSPHERE 2020年 242卷 125078页

作者： Liu, fuwen Zhang, Ying Zhang, Meng Luo, Qishi Cao, Xue Cui, Changzheng lin, Kuangfei Huang, Kai East China Univ Sci & Technol Sch Resource & Environm Engn State Environm Protect Key Lab Environm Risk Asse Shanghai 200237 Peoples R China Yonker Environm Protect Co Ltd Branch Shanghai Shanghai 200051 Peoples R China

The widespread use of tetrabromobisphenol A (TBBPA) in industries has resulted in its frequent detection in environmental matrices, and the mechanisms of its associated hazards need further investigation. In this study, the nematode Caenorhabditis elegans (C elegans) was exposed to environmentally relevant concentrations of TBBPA (0, 0.1, 1, 10, 100, 200 mu g/L) to determine its effects. At TBBPA concentrations above 1 mu g/L, the number of head thrashes, as the most sensitive physiological indicator, decreased significantly. Using the Illumina HiSeq (TM) 2000 sequencer, differentially expressed genes (DEGs) were determined, and 52 were down regulated and 105 were up regulated in the 200 mu g/L TBBPA treatment group versus the control group. Gene Ontology (GO) and Kyoto Encyclopedia of Genes and Genomes (KEGG) pathway database analysis demonstrated that dorso-ventral axis formation is related to neurotoxicity;metabolism of xenobiotics by Cytochrome P450 (CYP450) and glutathione-S-transferase (GST) was found to be the vital metabolic mechanisms and were confirmed by quantitative real-time polymerase chain reaction (qRT-PCR). GST was ascribed to the augmentation because mutations in cyp-13A7 were constrained under TBBPA exposure. Additionally, oxidative stress indicators accumulated in a dose-dependent relationship. These results will help understand the molecular basis for TBBPA-induced toxicity in C. elegans and open novel avenues for facilitating the exploration of more efficient strategies against TBBPA toxicity. (C) 2019 Elsevier Ltd. All rights reserved.

关键词： Caenorhabditis elegans TBBPA Neurotoxicity Transcriptome Cyp-13A7

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Preoperative Prediction of Ancillary Lymph Node Metastasis in Breast Carcinoma Using Radiomics Features Based on the Fat-Suppressed T2 Sequence

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ACADEMIC RADIOLOGY 2020年第9期27卷 1217-1225页

作者： Tan, Hongna Gan, fuwen Wu, Yaping Zhou, Jing Tian, Jie lin, Yusong Wang, Meiyun Zhengzhou Univ Dept Radiol Henan Prov Peoples Hosp 7 RdWeiwu Rd Zhengzhou 450003 Henan Peoples R China Zhengzhou Univ Imaging Diag Neurol Dis & Res Lab Henan Prov & Peoples Hosp 7 RdWeiwu Rd Zhengzhou 450003 Henan Peoples R China Zhengzhou Univ Collaborat Innovat Ctr Internet Healthcare Zhengzhou 450052 Henan Peoples R China Zhengzhou Univ Sch Informat Engn Zhengzhou 450052 Henan Peoples R China Chinese Acad Sci Inst Automat Beijing 100190 Peoples R China

