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effect of liquid product coverage on mass transfer and model development for gas-solid reaction in later reaction stage

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INTERNATIONAL JOURNAL OF HEAT AND MASS TRANSFER 2022年 184卷 122254-122254页

作者： Liu, Ming Shen, Zhongjie Xu, Jianliang Liang, Qinfeng Liu, Haifeng East China Univ Sci & Technol Natl Energy Adm Res Ctr Coal Gasificat Technol Shanghai 200237 Peoples R China East China Univ Sci & Technol Shanghai Engn Res Ctr Coal Gasificat Shanghai 200237 Peoples R China

The carbon conversion efficiency of coal is important performance index for gasifiers. Besides, the predic-tion of reaction rate of coal particle decides the operating residence time in gasifier. In this work, effect of molten slag covered on particle surface on mass transfer at high temperatures was investigated. In-situ gasification process of different char particles was analyzed and the molten slag enclosed residual carbon was found. The residual carbon inside fine slag and the core particle enclosed with slag from commercial entrained-flow gasifier were demonstrated. The carbon contents were up to 70% and 45% in gasification residual and fine slag. A critical point was found in the differential results of the reaction rate curve. The critical carbon conversion is about 0.93, 0.99 and 0.93 for three different coal chars. The reaction rates of different coal chars all showed linear decrease in the later reaction stage because of the diffusion re-sistance. Based on the reaction mode, the proposal of reaction model for carbon conversion prediction of high ash content coal chars in the later reaction stage was developed. The predicted carbon conversion of the proposed new model showed ideal agreement with the experimental data. This work introduced the formation of residual carbon in detail and supplies the new predictive reaction rate that considering ash fusion at high temperatures. (c) 2021 Elsevier Ltd. All rights reserved.

关键词： Gas-solid reaction product coverage effect Model development Reaction kinetics Coal gasification

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