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Exploring seasonal variability in water quality of Nyabarongo River in Rwanda via water quality indices and DPSIR modelling

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Environmental Science and pollution Research 2024年第31期31卷 44329-44347页

作者： Umuhoza, Mycline Niu, Dongjie Li, Fengting College of Environmental Science and Engineering Tongji University 1239 Siping Rd. Shanghai200092 China State Key Laboratory of Pollution Control and Resource Reuse College of Environmental Science and Engineering Tongji University 1239 Siping Rd. Shanghai200092 China Shanghai Institute of Pollution Control and Ecological Security North Zhongshan Rd. 1515 Shanghai200092 China

Understanding seasonal variations in water quality is crucial for effective management of freshwater rivers amidst changing environmental conditions. This study employed water quality index (WQI), metal index (MI), and pollution indices (PI) to comprehensively assess water quality and pollution levels in Nyabarongo River of Rwanda. A dynamic driver-pressure-state-impact-response model was used to identify factors influencing quality management. Over 4 years (201.–2021., 69 samples were collected on a monthly basis from each of the six monitoring stations across the Nyabarongo River throughout the four different seasons. Maximum WQI values were observed during dry long (52.90), dry short (21.478), long rain (93.66), and short rain (37.4) seasons, classified according to CCME 2001.guidelines. Ion concentrations exceeded WHO standards, with dominant ions being HCO3- and Mg2+. Variations in water quality were influenced by factors such as calcium bicarbonate dominance in dry seasons and sodium sulfate dominance in rainy seasons. Evaporation and precipitation processes primarily influenced ionic composition. Metal indices (MI) exhibited wide ranges: long dry (0.2–433.0), short dry (0.1.1.4.3), long rain (0.1.223.7), and short rain (0.3–252.5). The hazard index values for Cu2+, Mn4+, Zn2+, and Cr3+ were below 1. ranging from 8.89E − 08 to 7.68E − 07 for adults and 2.30E − 07 to 5.02E − 06 for children through oral ingestion, and from 6.68E − 1. to 5.07E − 07 for adults and 6.61. − 09 to 2.54E − 06 for children through dermal contact. With a total carcinogenic risk of less than 1.for both ingestion and dermal contact, indicating no significant health risks yet send strong signals to Governmental management of the Nyabarongo River. Overall water quality was classified as marginal in long dry, poor in short dry, good in long rain, and poor again in short rain seasons. Graphical Abstract: (Figure presented.) © The Author(s), under exclusive licence to Springer-Verlag GmbH Ger

关键词： Rain

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Effects of straw returning on photochemical process and imidacloprid degradation in paddy water through a field experiment

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Carbon Research 2024年第1期3卷 1-12页

作者： Li, Mabo Zeng, Yu Fu, Qinglong Zhang, Mingyang Chen, Ning Wang, Yujun Zhou, Dongmei Fang, Guodong State Key Laboratory of Soil and Sustainable Agriculture Institute of Soil Science Chinese Academy of Sciences Nanjing210008 China University of Chinese Academy of Sciences Beijing100049 China School of Environmental Studies China University of Geosciences Wuhan430074 China State Key Laboratory of Pollution Control and Resource Reuse School of the Environment Nanjing University Nanjing210023 China

Straw returning is an important strategy for effectively using straw resources to improve soil fertility and quality,&#1.0;but the effects of this process on reactive intermediates (RIs) formation in paddy water are n... 详细信息

Straw returning is an important strategy for effectively using straw resources to improve soil fertility and quality, but the effects of this process on reactive intermediates (RIs) formation in paddy water are not fully explored. In this study, we conducted a field experiment to explore the effects of straw returning on RIs formation including triplet chromophoric dissolved organic matter (3CDOM*), hydroxyl radicals (•OH), and singlet oxygen (1.2) in paddy water. It was found that straw returning considerably increased the steady-{1. concentration of RIs, and the application of rice straw with 25% and 75% organic replacement ratio increased RIs concentration by 2.52 and 2.25 times, respectively. The optical spectroscopy, Fourier transform ion cyclotron resonance mass spectrometry (FT-ICR-MS) analysis and structural equation model showed that straw returning produces abundant humified and aromatic DOM containing fulvic acid, lignin and protein-like substances, which could induce more RIs under irradiation. In addition, straw returning significantly accelerated imidacloprid (IMD) degradation, yielding degradation products that were highly toxic to aquatic animals (i.e., fish and daphnia) but less toxic to aquatic plants (i.e., green algae). This study would offer an innovative viewpoint on the effects of straw returning on the photochemistry of paddy water and the naturally occurring abiotic degradation pathway of organic contaminants. © The Author(s) 2024.

