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Hot-exciton effects on exciton diffusion and circular polarization dynamics in a single PbI_(2)nanoflake

science China(Technological sciences) 2024年第1期67卷 83-90页

作者： XU ChenYu WANG Lei CUI Lin GAO BingRong WANG HaiYu State Key Laboratory of Integrated Optoelectronics College of Electronic Science and EngineeringJilin UniversityChangchun 130012China

As one of the emerging two-dimensional lead halide materials,lead iodide(PbI_(2))nanosheets have proven to possess strong application potential in the fields of high-energy radiation detection and highly efficient perovskite solar ***,the underlying photophysical properties such as hot-exciton-related carrier dynamics remain unclear for PbI_(2)***,we report the exciton dynamics of a single PbI_(2)nanoflake prepared by an aqueous solution *** a three-dimensional(3D)diffusion model,we obtain the exciton annihilation radius and diffusion coefficient of a single PbI_(2)nanoflake under nonresonant and resonant excitation conditions of band-edge exciton *** initial exciton densities increase,we find the carrier recombination mechanism for a single PbI_(2)nanoflake gradually changes from exciton-exciton annihilation to free-carrier ***,we reveal the room-temperature circular polarization of a single PbI_(2)nanoflake is due to free-carrier recombination with a band-edge exciton dissociation time of~120 fs under the resonant excitation condition.

关键词： single PbI_(2)nanoflake exciton diffusion room-temperature circular polarization ultrafast spectroscopy

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Transient features of graphitization and nitrogen-vacancy color centers in a diamond fabricated by localization femtosecond laser direct writing

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science China(Technological sciences) 2024年第8期67卷 2530-2536页

作者： CUI Lin YIN SiYu HU ZiFan WANG Lei State Key Laboratory of Integrated Optoelectronics College of Electronic Science and EngineeringJilin UniversityChangchun 130012China

Femtosecond laser direct writing provides an efficient approach to fabricating single nitrogen vacancy(NV) color centers with a relatively high yield. Different from previously reported NV color centers with a random distribution in a bulk diamond or nanocrystals, this gives an opportunity to study the photophysical properties of single NV color centers with precise numbers and positions. However, ultrafast studies on single NV color centers prepared by localization femtosecond laser direct writing are still rare, especially for the graphitization inside a diamond and its relationship with single NV color centers. Here, we report the broadband transient absorption(TA) spectroscopic features of the graphitization and NV color centers in a diamond fabricated by localization femtosecond laser direct writing at room temperature under 400 nm excitation. In comparison with the graphene oxide film, the bleaching features of the graphitization point array in a diamond are similar to reduced graphene oxide,accompanied by excited state absorption signals from local carbon atom vacancy defects in graphene-like structures induced by laser writing. On the other hand, transient features of laser processing array containing single NV color centers with a yield of~50% are different from those of the graphitization point array. Our findings suggest that for ultrashort pulse processing of diamonds, broadband TA spectral signals are sensitive to the surrounding atomic environment of processing sites, which could be applied to laser writing point defects in other materials used as solid-state single photon sources.

关键词： nitrogen-vacancy color center graphitization diamond femtosecond laser direct writing ultrafast spectroscopy

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Nano-effect enhanced cooperative luminescence of Yb^(3+) clusters in bulk materials

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Journal of Rare Earths 2024年第3期42卷 473-478,I0002页

作者： Daguang Li Jiahao Cui Yanhui Dong Hao Cui Dan Zhao Weiping Qin State Key Laboratory on Integrated Optoelectronics College of Electronic Science and EngineeringJilin UniversityChangchun130012China

In order to improve the multi-ion cooperative transition, we proposed and exploited a novel nanoscale effect, namely the nanoshell effect in bulk materials. Based on the effect, an optimal material structure was designed by coating the surfaces of Ca F_(2):Yb^(3+)micron size particles with ZrO_(2). An about 2 times higher intensity of cooperative luminescence is observed upon laser excitation at 980 nm. Dynamical analysis exhibits that the novel effect plays a key role in improving the performance of cooperative transitions. Our results also suggest that the nanoshell effect in bulk materials is likely to be significant in some special cases, which have not been reported yet in the literature.

