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Hierarchical cobalt-molybdenum layered double hydroxide arrays power efficient oxygen evolution reaction

Nano Research 2024年第6期17卷 5080-5086页

作者： Xinyi Zhu Jiahui Lyu Shanshan Wang Xingchuan Li Xiaoyu Wei Cheng Chen Wanida Kooamornpattana Francis Verpoort Jinsong Wu Zongkui Kou State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China Sanya Science and Education Innovation Park of Wuhan University of Technology Sanya 572000China Nanostructure Research Center Wuhan University of TechnologyWuhan 430070China Department of Chemical Engineering Faculty of EngineeringMahidol UniversityNakhon Pathom 73170Thailand

Transition metal-based layered double hydroxides(LDHs)have been capable of working efficiently as catalysts in the basic oxygen evolution reaction(OER)for sustaining hydrogen production of alkaline water ***,exploring new LDH-based electrocatalysts featuring both remarkable activity and good stability is still in high demand,which is pivotal for comprehensive understanding and impressive improvement of the sluggish OER ***,a series of bimetallic(Co and Mo)LDH arrays were designed and fabricated via a facile and controlled strategy by incorporating a Mo source into presynthesized Co-based metal-organic framework(MOF)arrays on carbon cloth(CC),named as ZIF-67/CC *** found that tuning the Mo content resulted in gradual differences in the structural properties,surface morphology,and chemical states of the resulting catalysts,namely CoMox-LDH/CC(x representing the added weight of the Mo source).Gratifyingly,the best-performing CoMo_(0.20)-LDH/CC electrocatalyst demonstrates a low overpotential of only 226 mV and high stability at a current density of 10 mA·cm^(−2),which is superior to most LDH-based OER catalysts reported ***,it only required 1.611 V voltage to drive the overall water splitting device at the current density of 10 mA·cm^(−2).The present study represents a significant advancement in the development and applications of new OER catalysts.

关键词： layered double hydroxides(LDHs) metal-organic frameworks(MOFs) array catalysts Mo modification electrocatalytic oxygen evolution reaction(OER)

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Self-powered sensor based on compressible ionic gel electrolyte for simultaneous determination of temperature and pressure

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InfoMat 2024年第7期6卷 62-75页

作者： Junjie Zou Yanan Ma Chenxu Liu Yimei Xie Xingyao Dai Xinhui Li Shuxuan Li Shaohui Peng Yang Yue Shuo Wang Ce-Wen Nan Xin Zhang State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Center of Smart Materials and Devices&International School of Materials Science and EngineeringWuhan University of TechnologyWuhanthe People's Republic of China Hubei Key Laboratory of Energy Storage and Power Battery School of MathematicsPhysics and Optoelectronic EngineeringHubei University of Automotive TechnologyShiyanthe People's Republic of China Information Materials and Intelligent Sensing Laboratory of Anhui Province Key Laboratory of Structure and Functional Regulation of Hybrid Materials of Ministry of EducationInstitutes of Physical Science and Information TechnologyAnhui UniversityHefeithe People's Republic of China State Key Lab of New Ceramics and Fine Processing School of Materials Science and EngineeringTsinghua UniversityBeijingthe People's Republic of China

The simultaneous detection of multiple stimuli,such as pressure and temperature,has long been a persistent challenge for developing electronic skin(eskin)to emulate the functionality of human ***,the demand for integrated power supply units is an additional pressing concern to achieve its lightweightness and ***,we propose a self-powered dual temperature–pressure(SPDM)sensor,which utilizes a compressible ionic gel electrolyte driven by the potential difference between MXene and Al *** SPDM sensor exhibits a rapid and timely response to changes in pressure-induced deformation,while exhibiting a slow and hysteretic response to temperature *** distinct response characteristics enable the differentiation of current signals generated by different stimuli through machine learning,resulting in an impressive accuracy rate of 99.1%.Furthermore,the developed SPDM sensor exhibits a wide pressure detection range of 0–800 kPa and a broad temperature detection range of 5–75C,encompassing the environmental conditions encountered in daily human *** dual-mode coupled strategy by machine learning provides an effective approach for temperature and pressure detection and discrimination,showcasing its potential applications in wearable electronics,intelligent robots,human–machine interactions,and so on.