Rationale and Objectives: To investigate the value of radiomics method based on the fat-suppressed T2 sequence for preoperative predicting axillary lymph node (ALN) metastasis in breast carcinoma. Materials and Methods: The data of 329 invasive breast cancer patients were divided into the primary cohort (n = 269) and validation cohort (n = 60). Radiomics features were extracted from the fat-suppressed T2-weighted images on breast MRI, and ALN metastasis-related radiomics feature selection was performed using Mann-Whitney U-test and support vector machines with recursive feature elimination;then a radiomics signature was constructed by linear support vector machine. The predictive models were constructed using a linear regression model based on the clinicopathologic factors and radiomics signature, and nomogram was used for a visual prediction of the combined model. The predictive performances are evaluated with the sensitivity, specificity, accuracy, and area under the receiver operating characteristic curve. Results: A total of 647 radiomics features were extracted from each patient. About 23 ALN metastasis-related radiomics features were selected to construct the radiomics signature, including 17 texture features, 5 first-order statistical features, and one shape feature;patient age, tumor size, HER2 status, and vascular cancer thrombus accompanied or not were selected to construct the cilinicopathologic feature model. The sensitivity, specificity, accuracy, and are under the curve value of radiomics signature, clinicopathologic feature model, and the nomogram were 65.22%, 81.08%, 75.00%, and 0.819 (95% confidence interval [CI]: 0.776-0.861), 30.44%, 81.08%, 61.67%, and 0.605 (95% CI: 0.571-0.624) and 60.87%, 89.19%, 78.33%, and 0.810 (95% CI: 0.761-0.855), respectively. Conclusion: Radiomics methods based on the fat-suppressed T2 sequence and the nomogram are helpful for preoperative accurate predicting ALN metastasis.

关键词： Breast cancer Axillary lymph node Metastasis MRI Radiomics

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Trans-generational effect of neurotoxicity and related stress response in Caenorhabditis elegans exposed to tetrabromobisphenol A

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SCIENCE OF THE TOTAL ENVIRONMENT 2020年第0期703卷 134920-000页

作者： Liu, fuwen Luo, Qishi Zhang, Ying Huang, Kai Cao, Xue Cui, Changzheng lin, Kuangfei Zhang, Meng East China Univ Sci & Technol Sch Resource & Environm Engn State Environm Protect Key Lab Environm Risk Asse Shanghai 200237 Peoples R China Yonker Environm Protect Co Ltd Branch Shanghai Shanghai 200051 Peoples R China

Tetrabromobisphenol A (TBBPA), one of the most common brominated flame retardants, has been associated with immunotoxicity, neurotoxicity, and reproductive toxicity. However, little attention has been focused on understanding the trans-generational effects of TBBPA. The present study used the Caenorhabditis elegans (C. elegans) animal model to evaluate the trans-generational effects of neurotoxicity induced by environmentally relevant concentrations of TBBPA (0, 0.1, 1, 10, 100, and 1000 mu g/L). Multiple indicators including physiological effects (body length, brood size, head thrashes, body bends, and crawling trajectory), degree of neuronal damage (dopamine, GABAergic, and glutamatergic neurons), oxidative stress-related biochemical indicators (superoxide dismutase [SOD] activity, catalase [CAT] enzyme, malondialdehyde [MDA] production, and reactive oxygen species [ROS] accumulation), and stress-related gene expressions have been evaluated in the exposed parental C. elegans generation (G(1)) and their progeny (G(2)) under TBBPA-free conditions. The results showed that TBBPA exposure induced adverse effects on physiological endpoints, among which body bends and head thrashes were the most sensitive ones, detected above 1 mu g/L in G(1) and 100 mu g/L in G(2) nematodes, respectively. After contaminant exposure, the three neurons revealed damage related to neurobehavioral endpoints, with no hereditary effects in the progeny. The oxidative stress-related biochemical endpoints demonstrated that when the exposure concentrations were above 1 mu g/L in maternal worms, impairment can be detected in both generations, but the progeny recovered at low toxicity concentration (1-100 mu g/L). The integrated target gene expression profiles were clearly altered in G(1) and G(2) worms at concentrations between 1 and 1000 mu g/L, and a more significant difference existed in two generations of nematodes at low levels (1-10 mu g/L) of TBBPA. Studing trans-generational neurotoxicity a

关键词： TBBPA Caenorhabditis elegans Trans-generational effect Neurotoxicity Environmental risk

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Genomic evidence for low genetic diversity but purging of strong deleterious variants in snow leopards

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GENOME BIOLOGY 2025年第1期26卷 1-24页

