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Nanomaterials for renewable hydrogen production,storage and utilization

Progress in Natural Science:Materials International 2012年第6期22卷 522-534页

作者： Samuel S.Mao Shaohua Shen Liejin Guo Lawrence Berkeley National Laboratory and Department of Mechanical Engineering University of California at Berkeley.BerkeleyCA 94720United States Lawrence Berkeley National Laboratory and Department of Mechanical Engineering University of California at Berkeley.BerkeleyCA 94720.United States International Research Center for Renewable Energy.State Key Laboratory of Multiphase Flow in Power Engineering.Xi'an Jiaotong University International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power EngineeringXi'an Jiaotong University

An ever growing demand for energy coupled with increasing pollution is forcing us to seek environmentally clean alternative energy resources to substitute fossil *** rapid development of nanomaterials has opened up new avenues for the conversion and utilization of renewable *** article reviews nanostructured materials designed for selected applications in renewable energy conversion and *** review is based on the authors’ research,with particular focus on solar hydrogen production,hydrogen storage and hydrogen *** topics include photoelectrochemical(PEC) water splitting and photocatalytic hydrogen production, solid-state hydrogen storage,and proton exchange membrane fuel cells(PEMFCs).It is expected that the rational design of nanomaterials could play an important role in achieving a renewable energy based economy in the coming decades.

关键词： Nanomaterials Renewable energy Hydrogen production Fuel cell Hydrogen storage

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Novel Cu_3P/g-C_3N_4 p-n heterojunction photocatalysts for solar hydrogen generation

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Science China Materials 2018年第6期61卷 861-868页

作者： Zhixiao Qin Menglong Wang Rui Li Yubin Chen International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University

Developing efficient heterostructured photocatalysts to accelerate charge separation and transfer is crucial to improving photocatalytic hydrogen generation using solar energy. Herein, we report for the first time that p-type copper phosphide（Cu3P） coupled with n-type graphitic carbon nitride（g-C3N4） forms a p-n junction to accelerate charge separation and transfer for enhanced photocatalytic *** optimized Cu3P/g-C3N4 p-n heterojunction photocatalyst exhibits 95 times higher activity than bare g-C3N4, with an apparent quantum efficiency of 2.6% at 420 nm. A detail analysis of the reaction mechanism by photoluminescence,surface photovoltaics and electrochemical measurements revealed that the improved photocatalytic activity can be ascribed to efficient separation of photo-induced charge carriers. This work demonstrates that p-n junction structure is a useful strategy for developing efficient heterostructured photocatalysts.

关键词： photocatalysis copper phosphide p-n junction heterostructure hydrogen production

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On the Intelligent Optimization of the Crevice Structure in a Rapid Compression Machine

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Journal of Thermal Science 2024年第3期33卷 1200-1215页

作者： GUO Qiang LIU Jie WU Yingtao WANG Hewu TANG Chenglong YU Ruiguang Department of Power Mechanical Engineering Beijing Jiaotong UniversityBeijing100044China State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong UniversityXi’an710049China State Key Laboratory of Automotive Safety and Energy Tsinghua UniversityBeijing100084China Beijing Key Laboratory of New Energy Vehicle Powertrain Technology Beijing100044China National International Science and Technology Cooperation Base Beijing Jiaotong UniversityBeijing100044China

In this study,the multi-objective intelligent optimization of the crevice structure in a rapid compression machine(RCM)is carried out based on the RCM simulation model modified with the KIVA-3V program.A multi-objective optimization simulation model of the crevice structure based on the large eddy simulation model coupled with the genetic algorithm NSGA-Ⅲis *** optimization parameters and seven optimization objectives are selected in the optimization *** results show that the genetic algorithm can quickly find the values of the optimized *** crevice volume ratio shows a trade-off relationship with the dimensionless temperature ratio T_(max)/T_(aver)and the tumble ratio.A larger crevice volume can reduce the flow of boundary layer cryogenic gas into the combustion chamber,thus improving the temperature *** addition,the crevice entrance width and the connecting channel length should be smaller,while the volume of the crevice main chamber should be larger,so as to sufficiently introduce the low-temperature gas of the boundary layer into the crevice and reduce their influence on the temperature field of the combustion *** the crevice volume accounts for1.%of the total volume,the temperature uniformity of the combustor is significantly enhanced,and when the crevice volume accounts for 30.4%,there is almost no low-temperature vortex in the combustion chamber.

