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Design of Quantum Dot Color Convertors for Inkjet-Printed Optoelectronic Devices: Violet-Converted Full Color Mini-LED

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Advanced materials Technologies 2024年第3期9卷

作者： Lin, Chen-Te Zhuan, Yi-long Jung, Nian-Ting Hoang, Minh-Son Chen, Hsueh-Shih Ph.D. Program in Prospective Functional Materials Industry College of Engineering National Tsing Hua University Hsinchu30013 Taiwan Department of Materials Science and Engineering National Tsing Hua University Hsinchu30013 Taiwan College of Semiconductor Research National Tsing Hua University Hsinchu30013 Taiwan Department of Chemical Engineering & Materials Science College of Engineering Yuan Ze University Taoyuan32003 Taiwan

This study presents a strategy of design and development of inkjet-printable and UV-curable quantum dot (QD) polymer-based inks and color conversion (CC) film for use in optoelectronic devices. At first, the preparation of a QD ink is focused on two key aspects, that are QD chemical compatibility and ink printability. In the hybrid organic–inorganic polymer/QDs system, it must be formulated to a well-dispersed ink, in which a dispersant additive without negative effect on QDs is introduced to enhance the QD suspension. As the optical density of final dried QD film is one of the most critical concerns in color conversion, QD concentration should be as high as possible in the ink, which increases the ink viscosity. Consequently, a trade-off between QD concentration and the ink viscosity associated with the ink-jetting temperature is considered to ensure the ink printability. Finally, the designed QD ink is printed as color conversion film on a mini-LED panel composed of two violet mini-chips to produce red and green emissions, while blue emission directly comes from a blue mini-chip. The final conversion efficiency of QDCC on mini-LED panel are between 35% and 45%, showing the promising applications in optoelectronic devices. © 2023 Wiley-VCH GmbH.

关键词： Semiconductor quantum dots

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engineering H2O2 Self-Supplying Platform for Xdynamic Therapies via Ru-Cu Peroxide Nanocarrier: Tumor Microenvironment-Mediated Synergistic Therapy

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ACS Applied materials and Interfaces 2024年第19期16卷 24172-24190页

作者： Dirersa, Worku Batu Kan, Tzu-Chun Chang, Jungshan Getachew, Girum Ochirbat, Sonjid Kizhepat, Shamsa Wibrianto, Aswandi Rasal, Akash Chen, Hung-An Ghule, Anil Vithal Chou, Tzung-Han Chang, Jia-Yaw Department of Chemical Engineering National Taiwan University of Science and Technology Taipei106335 Taiwan Graduate Institute of Medical Sciences College of Medicine Taipei Medical University Taipei11031 Taiwan International Master/Ph.D. Program in Medicine College of Medicine Taipei Medical University Taipei11031 Taiwan International Ph.D. Program for Cell Therapy and Regeneration Medicine College of Medicine Taipei Medical University Taipei11031 Taiwan Green Nanotechnology Laboratory Department of Chemistry Shivaji University Kolhapur416004 India Department of Chemical and Materials Engineering National Yunlin University of Science and Technology Yunlin64002 Taiwan

Of the most common, hypoxia, overexpressed glutathione (GSH), and insufficient H2O2 concentration in the tumor microenvironment (TME) are the main barriers to the advancment of reactive oxygen species (ROS) mediated Xdynamic therapies (X = photo, chemodynamic, chemo). Maximizing Fenton catalytic efficiency is crucial in chemodynamic therapy (CDT), yet endogenous H2O2 levels are not sufficient to attain better anticancer efficacy. Specifically, there is a need to amplify Fenton reactivity within tumors, leveraging the unique attributes of the TME. Herein, for the first time, we design RuxCu1-xO2-Ce6/CPT (RCpCCPT) anticancer nanoagent for TME-mediated synergistic therapy based on heterogeneous Ru-Cu peroxide nanodots (RuxCu1-xO2 NDs) and chlorine e6 (Ce6), loaded with ROS-responsive thioketal (TK) linked-camptothecin (CPT). The Ru-Cu peroxide NDs (RCp NDs, x = 0.50) possess the highest oxygen vacancy (OV) density, which grants them the potential to form massive Lewis’s acid sites for peroxide adsorption, while the dispersibility and targetability of the NDs were improved via surface modification using hyaluronic acid (HA). In TME, RCpCCPT degrades, releasing H2O2, Ru2+/3+, and Cu+/2+ ions, which cooperatively facilitate hydroxyl radical (•OH) formation and deactivate antioxidant GSH enzymes through a cocatalytic loop, resulting in excellent tumor therapeutic efficacy. Furthermore, when combined with laser treatment, RCpCCPT produces singlet oxygen (1O2) for PDT, which induces cell apoptosis at tumor sites. Following ROS generation, the TK linkage is disrupted, releasing up to 92% of the CPT within 48 h. In vitro investigations showed that laser-treated RCpCCPT caused 81.5% cell death from PDT/CDT and chemotherapy (CT). RCpCCPT in cancer cells produces red-blue emission in images of cells taking them in, which allows for fluorescence image-guided Xdynamic treatment. The overall results show that RCp NDs and RCpCCPT are more biocompatible and have excellent Xdynamic the

