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Atomically ordered Rh₂P catalysts anchored within hollow mesoporous carbon for efficient hydrogen production

CHEMICAL COMMUNICATIONS 2021年第92期57卷 12345-12348页

作者： Guo, xuwen Chen, Xin huang, Yanping Min, Xiaowen Kong, Chuncai Tang, Yawen Liu, Ben Nanjing Normal Univ Jiangsu Collaborat Innovat Ctr Biomed Funct Mat Sch Chem & Mat Sci Jiangsu Key Lab New Power Batteries Nanjing 210023 Peoples R China ME Instruments Inc Huahan Sci & Technol Ind Pk Shenzhen 518118 Peoples R China Sichuan Univ Ctr Engn Expt Teaching Sch Chem Engn Chengdu 610065 Peoples R China Sichuan Univ Coll Chem Key Lab Green Chem & Technol Minist Educ Chengdu 610064 Peoples R China Shaanxi Prov Key Lab Adv Funct Mat & Mesoscop Phy Sch Phys Minist EducKey Lab Nonequilibrium Synth & Modula Xian Jiaotong Univ Xian 710049 Peoples R China

Atomically ordered Rh2P nanoclusters encapsulated within a high-surface-area hollow mesoporous carbon nanoreactor are catalytically active for hydrogen production via the electrocatalytic hydrogen evolution reaction a... 详细信息

关键词： Hydrogen production

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Memristive Artificial Synapses for Neuromorphic Computing

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Nano-Micro Letters 2021年第5期13卷 218-245页

作者： Wen huang xuwen Xia Chen Zhu Parker Steichen Weidong Quan Weiwei Mao Jianping Yang Liang Chu Xing’ao Li New Energy Technology Engineering Laboratory of Jiangsu Province and School of Science Nanjing University of Posts and Telecommunications(NJUPT)Nanjing 210023People’s Republic of China Key Laboratory for Organic Electronics and Information Displays and Institute of Advanced Materials Jiangsu National Synergistic Innovation Center for Advanced MaterialsSchool of Materials Science and EngineeringNanjing University of Posts and Telecommunications(NUPT)9 Wenyuan RoadNanjing 210023People’s Republic of China College of Electronic and Optical Engineering and College of Microelectronics Nanjing University of Posts and Telecommunications(NJUPT)Nanjing 210023People’s Republic of China Department of Materials Science and Engineering University of WashingtonSeattleWA 98195‑2120USA

Neuromorphic computing simulates the operation of biological brain function for information processing and can potentially solve the bottleneck of the von Neumann *** computing is realized based on memristive hardware neural networks in which synaptic devices that mimic biological synapses of the brain are the primary *** synaptic functions with these devices is critical in neuromorphic *** the last decade,electrical and optical signals have been incorporated into the synaptic devices and promoted the simulation of various synaptic *** this review,these devices are discussed by categorizing them into electrically stimulated,optically stimulated,and photoelectric synergetic synaptic devices based on stimulation of electrical and optical *** working mechanisms of the devices are analyzed in *** is followed by a discussion of the progress in mimicking synaptic *** addition,existing application scenarios of various synaptic devices are ***,the performances and future development of the synaptic devices that could be significant for building efficient neuromorphic systems are prospected.

关键词： Synaptic devices Neuromorphic computing Electrical pulses Optical pulses Photoelectric synergetic effects

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A graphene modified anode to improve the performance of microbial fuel cells

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JOURNAL OF POWER SOURCES 2011年第13期196卷 5402-5407页

作者： Zhang, Yezhen Mo, Guangquan Li, xuwen Zhang, Weide Zhang, Jiaqi Ye, Jianshan huang, Xiaodan Yu, Chengzhong S China Univ Technol Sch Chem & Chem Engn Guangzhou 510641 Peoples R China Tianjin Univ Technol Sch Environm Sci & Safety Engn Tianjin 300071 Peoples R China Fudan Univ Dept Chem Shanghai 200433 Peoples R China Fudan Univ Shanghai Key Lab Mol Catalysis & Innovat Mat Shanghai 200433 Peoples R China Univ Queensland ARC Ctr Excellence Funct Nanomat Brisbane Qld 4072 Australia Univ Queensland Australian Inst Bioengn & Nanotechnol Brisbane Qld 4072 Australia