关键词： rapid compression machine adiabatic core area ignition delay period crevice structure

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Progress and challenge of functional single-atom catalysts for the catalytic oxidation of volatile organic compounds

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Chinese Chemical Letters 2024年第9期35卷 83-91页

作者： Zeyu Jiang Yadi Wang Changwei Chen Chi He Department of Environmental Science and Engineering Xi’an Jiaotong UniversityXi’an 710049China State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power EngineeringXi’an Jiaotong UniversityXi’an 710049China National Engineering Laboratory for VOCs Pollution Control Material&Technology University of Chinese Academy of SciencesBeijing 101408China

The catalytic oxidation of volatile organic compounds(VOCs)is of considerable significance for the sustainable development of the chemical industry;thus,considerable efforts have been devoted to the exploration of efficient catalysts for use in this *** this regard,the development and utilization of single-atom catalysts(SACs)in VOCs decomposition is a rapidly expanding research *** can be employed as potential catalysts for oxidizing VOC molecules due to their optimal utilization efficiency,unique atomic bonding structures,and unsaturated *** has been achieved,while the challenges surrounding precise regulation of the microstructures of SACs for improving their low-temperature efficiency,stability,and product selectivity under practical conditions are ***,elucidating structure-performance relationships and establishing intrinsic modulating mechanisms are urgently required for guiding researchers on how to synthesize effective and stable functional SACs ***,recent advances in the design and synthesis of functional SACs for application in the catalytic oxidation of VOCs are *** experimental and theoretical studies revealing higher efficiency,stability,and selectivity of as-prepared functional SACs are being ***,the future perspectives in terms of promising catalysts with multi-sized composite active sites and the illustration of intrinsic mechanism are *** rapid intelligent screening of applicable SACs and their industrial applications are also discussed.

关键词： Single-atom catalysts VOCs catalytic oxidation Hydrocarbon activation Oxygen species transformation Surface chemistry Intrinsic mechanism

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Numerical Investigation on Isolated Moving Charged Droplet Evaporation in Electrostatic Field with Highly Volatile R1.4a 15

Numerical Investigation on Isolated Moving Charged Droplet E...

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1.th Triennial International Conference on Liquid Atomization and Spray Systems, ICLASS 2021

作者： Tian, Jiameng Wang, Junfeng Chen, Bin School of Energy and Power Engineering Jiangsu University Zhenjiang China State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an China

Fundamental investigations of the charged droplet evaporation are helpful in enhancing the cooling capability and advancing the electrostatic spray model, whereas the corresponding data with the highly volatile R1.4a under electric field is very scarce. In this work, an improved evaporation model accounting for the effects of the corona wind, Coulombic fission and electric force under the electric field was developed and validated to evaluate the importance of the electric field on the moving charged R1.4a droplet evaporation for the first time. Results demonstrated that the electrostatic field can improve the charged droplet evaporation by means of the heat and mass transfer enhancement by the corona wind and counteracting the drag force from air. The droplet lifetime was shortened by 20.8% (from 1.5.6 ms to 83.6 ms) when the applied voltage increased from 0 kV to 1. kV. Exponential decay in the charged droplet lifetime when the applied voltage increased was observed. © 2021.ICLASS 2021.- 1.th Triennial International Conference on Liquid Atomization and Spray Systems. All Rights Reserved.

