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Rare earth element Ce enables high thermoelectric performance in n-type SnSe polycrystals

Journal of Materials science & technology 2023年第12期143卷 234-241页

作者： Shan Li Li Yin Yijie Liu Xiaodong Wang Chen Chen Qian Zhang School of Civil Aviation Northwestern Polytechnical UniversityXi’an 710072China School of Materials Science and Engineering and Institute of Materials Genome&Big DataHarbin Institute of TechnologyShenzhen 518055China State Key Laboratory of Advanced Welding and Joining Harbin Institute of TechnologyHarbin 150001China

SnSe exhibits excellent thermoelectric performance in both n-and p-type single crystals,but its n-type polycrystals are restricted because of the lower electrical ***,we dually introduced rare earth element Ce and PbTe to optimize the thermoelectric properties of n-type SnSe *** is demonstrated that Ce is an effective cationic dopant to convert SnSe from p-to n-type conductor,and an enhanced peak zT value of∼0.9 at 823 K was obtained in Sn 0.97 Ce 0.03 Se due to the improved power ***,PbTe alloying not only reduced the band gap to increase the carrier concentration,but also enhanced the density-of-states effective mass,and hence further increased the power factor in the whole measured temperature ***,the lattice thermal conductivity was significantly reduced owing to the enhanced phonon scattering by the mass and strain *** a result,the peak zT value was increased to∼1.3 for Sn 0.9 Pb 0.07 Ce 0.03 Se 0.93 Te 0.07 together with a high average zT value of∼0.52 in the temperature range of 300 to 823 K.

关键词： Thermoelectric N-type SnSe Ce doping PbTe alloying

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Sign reversal and manipulation of anomalous Hall resistivity in facing-target sputtered Pt/Mn_(4)N bilayers

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Rare Metals 2023年第2期42卷 591-601页

作者： Ze-Yu Zhang Jia-Wei Jiang Xiao-Hui Shi Xiang Liu Xia Chen Zhi-Peng Hou Wen-Bo Mi Tianjin Key Laboratory of Low Dimensional Materials Physics and Preparation Technology School of ScienceTianjin UniversityTianjin300354China School of Physics and Electronic Engineering Linyi UniversityLinyi276000China College of Science Civil Aviation University of ChinaTianjin300300China Guangdong Provincial Key Laboratory of Optical Information Materials and Technology&Institute for Advanced Materials South China Academy of Advanced OptoelectronicsSouth China Normal UniversityGuangzhou510006China

The magnetic and electronic transport properties manipulated by spin-orbit torque have been devoted much attention as they show a great promise for future spintronic ***,the spin dependent transport properties of the facing-target sputtered Pt/Mn_(4)N bilayers on MgO(001)substrates have been investigated *** Hall resistivity of Pt/Mn_(4)N bilayers is strongly dependent on temperature,applied current intensity,Mn_(4)N and Pt layer *** temperature-dependent sign reversal of anomalous Hall resistivity appears in Pt/Mn_(4)N bilayers,which is dominated by the competition between the magnetic proximity and spin Hall ***,the magnitude of anomalous Hall resistivity can be manipulated by applied current *** critical and saturation currents are related to Mn_(4)N and Pt layer ***,a Dzyaloshinskii-Moriya interaction coefficient(D)of 5.63 mJ·m^(-2)is calculated in Pt/Mn_(4)N/MgO *** details of the anomalous Hall effects in Pt/Mn_(4)N bilayers are helpful to understand the interfacial effects between heavy metals and ferrimagnets.

关键词： Pt/Mn_(4)N bilayer Hall resistivity Magnetic proximity effect Spin Hall effect(SHE) DzyaloshinskiiMoriya interaction(DMI)

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A Grey Wolf Optimizer Variant with Weighted-leader Strategy 24

A Grey Wolf Optimizer Variant with Weighted-leader Strategy

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3rd International Conference on Signal Processing, Computer Networks and Communications, SPCNC 2024

作者： Liang, Yajun Yan, Su Ma, Qian Huang, Shunlun Liu, Xin China Aerodynamics Research & Development Center Sichuan Mianyang China Science and Technology on Complex Aviation Systems Simulation Laboratory Beijing China State Key Laboratory of Air Traffic Management System Beijing China Beijing Aviation Meteorological Institute Beijing China

ISBN: (纸本)9798400710834

To enhance the convergence capability of grey wolf optimizer (GWO), this research investigates an evolved GWO using weighted-leader strategy (WLS), namely WLSGWO. The key issue of WLS is realizing the adaptive adjustment of position weighting according to the control parameters, thus well overcoming the drawback of premature convergence in the basic GWO. The newly developed method’s performance is assessed through experiments conducted on a standardized test suite. Additionally, comparisons are made by utilizing GWO alongside other advanced optimization techniques. The results of non-parametric studies validate the outperformance of the WLSGWO, thus proving the efficiency of the proposed strategy. © 2024 Copyright held by the owner/author(s).

