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Black Phosphorus-Organic Framework-Derived Pei/Peg Nanohybrid Prepared by a One-Pot Method for a Wide Detection Range Co2 Gas Sensor

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SSRN 2022年

作者： Liu, Lulu Sang, Shengbo Han, Dan Liu, Zhihua Han, Xiaomei Li, Donghui Chen, Yi Liu, Dongming Liu, Xiaoru Zhuo, Kai Cheng, Yongqiang Yang, Kun Shanxi Key Laboratory of Micro Nano Sensors & Artificial Intelligence Perception College of Information and Computer Taiyuan University of Technology Taiyuan030024 China Key Lab of Advanced Transducers and Intelligent Control System of the Ministry of Education Taiyuan University of Technology Taiyuan030024 China Key Laboratory of Interface Science and Engineering in Advanced Materials Taiyuan University of Technology Ministry of Education Taiyuan030024 China

In this paper, we report a hybrid PEI/PEG-BP sensor (composite material of black phosphorus-organic framework-derived PEI/PEG nanohybrid) prepared by a one-pot method, in which the existence of PEI/PEG onto BP was confirmed by SEM, EDS, XPS and UPS. The gas sensing properties of the PEI/PEG-BP sensor, including the sensor response, response/recovery times, repeatability, selectivity, and effects of humidity on the sensor, were studied by exposure to several CO 2 gas concentrations ranging from 200 ppm to 300,000 ppm at room temperature (25 ℃). The results show that the PEI/PEG-BP sensor had an extremely wide detection range, with lower and upper detection limits of 200 ppm and 160,000 ppm, respectively. The response of the PEI/PEG-BP sensor to 200 ppm, and 160,000 ppm CO 2 gas at room temperature ( RT ) was 4.48%, and 254.02%, respectively, showing fast response/recovery time, excellent repeatability and high selectivity. The gas-sensing properties of the PEI/PEG-BP sensor are better than BP, PEI, PEG, PEI-BP and PEG-BP sensors. The superior properties of the PEI/PEG-BP sensor can be attributed to the BP framework, porous structure, electron doping, and surface reactive groups such as -NH 2 and -OH. The PEI/PEG-BP sensor, with its excellent gas-sensing performance will help us to further explore the changes of CO 2 concentration in microbial growth systems, natural environments, industrial production and so on. © 2022, The Authors. All rights reserved.

关键词： Carbon dioxide

A Novel Sensitization Mechanism of Stress-Electric-Coupled Biosensor Originated in Magnetostrictive Effect

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SSRN 2022年

作者： Sang, Shengbo Ge, Yang Ji, Jianglong Yuan, Zhongyun Dong, Xiushan Zhou, Chuangang Xiao, Pengli Tan, Qiuyun Zhao, Dong MicroNano System Research Center Key Lab of Advanced Transducers and Intelligent Control System The Ministry of Education College of Information and Computer Taiyuan University of Technology Taiyuan030024 China School of Electrical Engineering College of Engineering Science Hanyang University Seoul04763 Korea Republic of Shanxi Bethune Hospital Taiyuan030024 China Six-dimensional Artificial Intelligence Biomedical Research Institute Taiyuan030024 China

The stress-electric coupling based on receptor functionalization provides a new paradigm for the development of biosensor. However, the gravity factor of sensitive element usually shows difficult to be avoided due to its suppression to biosensor sensitivity. Herein, a magnetic-sensitization biosensing system with multi-physical field coupling of stress, magnetism and electricity was proposed to highly detect biomolecules. The gravitational interference of sensitive membrane was conquered by doping the TbDyFe with magnetostrictive effect into polydimethylsiloxane (PDMS) and applying magnetic field, showing great contributions to magnetic sensitization. The magnetic sensitization of the biosensor was proved by the collaboration of experiment and simulation. The detections of urine protein and urine sugar associated with kidney disease were realized with limits of detection (LOD) of 0.21 ng/mL and 0.45 nM by using the magnetic-sensitization biosensor. The prepared biosensor exhibited the high specificity, selectivity, stability and repeatability. Especially, the HSA and glucose in real samples can be accurately detect, showing good practicability of the prepared biosensor. This study provides a way to improve the sensitivity of the mechanical biosensor. © 2022, The Authors. All rights reserved.

