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物理化学学报 2021年第12期37卷 1-151页

作者：常诚陈伟陈也陈永华陈雨丁峰樊春海范红金范战西龚成宫勇吉何其远洪勋胡晟胡伟达黄维黄元季威李德慧李连忠李强林立凌崇益刘鸣华刘楠刘庄 Kian Ping Loh 马建民缪峰彭海琳邵明飞宋礼苏邵孙硕谭超良唐智勇王定胜王欢王金兰王欣王欣然 Andrew T.S.Wee 魏钟鸣吴宇恩吴忠帅熊杰熊启华徐伟高尹鹏曾海波曾志远翟天佑张晗张辉张其春张铁锐张翔赵立东赵美廷赵伟杰赵运宣周凯歌周兴周喻朱宏伟张华刘忠范 Institute of Science and Technology Austria Am Campus 13400 KlosterneuburgAustria Department of Chemistry National University of Singapore3 Science Drive 3117543Singapore Department of Chemistry The Chinese University of Hong KongShatinNew TerritoriesHong KongChina Key Laboratory of Flexible Electronics and Institute of Advanced Materials Nanjing Tech UniversityNanjing 211816China School of Life Sciences Shanghai UniversityShanghai 200444China Centre for Multidimensional Carbon Materials Institute for Basic ScienceUlsan 44919Korea School of Chemistry and Chemical Engineering Shanghai Jiao Tong UniversityShanghai 200240China School of Physical and Mathematical Sciences Nanyang Technological UniversitySingapore 637371Singapore Department of Chemistry City University of Hong KongKowloonHong KongChina Department of Electrical and Computer Engineering and Quantum Technology Center University of MarylandCollege ParkMaryland 20742USA School of Materials Science and Engineering Beihang UniversityBeijing 100191China Department of Materials Science and Engineering City University of Hong KongKowloonHong KongChina Center of Advanced Nanocatalysis(CAN) Hefei National Laboratory for Physical Sciences at the MicroscaleDepartment of Applied ChemistryUniversity of Science and Technology of ChinaHefei 230026China College of Chemistry and Chemical Engineering State Key Laboratory of Physical Chemistry of Solid SurfacesCollaborative Innovation Center of Chemistry for Energy Materials(iChEM)Xiamen UniversityXiamen361005Fujian ProvinceChina State Key Laboratory of Infrared Physics Shanghai Institute of Technical PhysicsChinese Academy of SciencesShanghai 200083China Advanced Research Institute of Multidisciplinary Science Beijing Institute of TechnologyBeijing100081China Beijing Key Laboratory of Optoelectronic Functional Materials&Micro-Nano Devices Department of PhysicsRenmin University of ChinaBeijing 100872China School of Optical and Electronic Information Wuhan National Laboratory

Research on two-dimensional(2D) materials has been explosively increasing in last seventeen years in varying subjects including condensed matter physics, electronic engineering, materials science, and chemistry since the mechanical exfoliation of graphene in 2004. Starting from graphene, 2D materials now have become a big family with numerous members and diverse categories. The unique structural features and physicochemical properties of 2D materials make them one class of the most appealing candidates for a wide range of potential applications. In particular, we have seen some major breakthroughs made in the field of 2D materials in last five years not only in developing novel synthetic methods and exploring new structures/properties but also in identifying innovative applications and pushing forward commercialisation. In this review, we provide a critical summary on the recent progress made in the field of 2D materials with a particular focus on last five years. After a brief backgroundintroduction, we first discuss the major synthetic methods for 2D materials, including the mechanical exfoliation, liquid exfoliation, vapor phase deposition, and wet-chemical synthesis as well as phase engineering of 2D materials belonging to the field of phase engineering of nanomaterials(PEN). We then introduce the superconducting/optical/magnetic properties and chirality of 2D materials along with newly emerging magic angle 2D superlattices. Following that, the promising applications of 2D materials in electronics, optoelectronics, catalysis, energy storage, solar cells, biomedicine, sensors, environments, etc. are described sequentially. Thereafter, we present the theoretic calculations and simulations of 2D materials. Finally, after concluding the current progress, we provide some personal discussions on the existing challenges and future outlooks in this rapidly developing field.

