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Performance of CO_2 absorption in a diameter-varying spray tower

Chinese Journal of Chemical engineering 2017年第8期25卷 1109-1114页

作者： Xiaomei Wu Yunsong Yu Zhen Qin Zaoxiao Zhang School of Chemical Engineering and Technology Xi'an Jiaotong University State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University

The application of spray towers for CO2 capture is a development trend in recent years. However, most of the previous jobs were conducted in a cylindrical tower by using a single spray nozzle, whose configuration and performance is not good enough for industrial application. To solve this problem, the present work proposed a diameter-varying spray tower and a new spray mode of dual-nozzle opposed impinging spray to enhance the heat and mass transfer of CO2 absorption process. Experiments were performed to investigate the mass transfer performance （in terms of the CO2 removal rate （η） and the overall mass transfer coefficient （KGae）） of the improved spray tower under various operating conditions. Experimental results showed that the liquid to gas ratio and mole ratio of MEA to C02 are major factors, which affect the absorption performance and the maximums of η and KGae that are 94.0% and 0.574 kmol. m^-3·h^-1.kPa^-1. respectively, under the experimental conditions. Furthermore, new correlations to predict the mass transfer coefficient of the proposed spray tower are developed in various CO2 concentrations with a Pearson Correlation Coefficient over 90%.

关键词： Carbon dioxide Absorption Diameter-varying spray tower Mass transfer

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Current Density Regulating Lithium Metal Directional Deposition for Long Cycle Life Lithium Metal Batteries

SSRN

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SSRN 2020年

作者： Mao, Heng Yu, Wei Cai, Zhuanyun Liu, Guixian Liu, Limin Wen, Rui Su, Yaqiong Xi, Kai Li, Benqiang Da, Xinyu Kou, Huari Yan, Wei Ding, Shujiang Xi'an Key Laboratory of Sustainable Energy Materials Chemistry School of Chemistry Xi’an Jiaotong University & Shaanxi Quantong Joint Research Institute of New Energy Vehicles Power Xi’an Jiaotong University Xi’an710049 China State Key Laboratory of Physical Chemistry of Solid Surfaces Department of Chemistry College of Chemistry and Chemical Engineering Xiamen University Xiamen361005 China Key Laboratory of Molecular Nanostructure and Nanotechnology Beijing National Laboratory for Molecular Sciences CAS Research/Education Center for Excellence in Molecular Sciences Institute of Chemistry Chinese Academy of Sciences Beijing100190 China Cambridge Graphene Centre Department of Engineering University of Cambridge CambridgeCB3 0FA United Kingdom Department of Mechanical Engineering University of Michigan-Dearborn DearbornMI48128 United States Department of Environmental Science and Engineering State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an710049 China

Uncontrolled dendrite formation in the high energy density of lithium metal batteries (LMBs) may pose serious safety risks. Numerous works have been reported to protect separator. However, these methods still couldn’t inhibit the dendrite upward growth to protect the separator, effectively. Here, we introduce a novel “orientated-growth” strategy that makes the depositional interface transfer to the anode/current collector interface from the anode/separator interface. We placed a layer of cellulose/graphene carbon composite aerogel (CCA) between the current collector and the anode (CCA-Li). This layer works as the charge organizer;it induces a higher current density distribution and makes Li prefer to deposit in the bottom CCA layer of CCA-Li electrode. Both in-situ and ex-situ images of the electrode demonstrate the anode part of the cell has been flipped;with the new deposited particles facing the current collector and smooth surface facing the separator. Electrochemical characterization of the electrode in half and full cells showed outstanding cyclic stability and rate capability, with the CCA-Li/LPF full cell able to maintain 94% of its initial capacity after 1.00 cycles. We believe that the innovative strategy would promote the leapfrog development for LMBs. © 2020, The Authors. All rights reserved.