关键词： Yb^(3+)cluster ZrO_(2) Nanoshell Enhancement Cooperative luminescence Rare earths

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Multipole higher-order topology in a multimode lattice

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Physical Review B 2024年第20期109卷 L201122-L201122页

作者： Maxim Mazanov Anton S. Kupriianov Roman S. Savelev Zuxian He Maxim A. Gorlach School of Physics and Engineering State Key Laboratory of Integrated Optoelectronics College of Electronic Science and Engineering International Center of Future Science

We put forward a two-dimensional multipolar higher-order topological insulator whose properties originate from the interference of the degenerate modes of the meta-atoms. This system features disorder-robust corner modes and cannot be reduced to the known crystalline topological phases, providing the example of multipolar topology in a C3-symmetric lattice. The multimode nature of the lattice gives rise to flat bands and corner states with extreme localization. We assemble the designed structure, observe multipolar topological corner states experimentally, and demonstrate their coherent control.

关键词： Topological effects in photonic systems Topological insulators Waveguide arrays Microwave techniques Tight-binding model

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Effect of annealing on the electrical performance of N-polarity GaN Schottky barrier diodes

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Journal of Semiconductors 2024年第4期45卷 48-55页

作者： Nuo Xu Gaoqiang Deng Haotian Ma Shixu Yang Yunfei Niu Jiaqi Yu Yusen Wang Jingkai Zhao Yuantao Zhang State Key Laboratory of Integrated Optoelectronics College of Electronic Science and EngineeringJilin UniversityChangchun 130012China

A nitrogen-polarity(N-polarity)GaN-based high electron mobility transistor(HEMT)shows great potential for high-fre-quency solid-state power amplifier applications because its two-dimensional electron gas(2DEG)density and mobility are mini-mally affected by device ***,the Schottky barrier height(SBH)of N-polarity GaN is *** leads to a large gate leakage in N-polarity GaN-based *** this work,we investigate the effect of annealing on the electrical characteristics of N-polarity GaN-based Schottky barrier diodes(SBDs)with Ni/Au *** results show that the annealing time and tem-perature have a large influence on the electrical properties of N-polarity GaN *** to the N-polarity SBD without annealing,the SBH and rectification ratio at±5 V of the SBD are increased from 0.51 eV and 30 to 0.77 eV and 7700,respec-tively,and the ideal factor of the SBD is decreased from 1.66 to 1.54 after an optimized annealing *** analysis results suggest that the improvement of the electrical properties of SBDs after annealing is mainly due to the reduction of the inter-face state density between Schottky contact metals and N-polarity GaN and the increase of barrier height for the electron emis-sion from the trap state at low reverse bias.

关键词： nitrogen polarity GaN Schottky barrier diodes annealing interface state

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The second near-infrared (NIR-II) window excitable/emissive organic/polymeric fluorescent molecules for bioimaging application

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Journal of Innovative Optical Health sciences 2025年第3期18卷 25-43页

作者： Guannan Liu Chenguang Wang Geyu Lu State Key Laboratory of Integrated Optoelectronics Key Laboratory of Advanced Gas Sensors of Jilin Province College of Electronic Science and Engineering Jilin UniversityChangchunP.R.China

The fluorescence imaging (FLI) in the second near-infrared window (NIR-II, 1000–1700nm) has attracted considerable attention in the past decade. In contrast to conventional NIR-I window excitation (808nm/980nm), FLI with NIR-II window excitation (1064nm/other wavelength beyond 1000nm) can afford deeper tissue penetration depth with high clarity due to the merits of suppressed photon scattering and diminished autofluorescence. In this review, we have summarized NIR-II window excitable/emissive organic/polymeric fluorophores recently developed. The characteristics of these fluorophores such as chemical structures and photophysical properties have also been critically discussed. Furthermore, the latest development of noninvasive in vivo FLI with NIR-II excitation was highlighted. The ideal imaging results emphasized the importance of NIR-II excitation of these fluorophores in enabling deep tissue penetration and high-resolution imaging. Finally, a perspective on the challenges and prospects of NIR-II excitable/emissive organic/polymeric fluorophores was also discussed. We expected this review will be served as a source of inspiration for researchers, stimulating the creation of novel NIR-II excitable fluorophores and fostering the development of bioimaging applications.

