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Photocatalytic bio-inspired PDA-RGO/g-C3N4 nanocomposite incorporated PES membrane for removal of environmental antibiotic pollutants

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Journal of Chemical technology and Biotechnology 2024年第6期99卷 1401-1413页

作者： Govardhanan, B. GokulaKrishnan, S.A. Arthanareeswaran, G. Ashok, M. Chen, Yong-Song Taweepreda, W. Membrane Research Laboratory Department of Chemical Engineering National Institute of Technology Tiruchirappalli Tiruchirappalli India New Generation Materials lab Department of Physics National Institute of Technology Tiruchirappalli Tiruchirappalli India Department of Mechanical Engineering and Advanced Institute of Manufacturing with High-tech Innovations National Chung Cheng University Chiayi County Taiwan Polymer Science Program Division of Physical Science Faculty of Science Prince of Songkla University Hat-Yai Thailand

BACKGROUND: Membrane technology makes it more suitable for the treatment of environmental polluted organic wastewater. Membrane fouling is one of the major concerns in commercial membranes. To overcome this issue, photocatalytic nanomaterials are embedded into the membrane to enhance its surface nature and reusability. In this investigation, polydopamine functionalized graphene oxide (PDA-RGO), graphite carbon nitride (g-C3N4) and PDA-RGO/g-C3N4 nanomaterials were incorporated within polyethersulfone membrane fabricated via a phase inversion technique. These as-prepared membranes’ functional groups and surface morphologies were investigated by Fourier transform infrared (FTIR) spectroscopy, atomic force microscopy (AFM) and field emission electron microscopy (FESEM). These as-prepared membranes were investigated for photocatalytic activity under visible-light-driven photodegradation by environmental pollutants such as Rhodamine B (RhB) and Norfloxacin (NOR). RESULTS: Compared with pristine PES membrane, the PDA-RGO/g-C3N4-PES nanocomposite membrane showed higher photocatalytic activity for Rhodamine B 94.6% and Norfloxacin 96.8%, also reached greater water flux 189 L m−2 h−1. Therefore, the bio-inspired nanocomposite-modified PDA-RGO/g-C3N4 photocatalytic membrane could have huge potential in processing environmentally polluted water. CONCLUSIONS: PDA-RGO/g-C3N4-PES nanocomposite membrane improved the membrane hydrophilicity, water flow, anti-fouling performance, rejection studies and photocatalytic degradation than the pristine membrane. The synergistic result of PDA-RGO and g-C3N4 exhibits better photodegradation efficiency of the membrane towards environmental pollutants. © 2024 Society of Chemical Industry (SCI). © 2024 Society of Chemical Industry (SCI).

关键词： Nanocomposites

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Observation of possible excitonic charge density waves and metal–insulator transitions in atomically thin semimetals

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Nature Physics 2024年第4期20卷 597-602页

作者： Gao, Qiang Chan, Yang-Hao Jiao, Pengfei Chen, Haiyang Yin, Shuaishuai Tangprapha, Kanjanaporn Yang, Yichen Li, Xiaolong Liu, Zhengtai Shen, Dawei Jiang, Shengwei Chen, Peng Shenyang National Laboratory for Materials Science Shanghai Center for Complex Physics School of Physics and Astronomy Shanghai Jiao Tong University Shanghai China Institute of Atomic and Molecular Sciences Academia Sinica Taipei Taiwan Physics Division National Center for Theoretical Sciences Taipei Taiwan Shanghai Synchrotron Radiation Facility Shanghai Advanced Research Institute Chinese Academy of Sciences Shanghai China College of Engineering International Advanced Technology Program National Taiwan University of Science and Technology Taipei Taiwan Chinese Academy of Sciences Shanghai China National Synchrotron Radiation Laboratory University of Science and Technology of China Hefei China

In solids, the condensation of electron and hole pairs with finite momentum leads to an ordered state known as a charge density wave, in which the charge has spatial modulation. However, lattice symmetry breaking and the accompanying relocation of the ions, which changes the charge distribution, can also occur simultaneously, making it difficult to disentangle the origin of the transition. Here we demonstrate a condensed phase in low-dimensional HfTe2. Angle-resolved photoemission spectroscopy measurements reveal a metal–insulator transition upon lowering the temperature. The observation of an opening gap, the renormalization of the bands and the emergence of replica bands in the low-temperature regime suggests that a charge density wave formed in the ground state. Raman spectroscopy shows no sign of lattice distortion within the detection limit. A small amount of electron doping substantially raises the transition temperature due to a reduced screening effect and a more balanced carrier density for electrons and holes. Our results indicate that the formation mechanism of the charge density wave is consistent with the excitonic insulator phase in low-dimensional HfTe2 without any structural modification. © The Author(s), under exclusive licence to Springer Nature Limited 2024.