关键词： Silicones

Physical-layer key distribution using synchronous complex dynamics of DBR semiconductor lasers

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arXiv

arXiv 2023年

作者： Wang, Anbang Du, Yicheng Li, Qingtian Wang, Longsheng Jia, Zhiwei Qin, Yuwen Wang, Yuncai Institute of Advanced Photonics Technology School of Information Engineering Guangdong University of Technology Guangzhou51006 China Key Laboratory of Photonic Technology for Integrated Sensing and Communication Ministry of Education of China Guangdong University of Technology Guangzhou51006 China Guangdong Provincial Key Laboratory of Information Photonics Technology Guangdong University of Technology Guangzhou51006 China Key Lab of Advanced Transducers and Intelligent Control System Ministry of Education Taiyuan University of Technology Taiyuan030024 China College of Optoelectronics Taiyuan University of Technology Taiyuan030024 China

Common-signal-induced synchronization of semiconductor lasers with optical feedback inspired a promising physical key distribution with information-theoretic security and potential in high rate. A significant challenge is the requirement to shorten the synchronization recovery time for increasing key rate without sacrificing operation parameter space for security. Here, open-loop synchronization of wavelength-tunable multi-section distributed Bragg reflector (DBR) lasers is proposed as a solution for physical-layer key distribution. Experiments show that the synchronization is sensitive to two operation parameters, i.e., currents of grating section and phase section. Furthermore, fast wavelength-shift keying synchronization can be achieved by direct modulation on one of the two currents. The synchronization recovery time is shortened by one order of magnitude compared to close-loop synchronization. An experimental implementation is demonstrated with a final key rate of 5.98 Mbit/s over 160 km optical fiber distance. It is thus believed that fast-tunable multi-section semiconductor lasers opens a new avenue of high-rate physical-layer key distribution using laser synchronization. Copyright © 2023, The Authors. All rights reserved.

关键词： Synchronization

Tuning Electrical Conductivity and Ultrafast Optical Nonlinearity of R-Go Films Ablated by Femtosecond Laser Direct Writing

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SSRN 2024年

作者： Tao, Youliang Nie, Zhongquan Zhang, Xuefeng Pan, Deng Wang, Han College of Aeronautics and Astronautics Taiyuan University of Technology Taiyuan030024 China Key Lab of Advanced Transducers and Intelligent Control System Ministry of Education and Shanxi Province College of Electronic Information and Optical Engineering Taiyuan University of Technology Taiyuan030024 China Institute of New Carbon Materials College of Materials Science and Engineering Taiyuan University of Technology Taiyuan030024 China Information Materials and Intelligent Sensing Laboratory of Anhui Province Anhui University 111 Jiu Long Road Hefei230601 China

Carbon-based nanomaterials with excellent electrical and optical properties are highly sought after for a plethora of hybrid applications ranging from advanced opto-electronic components to sustainable energy storage devices. In this contribution, we examine in detail the dependence of electrical conductivity and ultrafast optical nonlinearity of graphene oxide (GO) films on their degrees of reduction, as well as the link between the two properties. The GO films are first synthesized through the vacuum filtration method and then reduced partially controllably by the femtosecond laser direct writing with varying power doses. Subsequently, the 4-point probe measurements of the reduced GO (r-GO) films are demonstrated to exhibit superior resistivity and electrical conductivity compared with the pristine GO counterpart. It was found that the conductivity of the film increases and then decreases with increasing ablation laser power (P), GO was completely reduced at P = 100 mW with resistivity and electrical conductivity of 1.09 × 10-3Ω·m and 9.19 × 102s/m, respectively. GO was over reduced at P = 120 mW with resistivity and electrical conductivity being 3.72 × 10-3Ω·m and 2.69 × 102s/m, respectively. We further test the ultrafast optical nonlinearity (ONL) of the as-prepared pristine and reduced GO with the femtosecond Z-scan technique. The results show that the behavior of ONL is reversed whenever GO is reduced in a controlled manner. More interestingly, the higher the ablation laser power is, the stronger the optical nonlinearity of r-GO is. In particular, the nonlinear absorption and refraction coefficients of the r-GO films reach up to 3.26 × 10-8 m/W and -1.12 × 10-13 m2/W when P = 120 mW. The nonlinear absorption and refraction coefficients reach 1.9 × 10-8 m/W and -3 × 10-13 m2/W, respectively, for P = 70 mW. The GO/r-GO films endowing tunable electro-optical responses are potential building blocks for wide-ranging applications in microelectronic circuits, optoele

关键词： Femtosecond lasers

Study on Sensitization Mechanism of Novel Magnetorheological Composite Pdms Thin Film Based on Enhanced Magneto-Mechanical Effect

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SSRN 2023年

作者： Sang, Shengbo Tan, Qiuyun Jiang, Jiaolin Wu, Kaile Xiao, Pengli Zhao, Dong Guo, Xing Yang, Zhuoqing Dong, Xiushan Ge, Yang Shanxi Key Laboratory of Micro Nano Sensors & Artificial Intelligence Perception College of Information and Computer Taiyuan University of Technology Taiyuan030024 China Key Lab of Advanced Transducers and Intelligent Control System Ministry of Education Taiyuan University of Technology Taiyuan030024 China Shanghai200240 China Shanxi Academy of Medical Sciences China Shanxi Research Institute of 6D Artificial Intelligence Biomedical Science Taiyuan030024 China