Graphene with a Brunauer similar to Emmett-Teller (BET) specific surface area of 264 m(2) g(-1) has been used as anodic catalyst of microbial fuel cells (MFCs) based on Escherichia coli (ATCC 25922). The electrochemical activities of plain stainless steel mesh (SSM), polytetrafluoroethylene (PTFE) modified SSM (PMS) and graphene modified SSM (GMS) have been investigated by cyclic voltammetry (CV), discharge experiment and polarization curve measurement. The GMS shows better electrochemical performance than those of SSM and PMS. The MFC equipped with GMS anode delivers a maximum power density of 2668 mW m(-2), which is 18 times larger than that obtained from the MFC with the SSM anode and is 17 times larger than that obtained from the MFC with the PMS anode. Scanning electron microscopy (SEM) results indicate that the increase in power generation could be attributed to the high surface area of anode and an increase in the number of bacteria attached to anode. (C) 2011 Elsevier B.V. All rights reserved.

关键词： Graphene Biocatalyst Microbial fuel cells

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Transient Stability Evaluation of Independent Microgrid based on Message Passing Graph Neural Network 6

Transient Stability Evaluation of Independent Microgrid base...

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6th International Conference on Electronics Technology, ICET 2023

作者： Zhen, Jiubao huang, Shufan Jia, xuwen Du, Haocheng China Agricultural University College of Information and Electrical Engineering Beijing100083 China Shandong University Key Laboratory of Power System Intelligent Dispatch and Control of Ministry of Education Jinan250061 China

ISBN: (纸本)9798350337693

Virtual synchronous generator is used to control independent microgrid to provide inertia and damping support, but it often brings transient stability problems. Due to the large number of nonlinear and non-smooth characteristics of highly electronic independent microgrid, it is difficult to analyze it by the traditional transient stability analysis method. In this paper, the independent microgrid controlled by virtual synchronization is taken as the object. Firstly, we compare the impact of detailed modeling of energy storage and simplified modeling on the transient stability, and then discuss the impact of current limiting link of virtual synchronous machine on the transient stability. Secondary, combined with the idea of graph neural network, we propose an independent microgrid transient stability evaluation model based on message passing graph neural network. The information corresponding to bus and transmission lines in microgrid is aggregated and updated by message passing mechanism, so as to depict the topological connection relationship of microgrid, and then consider the influence of topology structure on transient stability evaluation. Last, a WSCC-9 system with virtual synchronous machine is taken as an example. The results show that considering the energy storage detailed model and current limiting link can effectively improve the accuracy of stability analysis. The proposed method has stronger generalization ability and is more applicable to the microgrid system with variable topological structure. © 2023 IEEE.

关键词： Stability

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Mesoporous Palladium-Boron-Sulfur Alloy Nanospheres for Efficient Hydrogen Evolution

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INORGANIC CHEMISTRY 2021年第7期60卷 4380-4384页

作者： Guo, xuwen Chen, Zhichao huang, Yanping Lv, Hao Wang, Yaru Sun, Lizhi Song, Kai Liu, Ben Nanjing Normal Univ Jiangsu Collaborat Innovat Ctr Biomed Funct Mat Sch Chem & Mat Sci Jiangsu Key Lab New Power Batteries Nanjing 210023 Peoples R China Shenzhen RELX Technol Co Ltd Shenzhen 518108 Peoples R China Sichuan Univ Coll Chem Chengdu 610064 Peoples R China Changchun Normal Univ Sch Life Sci Changchun 130032 Peoples R China Sichuan Univ Sch Chem Engn Ctr Engn Expt Teaching Chengdu 610065 Peoples R China

Ternary noble metal-metalloid-nonmetal PdBS alloy mesoporous nanospheres (MSs) with three-dimensional central-radial pore channels were prepared for an electrocatalytic hydrogen evolution reaction. The synthesis was performed via precise control in the reduction and nucleation growth of ternary PdBS alloy MSs along confined cylinder mesophases assembled by amphiphilic dioctadecyldimethylammonium chloride. The resultant PdBS alloy MSs disclosed a remarkably improved electrocatalytic performance due to their structural and compositional synergies. This finding extended our knowledge on the rational design and targeted synthesis of novel noble metal-metalloid-nonmetal alloys with desired structures and morphologies for catalysis and other applications.