关键词： e-skin gel electrolyte machine learning self-powered dual-mode sensor

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Multifactor roadmap for designing low-power-consumed micro thermoelectric thermostats in a closed-loop integrated 5G optical module

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Interdisciplinary materials 2024年第2期3卷 326-337页

作者： Dongwang Yang Yubing Xing Jiang Wang Kai Hu Yani Xiao Kechen Tang Jianan Lyu Junhao Li Yutian Liu Peng Zhou Yuan Yu Yonggao Yan Xinfeng Tang State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhanChina Nanostructure Research Center Wuhan University of TechnologyWuhanChina Research Center for Materials Genome Engineering Wuhan University of TechnologyWuhanChina Institute of Physics(IA) RWTH Aachen UniversityAachenGermany

As the core components of fifth-generation(5G)communication technology,optical modules should be consistently miniaturized in size while improving their level of *** inevitably leads to a dramatic spike in power consumption and a consequent increase in heat flow density when operating in a confined *** ensure a successful start-up and operation of 5G optical modules,active cooling and precise temperature control via the Peltier effect in confined space is essential yet *** this work,p-type Bi_(0.5)Sb_(1.5)Te_(3)and n-type Bi_(2)Te_(2.7)Se_(0.3)bulk thermoelectric(TE)materials are used,and a micro thermoelectric thermostat(micro-TET)(device size,2×9.3×1.1mm^(3);leg size,0.4×0.4×0.5mm^(3);number of legs,44)is successfully integrated into a 5G optical module with Quad Small Form Pluggable 28 *** a result,the internal temperature of this kind of optical module is always maintained at 45.7℃ and the optical power is up to 7.4 ***,a multifactor design roadmap is created based on a 3D numerical model using the ANSYS finite element method,taking into account the number of legs(N),leg width(W),leg length(L),filling atmosphere,electric contact resistance(Rec),thermal contact resistance(Rtc),ambient temperature(Ta),and the heat generated by the laser source(QL).It facilitates the integrated fabrication of micro-TET,and shows the way to enhance packaging and performance under different operating *** to the roadmap,the micro-TET(2×9.3×1mm^(3),W=0.3 mm,L=0.4 mm,N=68 legs)is fabricated and consumes only 0.89W in cooling mode(Q_(L)=0.7W,T_(a)=80℃)and 0.36Win heating mode(T_(a)=0℃)to maintain the laser temperature of 50℃.This research will hopefully be applied to other microprocessors for precise temperature control and integrated manufacturing.

关键词： 5G optical module finite element simulation micro thermoelectric thermostat Peltier effect

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ZnO-based micromotors fueled by CO2: the first example of self-reorientation-induced biomimetic chemotaxis

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National Science Review 2021年第11期8卷 102-109页

作者： Fangzhi Mou Qi Xie Jianfeng Liu Shengping Che Lamya Bahmane Ming You Jianguo Guan State Key Laboratory of Advanced Technology for Materials Synthesis and Processing International School of Materials Science and EngineeringWuhan University of Technology

Synthetic chemotactic micro/nanomotors are envisioned to actively 'seek out' targets by following specific chemicals,but they are mainly powered by bioincompatible fuels and only show pseudochemotaxis（or advanced chemokinesis） due to their weak self-reorientation *** we demonstrate that synthetic ZnO-based Janus micromotors can be powered by the alternative biocompatible fuel of CO;2;,and further provide the first example of self-reorientation-induced biomimetic chemotaxis using *** ZnO-based micromotors are highly sensitive to dissolved CO;2;in water,which enables the corrosion of ZnO to continuously occur by providing H;+;through ***,they can autonomously move even in water exposed to air based on ***,they can sense the local CO;2;gradient and perform positive chemotaxis by self-reorientations under the phoretic *** discovery opens a gate to developing intelligent micro/nanomotors powered by,and sensitive to,biocompatible atmospheric or endogenous gaseous chemicals for biomedical and environmental applications.