关键词： Fluorescence imaging near-infrared excitation wavelength organic fluorophores conjugated polymers

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Novel broad spectral response perovskite solar cells:A review of the current status and advanced strategies for breaking the theoretical limit efficiency

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Journal of Materials science & Technology 2023年第9期140卷 33-57页

作者： Bin Liu Yuqi Wang Yanjie Wu Biao Dong Hongwei Song State Key Laboratory on Integrated Optoelectronics College of Electronic Science and EngineeringJilin UniversityChangchun 130012China

Perovskite solar cells(PSCs)have revolutionized photovoltaic *** power conversion efficiency(PCE)of PSCs has now reached 25.7%,which is comparable to current state-of-the-art silicon-based ***,PSCs can only utilize light of 300-850 nm,resulting in wasted near-infrared(NIR)light,which occupies 45%-50%of entire solar spectrum,which is one of the main reasons limiting the development of *** strategies to broaden NIR spectroscopy to break the theoretical limit efficiency of PSCs have recently attracted extensive *** review firstly outlines theoretical basis for improving the NIR spectroscopy,then systematically summarizes some key strategies and research progress to improve NIR spectroscopy of *** firstly provided a comprehensive overview of historical research experiments on narrow-gap perovskite absorber layers,rare earth up-conversion,tandem devices,and integrated perovskite/organic solar cells and given constructive suggestions for exceeding limit efficiency of ***,based on the development status of PSCs with NIR utilization,the current issues,solutions and future development directions of important aspects to improve NIR utilization of PSCs are systematically *** review lays the foundation for the efficiency of PSCs beyond the Shockley-Queisser limit,and provides a certain development prospect.

关键词： Organic materials Up-conversion materials Perovskite solar cells Tandem cells integrated perovskite/organic heterojunction solar cells

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Multifunctional interfacial molecular bridge enabled by an aggregation-induced emission strategy for enhancing efficiency and UV stability of perovskite solar cells

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Journal of Energy Chemistry 2024年第8期95卷 588-595,I0013页

作者： Shuhang Bian Yuqi Wang Fancong Zeng Zhongqi Liu Bin Liu Yanjie Wu Long Shao Yongzhi Shao Huan Zhang Shuainan Liu Jin Liang Xue Bai Lin Xu Donglei Zhou Biao Dong Hongwei Song State Key Laboratory on Integrated Optoelectronics College of Electronic Science and EngineeringJilin UniversityChangchun 130012JilinChina College of Science Shanghai UniversityShanghai 200444China

The interface defects between the electron transport layer(ETL)and the perovskite layer,as well as the low ultraviolet(UV)light utilization rate of the perovskite absorption layer,pose significant challenges for the commercialization of perovskite solar cells(PSCs).To address this issue,this paper proposes an innovative multifunctional interface modulation strategy by introducing aggregation-induced emission(AIE)molecule 5-[4-[1,2,2-tri[4-(3,5-dicarboxyphenyl)phenyl]ethylene]phenyl]benzene-1,3-dicarboxylic acid(H_(8)ETTB)at the SnO_(2)ETL/perovskite ***,the interaction of H_(8)ETTB with the SnO_(2)surface,facilitated by its carboxyl groups,is effective in passivating surface defects caused by noncoord inated Sn and O *** interaction enhances the conductivity of the SnO_(2)film and adjusts energy levels,leading to enhanced charge carrier ***,H_(8)ETTB can passivate noncoord inated Pb^(2+)ions at the perovskite interface,promoting perovskite crystallization and reducing the interface energy barrier,resulting in a perovskite film with low defects and high crystalline *** importantly,the H_(8)ETTB molecule,can convert UV light into light absorbable by the perovskite,thereby reducing damage caused by UV light and improving the device's utilization of ***,the champion PSC based on SnO_(2)-H_(8)ETTB achieves an impressing efficiency of 23.32%and significantly improved photostability compared with the control device after continuous exposure to intense UV *** addition,the Cs_(0.05)(FA_(0.95)MA_(0.05))_(0.95)Pb(I_(0.95)Br_(0.05))_(3)based device can achieve maximum efficiency of 24.01%,demonstrating the effectiveness and universality of this ***,this innovative interface bridging strategy effectively tackles interface defects and low UV light utilization in PSCs,presenting a promising approach for achieving highly efficient and stable PSCs.