关键词： Swarm intelligence

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Outer delocalized electron aggregation of bromide bridged core–shell CuBr@C for hydrogen evolution reaction

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Nano Research 2023年第5期16卷 6608-6614页

作者： Tianyi Xu Ruoyu Li Lei Zhang Dongxu Jiao Yilong Dong Ming Gong Dantong Zhang Jinchang Fan Dewen Wang Yanhua Liu Xiao Zhao Wei Zhang Weitao Zheng Xiaoqiang Cui State Key Laboratory of Automotive Simulation and Control School of Materials Science and EngineeringKey Laboratory of Automobile Materials of MOEJilin Provincial International Cooperation Key Laboratory of High-Efficiency Clean Energy MaterialsElectron Microscopy CenterJilin UniversityChangchun 130012China College of Chemistry Jilin UniversityChangchun 130012China Center of Multiscale Crystal Materials Research Institute of Advanced Materials Science and EngineeringShenzhen Intitute of Advanced TechnologyChinese Academy of ScienceShenzhen 518055China

Modulation of the surface electron distribution is a challenging problem that determines the adsorption ability of catalytic ***,we address this challenge by bridging the inner and outer layers of the core–shell structure through the bridge Br *** shell wrapped copper bromide nanorods(CuBr@C)are constructed for the first time by chemical vapour deposition with hexabromobenzene(HBB).HBB pyrolysis provides both bridge Br atom and C *** C shell protects the stability of the internal halide structure,while the bridge Br atom triggers the rearrangement of the surface electrons and exhibits excellent electrocatalytic ***,the hydrogen evolution reaction(HER)activity of CuBr@C is significantly better than that of commercial N-doped carbon nanotubes,surpassing commercial Pt/C at over 200 mA·cm^(−2).Density functional theory(DFT)calculations reveal that bridge Br atoms inspire aggregation of delocalized electrons on C-shell surfaces,leading to optimization of hydrogen adsorption energy.

关键词： bridge Br atoms delocalized electron aggregation core–shell nanorods C-shell wrapped CuBr hydrogen evolution reaction

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Influence of Alloying Elements Content on High Temperature Properties of Ti-V-Cr and Ti-Al-V Series Titanium Alloys: A JMatPro Program Calculation Study

Influence of Alloying Elements Content on High Temperature P...

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Chinese Materials Conference 2022-2023

作者： Sun, Ruochen Mi, Guangbao Aviation Key Laboratory of Science and Technology on Advanced Titanium Alloys AECC Beijing Institute of Aeronautical Materials Beijing100095 China

For the issues of high temperature performance affected by the alloying elements content in Ti-V-Cr and Ti-V-Cr alloys, the thermodynamic calculation method based on JMatPro program was applied in this study. The research is mainly focused on the analysis of phase composition, thermodynamic parameters and mechanical properties of Ti-Al-V and Ti-V-Cr series alloys with different element proportions under high temperature environment. Those obtained results show that the proportion of Al in Ti-Al-V alloys has a great influence on the high temperature properties. Increasing the content of Al not only increases the transformation temperature of β single-phase structure and delays the transformation process of α/β microstructure to β single-phase structure, but also helps to improve the high temperature thermal conductivity and elastic deformation resistance of the alloy. In Ti-V-Cr alloys, the influence of V element on high temperature properties is mainly focused on the improvement of thermal conductivity and high temperature deformation properties, while the influence of Cr element is relatively weak. Besides, adding a small amount of Al element to Ti-V-Cr alloy can further improve the thermal conductivity of the alloy. The Young's modulus of the Ti-V-Cr alloy increases when 0.3%-1% of C element is added. Finally, the effect of Si element on the high temperature elastic deformation of the alloy is relatively weak. © Published under licence by IOP Publishing Ltd.

关键词： Titanium alloys

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Rubik’s cube as in-situ programmable matter and a reconfigurable mechanical metamaterial

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science China(Technological sciences) 2024年第10期67卷 3221-3234页

作者： ZHU ShaoWei CHEN Huan YANG XiaoQiang TAN Li JIN Shuai CHEN LiMing LIU Tao TAN XiaoJun WANG LianChao WANG Bing MUAMER Kadic State Key Laboratory of Coal Mine Disaster Dynamics and Control Chongqing UniversityChongqing 400030China College of Aerospace Engineering Chongqing UniversityChongqing 400030China School of Civil Aviation Northwestern Polytechnical UniversityXi’an 710129China National Key Laboratory of Science and Technology on Advanced Composites in Special Environments Harbin Institute of TechnologyHarbin 150080China Institut FEMTO-ST CNRS UMR 6174University BourgogneFranche-ComtBesan¸con 25000France