High sensitivity is key to expand the range of bio-detection, especially in realizing biological detection on single molecular level. Herein, we introduce a novel magnetorheological membrane with enhanced magneto-mechanical effect into the biosensor. Specifically, we made the magnetorheological composite PDMS film (MREF) strengthened by magnetostrictive particles (MSP), and the anisotropic TbDyFe-PDMS can be magnetically deformed to 90 °with 5.8 emu/g, which possesses an initial tensile modulus 55% higher than isotropic. In particular, the modified MR effect equations were proposed considering magnetic dipole interaction and nonlinear magnetostrictive pre-strain of MSP. Such formulae indicate that the enhanced MR effect of MSP-MREF is greatly determined by Ms, remanence, and the flux linkage-like structure. In addition, finite element simulations were carried out to validate and complementarily demonstrate the nonlinear magneto-mechanical behaviors of MSP-MREF theoretically. Finally, the biosensor based on MSP-MREF was fabricated to detect the low concentrations of human serum albumin (HSA), and its sensitivity is around 4 times that of the conventional biosensor. Furthermore, it exhibits high reliability in detecting HSA in real human urine samples, making it the ideal candidate as a practical and effective way for the detection of biomolecules at low concentrations in the future. © 2023, The Authors. All rights reserved.

关键词： Finite element method

Ultrafast Spin-to-Orbit and Orbit-to-Local-Spin Conversions of Tightly Focused Hybridly Polarized Light Pulses

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arXiv

arXiv 2021年

作者： Zhang, Yanxiang Zhang, Zijing Nie, Zhongquan Department of Physics Harbin Institute of Technology Harbin150001 China Key Lab of Advanced Transducers and Intelligent Control System Ministry of Education and Shanxi Province College of Physics and Optoelectronics Taiyuan University of Technology Taiyuan030024 China

Spin-orbit interaction (SOI) have provided a new viable roadmap for the development of spin-based photonics devices. However, existing strategies to control the SOI focus commonly on tailoring the spatial dimension of light fields yet neglecting the inherent temporal one. Herein, we first present ultrafast temporal effects on both spin-to-orbit and orbit-to-local-spin conversions based on the time-assistant vectorial diffractive theory and the fast Fourier transformation. Such interconversions depend upon whether the incident hybridly vectorial light pulse carries vortex phase or not in a single high numerical aperture geometry. For the case of the absence of vortex phase, we find that it enables orbit angular momentum-carrying transverse component fields, and the resultant orbit angular momentum embedded within focused light fields remains constantly revolving as time elapses, which indicates that the controllable spin-to-orbit conversion occurs. By contrast, it is revealed that hybridly polarized vectorial-vortex light pulses allow access to the locally excited circular polarization at the focus, and this induced local circular polarization is independent of ultrafast varying time, whereas the resulting spin angular momentum density components experience the alternation between the appearance and annihilation over time, thus giving rise to the tunable orbit-to-local-spin conversion. These exotic ultrafast interconversions not only breathe a new life into the area of ultrafast photonics, but refresh our understanding on the paradigm of photonic SOI. Copyright © 2021, The Authors. All rights reserved.

关键词： Circular polarization

controlled formation of GaN nanostructures through contactless photoelectrochemical etching for supercapacitor electrode applications

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International Journal of Electrochemical Science 2025年第8期20卷

作者： Yaya Ge Yihang Fan Yibiao Yang Mingda Zhang Xin Liu Binzhao Cao Yuan Tian Hongming Fei College of Physics and Optoelectronics Taiyuan University of Technology Taiyuan 030024 China Key Lab of Advanced Transducers and Intelligent Control System Ministry of Education and Shanxi Province College of Physics and Optoelectronics Taiyuan University of Technology Taiyuan 030024 China

Nanostructured n-type GaN layers were fabricated using the Contactless photoelectrochemical (PEC) etching method in KOH-based solutions under ultraviolet illumination. By adjusting the KOH concentration, distinct surface morphologies were obtained. Low-concentration KOH solutions led to the formation of nanorods at dislocation sites, whereas high-concentration solutions induced interconnected etch pits. Cathodoluminescence (CL) analysis confirmed a strong correlation between the resulting nanostructures and dislocation sites. The formation mechanisms of different nanostructures were discussed. Electrochemical characterization revealed significantly enhanced performance in etched GaN samples. In particular, the GaN layer treated with 0.02 M KOH and 0.02 M K 2 S 2 O 8 exhibited a 16-fold increase in specific capacitance compared to the pristine GaN layer.