作者： Yang, lin Jin, Hong Yang, Qien Poyarkov, Andrey Korablev, Miroslav Rozhnov, Viatcheslav Shao, Junjie Fu, Qiaomei Hernandez-Blanco, Jose Antonio Zhan, Xiangjiang Yu, Li Alexandrov, Dmitry Dai, Qingyan Munkhtsog, Bariushaa Du, Xin Munkhtsog, Bayaraa Ma, Liqing Chen, Wanlin Malykh, Sergei Jin, Yipeng He, Shunfu Zhang, Tongzuo Wu, Guosheng Shi, Yonghong Wei, fuwen Hu, Yibo Chinese Acad Sci Inst Zool CAS Key Lab Anim Ecol & Conservat Biol Beijing Peoples R China Jiangxi Agr Univ Coll Forestry Jiangxi Key Lab Conservat Biol Nanchang Jiangxi Peoples R China Southern Marine Sci & Engn Ctr Evolut & Conservat Biol Guangdong Lab Guangzhou Peoples R China Chinese Acad Sci Northwest Inst Plateau Biol Key Lab Adaptat & Evolut Plateau Biota Xining Qinghai Peoples R China Russian Acad Sci AN Severtsov Inst Ecol & Evolut Moscow Russia Univ Chinese Acad Sci Beijing Peoples R China Chinese Acad Sci Inst Vertebrate Paleontol & Paleoanthropol Key Lab Vertebrate Evolut & Human Origins Beijing Peoples R China Yunnan Univ State Key Lab Conservat & Utilizat Bioresource Kunming 650091 Yunnan Peoples R China Irbis Mongolia Ctr Ulaanbaatar Mongolia Mongolian Acad Sci Inst Biol Ulaanbaatar Mongolia Qinghai Univ Qinghai Acad Anim Sci & Vet Med Qinghai Prov Key Lab Pathogen Diag Anim Dis Xining 810016 Qinghai Peoples R China Qinghai Univ Green Techn Res Prevent & Control Xining Qinghai Peoples R China China Agr Univ Coll Vet Med Clin Dept Beijing Peoples R China Xining Wildlife Zoo Xining Qinghai Peoples R China Golmud Forestry & Grassland Stn Qinghai Prov Haixi 816000 Peoples R China

BackgroundLong-term persistence of species with low genetic diversity is the focus of widespread attention in conservation biology. The snow leopard, Panthera uncia, is a big cat from high-alpine regions of Asia. However, its subspecies taxonomy, evolutionary history, evolutionary potential, and survival strategy remain unclear, which greatly hampers their *** sequence a high-quality chromosome-level genome of the snow leopard and the genomes of 52 wild snow leopards. Population genomics reveal the existence of two large genetic lineages in global snow leopards, the northern and southern lineages, supported by the biogeography. The Last Glacial Maximum drove the divergence of two lineages. Microclimate differences and large rivers between the western and central Himalayas likely maintain the differentiation of two lineages. EPAS1 is positively selected in the southern lineage with almost fixed amino acid substitutions and shows an increased allele frequency with elevation. Compared to the southern lineage, the northern lineage exhibits a lower level of genomic diversity and higher levels of inbreeding and genetic load, consistent with its recent population decline. We find that snow leopards have extremely low genomic diversity and higher inbreeding than other Carnivora species;however, strong deleterious mutations have been effectively purged in snow leopards by historical population bottlenecks and inbreeding, which may be a vital genetic mechanism for their population survival and *** findings reveal the survival strategy of a species with low genetic diversity and highlight the importance of unveiling both genetic diversity and genetic burden for the conservation of threatened species.

