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SSRN 2024年

作者： Zhu, Lei Zhang, Jiaxin Wang, Jianan Liu, Jianwei Wang, Ze Yan, Wei Xi’an Key Laboratory of Solid Waste Resource Regeneration and Recycling State Key Laboratory of Multiphase Flow Engineering School of Energy and Power Engineering Xi’an Jiaotong University Xi’an710049 China School of Physics and Electrical Engineering Weinan Normal University Chaoyang Street Weinan714099 China School of Chemistry and Chemical Engineering Xi’an University of Science & Technology Xi’an710054 China

The construction of transition metal dichalcogenides (TMDs) heterojunctions for high performance gas sensors has garnered significant attention due to their capacity to operate at low temperature. Herein, we realize two-dimensional (2D) WS2 nanosheets in situ grown on one-dimensional (1.) In2O3 nanofibers to form heterostructures for formaldehyde (HCHO) gas sensors. Capitalizing on the p-n heterojunctions formed between WS2 and In2O3, coupled with the high surface-to-volume ratio characteristic of 1. nanostructures, the WS2/In2O3 NFs sensor demonstrated a high gas response value of 1..6 toward 1.0 ppm HCHO at operating temperature of 1.0 ℃, two times greater than that of the pristine In2O3 sensor. Meanwhile, the sensor presents remarkable repeatability, rapid response/ recovery time, and good long-term stability. The superior sensing capabilities of WS2/In2O3 NFs heterojunction are attributed to the combined impact of the increased charge transfer and the presence of more sites for gas adsorption. The research endows a potent approach for fabricating TMDs heterojunctions to significantly improve the performance of gas sensors. © 2024, The Authors. All rights reserved.

关键词： Tungsten compounds

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Gold/oxide heterostructured nanoparticles for enhanced SERS sensitivity and reproducibility

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Rare Metals 2020年第7期39卷 834-840页

作者： Qi-Kui Fan Ting-Zhuo Liu Hou-Shen Li Shu-Meng Zhang Kai Liu Chuan-Bo Gao Frontier Institute of Science and Technology and State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong UniversityXi’an 710054China College of Chemistry and Material Science Shandong Agricultural UniversityTaian 271018China

In surface-enhanced Raman scattering(SERS),it is highly desirable to obtain Raman signals with high sensitivity and reproducibility from noble metal nanoparticle substrates,which remains a great challenge due to the inhomogeneity of the plasmonic coupling that is sensitive to the interparticle *** this work,we report that the interparticle plasmonic coupling could be circumvented by first synthesizing Au/metal or nonmetal oxide heterostructured nanoparticles and then depositing them uniformly onto the substrates,leading to high reproducibility of the Raman *** plasmonic coupling has been found at the Au/oxide interface,which enables high sensitivity of the SERS analysis that accompanies the excellent signal *** different oxides investigated(SiO2,TiO2 and Fe2O3),the Au/Fe2O3 heterostructured nanoparticles demonstrate the highest Raman enhancement *** believe our strategy opens a promising route to fabricate SERS substrates that are capable of sensitively and quantitatively detecting molecules of interest in a much reliable manner.

关键词： Gold nanoparticles Au/oxide heterostructures Hot spots Surface-enhanced Raman scattering Reproducibility

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Interfacial Mass Transfer Enhancement for Photoelectrochemical Water Splitting Using 3d flow Field Structure

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SSRN 2022年

作者： Wang, Baoyuan Yang, Suyi Lai, Yongquan Su, Jinzhan International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Shaanxi Xi’an710049 China