关键词： Perovskite solar cells Aggregation-induced emission Defect passivation Efficiency UV stability

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Ship Weather Routing Based on Hybrid Genetic Algorithm Under Complicated Sea Conditions

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Journal of Ocean University of China 2023年第1期22卷 28-42页

作者： ZHOU Peng ZHOU Zheng WANG Yan WANG Hongbo State Key Laboratory on Integrated Optoelectronics College of Electronic Science and EngineeringJilin UniversityJilin 130012China

Considering the effects of increased economic globalization and global warming,developing methods for reducing shipping costs and greenhouse gas emissions in ocean transportation has become *** to its key role in modern navigation technology,ship weather routing is the research focus of several scholars in this *** study presents a hybrid genetic algorithm for the design of an optimal ship route for safe transoceanic navigation under complicated sea *** the basis of the basic genetic algorithm,simulated annealing algorithm is introduced to enhance its local search ability and avoid premature convergence,with the ship’s voyage time and fuel consumption as optimization ***,a mathematical model of ship weather routing is developed based on the grid system.A measure of fitness calibration is proposed,which can change the selection pressure of the algorithm as the population *** addition,a hybrid crossover operator is proposed to enhance the ability to find the optimal solution and accelerate the convergence speed of the ***,a multi-population technique is applied to improve the robustness of the algorithm using different evolutionary strategies.

关键词： genetic algorithm simulated annealing algorithm weather routing ship speed loss

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Upconversion-based chiral nanoprobe for highly selective dual-mode sensing and bioimaging of hydrogen sulfide in vitro and in vivo

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Light(science & Applications) 2024年第9期13卷 1878-1887页

作者： Yang Lu Xu Zhao Dongmei Yan Yingqian Mi Peng Sun Xu Yan Xiaomin Liu Geyu Lu State Key Laboratory of Integrated Optoelectronics College of Electronic Science and EngineeringJilin University130012 ChangchunChina Department of Immunology College of Basic Medical SciencesJilin University130021 ChangchunChina

Chiral assemblies have become one of the most active research areas due to their versatility,playing an increasingly important role in bio-detection,imaging and *** this work,chiral UCNPs/CuxOS@ZIF nanoprobes are prepared by encapsulating upconversion nanoparticles(UCNPs)and CuxOS nanoparticles(NPs)into zeolitic imidazolate framework-8(ZIF-8).The novel excited-state energy distribution-modulated upconversion nanostructure(NaYbF4@-NaYF4:Yb,Er)is selected as the fluorescence source and energy donor for highly efficient fluorescence resonance energy transfer(FRET).CuxOS NP is employed as chiral source and energy acceptor to quench upconversion luminescence(UCL)and provide circular dichroism(CD)*** the natural adsorption and sorting advantages of ZIF-8,the designed nanoprobe can isolate the influence of other common disruptors,thus achieve ultra-sensitive and highly selective UCL/CD dual-mode quantification of H2S in aqueous solution and in living ***,the nanoprobe is also capable of in vivo intra-tumoral H2S *** work highlights the multifunctional properties of chiral nanocomposites in sensing and opens a new vision and idea for the preparation and application of chiral nanomaterials in biomedical and biological analysis.

关键词： chiral sulfide donor

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