关键词： Snow leopards Population genomics Genetic structure Genomic diversity Deleterious variants EPAS1

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Evolutionary Conservation Genomics Reveals Recent Speciation and Local Adaptation in Threatened Takins

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MOLECULAR BIOLOGY AND EVOLUTION 2022年第6期39卷 msac111-msac111页

作者： Yang, lin Wei, fuwen Zhan, Xiangjiang Fan, Huizhong Zhao, Pengpeng Huang, Guangping Chang, Jiang Lei, Yinghu Hu, Yibo Chinese Acad Sci Inst Zool CAS Key Lab Anim Ecol & Conservat Biol Beijing Peoples R China Univ Chinese Acad Sci Beijing Peoples R China Chinese Acad Sci Ctr Excellence Anim Evolut & Genet Kunming Yunnan Peoples R China Shaanxi Louguantai Rescue & Breeding Ctr Rare Wil Xian Shaanxi Peoples R China Chinese Res Inst Environm Sci State Key Lab Environm Criteria & Risk Assessment Beijing Peoples R China

Incorrect species delimitation will lead to inappropriate conservation decisions, especially for threatened species. The takin (Budorcas taxicolor) is a large artiodactyl endemic to the Himalayan-Hengduan-Qinling Mountains and is well known for its threatened status and peculiar appearance. However, the speciation, intraspecies taxonomy, evolutionary history, and adaptive evolution of this species still remain unclear, which greatly hampers its scientific conservation. Here, we de novo assembled a high-quality chromosome-level genome of takin and resequenced the genomes of 75 wild takins. Phylogenomics revealed that takin was positioned at the root of Caprinae. Population genomics based on the autosome, X chromosome, and Y chromosome SNPs and mitochondrial genomes consistently revealed the existence of two phylogenetic species and recent speciation in takins: the Himalayan takin (B. taxicolor) and the Chinese takin (B. tibetana), with the support of morphological evidence. Two genetically divergent subspecies were identified in both takin species, rejecting three previously proposed taxonomical viewpoints. Furthermore, their distribution boundaries were determined, suggesting that large rivers play important roles in shaping the genetic partition. Compared with the other subspecies, the Qinling subspecies presented the lowest genomic diversity, higher linkage disequilibrium, inbreeding, and genetic load, thus is in urgent need of genetic management and protection. Moreover, coat color gene (PMEL) variation may be responsible for the adaptive coat color difference between the two species following Gloger's rule. Our findings provide novel insights into the recent speciation, local adaptation, scientific conservation of takins, and biogeography of the Himalaya-Hengduan biodiversity hotspot.

关键词： takins chromosome-level genome population genomics recent speciation adaptive evolution

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Different calcification responses of two hermatypic corals to CO2-driven ocean acidification

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ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH 2019年第30期26卷 30596-30602页

作者： Zheng, Xinqing Kuo, fuwen Pan, Ke Huang, Haining lin, Rongcheng State Ocean Adm Inst Oceanog 3 Xiamen Fujian Peoples R China Natl Museum Marine Biol & Aquarium Pingtung Taiwan Shenzhen Univ Inst Adv Study Shenzhen Guangdong Peoples R China

Understanding how calcification is influenced by the enhanced dissolution of CO2 in the oceans is the key to evaluating the effects of ocean acidification (OA) on coral reefs. In this study, two branching hermatypic corals widely distributed in the South China Sea, Pocillopora damicornis and Seriatopora caliendrum, were used to study the calcification responses to CO2-driven OA (7.77 +/- 0.07 vs. 8.15 +/- 0.12). Our results showed that the calcification rate (0.17 +/- 0.04%/day to 0.21 +/- 0.12%/day) in P. damicornis remained unchanged in the acidified seawaters, but that in S. caliendrum decreased significantly (0.62 +/- 0.21%/day to 0.44 +/- 0.11%/day). Our results suggested that reef corals with high calcification rates may be more susceptible to the enhanced dissolution of CO2. Differential calcified response to elevated CO2 may be closely attributed to coralline capacity of the upregulation at their site of calcification in acidified seawater.

关键词： Ocean acidification Pocillopora damicornis Seriatopora caliendrum Calcification

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