Hydrogen production using solar energy water splitting is an economical and feasible clean energy solution. It is recognized that the efficiency of photoelectrochemical water splitting is not only related to the electrode material, but also influenced by the mass transport at the electrode surface. To investigate that relationship, we design a novel photoelectrochemical water splitting reactor, which generates a turbulent flow at the electrode/electrolyte interface, and change the temperature of the electrolyte. It was found that the flow rate and temperature of the electrolyte mainly affect the mass transport and charge transfer at the photoelectrode/electrolyte interface. Based on the results of LSV, EIS, and the calculation of mass transfer coefficient, the photoelectrochemical performance of the system at flow rate ranging from 0 to 1.5 ml/min and temperature between 20-90 °C is analyzed. The influence of the flow rate on the photocurrent density is more significant during the transition of the flow state and at the high flow rate. The best performance is achieved at the flow rate of 1.7 ml/min, and the temperature of 90 °C. The electrochemical impedance spectroscopy results show that in the test range, ion transport impedance decreases with increasing electrolyte temperature, as a result, the photocurrent density at 90 °C is increased about 2.2 times compared to that at 20 °C. It is also shown that the design of the 3D step-like structure has a more significant effect on the electrolyte flow than the planar structure, and the photocurrent density is increased about 1.3 times. © 2022, The Authors. All rights reserved.

关键词： Mass transfer

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Unveiling micro- and nanoscale bubble dynamics for enhanced electrochemical water splitting

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Advances in Colloid and Interface Science 2025年 343卷 103544页

作者： Lu, Xinlong Yadav, Devendra He, Baichuan Zhou, Yu Zhou, Liwu Zeng, Zilong Ma, Lijing Jing, Dengwei International Research Center for Renewable Energy & State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Shaanxi Xi'an710049 China Department of Chemical Engineering Technion - Israel Institute of Technology Haifa3200003 Israel College of Mechanical Engineering Xi'an Shiyou University Shaanxi Xi'an710065 China

Bubbles generated during electrochemical and photoelectrochemical water splitting critically influence efficiency through complex factors, including chemical reactions, species transport, mass transfer at the three-phase interface, and bubble coverage. A detailed understanding of the nucleation, growth, coalescence, and detachment of micro- and nanoscale bubbles is vital for advancing water splitting technologies. Surface-attached bubbles significantly reduce the electrocatalytically active area of electrodes, leading to increased surface overpotential at a given current density. Consequently, their effective removal is pivotal for optimizing the electrolysis process. However, the intricate interplay among single bubble evolution, mass transport, bubble coverage, and overpotential remain inadequately understood. This review explores the fundamental mechanisms underpinning bubble evolution, with an emphasis on the Marangoni effect and its influence on bubble dynamics. Furthermore, recent advancements in understanding individual bubbles on micro and nano-electrodes are highlighted, offering valuable insights into scale-dependent bubble behavior. These findings enrich our knowledge of gas-liquid interfacial phenomena and underscore their industrial significance, presenting opportunities to enhance water splitting performance through optimized bubble dynamics. © 2025

关键词： Electrolysis

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General analytical equation of state for nanoconfined gases derived from statistical physics

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Physical Review E 2025年第2期111卷 025413-025413页

作者： Chengzhen Sun Haoxuan Li Zhixiang Zhao Mehdi Neek-Amal Bofeng Bai State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an Shaanxi 710049 China School of Urban Planning and Municipal Engineering Xi'an Polytechnic University Xi'an Shaanxi 710048 China Department of Physics Faculty of Sciences Shahid Rajaee Teacher Training University 16875-163 Lavizan Tehran Islamic Republic of Iran Department of Physics University of Antwerp Groenenborgerlaan 171 2020 Antwerp Belgium

The pressure prediction of nanoconfined gases is crucial for various industrial applications, yet existing equations of state (EOS) often compromise between accuracy and usability. This study derives a theoretical EOS in analytical form, combining precision and practicality through statistical physics. It begins by examining the pressure drop mechanism due to adsorbed molecules and refines molecular pairing and potential energy interactions. The resulting EOS accurately predicts the pressure of gases in nanoconfined spaces, especially with an average prediction error of about 5% for strongly adsorbing gases like nitrogen, oxygen, and argon. Additionally, it aligns with the Van der Waals EOS under macroscopic conditions, offering a unified framework across scales. This model enhances both {1. applications and the understanding of nanoconfined EOS.