关键词： micro/nanomotors zinc oxide carbon dioxide self-propulsion chemotaxis

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Bioinspired Additive Manufacturing of Hierarchical materials: From Biostructures to Functions

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Research 2024年第1期2023卷 533-559页

作者： Jingjiang Wei Fei Pan Hang Ping Kun Yang Yanqing Wang Qingyuan Wang Zhengyi Fu Institute for Advanced Materials Deformation and Damage from Multi-Scale Institute for Advanced StudyChengdu UniversityChengdu 610106P.R.China Department of Chemistry University of BaselBasel 4058Switzerland State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070P.R.China College of Polymer Science and Engineering Sichuan UniversityChengdu 610065P.R.China

Throughout billions of years,biological systems have evolved sophisticated,multiscale hierarchical structures to adapt to changing *** are synthesized under mild conditions through a bottom-up self-assembly process,utilizing substances from the surrounding environment,and meanwhile are regulated by genes and *** manufacturing,which mimics this natural process,provides a promising approach to developing new materials with advantageous properties similar to natural biological *** review presents an overview of natural biomaterials,emphasizing their chemical and structural compositions at various scales,from the nanoscale to the macroscale,and the key mechanisms underlying their ***,this review describes the designs,preparations,and applications of bioinspired multifunctional materials produced through additive manufacturing at different scales,including nano,micro,micro-macro,and macro levels.

关键词： materials structures utilizing

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Tristate ferroelectric memory in PZT-based films from antiferroelectric-ferroelectric phase transition

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Ceramics International 2025年第17期51卷 23680-23687页

作者： Liu, Yifei Hu, Yang Zhang, Huazhang Wang, Zhiqing Shen, Jie Wu, Zhi Chen, Wen Zhou, Jing State Key Laboratory of Advanced Technology for Materials Synthesis and Processing School of Materials Science and Engineering Wuhan University of Technology Wuhan430070 China Sanya Science and Education Innovation Park Wuhan University of Technology Hainan 572000 China School of Physics and Mechanics Wuhan University of Technology Wuhan430070 China School of Materials and Engineering Hunan Institute of Technology Hengyang421002 China

Ferroelectric random access memory (FeRAM) plays a vital role in information storage due to its unique advantages, driving the demand for high-capacity and high-density solutions. In this paper, a series of PbZr1-xTixO3 (x = 6 %, 8 %, 10 %, 12 %, 14 %) films were prepared using sol-gel and spin-coating methods. As the Ti content increases, the enhancement effect of the ferroelectric order is reflected structurally in XRD and Raman spectra, and electrically in the dielectric and ferroelectric properties. Notably, for x = 12 %, the P-E hysteresis loop exhibits slightly pinched and double-like, and the peaks of the I-V curve are split on both the positive and negative field sides. This ferroelectric behavior is caused by an underlying triple-well free-energy landscape, which is the basis of tristate ferroelectric memory. The measurement results show that the "±1" and "0" states of PbZr0.88Ti0.12O3 film under electric field cycling exhibit excellent programmability. It also achieves promising data retention up to 1000s and endurance up to 107 cycles. This investigation not only verifies the feasibility of applying tristate ferroelectric memory to PZT-based films but also provides a facile method for fabricating tristate ferroelectric memory devices. © 2025 Elsevier Ltd and Techna Group S.r.l.

