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Manipulating metal-oxygen local atomic structures in singlejunctional p-Si/WO_(3) photocathodes for efficient solar hydrogen generation

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Nano Research 2021年第7期14卷 2285-2293页

作者： Wu Zhou Chung-Li Dong Yiqing Wang Yu-Cheng Huang Lingyun He Han-Wei Chang Shaohua Shen International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power EngineeringXi’an Jiaotong UniversityShaanxi 710049China Department of Physics Tamkang UniversityTamsui 25137TaiwanChina

Self-passivation in aqueous solution and sluggish surface reaction kinetics significantly limit the photoelectrochemical(PEC)performances of silicon-based ***,a WO_(3) thin layer is deposited on the p-Si substrate by pulsed laser deposition(PLD),acting as a photocathode for PEC hydrogen *** to bare p-Si,the single-junctional p-Si/WO_(3) photoelectrodes exhibit excellent and stable PEC performances with significantly increased cathodic photocurrent density and exceptional anodic shift in onset potential for water *** is revealed that the WO_(3) layer could reduce the charge transfer resistance across the electrode/electrolyte interface by eliminating the effect of Fermi level pinning on the surface of *** importantly,by varying the oxygen pressures during PLD,the collaborative modulation of W–O bond covalency and WO6 octahedral structure symmetry contributes to the promoted charge carrier transport and ***,a large band bending at the p-Si/WO_(3) junction,induced by the optimized O vacancy contents in WO_(3),could provide a photovoltage as high as~500 mV to efficiently drive charge transfer to overcome the water reduction ***,by manipulating W–O local atomic structures in the deposited WO_(3) layer,a great improvement in PEC performance could be achieved over the singlejunctional p-Si/WO_(3) photocathodes for solar hydrogen generation.

关键词： silicon local atomic structure water splitting photocathodes hydrogen generation

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A calculation method for evaluating thermal loss of solar cavity receiver

A calculation method for evaluating thermal loss of solar ca...

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2009 Asia-Pacific power and Energy {1. Conference, APPEEC 2009

作者： Jiabin, Fang Jinjia, Wei Xunwei, Dong Yueshe, Wang State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an China

ISBN: (纸本)9781424424870

One of the most important components of solar thermal power system is the solar central receiver, which performance is in direct relation to the efficiency of the whole power generation system. The calculation of internal surface heat flux and thermal efficiency of receiver therefore plays a very important role in receiver design. A calculation method of heat loass of a cavity receiver is put forward in this paper. The first step of this method is to use the Monte Carlo method to simulate the track of solar beam and compute surface heat flux inside the receiver. The second step is to employ the correlations of flow boiling heat transfer to figure out the convective heat transfer coefficient inside the tubes and then the wall temperature of the boiling tubes laid inside the receiver. The last step is to simulate the air flow field inside the receiver to calculate convective thermal loss of the receiver. As every step can not be independently done, all steps are coupled and an iterative scheme is needed. Internal surface heat flux and thermal efficiency of the receiver can be finally gained with this method, and the result can provide theoretical guide for receiver design. © 2009 IEEE.

关键词： Monte Carlo methods

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Experimental and modeling study of low temperature ignition characteristics of methylcyclohexane/ethanol binary fuel 12

Experimental and modeling study of low temperature ignition ...

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1.th Asia-Pacific Conference on Combustion, ASPACC 201.

作者： Liu, Yang Tang, Chenglong Huang, Zuohua State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an China

The purpose of this work is to investigate the effect of ethanol blending into methylcyclohexane during the ignition at low temperatures. The ignition delay times of the binary fuels with ethanol blending ratio varied from 0% to 1.0% at = 1.0, Pc = 20 bar, Tc = 680 - 890 K were measured with the rapid compression machine, and the mechanism of Bissoonauth et al. (Proc Combust Inst 201.) well predicts the experimental results. Based on the high quality of the model, the effects of ethanol blending on the pressure and heat release are studied. Both of the maximum pressure and the heat release during the ignition decrease with the ethanol blending ratio increases. The interaction of MCH and ethanol happens in the competition of active radicals like OH, and MCH dominates the ignition process as it occupies about two thirds of the OH to form the fuel radical. © Asia-Pacific Conference on Combustion, ASPACC *** right reserved.

关键词： Ethanol

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A Novel One-step Hydrothermal Method for the Preparation of Cd1.xZnxS/Titanate Nanotubes Composites for Photocatalytic Hydrogen Production 18

A Novel One-step Hydrothermal Method for the Preparation of ...

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1.th World Hydrogen Energy Conference, WHEC 201.