关键词： Van der Waals forces

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Occurrence and flow Characteristics of Methane in High-Temperature and High-Pressure Nanopores of Deep Shale

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Kung Cheng Je Wu Li Hsueh Pao/Journal of engineering Thermophysics 2025年第4期46卷 1200-1204页

作者： Wang, Rui Sun, Chengzhen Yang, Xu State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an710049 China Petroleum Engineering School Southwest Petroleum University Chengdu610500 China

The understanding of gas transport in deep shale nanopores is still not clear. In this study, molecular simulations of methane occurrence and flow in illite slits of deep shales under the condition of high-temperature and high-pressure was carried out. The occurrence, diffusion and flow characteristics of methane molecules were analyzed. The effects of temperature and pressure on methane occurrence and flow were elucidated. The results show that the distribution of methane density in illite slits is nonuniform, and there are density peaks near the wall. Compared with Middle and Shallow shales, more methane molecules can exist in the pores of deep shale, and the diffusion ability is limited. The methane flow flux decreases with the decrease of pressure (5∼80 MPa) and increases with the decrease of temperature (60∼1.0◦C). Pressure is the main dominating factor of flow flux, and the flow flux decreases gradually during depressurization. © 2025 Science Press. All rights reserved.

关键词： Nanopores

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Evaluation of droplet drag force model on spray and atomization behaviours of R1.4a flashing spray 14

Evaluation of droplet drag force model on spray and atomizat...

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1.th International Conference on Liquid Atomization and Spray Systems, ICLASS 201.

作者： Zhou, Zhi-Fu Lu, Guan-Yu Zhang, Lu Chen, Bin State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an710049 China

Flashing spray is of great importance in a variety of engineering fields, which occurs as the pressurized liquid is released into a low-pressure environment below its saturation pressure. This paper conducts a systematically numerical study on the spray and thermal characteristics of R1.4a flashing spray with high volatility and low saturation temperature, using a modified sprayFoam solver in the open source tool OpenFOAM-2.4.0. {1. physics involved in the complex process, including droplet flash boiling, evaporation, droplet transport, breakup, heat transfer and interaction between droplet and gas phases are taken into consideration. The emphasis is put on the droplet drag force model and nozzle diameter on flashing spray including spray morphology, droplet diameter, velocity and temperature. The result indicates that most of the drag force models have little effect on droplet diameter, velocity and temperature distributions in flashing spray, except the Khan-Richardson (K-R) model. The K-R model predicts lower temperature, higher velocity and larger size of droplet, compared to other models. The nozzle diameter greatly affects R1.4a spray morphology and tip penetration, that smaller diameter contributes to a larger radial expansion at the near nozzle region while leading to a much smaller penetration distance. This research give a useful guidance that how people choose the appropriate drag force model for simulation of flashing spray. © 201. Solar Turbines Incorporated.

关键词： Morphology

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Experimental investigation on flash evaporation related to pipe leakage

Experimental investigation on flash evaporation related to p...

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作者： Cai, Benan Zhang, Qi Weng, Yu Gu, Hongfang Wang, Haijun State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an710049 China

Pipelines such as the surge line and main pipe are easily subjected to thermal stratification and thermal fatigue as a result of the nonuniform temperature distribution in the nuclear power plants. When the surge line or main pipe subjected to thermal stratification and thermal fatigue keeps operating for long time, the pipe leakage may happen due to the existence of pipeline crack. When the fluids with high temperature and pressure leak in the crack, the water will evaporate quickly, which means this process belongs to spray flash evaporation process. The flash evaporation related to pipe leak was experimentally studied in the paper. The experiment was carried out under high temperature and high pressure with low spray rate. The temperature and relative humidity (T&H) variations over time were monitored in the experiment with installing T&H detectors. The T&H variations at different measurement positions and with different spray rates were analyzed, respectively. In addition, the effect of the dimensionless parameters including the Weber number and Jakob number was also investigated. Results indicated that the response speed increased with the increase of the spray {1. rate. Higher Weber number and higher Jakob number led to higher evaporation rate. The slight pipe leakage can be predicted by using the (T&H) in the hazardous areas. Copyright © 2020 by ASME