关键词： Antiferroelectric Ferroelectric Phase transition PZT Tristate ferroelectric memory

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Hybrid ionic/electronic interphase enabling uniform nucleation and fast diffusion kinetics for stable lithium metal anode

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Chinese Chemical Letters 2024年第2期35卷 626-633页

作者： Lun Li Pengxia Ji Meng Huang Zixin Zhang Hong Wang Francis Verpoort Jinlong Yang Daping He State Key Laboratory of Advanced Technology for Materials Synthesis and Processing School of Materials Science and EngineeringWuhan University of TechnologyWuhan 430070China Guangdong Research Center for Interfacial Engineering of Functional Materials College of Materials Science and EngineeringShenzhen UniversityShenzhen 518060China Sanya Science and Education Innovation Park of Wuhan University of Technology Sanya 572000China Hubei Engineering Research Center of RF-Microwave Technology and Application Wuhan University of TechnologyWuhan 430070China State Key Laboratory of Silicate Materials for Architectures Wuhan University of TechnologyWuhan 430070China

Lithium(Li)dendrite issue,which is usually caused by inhomogeneous Li nucleation and fragile solid electrolyte interphase(SEI),impedes the further development of high-energy Li metal ***,the integrated construction of a high-stable SEI layer that can regulate uniform nucleation and facilitate fast Li-ion diffusion kinetics for Li metal anode still falls ***,we designed an artificial SEI with hybrid ionic/electronic interphase to regulate Li deposition by in-situ constructing metal Co clusters embedded in LiF *** generated Co and LiF both enable fast Li-ion diffusion kinetics,meanwhile,the lithiophilic properties of Co clusters can serve as Li-ion nucleation sites,thereby contributing to uniform Li nucleation and non-dendritic *** a result,a dendrite-free Li deposition with a low overpotential(16.1 mV)is achieved,which enables an extended lifespan over 750 h under strict *** full cells with high-mass-loading LiFePO_(4)(11.5 mg/cm^(2))as cathodes exhibit a remarkable rate capacity of 84.1 mAh/g at 5 C and an improved cycling performance with a capacity retention of 96.4%after undergoing 180 cycles.

关键词： Lithium metal anode Hybrid ionic/electronic interphase Solid electrolyte interphase Fast diffusion kinetics Dendritic growth of lithium

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Improvement of AlN Thermal Conductivity Based on Reductive Compound Additives

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Journal of Wuhan University of technology(materials Science) 2023年第5期38卷 1025-1033页

作者： LI Meijuan WANG Chuanyi WANG Gaoqiang WANG Chuanbin SHEN Qiang State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China School of Chemistry Chemical Engineering and Life SciencesWuhan University of TechnologyWuhan 430070China Nanchong Three-circle Electronics Co.LTD. Nanchong 637100China

AlN ceramics were prepared by plasma activation sintering(PAS)with compound additives yttrium acetylacetonate(Y(acac)_(3))and melamine(C_(3)H_(6)N_(6)).The effects of compound additives on the microstructure,density,and thermal properties of Al N ceramic were studied.Y(acac)3and C_(3)H_(6)N_(6)can form Y_(2)O_(3),residual organic carbon and reducing gas during the heating process,which improves the Al N sintering performance at a temperature of 1700℃and the bulk thermal *** the content of Y(acac)_(3)is 10 wt%and C_(3)H_(6)N_(6)is 3 wt%,the thermal conductivity of Al N ceramics is 105.6 W/(m·K),which is much higher than that of Al N ceramics with Y_(2)O_(3)under the same sintering *** work provides theoretical reference for the preparation of high-performance Al N ceramic.

关键词： reductive compound additives AlN ceramic thermal conductivity:plasma activated sintering

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Catalytic hosts with strong adsorption strength for long shelf-life lithium-sulfur batteries under lean electrolyte

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Nano Research 2023年第1期16卷 427-438页

作者： Siyuan Zhao Huayu Pei Quan Yang Kangli Liu Yuanyuan Huang Zhuo Wang Guosheng Shao Jinping Liu Junling Guo State Center for International Cooperation on Designer Low-carbon&Environmental Materials School of Materials Science and EngineeringZhengzhou UniversityZhengzhou 450001China Zhengzhou Materials Genome Institute Xingyang 450100China School of Chemistry Chemical Engineering and Life ScienceState Key Laboratory of Advanced Technology for Materials Synthesis and ProcessingWuhan University of TechnologyWuhan 430070China