关键词： Aquatic organisms

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Enhanced methane production from waste activated sludge by potassium ferrate combined with thermal hydrolysis pretreatment

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Environmental Science and pollution Research 2024年第33期31卷 45862-45874页

作者： Guo, Bing Zeng, Jiachen Hao, Yuchi Hu, Jiawei Li, Zhuo State Key Laboratory of Pollution Control and Resource Reuse College of Environmental Science & ampEngineering Tongji University 1239 Siping Road Shanghai200092 China CCCC National Engineering Research Center of Dredging Technology and Equipment Co. Ltd. Shanghai200082 China

Anaerobic digestion of waste activated sludge (WAS) was one of the directions of sludge treatment, but how to effectively improve the production of methane as a resource product of anaerobic digestion of sludge still needs further research. The study examined how the combination of potassium ferrate (PF) and thermal hydrolysis (TH) pretreatment affected methane production from sludge. The results demonstrated a positive synergistic effect on methane production with PF-TH pretreatment. Specifically, by employing a 0.05 g/g TSS (total suspended solids) PF in conjunction with TH at 80 °C for 30 min, the methane yield increased from 1.0.66 ± 0.92 to 232.73 ± 2.21.mL/g VSS (volatile suspended solids). The co-pretreatment of PF and TH has been substantiated by mechanism studies to effectively enhance the disintegration and biodegradability of sludge. Additionally, the variation of microbial community revealed an enrichment of active microorganisms associated with anaerobic digestion after treated with PF + TH, resulting in a total abundance increase from 1..87 to 20.45% in the PF + TH group. © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2024.

关键词： Anaerobic digestion

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Tuning the primary selective nanochannels of MOF thin-film nanocomposite nanofiltration membranes for efficient removal of hydrophobic endocrine disrupting compounds

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Frontiers of Environmental Science & Engineering 2022年第4期16卷 1-13页

作者： Ruobin Dai Hongyi Han Yuting Zhu Xi Wang Zhiwei Wang State Key Laboratory of Pollution Control and Resource Reuse Shanghai Institute of Pollution Control and Ecological SecuritySchool of Environmental Science and EngineeringTongji UniversityShanghai 200092China Tongji Architectural Design(Group)Co. Ltd.Environmental Engineering BranchShanghai 200092China

Metal organic framework(MOF)incorporated thin-film nanocomposite(TFN)membranes have the potential to enhance the removal of endocrine disrupting compounds(EDCs).In MOF-TFN membranes,water transport nanochannels include(i)pores of polyamide layer,(ii)pores in MOFs and(iii)channels around MOFs(polyamide-MOF interface).However,information on how to tune the nanochannels to enhance EDCs rejection is scarce,impeding the refinement of TFN membranes toward efficient removal of *** this study,by changing the polyamide properties,the water transport nanochannels could be confined primarily in pores of MOFs when the polyamide layer became ***,the improved rejection of EDCs was dependent on the water transport channels of the TFN *** low monomer concentration(i.e.,loose polyamide structure),the hydrophilic nanochannels of MIL-1.1.Cr)in the polyamide layer could not dominate the membrane separation performance,and hence the extent of improvement in EDCs rejection was relatively *** contrast,at high monomer concentration(i.e.,dense polyamide structure),the hydrophilic nanochannels of MIL-1.1.Cr)were responsible for the selective removal of hydrophobic EDCs,demonstrating that the manipulation of water transport nanochannels in the TFN membrane could successfully overcome the permeability and EDCs rejection *** results highlight the potential of tuning primary selective nanochannels of MOF-TFN membranes for the efficient removal of EDCs.