关键词： Contactless photoelectrochemical(PEC) etching KOH concentration Dislocations Nanostructures Specific capacitance

Biocompatible chitosan/polyethylene glycol/multi-walled carbon nanotube composite scaffolds for neural tissue engineering

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Journal of Zhejiang University-Science B(Biomedicine & Biotechnology) 2022年第1期23卷 58-73页

作者： Shengbo SANG Rong CHENG Yanyan CAO Yayun YAN Zhizhong SHEN Yajing ZHAO Yanqing HAN Shanxi Key Laboratory of Micro Nano Sensors&Artificial Intelligence Perception College of Information and ComputerTaiyuan University of TechnologyTaiyuan030024China Key Lab of Advanced Transducers and Intelligent Control System of the Ministry of Education Taiyuan University of TechnologyTaiyuan030024China College of Information Science and Engineering Hebei North UniversityZhangjiakou075000China Shanxi Six-Dimensional Artificial Intelligence Biomedical Research Institute Taiyuan030031China Department of Neurology Shanxi Provincial Cardiovascular HospitalTaiyuan030024China

Carbon nanotube(CNT)composite materials are very attractive for use in neural tissue engineering and biosensor *** scaffolds are excellent mimics of extracellular matrix due to their hydrophilicity,viscosity,and *** can also impart conductivity to other insulating materials improve mechanical stability guide neuronal cell behavior and trigger axon *** performance of chitosan(CS)/polyethylene glycol(PEG)composite scaffolds could be optimized by introducing multi-walled CNTs(MWCNTs).CS/PEG/CNT composite scaffolds with CNT content of 1%,3%,and 5%(1%=0.01 g/mL)were prepared by *** physical and chemical properties and biocompatibility were *** electron microscopy(SEM)showed that the composite scaffolds had a highly connected porous *** electron microscope(TEM)and Raman spectroscopy proved that the CNTs were well dispersed in the CS/PEG matrix and combined with the CS/PEG nanofiber *** enhanced the elastic modulus of the *** porosity of the scaffolds ranged from 83%to 96%.They reached a stable water swelling state within 24 h,and swelling decreased with increasing MWCNT *** electrical conductivity and cell adhesion rate of the scaffolds increased with increasing MWCNT *** showed that rat pheochromocytoma(PC12)cells grown in the scaffolds had characteristics similar to nerve *** measured changes in the expression of nerve cell markers by quantitative real-time polymerase chain reaction(qRT-PCR),and found that PC12 cells cultured in the scaffolds expressed growth-associated protein 43(GAP43),nerve growth factor receptor(NGFR),and class IIIβ-tubulin(TUBB3)*** research showed that the prepared CS/PEG/CNT scaffold has good biocompatibility and can be further applied to neural tissue engineering research.

关键词： Multi-walled carbon nanotube(MWCNT) Cell-scaffold PC12 cells Biocompatibility

An Improved Chimp Optimization Algorithm for Short-term Hydrothermal Scheduling

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IAENG International Journal of Computer Science

IAENG International Journal of Computer Science 2022年第3期49卷 666页

作者： Chen, Gonggui Wang, Shumin He, Yongsheng Shang, Wanfeng Long, Hongyu Key Laboratory of Industrial Internet of Things and Networked Control Ministry of Education Chongqing University of Posts and Telecommunications Chongqing400065 China Chongqing University of Posts and Telecommunications Chongqing400065 China State Grid Chongqing Electric Power Company Chongqing400015 China Guangdong Provincial Key Lab of Robotics and Intelligent System Shenzhen Institute of Advanced Technology Chinese Academy of Sciences Shenzhen Shenzhen518055 China Chongqing Key Laboratory of Complex Systems and Bionic Control Chongqing University of Posts and Telecommunications Chongqing400065 China

The short-term hydrothermal scheduling (STHS) is a complex non-linear, non-convex and high-dimensional mathematical optimization problem. Due to the fact that the original chimp optimization algorithm (ChOA) is likely to fall into local optimum and has the disadvantage of low population diversity, an improved chimp optimization algorithm (IChOA) is proposed to solve the STHS problem. Firstly, Logistic-Tent chaotic mapping is employed to initialize the population and increase the population diversity. Then a new nonlinear convergence factor is introduced to make the optimization search process more applicable to STHS problems. Next, particle swarm algorithm (PSO) and gravitational search algorithm (GSA) are combined to enhance the shortcoming and balance the global search ability and local exploration ability of ChOA. Moreover, Cauchy mutation and opposition-based learning strategy are supplemented as perturbation interference when the optimal position is not updated to improve the ability to leap out of the local optimum. Finally, a graded optimization strategy is adopted for the constraint handing of dynamic reservoir balance and thermal power balance. Three standard hydrothermal power systems are utilized to verify the practicability and validity of the proposed method. Results of simulations reveal that IChOA has significant competitive advantages in addressing the STHS problem. © 2022, IAENG International Journal of Computer Science. All Rights Reserved.

关键词： Particle swarm optimization (PSO)