关键词： Nuclear fuels

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flow and Thermal Analysis of the Transition Scheme between Micro-Channel and Micro-Jet Cooling Solution

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SSRN 2022年

作者： Guo, Yuming Fan, Liang-Liang Zhao, Liang State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'An710049 China School of Mechanical Engineering Xi'an Jiaotong University Xi'An China

With the rapid development of high-power electronics, the thermal management of these emerging devices is challenging&#1.0;due to the danger of ultra high heat flux and uneven temperature distribution. In this perspec... 详细信息

With the rapid development of high-power electronics, the thermal management of these emerging devices is challenging due to the danger of ultra high heat flux and uneven temperature distribution. In this perspective, as promising cooling technologies, micro-channel and micro-jet cooling designs have been extensively investigated. In the past decade, certain heat-dissipation technologies based on micro-channel and micro-jet cooling have utilized geometrically identical heat sinks;however, their corresponding {1. and thermal characteristics are dissimilar including micro-channel cooling technologies often have large temperature gradients as well as high heat transfer coefficients, while microjet technologies are more advantageous in terms of temperature distribution uniformity but larger pressure drop penalty. To characterize the enhanced heat-transfer mechanism driving this dissimilitude, a transition scheme between micro-channel and micro-jet was designed, featuring a gap on the channel fins top to provide extra {1. area, and investigated experimentally and numerically. By controlling the volumetric {1. ratio of the channel and jet, the {1. and thermal characteristics of the transition scheme could be interchangeably transformed between the micro-channel and micro-jet. Moreover, we investigated the effect of the vortex generated by the jet impingement on channel bottom and fins top, an important factor causing the distinctions between the two schemes. The results revealed that the vortex in the stagnation zone enhanced the local heat-transfer coefficient corresponding to the channel bottom and promoted temperature uniformity;however, it caused the thermal boundary layer on the fins top to thicken. Although the vortex was favorable for the forced convection in the acceleration zone, the vortex intersections formed by adjacent jets introduced a greater pressure-drop penalty and {1. blockage, which were not conducive to enhancing the heat transfer. Subsequently,

关键词： Vortex flow

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Dynamic modeling of an air-cooling supercritical power plant under temp oral variant ambient conditions 7

Dynamic modeling of an air-cooling supercritical power plant...

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7th International Conference on power {1., ICOPE 201.

作者： Yan, Wenchen Han, Xiaoqu Chen, Nana Wu, Wenxiang Zhou, Yan State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an710049 China

Air-cooling systems are widely used in coal-fired power plants, especially in areas rich in coal resources and short of water. To prompt its economic and safe operation, dynamic modeling is urgently required to acquire the power plant's characteristics under complex working conditions. In particular, the condensing pressure of the air-cooling unit is significantly affected by the ambient temperature, and the thermal power plant is a complicated energy system with serious nonlinearity. In many cases, it is difficult to establish the mathematical model of the system by traditional analytical methods. In the present work, a 1.00 MW supercritical power plant thermal system was modeled and simulated by GSE simulation software. The model was developed according to the structural characteristics, incorporating boiler system, steam turbine system and direct air-cooling system. The simulation results were compared with the actual operation data of the power plant to validate the model. The relative errors of the simulation models under steady-state conditions were less than 3%, which indicates that the models have high accuracy. On this basis, the influence of condensing pressure on the standard coal consumption rate was obtained. It was shown that when the condensing pressure ranged between 5 kPa and 20 kPa, the coal rate increased by 1.6 g/kW∙h with 1.kPa increase in the condensing pressure. Then the boundary conditions of the system were changed. When the parameters changed, the changes of condensing pressure and power were monitored, so as to study the dynamic characteristics of the system. © ICOPE 201. - 7th International Conference on power engineering, Proceedings. All rights reserved.

关键词： Coal

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