Low electrolyte/sulfur ratio(E/S)is an important factor in increasing the energy density of lithium-sulfur batteries(LSBs).Recently,the E/S has been widely lowered using catalytic hosts that can suppress“shuttle effect”during cycling by relying on a limited adsorption ***,the shelf-lives of these cathodes have not yet received ***,we show that the selfdischarge of sulfur cathodes based on frequently-used catalytic hosts is serious under low E/S because the“shuttle effect”during storage process caused by polysulfides(PSs)disproportionation cannot be suppressed using a limited adsorption *** further prove that the adsorption strength toward PSs,which is unfortunately weak in commonly-used catalytic hosts,is critical for effectively hindering the disproportionation of the ***,to verify this conclusion,we prepare a sulfur-doped titanium nitride(S-TiN)catalytic array *** the adsorption strength and catalytic activity of TiN can be improved by S doping simultaneously,the constructed S/S-TiN cathodes under a low E/S(6.5μL·mg−1)exhibit better shelf-life and cycle-stability than those of S/TiN *** work suggests that enhancing the adsorption strength of catalytic hosts,while maintaining their function to reduce E/S,is crucial for practical LSBs.

关键词： lithium-sulfur battery low electrolyte/sulfur ratio(E/S) self-discharge catalytic host adsorption strength

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Chiral effect on Aβ fibrillation from molecular-scale to nanoscale

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Nano Research 2022年第7期15卷 6721-6729页

作者： Guanbin Gao Guowei Zhu Liangchong Yu Zijun Zhang Ting Zhang Xinglin Liu Cheng Zhang Lin Zhou Taolei Sun State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China School of Chemistry Chemical Engineering and Life ScienceWuhan University of TechnologyWuhan 430070China

β-Amyloid(Aβ)peptide fibrillation,one of the characteristic hallmarks of Alzheimer’s disease,is determined by many interfacial physical-chemical factors,e.g.,charge,hydrophobicity,*** extensive research,chiral effect in different-scales on the fibrillation process of Aβremains ***,molecular-scale,sub-nanoscale,and nanoscale chiral-structures were constructed to investigate their chiral effect on the fibrillation of Aβ_(40) *** structures from molecular-scale to nanoscale were obtained from the different periods of the chemosynthesis process of chiral ZnS quantum-dots(QDs),confirmed by real-time monitoring of circular dichroism *** molecular-scale,both L-penicillamine(L-P)and D-P ligands accelerated the fibrillation of Aβ_(40),and the speed-up effect of D-P was slightly stronger than *** sub-nanoscale,both two chiral Zncomplexes(L-Zn and D-Zn)induced the agglomeration of Aβ_(40) without chirality *** nanoscale,both L-ZnS and DZnS QDs inhibited the fibrillation of Aβ_(40),and the inhibition effect of L-ZnS was notably better than that of ***-situ kinetics experiments of Aβ_(40) co-incubated with two chiral QDs demonstrated that L-ZnS completely prevents the misfolding of Aβ_(40) from unfolded toβ-sheet,while D-ZnS cannot achieve *** site-replacement experiments and simulation results revealed the underlying molecular mechanisms of the different inhibition efficiency of chiral ZnS QDs on Aβ_(40) fibrillation,which mainly attribute to the stereoselectivity interaction between the chiral ligands of ZnS QDs and electro-positive amino acid residues(R5,K16,and K28)of Aβ_(40).This work offers a microscopic insight of chiral effect on Aβfibrillation exerted by structures in different-scales,and provides a guidance in precise regulation of protein fibrillation via manipulating chiral structures in different-scales.

关键词： chirality molecular-scale sub-nanoscale nanoscale Aβ_(40) fibrillation

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