作者： Chen, Yubin Guo, Liejin State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi'an Jiaotong University China

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Base-or acid-assisted polystyrene plastic degradation in supercritical CO_(2)

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Waste Disposal and Sustainable Energy 2023年第2期5卷 165-175页

作者： Yanbing Liu Jinwen Shi Liuhao Mao Bingru Lu Xing Kang Hui Jin International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power EngineeringXi’an Jiaotong University28 West Xianning RoadXi’an710049ShaanxiChina

Plastic has caused serious"white pollution"to the environment,and the highly inert characteristics of plastic bring a major challenge for *** fluids have unique physical properties and have been widely used in various *** this work,supercritical CO_(2)(Sc-CO_(2))with mild conditions was selected and assisted by NaOH/HCl solution to degrade polystyrene(PS)plastic,and the reaction model was designed using response surface methodology(RSM).It was found that,regardless of the types of assistance solutions,the factors affecting PS degradation efficiencies were reaction temperature,reaction time,and NaOH/HCl *** the temperature of 400℃,time of 1.0 min,and base/acid concentration of 5%(in weight),0.1. g PS produced 1.6.88/1.6.99±5 mL of gases with 74.1./62.78±5 mL of H2,and consumed 81.2/71.5±5 mL of CO_(2).Sc-CO_(2)created a homogeneous environment,which made PS highly dispersed and uniformly heated,thus promoting the degradation of ***,Sc-CO_(2)also reacted with the degradation products to produce new CO and more CH_(4)and C_(2)H_(x)(x=4,6).Adding NaOH/HCl solution not only improved the solubility of PS in Sc-CO_(2),but also provided a base/acid environment that reduced the activation energy of the reaction,and effectively improved the degradation efficiencies of *** short,degrading PS in Sc-CO_(2)is feasible,and better results are obtained with the assistance of base/acid solution,which can provide a reference for the disposal of waste plastics in the future.

关键词： Plastic degradation Polystyrene Supercritical CO_(2) NaOH HCl

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Fabricating PdCe/OMS-2 catalysts with boosted low-temperature activity for toluene deep degradation

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Journal of Rare Earths 2023年第6期41卷 839-849,I0002页

作者： Lin Yue Zhihua Xu Minghua Hu Mingjiao Tian Mudi Ma Bijie Huang Chi He State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power EngineeringXi'an Jiaotong UniversityXi'an 710049China State Key Laboratory of Precision Blasting and Hubei Key Laboratory of Industrial Fume and Dust Pollution Control Jianghan UniversityWuhan 430056China National Engineering Laboratory for VOCs Pollution Control Material&Technology University of Chinese Academy of SciencesBeijing 101408China

Porous cryptomelane-type octahedral molecular sieve(OMS-2)with mixed Mn valence and abundant lattice oxygen species has attracted much attention in volatile organic compounds(VOC)catalytic ***,complete conversion of arene over OMS-2 catalysts at relatively low temperature is still a challenge due to its limited crystal structure and inferior ***,a series of PdCe/OMS-2 catalysts with different Pd/Ce molar ratios was fabricated by a facile impregnation method and the physicochemical properties of which were extensively characterized by X-ray diffraction(XRD),scanning electron microscopy(SEM),high-resolution transmission electron microscopy(HR-TEM),B runauer-Emmett-Teller(BET)method,X-ray fluorescence(XRF),X-ray photoelectron spectroscopy(XPS),temperature programmed reduction of H2(H2-TPR),Raman,In situ diffused reflectance infrared Fourier transform spectra(DRIFTS),and density functional theory(DFT)*** show that the total conversion of toluene can be achieved at 207℃ over PdCe2 with apparent activation energy as low as 62.6 kJ/*** strong synergistic effect between Pd and Ce remarkably boosts the catalytic activity of OMS-2,attributed to the abundant Mn^(3+)-O bands and active surface oxygen *** results reveal that oxygen vacancy can be formed over PdCe2 much easily than that of Pd/OMS-2 and Ce/OMS-2 with the oxygen vacancy formation energy of2.42,2.83 and 2.68 eV,*** increasing the Pd content cannot promote the catalytic activity although PdO is a critical active center in toluene *** vacancy attributed to the integrative effect of Pd,Ce and Mn species plays a promine nt role over prepared catalysts in toluene activation *** findings reported in this work showed new insights into the designing of highly efficient OMS-2catalysts for VOC deep oxidation by tuning oxygen vacancy concentration.

关键词： PdCe/OMS-2 Toluene Catalytic oxidation Oxygen vacancy Rare earths

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Experimental study on a linear concentrating solar photovoltaic/thermal system

Experimental study on a linear concentrating solar photovolt...

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26th International Conference on Efficiency, Cost, Optimization, Simulation and Environmental Impact of Energy Systems, ECOS 201.

作者： Ma, Qiuming Cao, Fei Zhao, Liang State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an China

A set of solar photovoltaic and thermal combined (PV/T) system is installed and tested in the present study. The PV/T system is designed and constructed by integrating coiled-channel flat-plate collectors with polycrystalline silicon PV modules. The linear Fresnel lens acts as the concentrator. Three systems, i.e. the non-cooling PV system, the non-concentrating PV/T system and the concentrating PV/T system, are tested and analyzed. Experimental results show that a high thermal and electrical combined efficiency, over 65%, is achieved by the PV/T system. Water in the flat plate can significantly decrease the PV module temperature and improve the electricity-conversion efficiency. Comparing with the non-concentrating PV/T system, the concentrating PV/T system can increase the total utilization of solar energy.

