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Influence of Salts on Morphology of Structures in Surfactant-Polymer Solutions Explored by Coarse Grained Dynamic Simulation

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Influence of Salts on Morphology of Structures in Surfactant...

作者： Liu, Dongjie Liu, Fei Zhou, Wenjing Chen, Fei Wei, Jinjia State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an710049 China School of Chemical Engineering and Technology Xi’an Jiaotong University Xi’an710049 China

In this study, a coarse-grained molecular dynamic simulation was employed to test the influence of salts in morphology of structures in surfactant-polymer solutions. The surfactant was cetyltrimethyl ammonium chloride (CTAC) and the polymer was polyacrylamide (PAM). Six different salt concentrations were studied in the mixed surfactant-polymer solutions, and pure surfactant solutions with salts were also tested as control groups. By analyzing the shapes of micelles and the CTA+ aggregation number of micelles, we noted that the proper salt concentration can facilitate the formation of large micelles. In too high or too low salt concentration solutions only spherical or short rodlike micelles exist. The existence of PAM can also facilitate the formation of large micelles because polymers act as "bridges" and increase the probability of touch and coalescence of micelles. © Springer Nature Switzerland AG 2020.

关键词： Morphology

Experimental Investigations of Liquid Immersion Cooling for 1.650 Lithium-Ion Battery Pack Under Fast Charging Conditions

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SSRN 2022年

作者： Li, Yang Bai, Minli Zhou, Zhifu Wu, Wei-Tao Lv, Jizu Gao, Linsong Huang, Heng Li, Yulong Li, Yubai Song, Yongchen Key Laboratory of Ocean Energy Utilization and Energy Conservation of Ministry of Education Dalian University of Technology Dalian116023 China State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi’an710049 China School of Mechanical Engineering Nanjing University of Science and Technology Nanjing210094 China

In this study, a novel battery thermal management system (BTMS) based on FS49 is proposed and tested for cooling the cylindrical lithium-ion battery (LIB) module under fast charging conditions. Firstly, the temperature response of the battery module under 3 C rate charging with forced air cooling (FAC) and liquid immersion cooling (LIC) is compared. The results indicate that the LIC has excellent heat dissipation performance, and the peak temperature and peak temperature difference of the module are reduced by 1..6 °C and 8.99 °C, respectively, compared with the FAC, while the cooling energy consumption of LIC is only 40.4% of the FAC. It is found that the LIC embraces advantages of efficient cooling and minimizing the temperature non-uniformity in battery pack. Subsequently, the thermal management performance of the proposed LIC is investigated under conventional C rate discharging and different fast charging schemes. Finally, effect of condenser flow rate and cooling water temperature were investigated. This study demonstrates the application prospect of the LIC in the field of LIB fast charging. © 2022, The Authors. All rights reserved.

关键词： Lithium-ion batteries

A Subchannel Analysis Code Star for Sodium-Cooled Fast Reactor

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SSRN 2022年

作者： Liang, Yu Zhang, Dalin Zhang, Jing Liu, Xiao Liu, Yapeng Zhou, Lei Chen, Yutong Mikityuk, Konstantin Wang, Xiaoyu Tian, Wenxi Qiu, Suizheng Su, Guanghui School of Nuclear Science and Technology Shaanxi Key Laboratory of Advanced Nuclear Energy and Technology State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'An710049 China Nuclear Power Institute of China 328 Changshun Avenue Chengdu610213 China Paul Scherrer Institute Villigen PSI5232 Switzerland

The strong coupling heat transfer between subassemblies and inter-wrapper gaps is closely related to the safety of the sodium-cooled fast reactor (SFR). Therefore, it is very important to carry out a detailed thermal hydraulic analysis of the core. In this paper, the inter-wrapper channel is modeled using the subchannel method, and a two-fluid subchannel analysis model is developed based on the staggered grid method. The core thermal-hydraulic analysis code STAR (Subchannel Thermal-hydraulic Analysis code for SFR) is developed by using SIMPLE algorithm. © 2022, The Authors. All rights reserved.

关键词： Sodium-cooled fast reactors

Supercritical Water Gasification of Phenol with Metal Cations-A Way to Degrade Coal Industrial Wastewater and Metal-Contaminated Wastewater Simultaneously

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SSRN 2022年

作者： Cao, Wen Wang, Shaoqi Ma, Lujing Liu, Shi Jin, Hui Wei, Wenwen Guo, Liejin State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xianning West Road Xi’an710049 China Suzhou Academy of Xi’an Jiaotong University No.99 Ren’ai Road Jiangsu Suzhou215123 China