关键词： Two-dimensional materials Transition metal dichalcogenides Phase engineering of nanomaterials Electronics Optoelectronics Catalysis Energy storage and conversion

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Water Splitting: Optical and Electrical Enhancement of Hydrogen Evolution by MoS2@MoO3Core–Shell nanowires with Designed Tunable Plasmon Resonance (Adv. Funct. Mater. 32/2018)

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advanced Functional Materials 2018年第32期28卷

作者： Shaohui Guo Xuanhua Li Xingang Ren Lin Yang Jinmeng Zhu Bingqing Wei State Key Laboratory of Solidification Processing Center for Nano Energy Materials School of Materials Science and Engineering Northwestern Polytechnical University and Shaanxi Joint Lab of Graphene (NPU) Xi'an 710072 China Northwestern Polytechnical University‐Queen Mary University of London (NPU‐QMUL) Joint Research Institute of Advanced Materials and Structures (JRI‐AMAS) Xi'an 710072 China Key Laboratory of Intelligent Computing and Signal Processing Ministry of Education Anhui University No. 3 Feixi Road Hefei Anhui Province 230039 P. R. China Department of Mechanical Engineering University of Delaware Newark DE 19716 USA

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Localized Ligands Assist Ultrafast Multivalent-Cation Intercalation Pseudocapacitance

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Angewandte Chemie 2023年第26期135卷

作者： Luting Xie Prof. Kui Xu Wenlu Sun Yingzhu Fan Dr. Junyu Zhang Dr. Yixiao Zhang Dr. Hui Zhang Jun Chen Prof. Yanbin Shen Prof. Fang Fu Dr. Huabin Kong Prof. Guan Wu Prof. Jihuai Wu Prof. Liwei Chen Prof. Hongwei Chen College of Materials Science and Engineering Huaqiao University Xiamen 361021 China School of Flexible Electronics (Future Technologies) & Institute of Advanced Materials (IAM) Nanjing University of Technology Nanjing 211816 China i-Lab CAS Center for Excellence in Nanoscience Suzhou Institute of Nano-Tech and Nano-Bionics Chinese Academy of Sciences Suzhou 215123 Jiangsu Province China Instrumental Analysis Center Laboratory and Equipment Management Department Huaqiao University Xiamen Fujian 361021 China In-Situ Center for Physical Science School of Chemistry and Chemical Engineering Shanghai Jiaotong University Shanghai 200240 China National Key Laboratory of High-efficiency Utilization of Coal and Green Chemical Engineering Ningxia University Yinchuan 750021 China National Engineering Lab for Textile Fiber Materials and Processing Technology School of Materials Science and Engineering Zhejiang Sci-Tech University Hangzhou 310018 China Department of Xiamen Key Laboratory of Optoelectronic Materials and Advanced Manufacturing College of Materials Science and Engineering Huaqiao University Xiamen 361021 China

Rechargeable batteries based on multivalent cation (Mv n + , n >1) carriers are considered potentially low-cost alternatives to lithium-ion batteries. However, the high charge-density Mv n + carriers generally lead to sluggish kinetics and poor structural stability in cathode materials. Herein, we report an Mv n + storage via intercalation pseudocapacitance mechanism in a 2D bivalve-like organic framework featured with localized ligands. By switching from conventional intercalation to localized ligand-assisted-intercalation pseudocapacitance, the organic cathode exhibits unprecedented fast kinetics with little structural change upon intercalation. It thus enables an excellent power density of 57 kW kg −1 over 20000 cycles for Ca 2+ storage and a power density of 14 kW kg −1 with a long cycling life over 45000 cycles for Zn 2+ storage. This work may provide a largely unexploited route toward constructing a local dynamic coordination microstructure for ultrafast Mv n + storage.