As part of the 4th industrial revolution,programmable mechanical metamaterials exhibit great application potential in flexible robotics,vibration control,and impact ***,maintaining a programmed state without sustaining the external stimulus is often challenging and leads to additional energy *** by Rubik’s cube,we design and study an in-situ programmable and distribution-reconfigurable mechanical metamaterial(IPDR-MM).A matrix model is developed to model IPDR-MMs and describe their morphological *** on this model,the reinforcement learning method is employed to find the pathways for morphological *** find that IPDR-MMs have controllable stiffness across several orders of magnitude and a wide range of adjustable anisotropies through morphology ***,because of the independence of the directions of morphology transformation and bearing,IPDR-MMs exhibit good stability in bearing and can readily achieve high *** Rubik’s cube-inspired design concept is also instructive for other deformable structures and metamaterials,and the current version of the proposal should be sufficiently illustrative to attract and broaden interdisciplinary interests.

关键词： mechanical metamaterials in-situ programmable distribution-reconfigurable Rubik’s cube controllable stiffness and anisotropy

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Efficient and selective recovery of Gd(Ⅲ)via polyethyleneimine modification of lanthanum-based metal-organic frameworks

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Journal of Rare Earths 2024年第1期42卷 210-219,I0007页

作者： Wenhao Li Lijinhong Huang Bin Xiao Xiaoguang Duan Haike Li Lang Li Wanfu Huang Ganzhou Key Laboratory of Basin Pollution Simulation and Control Jiangxi University of Science and TechnologyGanzhou341000China Innovation Center for Water Quality Security Technology at Ganjiang River Basin Jiangxi University of Science and TechnologyGanzhou341000China Faculty of Science and Engineering WA School of Mines:MineralsEnergy and Chemical EngineeringCurtin UniversityWAAustralia School of Architecture and Design Jiangxi University of Science and TechnologyGanzhou341000China School of Resources and Architectural Engineering Gannan University of Science and TechnologyGanzhou341000China School of Chemical Engineering and Advanced Materials The University of AdelaideAdelaideSA5005Australia School of Resource and Environmental Engineering Jiangxi University of Science and TechnologyGanzhou341000China

With the development of the economy and the increasing demand for environmental protection,the efficient and selective recovery of Gd(Ⅲ)from actual wastewater is of critical *** this work,lanthanum-based metal-organic framework(LaBDC)materials were prepared by a hydrothermal method,and then polyethyleneimine(PEI)and LaBDC were combined by an impregnation method to form a novel LaBDC@xPEI *** prepared materials were characterized using Fourier transfo rm infrared spectroscopy(FTIR),X-ray diffraction(XRD),scanning electron microscopy(SEM),energy dispersive X-ray spectroscopy(EDX),B runauer-Emmett-Teller(BET),thermogravimetric analysis(TGA)and X-ray photoelectron spectroscopy(XPS).Experiments show that LaBDC@50%PEI has the highest adsorption capacity(181.77 mg/g)among lanthanum-based MOFs with different PEI loadings at pH=5.5,which is about 5.1 times that of bare *** adsorption isotherm analysis shows that LaBDC@50%PEI follows the Langmuir *** addition,the adsorption kinetics of LaBDC@50%PEI follows a pseudo-second-order kinetic model,indicating that the adsorption process is chemical *** is worth noting that LaBDC@50%PEI maintains good adsorption performance and stability after three recycling tests,and exhibits excellent selectivity in cation interference ***,the LaBDC@50%PEI composites possess good stability and hold great promises in rapid recovery of Gd(Ⅲ)from practical aqueous environments.

关键词： Wet-impregnation method Polyethylene imine Metaleorganic frameworks Lanthanum Recovery of Gd(Ⅲ) Rare earths

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An architecture decomposition method of pneumatic catapult system based on OPM and DSM

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Chinese Journal of Aeronautics 2023年第8期36卷 168-181页

作者： Lu GAN Gang YANG Xianhui LI Enze ZHU Hu CHEN Xiaohui WEI State Key Laboratory of Mechanics and Control of Aerospace Structures Nanjing University of Aeronautics and AstronauticsNanjing 210016China Key Laboratory of Fundamental Science for National Defense-Advanced Design Technology of Flight Vehicle Nanjing University of Aeronautics and AstronauticsNanjing 210016China College of General Aviation and Flight Nanjing University of Aeronautics and AstronauticsNanjing 210016China

The architecture strategy of the Unmanned Aerial Vehicle(UAV)pneumatic launch system should continue to evolve to adapt to complex and variable operating *** representation,decomposition perspective,and cluster analysis play a vital role in the early phase of system architecture *** order for the system to emerge anticipated and desirable intrinsic functional properties,an architecture decomposition method based on the ObjectProcess Methodology(OPM)and Design Structure Matrix(DSM)is put forward in this *** OPM is proposed to model the UAV launch process formally,and the matrix representation of the architecture of the pneumatic launch system is *** the extension of the definition and operations of DSM,with the Idicula-Gutierrez-Thebeau Algorithm plus(IGTA+)clustering algorithm,the transformation of the pneumatic launch system architecture from process decomposition to function decomposition is demonstrated in this *** analysis shows that the architecture decomposition of the pneumatic launch system meets the functional requirements of stakeholders.