关键词： Palladium Alloys Genetics Evolution reactions Transmission electron microscopy

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Membrane Fouling mechanism and Its Control in the Treatment of Brackish Water with Reverse Osmosis Process

Membrane Fouling mechanism and Its Control in the Treatment ...

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International Conference on Material Engineering, Chemistry and Environment (MECE 2013)

作者： Wang, Jianbing Cheng, Junyang Shi, Ting huang, Qing He, xuwen China Univ Min & Technol Sch Chem & Environm Engn Beijing 100083 Peoples R China

ISBN: (纸本)9783037858226

Brackish water was treated with reverse osmosis process. The fouling mechanism of RO and its control method was studied. In the treatment of brackish water, the salt removal efficiency was above 95% and the effluent quality was up to the standard for drinking water quality (GB5749-2006). The SDI of the influent of RO was less than 5 after the raw water was pretreated by the combination of coagulation and sedimentation process and filtration process, which met the demand of the water quality of the RO influent. If ultrafiltration was added, the water quality of the pre-treatment was better. Coagulation and precipitation was not very effective for the removal of dissolved organic compounds, especially for the removal of organic compounds with molecular amount ranging from 1000 to 10000. The formation of RO membrane fouling can be divided into five stages, which is membrane surface coarseness stage by inorganic substrate, organic compounds adsorption stage, organism adhesion stage, microbial film development stage, and irreversible membrane block stage. The membrane fouling was effectively alleviated by the strategy of first alkali solution cleaning and then acid solution cleaning.

关键词： Reverse Osmosis Brackish water from coal mines membrane fouling

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High power input coupler development for BEPCII 500 MHz superconducting cavity

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NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT 2010年第3期623卷 895-902页

作者： huang, Tongming Pan, Weimin Ma, Qiang Wang, Guangwei Dai, xuwen Zhang, Zhanjun Furuya, T. Mitsunobu, S. Chinese Acad Sci Inst High Energy Phys Beijing 100049 Peoples R China KEK Tsukuba Ibaraki 3050801 Japan

A high power input coupler for a 500 MHz superconducting cavity (SCC) of the upgrade project of Beijing Electron Positron Collider (BEPCII) has been developed in China. Several prototypes have been fabricated and tested successfully. A maximum of 420 kW continuous wave (CW) RF power in traveling wave (TW) mode was achieved in the high power test. The detailed design, fabrication and test of the coupler are described in this paper. (C) 2010 Elsevier B.V. All rights reserved.

关键词： High power input coupler Superconducting cavity High power conditioning

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2D-Material-Based Volatile and Nonvolatile Memristive Devices for Neuromorphic Computing

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ACS MATERIALS LETTERS 2023年第4期5卷 1109-1135页

作者： Xia, xuwen huang, Wen Hang, Pengjie Guo, Tao Yan, Yong Yang, Jianping Yang, Deren Yu, Xuegong Li, Xing'ao Nanjing Univ Posts & Telecommun NJUPT New Energy Technol Engn Lab Jiangsu Prov Nanjing 210023 Peoples R China Nanjing Univ Posts & Telecommun NJUPT Sch Sci Nanjing 210023 Peoples R China Zhejiang Univ State Key Lab Silicon Mat Hangzhou 310027 Zhejiang Peoples R China Zhejiang Univ Sch Mat Sci & Engn Hangzhou 310027 Zhejiang Peoples R China Univ Waterloo Waterloo Inst Nanotechnol Ctr Adv Mat Joining Dept Mech & Mechatron Engn Waterloo ON N2L 3G1 Canada Henan Normal Univ Sch Phys Henan Key Lab Photovolta Mat Xinxiang 453007 Peoples R China Zhejiang Univ Sci & Technol Sch Sci Hangzhou 310027 Peoples R China