关键词： Drops

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MHD Simulations Preliminarily Predict The Habitability and Radio Emission of TRAPPIST-1.

arXiv

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arXiv 2025年

作者： Wang, BoRui Ye, ShengYi Varela, J. Luo, XinYi Department of Earth and Space Sciences Southern University of Science and Technology Shenzhen518055 China Institute for Fusion Studies University of Texas AustinTX78712 United States State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an710049 China

Context. As the closest Earth-like exoplanet within the habitable zone of the M-dwarf star TRAPPIST-1. TRAPPIST-1. exhibits a magnetic field topology that is dependent on space weather conditions. Variations in these conditions influence its habitability and contribute to its radio emissions. Aims. Our objective is to analyze the response of different terrestrial magnetosphere structures of TRAPPIST-1. to various space weather conditions, including events analogous to coronal mass ejections (CMEs). We assess its habitability by computing the magnetopause standoff distance and predict the resulting radio emissions using scaling laws. This study provides some priors for future radio observations. Methods. We perform three-dimensional magnetohydrodynamic (MHD) simulations of the TRAPPIST-1. system using the PLUTO code in spherical coordinates. Assuming TRAPPIST-1. possesses various Earth-like magnetospheres, we analyze the impact of four distinct space weather conditions on its magnetospheric topology. The space weather parameters range from sub-Alfvénic conditions to CMEs. Results. Our analysis indicates that the predicted habitability and radio emission of TRAPPIST-1. strongly depend on the planet’s magnetic field intensity and magnetic axis inclination. Within sub-Alfvénic, super-Alfvénic, and transitional stellar wind regimes, the radio emission intensity positively correlates with both planetary magnetic field strength and axial tilt, while planetary habitability, quantified by the magnetopause standoff distance, shows a positive correlation with magnetic field strength and a negative correlation with magnetic axis tilt. If TRAPPIST-1. possesses a magnetic field strength and axial tilt comparable to Earth’s (∼ 0.32G and ∼ 23.5◦). its magnetosphere can effectively shield the planetary surface from stellar wind erosion even under severe space weather conditions (e.g., CME events). However, for larger axial tilts (∼ 45◦), a stronger planetary magnetic field would be

关键词： Plasma magnetohydrodynamic waves

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Evaluation of R51.A as an environmentally friendly alternative to R1.4a in spray cooling for laser surgery: Heat transfer performance and optimization

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International Journal of Thermal Sciences 2025年 215卷

作者： Zhi-Zhong He Xiang-Wei Lin Chen-Xi Li Chen Kong Lin-Xin Shen Zhi-Fu Zhou State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an 710049 Shaanxi China School of Future Technology Xi'an Jiaotong University Xi'an 710049 Shaanxi China Xi'an Jiaotong University Health Science Center Xi'an 710049 Shaanxi China

Spray cooling plays a pivotal role in mitigating thermal injuries to the epidermis during laser surgery. However, the widespread use of R1.4a, a refrigerant with a high global warming potential (GWP) of 1.00, poses significant environmental concerns. In this study, R51.A, a more environmental-friendly cryogen with a GWP of 573, is used to investigate the feasibility of replacing R1.4a and the effects of spray height, spurt duration, nozzle orifice diameter, and spray pressure on R51.A spray cooling through a self-built open-loop spray system. Experimental results demonstrate that R51.A exhibits superior cooling performance, achieving a minimum surface temperature ( T min ) 1. °C lower and a maximum heat flux ( q max ) 27.5 % higher than R1.4a. Additionally, R51.A offers a broader optimal spray height range (30–50 mm) in which T min is 4 °C and 1. °C lower than those at 20 mm and 1. mm, respectively. q max in this range is 1. % and 1. % higher than those at 20 mm and 1. mm, respectively. While extending the spurt duration consumes more cryogen and prolongs the liquid film lifetime, the differences in T min and q max are less than 4 °C and 1. kW/m 2 . With the nozzle orifice increasing from 0.6 mm to 1.0 mm, T min remains approximately −42 °C but q max gradually increases by 6 kW/m 2 . Macroscopic analysis reveals that higher spray pressure induces a more dispersive spray, though this does not significantly improve cooling efficiency. To advance the understanding of R51.A spray cooling dynamics, a dimensionless correlation was developed to predict the dynamic heat transfer coefficient across diverse conditions. This study not only highlights the potential of R51.A as a sustainable alternative but also provides critical insights into optimizing spray cooling parameters for enhanced thermal management in laser surgery.