关键词： Electric current collectors

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Dynamic modeling of a NG-fueled SOFC-PEMFC hybrid system coupled with TSA process for fuel cell vehicle

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Energy Procedia 2019年 158卷 2215-2224页

作者： Zhen Wu Meng Ni Pengfei Zhu Zaoxiao Zhang Building Energy Research Group Department of Building and Real Estate The Hong Kong Polytechnic University Hong Kong P.R. China State Key Laboratory of Multiphase Flow in Power Engineering School of Chemical Engineering and Technology Xi’an Jiaotong University Xi’an 710049 P.R. China

Fuel cell power technology has drawn extensive attentions due to its high efficiency, low emission and noise. Solid oxide fuel cell (SOFC) could generate the power by diverse fuels, such as natural gas (NG), while proton exchange membrane fuel cell (PEMFC) only feeds on pure H 2 . More and more attentions are paid on the combination of SOFC and PEMFC for high efficiency and convenient refueling in the practical applications. To obtain H 2 fuel with high purity from SOFC as a reformer, the gas processing subsystem for H 2 separation and purification should be applied between SOFC and PEMFC. In this present study, the gas processing subsystem, consisting of water gas shift (WGS) and thermal swing adsorption (TSA), is introduced into the SOFC-PEMFC hybrid system. Then, the SOFC-WGS-TSA-PEMFC hybrid system is modelled to investigate the transient behaviors under different operations. The simulation results show that the SOFC-WGS-TSA-PEMFC hybrid system has an improved energy conversion efficiency of approximately 64%, which is higher than the only-SOFC and the reform-PEMFC. The waste heat recovery for driving the TSA reaction accounts for the higher net electricity efficiency compared with the SOFC-PEMFC hybrid system based on the pressure swing adsorption (PSA) for H 2 separation. Since the SOFC and PEMFC have completely different transient responses to the change of the loading, the influences of operating conditions of fuel cell vehicles on the transient behaviors of single SOFC and PEMFC and the overall performance of the SOFC-WGS-TSA-PEMFC hybrid system are further investigated. Through the analysis and discussion based on the dynamic modelling, the operation strategy is unveiled in this paper for the performance optimization of the hybrid system when installed in the fuel cell vehicles.

关键词： SOFC PEMFC Metal hydride Transient behavior High efficiency

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Influence of(Mg_(1.3)Nb_(2/3))complex substitutions on crystal structures and microwave dielectric properties of Li2TiO3 ceramics with extreme low loss

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Journal of Materiomics 2018年第4期4卷 368-382页

作者： Huan-Huan Guo Di Zhou Li-Xia Pang Jin-Zhan Su Electronic Materials Research Laboratory Key Laboratory of the Ministry of Education&International Center for Dielectric ResearchSchool of Electronic and Information EngineeringXi'an Jiaotong UniversityXi'an710049China Micro-optoelectronic Systems Laboratories Xi'an Technological UniversityXi'an710032ShaanxiChina International Research Centre for Renewable Energy State Key Laboratory of Multiphase Flow in Power EngineeringXi'an Jiaotong UniversityXi'anShaanxi710049China

A systematic investigation of the Li2Ti1.x(Mg_(1.3)Nb_(2/3))xO_(3)(0.1.x≤0.35)solid solutions synthesized by traditional solid-state reaction method is reported in this *** the composition range of 0.1.x≤0.25,a monoclinic rock salt structured solid solution was *** x increased to 0.3,a phase transition from monoclinic to cubic phase,along with an order-disorder phase transition,was *** x increased from 0.1.to 0.35,the microwave permittivity(εr)and temperature coefficient of resonant frequency(TCF)of the Li2Ti1.x(Mg_(1.3)Nb_(2/3))xO_(3)ceramics decreased linearly from 21.0 to 1..6,+27.1.to-1..4 ppm/℃,*** Li_(2)Ti_(0.75)(Mg_(1.3)Nb_(2/3))0.25O_(3)ceramic sintered at 1.70℃shows high performance of microwave dielectric properties with aεr~1..6,a Qf(Q=quality factor=1.dielectric loss;f=resonant frequency)~1.9,770 GHz(at 7.7 GHz)and a near zero TCF~t 1.2 ppm/℃.Moreover,the burying sintering process can reduce the volatilization of lithium so that the porosity of Li_(2)Ti_(0.75)(Mg_(1.3)Nb_(2/3))0.25O_(3)ceramic was reduced effectively,which made Li_(2)Ti_(0.75)(Mg_(1.3)Nb_(2/3))0.25O_(3)ceramic promising for future *** area electron diffraction patterns,high-resolution transmission electron microscopy,Raman and far-infrared spectra were employed to study the relation between crystal structure and microwave dielectric properties in detail.