关键词： Cathodes Intercalation Pseudocapacitance Multivalent Ion Batteries Organic Frameworks Stability

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Perovskite Solar Cells: Unique Seamlessly Bonded CNT@Graphene Hybrid nanostructure Introduced in an Interlayer for Efficient and Stable Perovskite Solar Cells (Adv. Funct. Mater. 32/2018)

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advanced Functional Materials 2018年第32期28卷

作者： Xuanhua Li Tengteng Tong Qinjiang Wu Shaohui Guo Qiang Song Jian Han Zhixiang Huang State Key Laboratory of Solidification Processing Research and Development Institute of Northwestern Polytechnical University In Shenzhen Center for Nano Energy Materials School of Materials Science and Engineering Northwestern Polytechnical University and Shaanxi Joint Lab of Graphene (NPU) Xi'an 710072 China Northwestern Polytechnical University‐Queen Mary University of London (NPU‐QMUL) Joint Research Institute of Advanced Materials and Structures (JRI‐AMAS) Xi'an 710072 China Key Laboratory of Intelligent Computing and Signal Processing Ministry of Education Anhui University No. 3 Feixi Road Hefei Anhui Province 230039 P. R. China

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Cover Feature: Ultrasensitive, Sustainable, and Selective Electrochemical Hydrazine Detection by ALD-Developed Two-Dimensional WO3(ChemElectroChem 2/2018)

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ChemElectroChem 2017年第2期5卷

作者： Zihan Wei Zhenyin Hai Mohammad Karbalaei Akbari Prof. Jie Hu Lachlan Hyde Prof. Stephen Depuydt Prof. Francis Verpoort Prof. Serge Zhuiykov Ghent University Global Campus Department of Applied Analytical & Physical Chemistry 119 Songdomunhwa-ro Yeonsu-gu Incheon South Korea Micro and Nano System Research Center Key Lab of Advanced Transducers and Intelligent Control System (Ministry of Education) & College of Information Engineering Taiyuan University of Technology Taiyuan 030024 Shanxi PR China Factory of the Future Swinburne University of Technology Hawthorn Australia National Research Tomsk Polytechnic University Lenin Avenue 30 634050 Tomsk Russian Federation Laboratory of Organometallics Catalysis and Ordered Materials State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Center for Chemical and Material Engineering Wuhan University of Technology Wuhan P.R. China

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Graphene Foams: A Bubble‐Derived Strategy to Prepare Multiple Graphene‐Based Porous Materials (Adv. Funct. Mater. 23/2018)

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advanced Functional Materials 2018年第23期28卷

作者： Rujing Zhang Ruirui Hu Xinming Li Zhen Zhen Zhenhua Xu Na Li Limin He Hongwei Zhu Aviation Key Laboratory of Science and Technology on Advanced Corrosion and Protection for Aviation Material Department 5 P.O. Box 81‐5 AECC Beijing Institute of Aeronautical Materials Beijing 100095 China State Key Lab of New Ceramics and Fine Processing School of Materials Science and Engineering and Center for Nano and Micro Mechanics Tsinghua University Beijing 100084 China International Center for Materials Nanoarchitectonics (WPI‐MANA) National Institute for Materials Science (NIMS) 1‐1 Namiki Tsukuba Ibaraki 305‐0044 Japan

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Regulating Non-Equilibrium Solvation Structure in Locally Concentrated Ionic Liquid Electrolytes for Wide-Temperature and High-Voltage Lithium Metal Batteries

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Angewandte Chemie 2024年第1期137卷

作者： Haifeng Tu Zhicheng Wang Jiangyan Xue Zhiyong Tang Yang Liu Xiaofang Liu Lingwang Liu Suwan Lu Shixiao Weng Yiwen Gao Guochao Sun Zheng Liu Keyang Peng Xin Zhang Dejun Li Guangye Wu Meinan Liu Jianchen Hu Hong Li Jingjing Xu Xiaodong Wu School of Nano-Tech and Nano-Bionics University of Science and Technology of China Hefei Anhui 230026 China i-lab Suzhou Institute of Nano-Tech and Nano-Bionics Chinese Academy of Sciences Suzhou Jiangsu 215123 China These authors contributed equally to this work: Haifeng Tu Zhicheng Wang Institute of Physics Chinese Academy of Sciences Beijing 100190 China Tianmu Lake Institute of Advanced Energy Storage Technologies Liyang 213300 China Jiangxi Key Laboratory of Flexible Electronics Jiangxi Science & Technology Normal University Nanchang 330013 Jiangxi China State Key Laboratory of Featured Metal Materials and Life-cycle Safety for Composite Structures Guangxi Key Laboratory of Processing for Non-Ferrous Metals and Featured Materials School of Resources Environment and Materials Guangxi University Nanning 530004 China National Engineering Laboratory for Modern Silk College of Textile and Clothing Engineering Research Center of Cooperative Innovation for Functional Organic/Polymer Material Micro/Nanofabrication Soochow University Suzhou 215123 China College of Material Science and Engineering Hohai University Nanjing Jiangsu 210024 China