Phenol is a representative compound in coal industrial wastewater. Metal cations are the main harmful components in the wastewater of the electroplating and dyeing industries. Supercritical water gasification (SCWG) of phenol with metal cations could provide a promising way to degrade coal chemical wastewater and metal-containing wastewater simultaneously. In this study, SCWG of phenol with Mg2+, Mn2+, and Ni2+ was carried out to investigate the effect of metal cations on gasification results. Results showed that gaseous product was mainly composed of H2, CO, CH4 and CO2, and CO2 was the dominant one. Prolonging residence time and increasing the concentration of metal cations significantly increased the gas yield of CO2 and carbon gasification efficiency. Higher concentrations of metal cations facilitated methane-reforming reaction and water-gas shift reaction. Metal cations promoted the generation of 1.Ethoxybutane by the ring-breaking reaction and prevented the polymerization reaction. The order of catalytic effect was ranked as Ni2+>Mn2+>Mg2+. Mg2+, Mn2+ and Ni2+ were finally transformed into the corresponding metal hydroxides and metal oxides which could be recycled for reutilization. NiO could be reduced into metallic Ni, which consumed the H2 but effectively catalyzed SCWG of phenol. © 2022, The Authors. All rights reserved.

关键词： Phenols

Capillary Limit of a Sodium Screen-Wick Heat Pipe

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SSRN 2022年

作者： Ma, Yugao Wang, Xueqing Yu, Hongxing Huang, Shanfang Zhang, Yingnan Huang, Jian Su, Guanghui Deng, Jian Chai, Xiaoming Hu, Wenzhen School of Nuclear Science and Technology Xi’an Jiaotong University Shanxi Xi’an710049 China Science and Technology on Reactor System Design Technology Laboratory Nuclear Power Institute of China Chengdu610213 China Department of Engineering Physics Tsinghua University Beijing100084 China State Key Laboratory of Multiphase Flow in Power Engineering China

High-temperature alkali-metal heat pipes are passive heat transfer devices, where the capillary pressure created by the menisci in the wick pumps the condensed fluid back to the evaporator. Thus, the heat pipe heat transfer capacity is limited by the maximum capillary pressure at high heat fluxes. This work presents a two-dimensional heat and mass transfer model that includes the capillary and gravitational forces that are used to predict the capillary limit which is then validated by experimental data. The predicted critical heat flux temperature has an error of less than 20℃ and a relative error of 6%. The predicted transient sequences are consistent with the measurements. The model shows that capillary limit is affected by inclination angle, heat flux, and wick structure. For inclinations, the critical heat flux at the capillary limit is linearly related to the inclination angle with the predicted temperature rising 2 ~1.℃/s during the early stage of the capillary limit critical heat flux condition. The evaporator temperature oscillates before the capillary limit with positive inclinations. For heat fluxes, increasing the heat flux by 1.% increases the temperature increase rate 1. fold with a longer dryout length. The evaporator exhibits hysteresis after the capillary limit due to partial dryout of evaporator. For wick structures, reducing the mesh screen pitch from 80 μm to 1. μm reduces the critical heat flux to 1.% of the CHF at 80 μm. This model can accurately predict the heat pipe temperature variations at the capillary limit and can explain the physical mechanisms for the dryout oscillations and recovery hysteresis at the capillary limit. Thus, the measurements and model provide analytical guidelines for designing heat pipe cooling systems. © 2022, The Authors. All rights reserved.

关键词： Heat flux

Oxidation of Typical Zr-1.b Alloy in High-Temperature Air Under 700–900 °C

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SSRN 2022年

作者： Jiang, Guanyu Xu, Donghai Liu, Lu Ding, Xin Kuang, Wenjun Wang, Mingjun Key Laboratory of Thermo-Fluid Science & Engineering Ministry of Education School of Energy and Power Engineering Xi’an Jiaotong University Shaanxi Province Xi’an710049 China School of Materials Science and Engineering Xi’an Jiaotong University Shaanxi Province Xi’an710049 China State Key Laboratory of Multiphase Flow in Power Engineering Department of Nuclear Science and Technology Xi'an Jiaotong University Xi’an China

m-ZrO2 is always the dominant phase, while oxide shapes, the integrity and roughness of oxide films share evident differences. At 900 &#1.6;C, M5 alloy exhibits kinetics transition and breakaway oxidation at approxima... 详细信息

m-ZrO2 is always the dominant phase, while oxide shapes, the integrity and roughness of oxide films share evident differences. At 900 °C, M5 alloy exhibits kinetics transition and breakaway oxidation at approximately 80 min. The pre-transition oxidation follows a parabola kinetics with the rate exponent n being 1.65. The presence of ZrO and ZrO0.35 sub-oxides accounts for the high reaction activation energy (1.9.6 kJ/mol). During the kinetics transition, some intergranular cracks turn transgranular, and pores distribute on the oxide layer and O/M interface. Air ingress through the oxide layer is jointly affected by air transport and ion diffusion. © 2022, The Authors. All rights reserved.