关键词： Oxidation

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AI for organic and polymer synthesis

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science China Chemistry 2024年第8期67卷 2461-2496页

作者： Xin Hong Qi Yang Kuangbiao Liao Jianfeng Pei Mao Chen Fanyang Mo Hua Lu Wen-Bin Zhang Haisen Zhou Jiaxiao Chen Lebin Su Shuo-Qing Zhang Siyuan Liu Xu Huang Yi-Zhou Sun Yuxiang Wang Zexi Zhang Zhunzhun Yu Sanzhong Luo Xue-Feng Fu Shu-Li You Center of Chemistry for Frontier Technologies Department of ChemistryZhejiang UniversityHangzhou 310027China Center of Basic Molecular Science Department of ChemistryTsinghua UniversityBeijing 100084China Guangzhou National Laboratory Guangzhou 510005China Center for Quantitative Biology Academy for Advanced Interdisciplinary StudiesPeking UniversityBeijing 100871China State Key Laboratory of Molecular Engineering of Polymers Department of Macromolecular ScienceFudan UniversityShanghai 200433China School of Materials Science and Engineering Peking UniversityBeijing 100871China Beijing National Laboratory for Molecular Sciences Center for Soft Matter Science and EngineeringKey Laboratory of Polymer Chemistry and Physics of Ministry of EducationCollege of Chemistry and Molecular EngineeringPeking UniversityBeijing 100871China AI for Science(AI4S)-Preferred Program Shenzhen Graduate SchoolPeking UniversityShenzhen 518055China State Key Laboratory of Chemical Biology Shanghai Institute of Organic ChemistryUniversity of Chinese Academy of SciencesChinese Academy of SciencesShanghai 200032China Department of Chemical Sciences National Natural Science Foundation of ChinaBeijing 100085China State Key Laboratory of Organometallic Chemistry Shanghai Institute of Organic ChemistryChinese Academy of SciencesShanghai 200032China

Recent years have witnessed the transformative impact from the integration of artificial intelligence with organic and polymer synthesis. This synergy offers innovative and intelligent solutions to a range of classic problems in synthetic chemistry. These exciting advancements include the prediction of molecular property, multi-step retrosynthetic pathway planning, elucidation of the structure-performance relationship of single-step transformation, establishment of the quantitative linkage between polymer structures and their functions, design and optimization of polymerization process, prediction of the structure and sequence of biological macromolecules, as well as automated and intelligent synthesis platforms. Chemists can now explore synthetic chemistry with unprecedented precision and efficiency, creating novel reactions, catalysts, and polymer materials under the datadriven paradigm. Despite these thrilling developments, the field of artificial intelligence(AI) synthetic chemistry is still in its infancy, facing challenges and limitations in terms of data openness, model interpretability, as well as software and hardware support. This review aims to provide an overview of the current progress, key challenges, and future development suggestions in the interdisciplinary field between AI and synthetic chemistry. It is hoped that this overview will offer readers a comprehensive understanding of this emerging field, inspiring and promoting further scientific research and development.

关键词： organic synthesis polymer synthesis machine learning prediction chemical database automated synthesis

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Carrier dynamics in semi-insulating and low-temperature-grown gallium arsenide photoconductive antenna devices under above-bandgap and below-bandgap photoexcitation

Carrier dynamics in semi-insulating and low-temperature-grow...