关键词： Charge density waves

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Concentrated ternary ether electrolyte allows for stable cycling of a lithium metal battery with commercial mass loading high-nickel NMC and thin anodes

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Carbon Energy 2023年第3期5卷 2-18页

作者： Jun Yang Xing Li Ke Qu Yixian Wang Kangqi Shen Changhuan Jiang Bo Yu Pan Luo Zhuangzhi Li Mingyang Chen Bingshu Guo Mingshan Wang Junchen Chen Zhiyuan Ma Yun Huang Zhenzhong Yang Pengcheng Liu Rong Huang Xiaodi Ren David Mitlin School of New Energy and Materials Southwest Petroleum UniversityChengduChina Energy Storage Research Institute Southwest Petroleum UniversityChengduChina Shenzhen Key Laboratory of Nanobiomechanics Shenzhen Institutes of Advanced TechnologyChinese Academy of SciencesShenzhenChina China Key Laboratory of Polar Materials and Devices(MOE) Department of ElectronicsEast China Normal UniversityShanghaiChina Materials Science Program and Texas Materials Institute The University of Texas at AustinAustinTexasUSA Beijing Computational Science Research Center BeijingChina School of Materials Science and Engineering Center for Green Innovation University of Science and Technology BeijingBeijingChina Department of Materials Science and Engineering Hefei National Research Center for Physical Sciences at the MicroscaleUniversity of Science and Technology of ChinaHefeiAnhuiChina

A new concentrated ternary salt ether-based electrolyte enables stable cycling of lithium metal battery(LMB)cells with high-mass-loading(13.8 mg cm^(−2),2.5 mAh cm^(−2))NMC622(LiNi_(0.6)Co_(0.2)Mn_(0.2)O_(2))cathodes and 50μm Li ***“CETHER-3,”this electrolyte is based on LiTFSI,LiDFOB,and LiBF4 with 5 vol%fluorinated ethylene carbonate in 1,***-cial carbonate and state-of-the-art binary salt ether electrolytes were also tested as *** CETHER-3,the electrochemical performance of the full-cell battery is among the most favorably reported in terms of high-voltage cycling *** example,LiNi_(x)Mn_(y)Co_(1-x-y)O_(2)(NMC)-Li metal cells retain 80%capacity at 430 cycles with a 4.4 V cut-off and 83%capacity at 100 cycles with a 4.5 V cut-off(charge at C/5,discharge at C/2).According to simulation by density functional theory and molecular dynamics,this favorable performance is an outcome of enhanced coordination between Li^(+)and the solvent/salt *** advanced microscopy(high-resolution transmission electron microscopy,scanning electron microscopy)and surface science(X-ray photoelectron spectroscopy,time-of-fight secondary ion mass spectroscopy,Fourier-transform infrared spectroscopy,Raman spectroscopy),it is demonstrated that a thinner and more stable cathode electrolyte interphase(CEI)and solid electrolyte interphase(SEI)are *** CEI is rich in lithium sulfide(Li_(2)SO_(3)),while the SEI is rich in Li_(3)N and *** cycling,the CEI/SEI suppresses both the deleterious transformation of the cathode R-3m layered near-surface structure into disordered rock salt and the growth of lithium metal dendrites.

关键词： concentrated electrolyte density functional theory ether electrolyte high‐nickel cathode high‐voltage battery molecular dynamics

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Multi-Panel Extra-Large Scale MIMO Based Joint Activity Detection and Channel Estimation for Near-Field Massive IoT Access

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China Communications 2023年第5期20卷 232-243页

作者： Zhen Gao Hanlin Xiu Yikun Mei Anwen Liao Malong Ke Chun Hu Mohamed-Slim Alouini School of Information and Electronics Beijing Institute of TechnologyBeijing 100081China MIIT Key Laboratory of Complex-Field Intelligent Sensing Beijing Institute of TechnologyBeijing 100081China The Advanced Technology Research Institute of Beijing Institute of Technology Jinan 250307China Yangtze Delta Region Academy of Beijing Institute of Technology(Jiaxing) Jiaxing 314019China Electrical Engineering Program Division of Physical Sciences and EngineeringKing Abdullah University of Science and TechnologyThuwal 23955Saudi Arabia