关键词： Microwave dielectric properties Phase evolution Crystal structure High quality

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Synthesis and application of transition metal phosphides as electrocatalyst for water splitting

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Science Bulletin 2017年第9期62卷 633-644页

作者： Jinzhan Su Jinglan Zhou Lu Wang Cong Liu Yubin Chen International Research Center for Renewable Energy (IRCRE) State Key Laboratory for Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an 710049 China

With continuous research on photocatalytic water splitting, searching for efficient catalyst for hydrogen evolution reaction(HER) becomes popular topic in addition to main catalyst research. Transition metal phosphides are receiving intense attention due to its abundance in the Earth's crust and comparable catalytic properties to noble metals. In this review, the synthesis approaches, HER reaction mechanism,photocatalytic activity, approaches to improve the activity of transition metal phosphides were reviewed and discussed. It was showed that the transition metal phosphides have great potential to reduce the cost of photocatalyst and promising application on water splitting. The stability problem and participation of poisonous reactant and product in its synthesis reaction limit its application and developing in a certain extent, but with the continuous efforts on the development and improvement of the synthesis methods,transition metal phosphides will find wide application in water splitting.

关键词： Transition metal phosphide Electrocatalyst HER Photocatalytic water splitting

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Three-dimensional analysis of condensation nanofluid film on an inclined rotating disk by efficient analytical methods

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Arab Journal of Basic and Applied Sciences 2018年第1期25卷 28-37页

作者： Hatami, M. Jing, D. Yousif, Majeed A. Department of Mechanical Engineering Esfarayen University of Technology Esfarayen Iran State Key Laboratory of Multiphase Flow in Power Engineering & International Research Center for Renewable Energy Xi’an Jiaotong University Xi’an China Department of Mathematics Faculty of Science University of Zakho Zakho Iraq

In this study, least square method (LSM) and differential transform method (DTM) applied to solve the three dimensional problem of steady nanofluid deposition on an inclined rotating disk is illustrated. The governing non-linear partial differential equations are reduced to the nonlinear ordinary differential equations system by similarity transform. There is a good agreement between the present analytical and numerical results. Results indicate that increasing nanofluid volume fraction leads to increase in temperature profile and highest temperature obtained for aluminium oxide (Al₂O₃)-water case. © 201., © 201. The Author(s). Published by Informa UK Limited, trading as Taylor & Francis Group on behalf of the University of Bahrain.

关键词： condensation film DTM film thickness LSM Nanofluid rotating disk

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Calcined [email protected] @Rh x Ni 1. x : A novel hierarchically oriented composition tunable catalyst for green and sustainable hydrogen generation

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Journal of Environmental Chemical engineering 2022年第3期10卷

作者： Yasir Abbas Zareen Zuhra Sahresh Majeed Muhammad Shuaib Khan Majid Basharat Deependra Tyagi Shafqat Ali Zhanpeng Wu Zhaojun Liu Department of Electrical and Electronic Engineering Southern University of Science and Technology 1088 Xueyuan Blvd Nanshan District Shenzhen 518055 PR China State Key Laboratory of Organic-Inorganic Composites Beijing University of Chemical Technology Beijing 100029 PR China Department of Environment and Civil Engineering Dongguan University of Technology Dongguan 523808 PR China Institute of Chemical Sciences Bahauddin Zakariya University Multan 60800 Pakistan International Research Center for Renewable Energy (IRCRE) State Key Laboratory of Multiphase Flow in Power Engineering (MPFE) Xi’an Jiaotong University Xi’an 710049 PR China Institute for Advanced Study Shenzhen University Nanhai Avenue 3688 Shenzhen 518060 PR China

The ever decreasing amount of fossil fuels and increasing environmental pollution are alarming threats for green and sustainable future. Designing a new catalyst is, therefore, of paramount significance in the quest to discover sustainable, robust, and environmentally benign materials for clean and sustainable energy generation. Herein, we developed a hierarchically oriented catalyst of calcined poly(ferrocenedimethano)-cyclotriphosphazene-microspheres (CPFC-MS) supported with nickel-aluminum layered double hydroxide and decorated with nanoparticles (NPs) of rhodium-nickel, [email protected] x Ni 1.- x ( x = 2.06–6.75), for H 2 generation from ammonia borane (AB) hydrolysis . The highly active catalyst was characterized by scanning electron microscopy (SEM), Raman spectroscopy , high-resolution transmission electron microscopy (HRTEM) and TEM, energy dispersive X-ray spectroscopy (EDX), fourier transform infrared (FTIR), X-ray diffraction (XRD), X-ray photoelectron spectroscopy (XPS). The as-fabricated [email protected] @Rh x Ni 1. x ( x = 2.06–6.75) catalysts were tested for AB hydrolysis and the results showed remarkable performance and higher stability for H 2 generation. The [email protected] @Rh 2.06 Ni 7.32 catalyst, having the lowest Rh-contents, exhibited maximum H 2 generation with a turn over frequency (TOF) of 780 mol H 2 hr −1.mol Rh −1.and an activation energy (E a ) of 40.3 kJ/mol with excellent sustainability . The superior activity is ascribed to the synergetic effect between RhNi NPs and their well-dispersion over hierarchically oriented [email protected] support, while higher stability due to LDH-AlNi/RhNi attractions. This work will provide new opportunities for polyphosphazenes and LDH derived hierarchically oriented sustainable catalysts for green energy production for sustainable future.