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2022 JSAP-Optica Joint Symposia, JSAP 2022

作者： De Los Reyes, Alexander Publico, Jairrus Verona, Ivan Cedric Ferrolino, John Paul Juguilon, Vince Paul Rosa, Lourdes Nicole Dela Bardolaza, Hannah Cabello, Neil Irvin Estacio, Elmer National Institute of Physics University of the Philippines Diliman Quezon City1101 Philippines Materials Science and Engineering Program University of the Philippines Diliman Quezon City1101 Philippines

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Low-loss, nonvolatile tuning of Bragg structures with Sb2Se3

Low-loss, nonvolatile tuning of Bragg structures with Sb2Se3

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2024 Conference on Lasers and Electro-Optics, CLEO 2024

作者： Nobile, Nicholas A. Lian, Chuanyu Sun, Hongyi Huang, Yi-Siou Mills, Brian Popescu, Cosmin Constantin Callahan, Dennis Hu, Juejun Ríos Ocampo, Carlos A. Youngblood, Nathan Electrical & Computer Engineering Department University of Pittsburgh PittsburghPA15213 United States Department of Materials Science & Engineering University of Maryland College ParkMD20742 United States Institute for Research in Electronics and Applied Physics University of Maryland College ParkMD20742 United States Department of Materials Science & Engineering Massachusetts Institute of Technology CambridgeMA02139 United States Draper Scholar Program The Charles Stark Draper Laboratory Inc CambridgeMA02139 United States The Charles Stark Draper Laboratory Inc CambridgeMA02139 United States

Sb2Se3 is used to switch between broadband transparency and enhanced index contrast in two device types leveraging Bragg gratings for tunable stop- and pass-band functionalities. Experimental results highlight fabrica... 详细信息

ISBN: (纸本)9781957171395

关键词： Fabry-Perot interferometers

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Electro-Polymerization Process with Double-Sided Electrodes for Supercapacitors 5

Electro-Polymerization Process with Double-Sided Electrodes ...

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5th IEEE International Flexible Electronics Technology Conference, IFETC 2023

作者： Koripally, Nandu Yao, Lulu Eedugurala, Naresh Azoulay, Jason D. Ng, Tse Nga University of California San Diego Department of Electrical and Computer Engineering La Jolla CA United States University of California San Diego Materials Science Engineering Program La Jolla CA United States Georgia Institute of Technology Chemisty Department AtlantaGA United States

ISBN: (纸本)9798350332094

Supercapacitors are known for longer cycle life and faster charging rate compared to batteries. However, the energy density of supercapacitors requires improvement to expand their application space. To raise the energy density of redox supercapacitors, this work demonstrates electro-polymerization on both sides of electrodes to increase material loading, reduce overall device mass, and consequently increase the capacitance, power, and energy density of supercapacitors. We achieved an energy density of 1823 mWh kg-1 and a power density of 16.5 W kg-1 with a wide potential window of 3 V. © 2023 IEEE.

关键词： Supercapacitor

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Development of Flame Retardant Property on Sodium Silicate Treated Paper Based materials 21

Development of Flame Retardant Property on Sodium Silicate T...

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21st International Union of materials Research Societies International Conference in Asia, IUMRS-ICA 2021

作者： Suttipintu, Thitiporn Lhosupasirirat, Siraprapa Osotchan, Tanakorn Srikhirin, Toemsak Materials Science and Engineering Program School of Materials Science and Innovation Faculty of Science Mahidol University Bangkok10400 Thailand Research Network of NANOTEC Mahidol University National Nanotechnology Center Thailand Department of Physics Faculty of Science Mahidol University 272 Rama VI Road Ratchathewi District Bangkok10400 Thailand

The preparation of cellulose-based flame retardant paper treated with sodium silicate and silicon dioxide (SiO2) colloidal particle by simple immersion process is reported. Cellulose-based paper was preheated at 90°C for surface preparation. The heat treated paper was immersed in solution of sodium silicate-SiO2 at different immersion time ranging from 15 min to 24 hrs. Treated solution diffused into paper coated on the paper fiber and filled the void in the paper microstructure. Treated paper was heated at 90°C to convert an impregnated sodium silicate-SiO2 precursor into silicate framework. The treated paper showed Vsym Si-O-Si from siloxane bond at 792 cm-1 which confirmed a presence of SiO2 in paper. Treated paper at 1 hr immersion showed the highest weight percent gain (WPG) of 40% and total combustion time was improved to 14 sec. © Published under licence by IOP Publishing Ltd.