The extra-large scale multiple-input multiple-output(XL-MIMO)for the beyond fifth/sixth generation mobile communications is a promising technology to provide Tbps data transmission and stable access ***,the extremely large antenna array aperture arouses the channel near-field effect,resulting in the deteriorated data rate and other challenges in the practice communication ***,multi-panel MIMO technology has attracted extensive attention due to its flexible configuration,low hardware cost,and wider *** combining the XL-MIMO and multi-panel array structure,we construct multi-panel XL-MIMO and apply it to massive Internet of Things(IoT)***,we model the multi-panel XL-MIMO-based near-field channels for massive IoT access scenarios,where the electromagnetic waves corresponding to different panels have different angles of arrival/departure(AoAs/AoDs).Then,by exploiting the sparsity of the near-field massive IoT access channels,we formulate a compressed sensing based joint active user detection(AUD)and channel estimation(CE)problem which is solved by AMP-EM-MMV *** simulation results exhibit the superiority of the AMP-EM-MMV based joint AUD and CE scheme over the baseline algorithms.

关键词： extra-large scale MIMO massive IoT access active user detection channel estimation multipanel approximate message passing

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A model of service-oriented architecture of e-certification system to support boat registration and site visit inspection to support maritime safety and crew health inspection

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Marine Systems and Ocean technology 2023年第1-2期18卷 45-63页

作者： Saputra, Diaz Gaol, Ford Lumban Abdurachman, Edi Sensuse, Dana Indra Matsuo, Tokuro Department of Computer Science BINUS Graduate Program - Doctor of Computer Science Bina Nusantara University Jakarta11480 Indonesia Department of Computer Science Binus Graduate Program - Master in Information System Bina Nusantara University Jakarta11480 Indonesia Department of Research in Management Bina Nusantara University Jakarta Indonesia Faculty of Computer Science University of Indonesia Jakarta Indonesia Advanced Institute of Industrial Technology Tokyo Japan City University of Macau China Asia University Taichung Taiwan

This article describes the architecture of software services that provide registration of small boat data to build maritime safety. The proposed system architecture which so-called SIMKAPEL aims to support small boat registration for maritime safety. It is developed from a conventional service-oriented architecture (SOA) with an open standard for data interoperability between elements. The goal of this research is to implement and evaluate the proposed architecture to support small boat registration and e-certification. Several parts of the architecture have been implemented as a platform that provides core services and data sources to be used by Ministry of Transportation, Directorate General of Sea Transportation, and other government agencies. Finally, the proposed SIMKAPEL platform with the SOA architecture is evaluated for its benefits to users through the expert opinion survey to measure its efficiency. The analysis results showed that SOA-based SIMKAPEL is feasible to use as a boat e-certification system. Furthermore, experiment results provide three parameters (e.g., maritime safety, namely, cargo/passengers, boat safety facilities, and maritime safety systems) with efficiency values of 42%, 46%, and 42%, respectively. The parameter with the highest efficiency shows a big effect on the level of safety of the boat and passengers. Thus, the parameters that need to be prioritized and need boat owners’ attention are cargo/passenger, boat safety equipment, and maritime safety system. © 2023, The Author(s).

关键词： Boat e-certification Boat online certification Cloud-based service Integrated system SOA architecture

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AllWeather-UsableWearable Dual Energy Harvester for Outdoor Sustainable Operation

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SusMat 2025年第1期5卷 159-170页

作者： Yeongju Jung Jiyong Ahn Ji-Seok Kim Junhyuk Bang Minwoo Kim Seongmin Jeong Jinwoo Lee Seonggeun Han Il-Kwon Oh Seung Hwan Ko Applied Nano and Thermal Science Lab Department of Mechanical EngineeringSeoul National UniversitySeoulRepublic of Korea National Creative Research Initiative for Functionally Antagonistic Nano-Engineering Department of Mechanical EngineeringSchool of Mechanical and Aerospace EngineeringKorea Advanced Institute of Science and Technology(KAIST)DaejeonRepublic of Korea Department of Mechanical Roboticsand Energy EngineeringDongguk UniversitySeoulRepublic of Korea Device Solutions Research Samsung ElectronicsHwaseong-siRepublic of Korea Institute of Engineering Research/Institute of Advanced Machinery and Design(SNU-IAMD) Seoul National UniversitySeoulRepublic of Korea Interdisciplinary Program in Bioengineering Seoul National UniversitySeoulRepublic of Korea