关键词： Porous metal organic framework Thin-film nanocomposite membrane Primary selective nanochannels Nanofiltration Endocrine disrupting compounds

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A Multi-Stage Green Barrier Strategy for the control of Global SARS-CoV-2 Transmission via Cold Chain Goods

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Engineering 2022年第2期8卷 13-16页

作者： Xu He Xinwang Liu Pan Li Panpan Wang Haijun Cheng Wenqian Li Boda Li Ting Liu Jun Ma State Key Laboratory of Urban Water Resource and Environment Harbin Institute of TechnologyHarbin 150090China State Key Laboratory of Pollution Control and Resource Reuse College of Environmental Science and EngineeringTongji UniversityShanghai 200092China

*** object-to-human transmission route of SARS-CoV-2 At the time of writing,coronavirus disease 201.(COVID-1.),which is caused by the severe acute respiratory syndrome coron-avirus 2(SARS-CoV-2),has been a global pandemic for more than a *** of 22 September 2021.the global cumulative incidence exceeds 229 million cases,and the number of deaths has exceeded 4.75 million[1..The current situation of epidemic prevention and control within the countries around the world can be roughly divided into two stages:the pandemic stage that the United {1.s,the United Kingdom,and India are still experiencing(as of 23 September 2021.newly reported cases in the last 24 h in the United {1.s,United Kingdom,and India are 202840,31.95,and 26964,respectively[1.);and the normalized epidemic pre-vention and control stage that countries such as China and New Zealand are currently in.

关键词： prevention Strategy Chain

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Biochar nanoparticles-mediated transport of organic contaminants in porous media: dependency on contaminant properties and effects of biochar aging

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Carbon Research 2023年第1期2卷 1-15页

作者： Ma, Pengkun Qi, Zhichong Wu, Xuan Ji, Rong Chen, Wei College of Environmental Science and Engineering Ministry of Education Key Laboratory of Pollution Processes and Environmental Criteria Tianjin Key Laboratory of Environmental Remediation and Pollution Control Nankai University Tianjin300350 China China Water Resources Beifang Investigation Design and Research Co. Ltd. Tianjin300222 China College of Chemistry and Chemical Engineering Henan Joint International Research Laboratory of Environmental Pollution Control Materials Henan University Kaifeng475004 China State Key Laboratory of Pollution Control and Resource Reuse School of the Environment Nanjing University Nanjing210023 China

Land application of biochar has been recommended as an effective soil amendment measure. Nonetheless, the applied biochar can accumulate co-existing contaminants. Meanwhile, nanoparticles formed due to biochar disintegration may facilitate contaminant transport in vadose zone and groundwater, posing a potential risk to the subsurface environment. Here, we show that the presence of pinewood- and rice straw-derived biochar nanoparticles (BCNPs) at parts per million level (~ 20 mg/L) can result in significant mobilization of hydrophobic, nonpolar contaminants (naphthalene and pyrene) and positively charged polar contaminants (trimethoprim and ciprofloxacin) in saturated sandy soil, but slightly inhibits the transport of negatively charged or neutral hydrophilic compounds (sulfamethoxazole and bisphenol A). With supplemental adsorption and desorption experiments we show that the ability of BCNPs in mediating contaminant transport (either enhancing or inhibiting) relies primarily on the extent of irreversible binding of a contaminant to the BCNPs. Sulfide reduction and leaching of organic carbon, two relatively mild (in terms of modification of physicochemical properties, e.g., surface O/C ratio) but widely occurring aging processes, facilitate co-transport of pyrene and bisphenol A with the BCNPs. However, this is mainly the result of increased mobility of the BCNPs (i.e., the carrier), rather than enhanced interactions between the BCNPs and the contaminants being carried. The findings underline the significant effects of BCNPs on the fate and transport of environmental contaminants, and further highlight the important role of aging in affecting environmental behaviors and effects of biochar materials. Graphical Abstract: [Figure not available: see fulltext.] © 2023, The Author(s).