关键词： Silica

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Green Synthesis of Hierarchical Ag Nanostructures for Sers Detection of Rhodamine Dye

SSRN

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SSRN 2024年

作者： Sayson, Luce Vida A. Taaca, Kathrina Lois M. Madera, Rozen Grace B. Vasquez, Magdaleno R. Regulacio, Michelle D. Materials Science and Engineering Program College of Science University of the Philippines Diliman Quezon City1101 Philippines Department of Mining Metallurgical and Materials Engineering College of Engineering University of the Philippines Diliman Quezon City1101 Philippines Institute of Chemistry College of Science University of the Philippines Diliman Quezon City1101 Philippines

This study presents a simple benchtop synthetic protocol for the fabrication of silver (Ag) nanostructures in aqueous media using environmentally friendly and inexpensive reagents under mild experimental conditions. Natural organic acids that are known to be present in plants were employed as reducing and morphology-directing reagents. SEM and TEM imaging revealed that the resultant nanostructures are three-dimensional hierarchical structures that were formed from self-assembly of smaller nanoparticles. They are generally spherical in shape and possess highly roughened surfaces due to the interstitial gaps between their nanoparticle subunits. Their hierarchical architecture allows for strong absorption of light in a broad range of wavelengths that extends to the near-infrared region. In addition, their surface morphology has an abundance of hot spot regions, which are capable of inducing strong SERS enhancement effects. The green-synthesized Ag nanostructures showed remarkable SERS activity when used as substrates for the detection of rhodamine 6G dye, a highly toxic water contaminant. Overall, this study does not only provide a greener approach to hierarchical Ag nanostructures, but also demonstrates theimmense potential of these nanostructures in the sensitive detection of organic dyepollutants. © 2024, The Authors. All rights reserved.

关键词： Substrates

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A mini review on two-dimensional nanomaterial assembly

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Nano Research 2020年第5期13卷 1179-1190页

作者： Zhiwei Fang Qiyu Xing Desiree Fernandez Xiao Zhang Guihua Yu Materials Science and Engineering Program and Department of Mechanical Engineering The University of Texas at AustinAustinTexas 78712USA 2 School of Chemistry and Materials ScienceUniversity of Science&Technology of ChinaHefei 230026China

Two-dimensional(2D)nanomaterials have attracted a great deal of attention since the discovery of graphene in 2004,due to their intriguing physicochemical properties and wide-ranging applications in catalysis,energy-related devices,electronics and *** maximize the potential of 2D nanomaterials for their technological applications,controlled assembly of 2D nanobulding blocks into integrated systems is critically *** mini review summarizes the reported strategies of 2D materials-based assembly into integrated functional nanostructures,from in-situ assembly method to post-synthesis *** applications of 2D assembled integrated structures are also covered,especially in the areas of energy,electronics and sensing,and we conclude with discussion on the remaining challenges and potential directions in this emerging field.

关键词： two-dimensional materials assembly self-assembly post-synthesis assembly integrated nanostructures

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Stretchable and self-healable spoof plasmonic meta-waveguide for wearable wireless communication system

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Light(science & Applications) 2022年第11期11卷 2725-2737页

作者： Bu-Yun Yu De-Wei Yue Ke-Xin Hou Lu JU Hao Chen Cong Ding Zhen-Guo Liu Yun-Qian Dai Hari Krishna Bisoyi Ying-Shi Guan Wei-Bing Lu Cheng-Hui Li Quan Li State Key Laboratory of Millimeter Waves School of Information Science and EngineeringSoutheast UniversityNanjing 210096China Center for Flexible RF Technology Frontiers Science Center for Mobile Information Communication and SecuritySoutheast UniversityNanjing 210096China Purple Mountain Laboratories Nanjing 21111China State Key Laboratory of Coordination Chemistry School of Chemistry and Chemical EngineeringNanjing UniversityNanjing 210023China Institute of Advanced Materials and School of Chemistry and Chemical Engineering Southeast UniversityNanjing 211189China Advanced Materials and Liquid Crystal Institute and Chemical Physics Interdisciplinary Program Kent State UniversityKentOH 44242USA

Microwave transmission lines in wearable systems are easily damaged after frequent mechanical deformation,posing a severe threat to wireless ***,we report a new strategy to achieve stretchable microwave transmission lines with superior reliability and durability by integrating a self-healable elastomer with serpentine-geometry plasmonic meta-waveguide to support the spoof surface plasmon polariton(SSPP).After mechanical damage,the self-healable elastomer can autonomously repair itself to maintain the electromagnetic performance and mechanical ***,the specially designed SSPP structure exhibits excellent stability and damage *** if the self-healing process has not been completed or the eventual repair effect is not ideal,the spoof plasmonic meta-waveguide Can still maintain reliable ***-healing material enhances strength and durability,while the SSPP improves stability and gives more tolerance to the self-healing *** design coordinates the structural design with material synthesis to maximize the advantages of the SSPP and self-healing material,signifcantly improving the relability and durability of stretchable microwave transmission *** also perform communication quality experiments to demonstrate the potential of the proposed meta-waveguide as interconnects in future body area network systems.

关键词： process durability maintain

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