Sustainable power sources for outdoor wearable electronics are essential for the continuous operation of wearable ***,the current lack of engineering design that can harvest energy regardless of weather conditions presents a significant *** this regard,this study introduces a wearable,breathable all-weather usable dual energy harvester(AWuDEH)that can seamlessly generate electrical energy regardless of weather *** this study,the AWuDEH integrated with the thermoelectric generator and the droplet-based electricity generator is *** AWuDEH,especially engineered with a bi-functional top substrate for radiative cooling and electrification,achieves sustainable energy harvesting outdoors,thereby addressing the conventional challenge associated with the necessity for separate energy harvesters tailored to outdoor usage contingent on weather *** device reaches a maximum power output of 14.6μW cm^(-2)under simulated sunny conditions and generates a much more enhanced thermoelectric power of 74.78μW cm^(-2)and a droplet-based electric power of 256.25 mW m^(-2)in rainy *** proof,this study developed self-powered wearable electronics capable of acquiring physiological signals in simulated outdoor *** study presents a promising advancement in wearable technology,offering a potent solution for sustainable energy harvesting independent of weather conditions.

关键词： all-weather usable droplet-based electricity generator hybrid architecture outdoor sustainable operation thermoelectric generator

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X-photon 3D lithography by fs-oscillators:wavelength-independent and photoinitiator-free

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Light(advanced Manufacturing) 2024年第4期5卷 89-101页

作者： Dimitra Ladika Antanas Butkus Vasileia Melissinaki Edvinas Skliutas Elmina Kabouraki Saulius Juodkazis Maria Farsari Mangirdas Malinauskas Institute of Electronic Structure and Laser Foundation for Research and Technology-Hellas70013 HeraklionGreece Department of Materials Science and Technology University of Crete70013HeraklionCrete Laser Research Center Faculty of PhysicsVilnius UniversitySaulėtekio Ave.10LT-10223 VilniusLithuania Optical Sciences Centre and ARC Training Centre in Surface Engineering for Advanced Materials(SEAM) School of ScienceSwinburne University of TechnologyMelbourneAustralia WRH Program International Research Frontiers Initiative(IRFI)Tokyo Institute of Technology Nagatsuta-choMidori-kuYokohamaJapan

Laser direct writing employing multi-photon 3D polymerisation is a scientific and industrial tool used in various fields such as micro-optics,medicine,metamaterials,programmable materials,etc.,due to the fusion of highthroughput and fine features down to hundreds of *** limitations of technology applicability emerge from photo-resin properties,however any material modifications can strongly affect its printability,as photoexcitation conditions alter as *** we present wavelength-independent 3D polymerisation using low peak power laser *** pulse repetition rate and fast laser direct writing was employed for advancing additive manufacturing out of the SZ2080^(TM)photo-resist without any *** of 517 nm,780 nm,and 1035 nm are shown to be suitable for producing 300 nm polymerized features even at high-up to 10^(5)μm/s-writing *** of organic-inorganic ratio in hybrid material results in shift and decrease of the dynamic fabrication window,yet not prohibiting the *** energy deposition per focal volume is achieved due to localized heating enabling efficient 3D *** spatio-selective photo-chemical crosslinking widens optical manufacturing capacity of non-photo-sensitive materials.

关键词： 3D polymerisation Nonlinear absorption Multi-photon absorption Laser direct writing Additive manufacturing Material engineering Organic-inorganic polymers SZ2080^(TM) Photosensitizer

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AI Fairness-From Machine Learning to Federated Learning

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Computer Modeling in Engineering & sciences 2024年第5期139卷 1203-1215页

作者： Lalit Mohan Patnaik Wenfeng Wang Consciousness Studies Program School of HumanitiesNational Institute of Advanced StudiesBangalore560012India Research Institute of Intelligent Engineering and Data Applications Shanghai Institute of TechnologyShanghai201418China Research Center of Ecology and Environment of Central Asia Chinese Academy of SciencesUrumqi830011China Applied Nonlinear Science Lab Anand International College of EngineeringJaipur391320India London Institute of Technology The ASE-London CTI of SCOLondonCR26EQUK Sino-Indian Joint Research Center of AI and Robotics The IMT InstituteBhubaneswar752054India

This article reviews the theory of fairness in AI-frommachine learning to federated learning,where the constraints on precision AI fairness and perspective solutions are also *** a reliable and quantitative evaluation of AI fairness,many associated concepts have been proposed,formulated and ***,the inexplicability of machine learning systems makes it almost impossible to include all necessary details in the modelling stage to ensure *** privacy worries induce the data unfairness and hence,the biases in the datasets for evaluating AI fairness are *** imbalance between algorithms’utility and humanization has further reinforced *** for federated learning systems,these constraints on precision AI fairness still *** solution is to reconcile the federated learning processes and reduce biases and imbalances accordingly.