关键词： Solar energy

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Dynamic simulation of coal-fired power plant integrated with trough solar collector operating in parallel with high pressure heaters

Dynamic simulation of coal-fired power plant integrated with...

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201. Canadian Society for Civil engineering Annual Conference, CSCE 201.

作者： Yan, Hui Li, Xin Liu, Ming Chong, Daotong Yan, Junjie State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an China

ISBN: (纸本)9780791883747

Solar-aided coal-fired power plant (SACFPP) is a costeffective approach to overcome solar energy intermittency. SACFPPs frequently operate in dynamic processes due to power load and solar energy fluctuations. This study investigated the dynamic characteristics of SACFPPs;such characteristics are important for flexibility evaluation and control system design. The SACFPP used in this study was based on a 660 MW coalfired power plant, and a trough collector system (TCS) operates in parallel with high pressure (HP) heaters. After model development and validation, the dynamic performance of the SACFPP was analyzed under four load ratios of power plant, with disturbances of two parameters: direct normal irradiance (DNI) and mass flowrate ratio to TCS. The performance was also compared with three parallel TCS connection modes. Results showed that the magnitude and response time for power variation under DNI disturbance increased with load ratio. With 500 W/m2 DNI step increments, power increased by approximately 1..4, 21.2, 24.7, and 29.8 MW in 2200, 2330, 2550 and 2620 s at 70%, 80%, 90%, and 1.0% load ratios, respectively, when all the HP heaters were replaced. The serial number and the number of HP heaters replaced also increased the power variation and response time. Under mass flowrate ratio to TCS increase disturbance, the power rapidly changed to its maximum and then slowly decreased, but the variation value depended on the load ratio. Copyright © 2020 ASME.

关键词： Coal fired power plant

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Au@SiO_2 core/shell nanoparticle-decorated TiO_2 nanorod arrays for enhanced photoelectrochemical water splitting

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Chinese Science Bulletin 2014年第18期59卷 2191-2198页

作者： Jianan Chen Miao Yu Yuhao Wang Shaohua Shen Meng Wang Liejin Guo International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power EngineeringXi’an Jiaotong University School of Chemical Engineering and Technology Harbin Institute of Technology

To improve the separation efficiency of photoinduced charge carries,Au@SiO2nanoparticles(NPs)with core–shell structure were loaded onto the surface of TiO2nanorods grown on fluorine-doped tin oxide substrate by a facile two-step *** resulted Au@SiO2/TiO2photoanodes were characterized by X-ray diffraction,scanning electron microscopy,transmission electron microscopy,as well as photoelectrochemical *** with pristine TiO2nanorod film,the Au@SiO2/TiO2films showed remarkable enhancement in photoelectrochemical water splitting,with incident photonto-current conversion efficiency increasing from 31.to37%at 380 nm at 0.7 V versus saturated calomel *** could be interpreted by the effect of metallic surface plasmon resonance of Au@SiO2NPs,which would generate an intense electromagnetic field with spatially nonhomogenous distributed *** a result,the charge carriers generated in the near-surface region of TiO2nanorods could be easily *** modification method based on the effect of metallic surface plasmon resonance for promoted charge carrier separation provides a promising way to develop semiconductor photoelectrodes with high solar water-splitting performance.

关键词：二氧化硅纳米粒子二氧化钛纳米棒电解水表面等离子体共振效应纳米颗粒金属 TiO2薄膜

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Research on the effects of diluents and dilution ratios on laminar burning velocities and flame instabilities of hydrogen flame 11

Research on the effects of diluents and dilution ratios on l...

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1.th Asia-Pacific Conference on Combustion, ASPACC 201.

作者： Lu, Xin Hu, Erjiang Li, Xiaotian Huang, Zuohua State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an China

Laminar burning velocities and flame instabilities of H2/O2/diluents mixture were studied at initial pressure of 0.3 MPa, initial temperature of 373 K and equivalence ratio of 1.0. The He diluted mixtures have the largest laminar burning velocities and the N2 diluted mixtures have the smallest, while He diluted mixtures have the largest mole fraction of H and OH radical and N2 diluted mixtures have the smallest. And laminar burning velocities fall when the dilution ratio rises, due to the mole fractions of H and OH radical fall with increasing dilution ratio. The cellular structure appeared on both N2 and Ar diluted mixture, while only wrinkles grew on He diluted mixtures. When dilution ratio rose, the appearance of cellular structure deferred. Thus, He diluted mixtures are more stable than N2 and Ar diluted mixtures, and higher dilution ratios restrain the flame instabilities. © 201. Combustion Institute. All rights reserved.

关键词： Hydrogen

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