The development of high-voltage lithium metal batteries (LMBs) encounters significant challenges due to aggressive electrode chemistry. Recently, locally concentrated ionic liquid electrolytes (LCILEs) have garnered attention for their exceptional stability with both Li anodes and high-voltage cathodes. However, there remains a limited understanding of how diluents in LCILEs affect the thermodynamic stability of the solvation structure and transportation dynamics of Li + ions. Herein, we propose a wide-temperature LCILEs with 1,3-dichloropropane (DCP13) diluent to construct a non-equilibrium solvation structure under external electric field, wherein the DCP13 diluent enters the Li + ion solvation sheath to enhance Li + ion transport and suppress oxidative side reactions at high-nickel cathode (LiNi 0.9 Co 0.05 Mn 0.05 O 2 , NCM90). Consequently, a Li/NCM90 cell utilizing this LCILE achieves a high capacity retention of 94 % after 240 cycles at 4.3 V, also operates stably at high cut-off voltages from 4.4 V to 4.6 V and over a wide temperature range from −20 °C to 60 °C. Additionally, an Ah-level pouch cell with this LCILE simultaneously achieves high-energy-density and stable cycling, manifesting the practical feasibility. This work redefines the role of diluents in LCILEs, providing inspiration for electrolyte design in developing high-energy-density batteries.

关键词： Lithium metal batteries locally concentrated ionic liquid electrolyte chloroalkane diluent non-equilibrium solvation structure external electric field

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Managing Secondary Phase Lead Iodide in Hybrid Perovskites via Surface Reconstruction for High-Performance Perovskite Solar Cells with Robust Environmental Stability

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Angewandte Chemie 2023年第18期135卷

作者： Linfeng Ye Dr. Pengfei Guo Dr. Jie Su Kaiyuan Zhang Chen Liu Penghui Yang Wenhao Zhao Pengzhen Zhao Prof. Zhe Liu Prof. Jingjing Chang Dr. Qian Ye Prof. Hongqiang Wang State Key Laboratory of Solidification Processing Center for Nano Energy Materials School of Materials Science and Engineering Northwestern Polytechnical University and Shaanxi Joint Laboratory of Graphene (NPU) Xi'an 710071 China Contribution: Investigation (lead) Methodology (lead) Writing - original draft (equal) Writing - review & editing (equal) Chongqing Innovation Center Northwestern Polytechnical University Chongqing 401135 China Contribution: Investigation (equal) Writing - original draft (equal) Writing - review & editing (equal) School of Microelectronics State Key Discipline Lab of Wide Band Gap Semiconductor Technology Shaanxi Joint Key Lab of Graphene Advanced Interdisciplinary Research Center for Flexible Electronics Xidian University Xi'an 710071 China

Rationally managing the secondary-phase excess lead iodide (PbI 2 ) in hybrid perovskite is of significance for pursuing high performance perovskite solar cells (PSCs), while the challenge remains on its conversion to a homogeneous layer that is robust stable against environmental stimuli. We herein demonstrate an effective strategy of surface reconstruction that converts the excess PbI 2 into a gradient lead sulfate-silica bi-layer, which substantially stabilizes the perovskite film and reduces interfacial charge transfer barrier in the PSCs device. The perovskite films with such bi-layer could bear harsh conditions such as soaking in water, light illumination at 70 % relative humidity, and the damp-thermal (85 °C and 30 % humidity) environment. The resulted PSCs deliver a champion efficiency up to 24.09 %, as well as remarkable environmental stability, e.g., retaining 78 % of their initial efficiency after 5500 h of shelf storage, and 82 % after 1000 h of operational stability testing.