Neuromorphic computing can process large amounts of information in parallel and provides a powerful tool to solve the von Neumann bottleneck. Constructing an artificial neural network (ANN) is a common means to realize neuromorphic computing, which has exhibited potential applications in pattern recognition, complex sensing, and other areas. Reservoir computing (RC), which is another approach to realize neuromorphic computing, has shown some progress and attracted researchers' attention. Neuromorphic computing can be generally implemented by fabricating memristive array systems. 2D-material-based memristive systems and their applications in ANN and RC have been investigated substantially in recent years due to the unique properties of these systems, such as atomic-level thickness and high carrier mobility. In this Review, we first discuss the volatility and nonvolatility properties of memristive devices and their applications in ANN and RC. Second, 2D materials that can be used to fabricate these devices are introduced, and their classification, physical properties, and preparation methods are presented. Third, we discuss the working mechanisms of 2D-material-based synaptic devices, the mimicked synaptic functions, and the applications of these devices in neuromorphic computing through ANN and RC. Lastly, the performance, progress, and future development directions of 2D-material-based synaptic devices are analyzed. This work systematically investigates the status of 2D-material-based synaptic devices and promotes their utilization in neuromorphic computing.

关键词： Electrical conductivity Layers Memristors Polarization Two dimensional materials

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Adsorption of Orange G on Activated Porous Carbon Derived from Coal Tar Pitch: Experimental and DFT Study

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LANGMUIR 2024年第48期40卷 25471-25482页

作者： huang, Linlin Zhang, xuwen Liu, Tingting Wang, Lin Li, Lixin Li, Da Sheng, Tao Dong, Zilong Zhao, Xinyue Heilongjiang Univ Sci & Technol Coll Environm & Chem Engn Harbin 150022 Peoples R China Harbin Inst Technol State Key Lab Urban Water Resource & Environm Harbin 150000 Peoples R China Northeast Agr Univ Sch Resources & Environm Harbin 150030 Peoples R China

A coal tar pitch-based porous carbon adsorbent (CPA) was synthesized through a straightforward method involving the heating of a mixture of KOH and coal tar pitch (CTP). This CPA exhibited a high surface area of 1811.2 m2 g-1 and a large pore volume of 0.94 cm3 g-1 when prepared with a CTP to KOH mass ratio of 1:4 at 800 degrees C. Parameters such as the heating temperature and activator dose were optimized to enhance the adsorption efficiency. The prepared CPA was extensively characterized by SEM, XRD, FTIR, and BET measurements. Notably, CPA presented a distinct adsorption performance for Orange G (OG), achieving a maximum adsorption capability of 449.7 mg g-1. Kinetic studies indicated that the adsorption process followed the pseudo-second-order model, while the adsorption isotherm data demonstrated that both chemical and physical interactions favored OG adsorption. Thermodynamic analysis revealed that the adsorption of OG on CPA was spontaneous and exothermic and increased the entropy. Density functional theory (DFT) calculations provided insights into the adsorption mechanism, highlighting electrostatic interactions, hydrogen bonds, and pi-pi interactions as the dominant processes governing OG adsorption onto the adsorbent.

关键词： Potassium hydroxide

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IVDETR: A Multi-Source Image Pig Detection Method Based on Cross-Domain Feature Fusion 7

IVDETR: A Multi-Source Image Pig Detection Method Based on C...

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7th International Conference on Pattern Recognition and Artificial Intelligence, PRAI 2024

作者： Song, Rui Li, Hao huang, Mengzhen huang, Zihan Li, Peng He, xuwen Wuhan Polytechnic University School of Mathematics and Computer Science Wuhan China

ISBN: (纸本)9798350350890

In large-scale centralised pig farming, object detection algorithms can accurately track and monitor each pig. However, a significant proportion of current detection methods are based on visible images, and the colour differences between different pig breeds limit the applicability of the models. Furthermore, complex background interference, low illumination conditions, or high illumination intensity noise in visible scenes can likewise lead to reduced accuracy during detection. Therefore, we propose a cross-domain encoder based on the self-attention and design the IVDETR model, which integrates features from infrared and visible light images for pig object detection. In order to facilitate the training and evaluation of the model, we constructed a comprehensive, standardised infrared-visible light dataset for the first time. The experimental outcomes demonstrated that the detection accuracy was increased from 0.939 to 0.998 in a real pig breeding environment. © 2024 IEEE.

关键词： Mammals

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