关键词： Naphthalene

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Mechanisms of allicin exposure for the sludge fermentation enhancement:Focusing on the fermentation processes and microbial metabolic traits

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Journal of Environmental Sciences 2022年第5期34卷 253-264页

作者： Feng Wang Jingyang Luo Shiyu Fang Wenxuan Huang Yunqi Zhang Le Zhang Xiaoshi Cheng Wei Du Fang Fang Jiashun Cao Yang Wu Key Laboratory of Integrated Regulation and Resource Development on Shallow Lakes Ministry of EducationHohai UniversityNanjing 210098China College of Environment Hohai UniversityNanjing 210098China State Key Laboratory of Pollution Control and Resource Reuse School of Environmental Science and EngineeringTongji UniversityShanghai 200092China

As a frequently used product with antimicrobial activity,consumed allicin might be dis-charged and concentrated in waste-activated sludge(WAS).However,the influence of al-licin(as an exogenous pollutant)on WAS fermentation has not been clearly *** study aimed to disclose the impacts of allicin on volatile fatty acid(VFA)generation dur-ing WAS *** results showed that the appropriate presence of allicin(1. mg/g TSS)significantly enhanced the VFA yield(1.94 versus 575 mg COD/L in the control)with increased acetate proportion(24.3%).Further exploration found that allicin promoted WAS solubilization,hydrolysis and acidification *** analysis revealed that the {1. genes involved in extracellular hydrolysis metabolism(i.e.,CAZymes),mem-brane transport(i.e.,gtsA and ytfT),substrate metabolism(i.e.,yhdR and pfkC)and fatty acid synthesis(i.e.,accA and accD)were all highly *** also induced the bacteria to produce more signalling molecules and regulate cellular functions,thereby enhancing the microbial adaptive and regulatory capacity to the unfavourable ***,the variations in fermentative microbes and their contributions to the upregulation of func-tional genes(i.e.,ytfR,gltL,INV,iolD and pflD)for VFA generation were ***,the simultaneous stimulation of functional microbial abundances and metabolic activities contributed to VFA production in allicin-conditioned reactors.

关键词： Allicin Waste activated sludge(WAS) Anaerobic fermentation Metagenomic analysis Functional genes

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The response of structure and nitrogen removal function of the biofilm on submerged macrophytes to high ammonium in constructed wetlands

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Journal of Environmental Sciences 2024年第8期142卷 129-141页

作者： Xue Jiang Mengmeng Wang Shunqing Yang Di He Fei Fang Liuyan Yang State Key Laboratory of Pollution Control and Resource Reuse School of the EnvironmentNanjing UniversityNanjing 210023China School of Resources and Environment Anqing Normal UniversityAnqing 246133China

The ammonium exceedance discharge from sewage treatment plants has a great risk to the stable operation of subsequent constructed wetlands(CWs).The effects of high ammonium shocks on submerged macrophytes and epiphytic biofilms on the leaves of submerged macrophytes in CWs were rarely mentioned in previous *** this paper,the 1.S rRNA sequencing method was used to investigate the variation of the microbial communities in biofilms on the leaves of Vallisneria natans plants while the growth characteristics of *** plants were measured at different initial ammonium *** results demonstrated that the total chlorophyll and soluble sugar synthesis of *** plants decreased by 51.45%and 57.1.%,respectively,and malondialdehyde content increased threefold after8 days if the initial NH_(4)^(+)-N concentration was more than 5 mg/*** density,bacterial quantity,dissolved oxygen,and pH increased with high ammonium *** average removal efficiencies of total nitrogen and NH_(4)^(+)-N reached 73.26%and 83.94%,*** heat map and relative abundance analysis represented that the relative abundances of phyla Proteobacteria,Cyanobacteria,and Bacteroidetes *** numbers of autotrophic nitrifiers and heterotrophic nitrification aerobic denitrification(HNAD)bacteria expanded in *** particular,HNAD bacteria of Flavobacterium,Hydrogenophaga,Acidovorax,Acinetobacter,Pseudomonas,Aeromonas,and Azospira had higher abundances than autotrophic nitrifiers because there were organic matters secreted from declining leaves of *** *** analysis of the nitrogen metabolic pathway showed aerobic denitrification was the main nitrogen removal ***,the nitrification and denitrification bacterial communities increased in epiphytic biofilms on submerged macrophytes in constructed wetlands while submerged macrophytes declined under ammonium shock loading.