关键词： Chilling

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Improved filtered mesoscale interphase heat transfer model

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Particuology 2021年第4期19卷 176-186页

作者： Yu Li Yaxiong Yu Chi Zhang Zheqing Huang Qiang Zhou School of Chemical Engineering and Technology Xi’an Jiao Tong UniversityXi’an 710049China AVIC Xi’an Flight Automatic Control Research Institute Xi’an 710049China State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiao Tong UniversityXi’an 710049China

Mesoscale structures that form in gas-solid flows considerably affect interphase heat transfer.A filtered interphase heat transfer model accounts for the effects of unresolved mesoscale structures is required in coarse-grid *** the literature,researchers obtain the filtered interphase heat transfer coefficient using a correction(Q)to the microscopic interphase heat transfer *** models are based on filtered data in the range 01.is *** percentage can reach approximately 20%when the dimensionless filter size is smaller than 1.028(66.7×the particle diameter).We proposed an improved filtered interphase heat transfer model by considering the data in the range Q<0 and Q>*** evaluated the predictive {1. of our model in an a priori *** model has much better performance than other models when the dimensionless filter size△<8.222.

关键词： Gas-solid flows Two-fluid model Interphase heat transfer Filtered model Mesoscale

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Experimental studies of ash film fractions based on measurement of cenospheres geometry in pulverized coal combustion

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Frontiers in Energy 2021年第1期15卷 91-98页

作者： Siqi LIU Yanqing NIU Liping WEN Yang LIANG Bokang YAN Denghui WANG Shi'en HUI State Key Laboratory of Multiphase Flow in Power Engineering Department of Thermal EngineeringSchool of Energy and Power EngineeringXi'an Jiaotong UniversityXi'an 710049China

In pulverized coal particle combustion, part of the ash forms the ash film and exerts an inhibitory influence on combustion by impeding the diffusion of oxygen to the encapsulated char core, while part of the ash diffuses toward the char core. Despite the considerable ash effects on combustion, the fraction of ash film still remains unclear. However, the research of the properties of cenospheres can be an appropriate choice for the fraction determination, being aware that the formation of cenospheres is based on the model of coal particles with the visco-plastic ash film and a solid core. The fraction of ash film X is the ratio of the measuring mass of ash film and the total ash in coal particle. In this paper, the Huangling bituminous coal with different sizes was burnt in a drop-tube furnace at 1.73, 1.73, and 1.73 K with air as oxidizer. A scanning electron microscope (SEM) and cross-section analysis have been used to study the geometry of the collected cenospheres and the effects of combustion parameters on the fraction of ash film. The results show that the ash film fraction increases with increasing temperature and carbon conversion ratio but decreases with larger sizes of coal particles. The high fraction of ash film provides a reasonable explanation for the extinction event at the late burnout stage. The varied values of ash film fractions under different conditions during the dynamic combustion process are necessary for further development of kinetic models.

关键词： ash film fraction cenospheres coal combustion fly ash

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Phase identification by a novel needle-contact capacitance probe in gas-liquid two-phase flows

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Nuclear Science and Techniques 2010年第5期21卷 316-320页

作者： HUANG Shanfang LU Jun ZHANG Bingdong WANG Dong Department of Engineering Physics Tsinghua University Beijing 100084 China State Key Laboratory of Multiphase Flow in Power Engineering Xi 'an Jiaotong University Xi'an 710049 China Beijing Aerospace Institute for Metrology and Measurement Technology Beijing 100076 China

In this paper,we propose a novel probe to identify phases in any two-phase flows where one phase is conductive and the other *** can further obtain many parameters such as void fraction,bubble velocity,and interfacial area *** with the traditional probe,the novel probe has unique advantages that it is less dependent on water conductance or distance between the electrodes,and that the amplitude is bigger between high and low *** analyses showed that the measurement error became higher when water conductance decreases or distance increases,which is consistent with the theoretical *** results showed that the output signal kept constant with salt content of 0-5% and electrode distance of 0-30 mm in tap *** level difference was up to 6.4 V,resulting in identifying two phases *** traces of phase identification were completely consistent with the flow structures.

关键词：气液两相流探头接触式鉴定一阶电导电极水电导率气泡速度

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