关键词： Environmental Stability Hybrid Perovskite Lead Iodide Perovskite Solar Cells Surface Reconstruction

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Publisher Correction: Twisted moiré conductive thermal metasurface

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Nature communications 2024年第1期15卷 2876页

作者： Huagen Li Dong Wang Guoqiang Xu Kaipeng Liu Tan Zhang Jiaxin Li Guangming Tao Shuihua Yang Yanghua Lu Run Hu Shisheng Lin Ying Li Cheng-Wei Qiu Department of Electrical and Computer Engineering National University of Singapore Kent Ridge 117583 Republic of Singapore. State Key Laboratory of Extreme Photonics and Instrumentation ZJU-Hangzhou Global Scientific and Technological Innovation Center Zhejiang University Hangzhou 310027 China. International Joint Innovation Center Key Lab. of Advanced Micro/Nano Electronic Devices & Smart Systems of Zhejiang The Electromagnetics Academy of Zhejiang University Zhejiang University Haining 314400 China. Wuhan National Laboratory for Optoelectronics and State Key Laboratory of Material Processing and Die and Mould Technology School of Materials Science and Engineering Huazhong University of Science and Technology Wuhan 430074 China. Smart Materials for Architecture Research Lab Innovation Center of Yangtze River Delta Zhejiang University Jiaxing 314100 China. State Key Laboratory of Coal Combustion School of Energy and Power Engineering Huazhong University of Science and Technology Wuhan 430074 China. Chongqing 2D Materials Institute Chongqing 400015 China. State Key Laboratory of Extreme Photonics and Instrumentation ZJU-Hangzhou Global Scientific and Technological Innovation Center Zhejiang University Hangzhou 310027 China. eleying@***. International Joint Innovation Center Key Lab. of Advanced Micro/Nano Electronic Devices & Smart Systems of Zhejiang The Electromagnetics Academy of Zhejiang University Zhejiang University Haining 314400 China. eleying@***. Department of Electrical and Computer Engineering National University of Singapore Kent Ridge 117583 Republic of Singapore. chengwei.qiu@nus.edu.sg.

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Author Correction: Activation of subnanometric Pt on Cu-modified CeO2 via redox-coupled atomic layer deposition for CO oxidation

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Nature communications 2020年第1期11卷 5879页

作者： Xiao Liu Shuangfeng Jia Ming Yang Yuanting Tang Yanwei Wen Shengqi Chu Jianbo Wang Bin Shan Rong Chen State Key Laboratory of Digital Manufacturing Equipment and Technology School of Mechanical Science and Engineering Huazhong University of Science and Technology 430074 Wuhan Hubei People's Republic of China. State Key Laboratory of Materials Processing and Die and Mould Technology School of Materials Science and Engineering Huazhong University of Science and Technology 430074 Wuhan Hubei People's Republic of China. School of Physics and Technology Center for Electron Microscopy MOE Key Laboratory of Artificial Micro- and Nano-structures and Institute for Advanced Studies Wuhan University 430072 Wuhan Hubei People's Republic of China. General Motors Global Research and Development Chemical Sciences and Materials Systems Lab 3500 Mound Road Warren MI 48090 USA. Department of Chemical and Biomolecular Engineering Clemson University Clemson SC 29634 USA. Institute of High Energy Physics Chinese Academy of Sciences 100049 Beijing People's Republic of China. State Key Laboratory of Materials Processing and Die and Mould Technology School of Materials Science and Engineering Huazhong University of Science and Technology 430074 Wuhan Hubei People's Republic of China. bshan@***. State Key Laboratory of Digital Manufacturing Equipment and Technology School of Mechanical Science and Engineering Huazhong University of Science and Technology 430074 Wuhan Hubei People's Republic of China. rongchen@***.

A Correction to this paper has been published: https://***/10.1038/s41467-020-19663-3 .

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