关键词： Formulation evaluation classification constraints imbalance biases

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Erosion-corrosion resistance of Mo-Ti- and Ni-Cr-Mo-alloyed medium-carbon martensitic steels: a critical analysis of synergistic effect of erosion and corrosion

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Journal of Iron and Steel research International 2022年第8期29卷 1299-1311页

作者： De-fa Li Hang-yu Dong Cheng-yang Hu Kai-ming Wu Serhii Yershov Oleg Isayev School of Mechanical and Vehicle Engineering West Anhui UniversityLuan 237012AnhuiChina The State Key Laboratory of Refractories and Metallurgy Hubei Province Key Laboratory of Systems Science on Metallurgical ProcessingInternational Research Institute for Steel TechnologyWuhan University of Science and TechnologyWuhan 430081HubeiChina Laboratory for Excellence in Advanced Steel Research Materials Science and Engineering ProgramDepartment of MetallurgicalMaterials and Biomedical EngineeringUniversity of Texas at El PasoEl PasoTX 79968USA

Grain refinement renders Mo-Ti-alloyed medium-carbon martensitic steel to exhibit high hardness,high strength,and good toughness,but the erosion-corrosion resistance of steel in a corrosive slurry environment is not ***-Ti-alloyed medium-carbon martensitic steel is compared with Ni-Cr-Mo-alloyed medium-carbon martensitic steel,and the erosion-corrosion resistance of those two steels under impingement by NaCl solution with gravels has been *** components,pure-corrosion rate,pure-erosion rate,and synergistic effect of erosion and corrosion(SEEC)of erosion-corrosion rate,were *** pure-corrosion and pure-erosion rates of Mo-Ti-alloyed steel were higher than those of Ni-Cr-Mo-alloyed one;however,its erosion-corrosion rate was relatively lower because of a weak *** plastic deformation and work hardening due to gravel impingement were the essential reason for SEEC,which could be reduced by grain refinement,and consequently,Mo-Ti-alloyed steel with finer grains had better erosion-corrosion *** refinement could be an effective way to improve the erosion-corrosion resistance of martensitic steels.

关键词： Grain refinement Mo-Ti alloying Ni-Cr-Mo alloying Martensite Erosion-corrosion

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Unified throughout-pore microstructure enables ultrahigh separator porosity for robust high-flux lithium batteries

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Electron 2023年第1期1卷 37-49页

作者： Dongjiang Chen Yuanpeng Liu Chao Feng Yuhui He Shengyu Zhou Botao Yuan Yunfa Dong Haodong Xie Guangfeng Zeng Jiecai Han Weidong He National Key Laboratory of Science and Technology on Advanced Composites in Special Environments Harbin Institute of TechnologyHarbinChina Center for Composite Materials and Structures Harbin Institute of TechnologyHarbinChina State Key Laboratory of Electronic Thin Film and Integrated Devices University of Electronic Science and Technology of ChinaChengduChina Chongqing Research Institute Harbin Institute of TechnologyChongqingChina Interdisciplinary Graduate Program in Materials Science Vanderbilt UniversityNashvilleTennesseeUSA

With small thickness,commercial polyolefin separators own low porosity to ensure sufficient thermomechanical properties,resulting in tortuous and enlarged Li+diffusion pathways that induce large overpotentials and detrimental dendrite *** a dilemma,the exploration of highly porous separators has been challenged by their large thickness,impairing the applicability of such ***,an ultraporous architecture is designed to shorten Li+transfer pathways by impregnating electrolyteaffinitive poly(vinylidene fluoride-co-hexafluoropropylene)into ultralight~3μm 3D-polytetrafluoroethylene scaffold(abbreviated as UP3D).The UP3D separator with a porosity of 74%gives rise to 70%enhancement in Li+transference and 77%reduction in Li+transfer resistance(2.67 mΩmm^(−1))and thus enables an ultrahigh Li+flux of 22.7 mA cm^(−2),effectively alleviating Li+concentration gradient across the *** the separator,the LiFePO4 half cell delivers a capacity of 118 mAh g^(−1) with an unparalleled capacity retention of 90%after 1000 cycles at 2 C,and a graphite||LiNi_(0.6)Co_(0.2)Mn_(0.2)O_(2)pouch full cell delivers an areal energy density of 6.8 mWh cm^(−2)at 8.848 mA(1.4 mA cm^(−2))with a high cathode loading of 134.9 *** results,together with the scalable production of the separator,reflect its promising potential in high-flux battery applications of separators that require both ultrahigh porosity and reliability.

关键词： Li deposition Li-ion batteries polytetrafluoroethylene separator ultrahigh porosity

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