关键词： Oxidation

Evaluation of stability and catalytic activity of Ni catalysts for hydrogen production by biomass gasification in supercritical water

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Carbon Resources Conversion 2019年第1期2卷 95-101页

作者： Youjun Lu Hui Jin Rui Zhang State Key Laboratory of Multiphase Flow in Power Engineering(SKLMFPE) Xi’an Jiaotong UniversityXi’an 710049ShaanxiChina

Supercritical water gasification is a promising technology for wet biomass *** this paper,Ni and other metal catalysts were synthesized by wet *** stability and catalytic activities of Ni catalysts were ***,catalytic activities of Ni,Fe,Cu catalysts supported on MgO were tested using wheat straw as raw material in a batch reactor at 723 K and water density of 0.07 cm^(3)/*** results showed that the order of metal catalyst activity for hydrogen generation was Ni/MgO>Fe/MgO>Cu/***,the influence of different supports on Ni catalysts performance was *** results showed that the order of the Ni catalysts’activity with different supports was Ni/MgO>Ni/ZnO>Ni/Al_(2)O_(3)>Ni/ZrO_(2).Finally,the effects of Ni loading and the amount of Ni catalyst addition on hydrogen production,and the stability of Ni/MgO catalyst were *** was found that serious deactivation of Ni catalyst in the process of supercritical water gasification took *** if carbon deposited on the catalyst surface was removed by high temperature calcination and the catalyst was reduced with hydrogen,the activity of used catalyst was only partially restored.

关键词： Ni catalyst Deactivation Biomass gasification Supercritical water Hydrogen production

PREFACE: SPECIAL ISSUE FOR THE 2ND INTERNATIONAL SYMPOSIUM ON THERMAL-FLUID DYNAMICS (ISTFD2021.

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Heat Transfer Research 2022年第8期53卷 V-VI页

作者： Cheng, Lixin Bai, Bofeng Guo, Zhixiong School of Energy and Power Engineering Beijing University of Technology Beijing100124 China Department of Engineering and Mathematics Sheffield Hallam University SheffieldS1 1WB United Kingdom State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an710049 China Department of Mechanical and Aerospace Engineering Rutgers The State University of New Jersey PiscatawayNJ08854 United States

Comparison of chemical composition and acidity of size-resolved inorganic aerosols at the top and foot of Mt. Hua, Northwest China: The role of the gas-particle distribution of ammonia

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Science of the Total Environment 2023年 905卷 166985页

作者： Feng, Qiao Liu, Haijiao Dai, Wenting Cao, Yue Shen, Minxia Liu, Yali Qi, Weining Chen, Yukun Guo, Xiao Zhang, Yifan Li, Lu Zhou, Bianhong Li, Jianjun State Key Laboratory of Loess and Quaternary Geology Key Lab of Aerosol Chemistry and Physics Institute of Earth Environment Chinese Academy of Sciences Xi'an710061 China College of Geography and Environment Baoji University of Arts and Sciences Shaanxi Key Laboratory of Disaster Monitoring and Mechanism Simulation Baoji721013 China Xi'an Institute for Innovative Earth Environment Research Xi'an710061 China National Observation and Research Station of Regional Ecological Environment Change and Comprehensive Management in the Guanzhong Plain Shaanxi China State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an710049 China

Aerosol pH is not only a diagnostic indicator of secondary aerosol formation, but also a key factor in the specific chemical reaction routes that produce sulfate and nitrate. To understand the characteristics of aerosol acidity in the Mt. Hua, the chemical fractions of water-soluble inorganic ions in the atmospheric PM2.5 and size-resolved particle at the top and foot of Mt. Hua in summer 2020 were studied. The results showed the mass concentrations of PM2.5 and water-soluble ions at the foot were 2.0–2.6 times higher than those at the top. The secondary inorganic ions, i.e., SO42−, NO3−, and NH4+ (SNA) were 56 %–61.% higher by day than by night. SO42− was mainly distributed in the fine particles (Dp 3− showed a unimodal size distribution (peaking at 0.7–1.1.μm) at the foot and a bimodal (0.7–1.1.μm and 4.7–5.8 μm) size distribution at the top. At the top site, the distribution of NO3− in coarse particles (> 2.1.μm) was mainly attributed to the gaseous HNO3 volatilized from fine particles reacting with cations in coarse particles to form non-volatile salts (such as Ca(NO3)2). The pH values of PM2.5 were 2.7 ± 1.3 and 3.3 ± 0.42 at the top and foot, respectively. NH4+/NH3(g) plays a decisive role in stabilizing aerosol acidity. In addition, the increase of the liquid water content (LWC) at the foot facilitates the gas-particle conversion of NH3, while the H+ concentration was diluted, resulting in a decrease in acidity at the foot. NH4+/NH3 had good linear correlations with SO42−, NO3−, and LWC during the daytime at both sites, indicating that SO42−, NO3−, and LWC together affect the gas-particle distribution of ammonia by day: however, the effect of LWC at night was not evident. © 2023

关键词： Ammonia