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Cover Feature: Hollow Carbon Sphere-Modified Graphitic Carbon Nitride for Efficient Photocatalytic H2Production (Chem. Eur. J. 68/2021.

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Chemistry – A European Journal 2021年第68期27卷

作者： Dr. Jinghua Li Dr. Lunqiao Xiong Dr. Bing Luo Prof. Dengwei Jing Dr. Jiamei Cao Prof. Junwang Tang International Research Center for Renewable Energy & State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an Shaanxi 710049 P. R. China Department of Chemical Engineering University College London London WC1E 7JE UK School of Chemical Engineering and Technology Xi'an Jiaotong University Xi'an Shaanxi 710049 P. R. China

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A mixed discontinuous galerkin method for linear elasticity with strongly imposed symmetry

arXiv

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arXiv 2019年

作者： Wang, Fei Wu, Shuonan Xu, Jinchao School of Mathematics and Statistics and State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an Shaanxi710049 China School of Mathematical Sciences Peking University Beijing100871 China Department of Mathematics Pennsylvania State University University ParkPA16802 United States

In this paper, we study a mixed discontinuous Galerkin (MDG) method to solve linear elasticity problem with arbitrary order discontinuous finite element spaces in d-dimension (d = 2, 3). This method uses polynomials of degree k + 1.for the stress and of degree k for the displacement (k > 0). The mixed DG scheme is proved to be well-posed under proper norms. Specifically, we prove that, for any k > 0, the H(div)-like error estimate for the stress and L2 error estimate for the displacement are optimal. We further establish the optimal L2 error estimate for the stress provided that the Pk+2 - P-1.k+1.Stokes pair is stable and k > d. We also provide numerical results of MDG showing that the orders of convergence are actually sharp.65N30, 65M60 Copyright © 201., The Authors. All rights reserved.

关键词： Galerkin methods

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Theoretical insights into the hydrophobicity of low index CeO2 surfaces

arXiv

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arXiv 2019年

作者： Fronzi, Marco N. Assadi, M. Hussein Hanaor, Dorian A.H. International Research Centre for Renewable Energy State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’anShaanxi710049 China 1-1 Namiki TsukubaIbaraki305-0044 Japan Chair of Advanced Ceramic Materials Institute for Materials Science and Technology Technische Universität Berlin Berlin10653 Germany

The hydrophobicity of CeO2 surfaces is examined here. Since wettability measurements are extremely sensitive to experimental conditions, we propose a general approach to obtain contact angles between water and ceria surfaces of specified orientations based on density functional calculations. In particular, we analysed the low index surfaces of this oxide to establish their interactions with water. According to our calculations, the CeO2 (1.1. surface was the most hydrophobic with a contact angle of Θ = 1.2.53° followed by (1.0) with Θ = 93.91.. The CeO2 (1.0) surface was, on the other hand, mildly hydrophilic with Θ = 64.09°. By combining our calculations with an atomistic thermodynamic approach, we found that the O terminated (1.0) surface was unstable unless fully covered by molecularly adsorbed water. We also identified a strong attractive interaction between the hydrogen atoms in water molecules and surface oxygen, which gives rise to the hydrophilic behaviour of (1.0) surfaces. Interestingly, the adsorption of water molecules on the lower-energy (1.1. surface stabilises oxygen vacancies, which are expected to enhance the catalytic activity of this plane. The findings here shed light on the origin of the intrinsic wettability of rare earth oxides in general and CeO2 surfaces in particular and also explain why CeO2 (1.0) surface properties are so critically dependant on applied synthesis methods. Copyright © 201., The Authors. All rights reserved.

关键词： Density functional theory

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