关键词： Ammonium shock loading Biofilm Autotrophic nitrifiers Heterotrophic nitrification aerobic denitrification bacteria Submerged macrophyte

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control of Effluent Organic Matter, Cytotoxicity, and Disinfection Byproducts in Wastewater with Biological Anion Exchange Resins: Enhanced Performance through Skeleton Design

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Environmental science & technology 2025年第22期59卷 2025 May 28页

作者： Xingqi Zhu Lu Jiang Ye-Chao Tian Yang Pan Wen-Tao Li Chendong Shuang Rong Ji Aimin Li State Key Laboratory of Pollution Control and Resource Reuse School of the Environment Nanjing University Nanjing 210023 Jiangsu China.

Effluent organic matter (EfOM) in wastewater threatens ecosystems and drinking water safety via the urban water cycle. Biofiltration using adsorbents with dual adsorption-biodegradation functions, such as biological anion exchange resins (BAERs), offers a promising solution. Compared to biological activated carbon (BAC), BAERs' adjustable skeletons enable targeted EfOM removal. This study designed two BAERs with polystyrene (PS-AER) and magnetic polyacrylic (MPA-AER) skeletons and compared them with conventional polyacrylic BAER (PA-AER) and BACs. During 1. 000-bed-volume field applications, BAERs demonstrated 1.7-2.6 and 1.6-2.6 times higher dissolved organic carbon (DOC) and UV removal rates than BACs. This efficacy stemmed from the high concentration of negatively charged components, which BAERs effectively attract. Furthermore, skeleton modifications improved DOC removal by 1..3-1..2% and UV removal by 7.3-1..2% for PS-AER and MPA-AER, compared to PA-AER. The MPA-AER's open pore structure enhanced diffusion of high molecular weight components, while PS-AER's enhanced hydrophobicity improved aromatic component removal. These structural changes also influenced the biological effects of BAERs. Notably, the enhanced performance of PS-AER and MPA-AER reduced wastewater cytotoxicity and controlled the production of disinfection byproducts. Overall, this study confirms the potential of BAERs in wastewater treatment and highlights strategies for performance enhancement through skeleton modification.

关键词： biological anion exchange resin disinfection byproducts (DBPs) effluent organic matter (EfOM) reclaimed wastewater wastewater

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Enhanced methane production during long-term UASB operation at high organic loads as enabled by the immobilized Fungi

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Frontiers of Environmental Science & Engineering 2022年第6期16卷 47-59页

作者： Qiong Guo Zhichao Yang Bingliang Zhang Ming Hua Changhong Liu Bingcai Pan State Key Laboratory of Pollution Control and Resource Reuse School of EnvironmentNanjing UniversityNanjing 210023China Research Center for Environmental Nanotechnology(ReCENT) Nanjing UniversityNanjing 210023China School of Life Sciences Nanjing UniversityState Key Laboratory of Pharmaceutical BiotechnologyNanjing 210023China

Anaerobic digestion is widely applied in organic wastewater treatment coupled with bioenergy production,and how to stabilize its work at the high organic loading rate(OLR)remains a ***,we proposed a new strategy to address this issue via involving the synergetic role of the Aspergillus sydowii 8L-9-F02 immobilized beads(AEBs).A long-term(21.-day)continuous-mode operation indicated that the upflow anaerobic sludge bed(UASB)reactor(R1.with AEBs added)could achieve the OLR as high as 25.0 kg/(m^(3)×d),whereas the control reactor(R0,with AEBs free)could only tolerate the maximum OLR of 1..3 kg/(m^(3)×d).Remarkably,much higher COD removal(85.9%vs 23.9%)and methane production(5.4 m^(3)/(m^(3)×d)vs 2.2 m^(3)/(m^(3)×d))were achieved in R1.than R0 at the OLR of 25.0 kg/(m^(3)×d).Such favorable effect results from the facts that fungi inhibit VFAs accumulation,favor the pH stabilization,promote the generation of more extracellular polymeric substance,and enhance the sludge granulation and ***,fungi may enhance the secretion of acetyl-coenzyme A,a {1. compound in converting organic matters to CO_(2).In addition,fungi are favorable to enrich methanogenic archaea even at high OLR,improving the activity of acetate kinase and coenzyme F_(420) for more efficient methanogenic *** work may shed new light on how to achieve higher OLR and methane production in anaerobic digestion of wastewater.

关键词： Anaerobic digestion Fungi Methane production High OLR Microbial community

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