关键词： Architecture decomposition Cluster analysis Design structure matrix Object-process methodology Pneumatic catapult system

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Applying machine-learning screening of single transition metal atoms anchored on N-dopedγ-graphyne for carbon monoxide electroreduction toward C_(1)products

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Nano Research 2023年第8期16卷 11511-11520页

作者： Dongxu Jiao Dantong Zhang Dewen Wang Jinchang Fan Xingcheng Ma Jingxiang Zhao Weitao Zheng Xiaoqiang Cui State Key Laboratory of Automotive Simulation and Control School of Materials Science and Engineeringand Key Laboratory of Automobile Materials of MOEJilin UniversityChangchun 130012China College of Chemistry and Chemical Engineering and Key Laboratory of Photonic and Electronic Bandgap MaterialsMinistry of EducationHarbin Normal UniversityHarbin 150025China Multiscale Crystal Materials Research Center Shenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhen 518055China

Carbon monoxide electroreduction(COER)has been a key part of tandem electrolysis of carbon dioxide(CO_(2)),in which searching for high catalytic performance COER electrocatalysts remains a great ***,by means of density functional theory(DFT)computations,we explored the potential of a series of transition metal atoms anchored on N-dopedγ-graphyne(TM@N-GY,TM from Ti to Au)as the COER *** found that the final product selectivity of these single-atom catalysts depended on the position of the metal atom in the periodic table,with metals in the front and middle of each periodic period exhibiting high selectivity for CH_(4),while metals in the back producing CH_(3)*** learning(ML)found that metal atomic number was intrinsic to the difference in COER performance of these single-atom catalysts(SACs).The free energy changes showed that Mn@N-GY and Ni@N-GY exhibited outstanding COER catalytic performance for producing CH_(4)and CH_(3)OH,*** results provide theoretical and experimental guidance for designing efficient COER catalysts to generate C_(1)products.

关键词： CO electroreduction single atom catalysts γ-graphyne density functional theory machine learning

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Ordered mesoporous materials for water pollution treatment:Adsorption and catalysis

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Green Energy & Environment 2024年第8期9卷 1239-1256页

作者： Peng Zhang Mingming He Wei Teng Fukuan Li Xinyuan Qiu Kexun Li Hao Wang College of Environmental Science and Engineering MOE Key Laboratory of Pollution Processes and Environmental CriteriaTianjin Key Laboratory of Environmental Remediation and Pollution TreatmentTianjin Key Laboratory of Environmental Technology for Complex Trans-Media PollutionNankai UniversityTianjin300350China Department of Chemistry and State Key Laboratory Marine Pollution Hong Kong Institute for Advanced Study City University of Hong KongHong Kong999077China State Key Laboratory for Pollution Treatment College of Environmental Science and EngineeringShanghai Institute of Pollution Treatment and Ecological SecurityTongji UniversityShanghai200092China State Key Laboratory of Simulation and Regulation of Water Cycles in River Basins China Institute of Water Resources and Hydropower ResearchBeijing100038China

To meet the growing emission of water contaminants,the development of new materials that enhance the efficiency of the water treatment system is *** mesoporous materials provide opportunities in environmental processing applications due to their exceptionally high surface areas,large pore sizes,and enough pore *** properties might enhance the performance of materials concerning adsorption/catalysis capability,durability,and *** this review,we enumerate the ordered mesoporous materials as adsorbents/catalysts and their modifications in water pollution treatment from the past decade,including heavy metals(Hg^(2+),Pb^(2+),Cd^(2+),Cr^(6+),etc.),toxic anions(nitrate,phosphate,fluoride,etc.),and organic contaminants(organic dyes,antibiotics,etc.).These contributions demonstrate a deep understanding of the synergistic effect between the incorporated framework and homogeneous active ***,the challenges and perspectives of the future developments of ordered mesoporous materials in wastewater treatment are *** work provides a theoretical basis and complete summary for the application of ordered mesoporous materials in the removal of contaminants from aqueous solutions.

关键词： Water pollution treatment Ordered mesoporous materials Toxic contaminants Adsorption Catalysis

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