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arXiv 2023年

作者： Zheng, Ru-You Sun, Xiang-Xiang Shen, Guo-Fang Geng, Li-Sheng School of Physics Beihang University Beijing102206 China School of Nuclear Science and Technology University of Chinese Academy of Sciences Beijing100049 China Institut für Kernphysik Institute for Advanced Simulation Jülich Center for Hadron Physics Forschungszentrum Jülich JülichD-52425 Germany CAS Key Laboratory of Theoretical Physics Institute of Theoretical Physics Chinese Academy of Sciences Beijing100190 China Peng Huanwu Collaborative Center for Research and Education Beihang University Beijing100191 China Beijing Key Laboratory of Advanced Nuclear Materials and Physics Beihang University Beijing102206 China Institute of Modern Physics Chinese Academy of Sciences Guangdong Province Huizhou516000 China

Magicity, or shell closure, plays an important role in our understanding of complex nuclear phenomena. In this work, we employ one of the state-of-the-art density functional theories, the deformed relativistic Hartree-Bogoliubov theory in continuum (DRHBc) with the density functional PC-PK1, to investigate the evolution of the N = 20, 28, 50 shell closures in the 20 6 Z 6 30 region. We show how these three conventional shell closures evolve from the proton drip line to the neutron drip line by studying the charge radii, two-neutron separation energies, two-neutron gaps, quadrupole deformations, and single-particle levels. In particular, we find that in the 21 6 Z 6 27 region, the N = 50 shell closure disappears or becomes quenched, mainly due to the deformation effects. Similarly, both experimental data and theoretical predictions indicate that the N = 28 shell closure disappears in the Mn isotopic chain, also predominantly due to the deformation effects. The DRHBc theory predicts the existence of the N = 20 shell closure in the Ca, Sc, and Ti isotopic chains, but the existing data for the Ti isotopes suggests the contrary, and therefore more investigations are needed. Copyright © 2023, The Authors. All rights reserved.

关键词： Neutrons

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Roof greening in major Chinese cities possibly afford a large potential carbon sink

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science Bulletin 2024年第20期69卷 3216-3220页

作者： Chao Yang Yinghui Zhang Min Chen Song Zhu Yuzhi Tang Zhixin Zhang Wei Ma Huizeng Liu Junyi Chen Bohui Tang Dejin Zhang Zhengdong Huang Xuqing Wang Wei Tu Cuiling Liu Tiezhu Shi Haiying Xu Aihong Cui Fanyi Meng Tianhong Zhao Kai Guo Wenhao Guo Bi Fan Quande Qin Wuyang Hong Haishan Wu Bing Wang Jinrong Zeng Ka Wai Wu Qingquan Li Key Laboratory for Geo-Environmental Monitoring of Great Bay Area Ministry of Natural Resources&Guangdong Key Laboratory of Urban InformaticsShenzhen UniversityShenzhen 518060China School of Architecture and Urban Planning Shenzhen UniversityShenzhen 518060China Key Laboratory of Virtual Geographic Environment Ministry of EducationNanjing Normal UniversityNanjing 210023China Jiangsu Center for Collaborative Innovation in Geographical Information Resource Development and Application Nanjing 210023China International Research Center of Big Data for Sustainable Development Goals Beijing 100094China Shenzhen Zhiyuan Space Innovation Technology Co. LtdShenzhen 518060China Guangdong Laboratory of Artificial Intelligence and Digital Economy(SZ) Shenzhen 518107China School of Geography and Ocean Science Nanjing UniversityNanjing 210008China School of Geography Nanjing Normal UniversityNanjing 210023China School of Civil Engineering Chongqing Jiaotong UniversityChongqing 400074China Institute for Advanced Study&Shenzhen University Shenzhen 518060China Tiandu-Shenzhen University Deep Space Joint Laboratory Shenzhen UniversityShenzhen 518060China Faculty of Land Resource Engineering Kunming University of Science and TechnologyKunming 650093China Center for Hydrogeology and Environmental Geology China Geological SurveyBaoding 071051China Department of Landscape Architecture and Urban Planning Texas A&M UniversityTX 77840USA Department of Geography Hong Kong Baptist UniversityHong Kong 999077China College of Civil and Transportation Engineering Shenzhen UniversityShenzhen 518060China College of Big Data and Internet Shenzhen Technology UniversityShenzhen 518118China Faculty of Geosciences and Environmental Engineering Southwest Jiaotong UniversityChengdu 611756China College of Management Shenzhen UniversityShenzhen 518060China WeBank(Shenzhen)Co. LtdShenzhen 518060China Department of Aeronautical and Aviation Engineering The Hong Kong Polytechnic UniversityHong Kong 100872China Esri C

China is experiencing accelerated urbanisation,with a large number of people moving from rural to urban areas[1].It has resulted in large losses in the net primary production(NPP),biodiversity and carbon stocks and an increase in environmental pollution and CO_(2)emissions[2–4].In 2015,196 countries signed the Paris Agreement and committed to setting long-term goals to jointly manage climate change and reduce their individual emissions,aiming to control the increase in global average temperature from the pre-industrial level to below 2℃and to curtail the temperature rise within 1.5℃till the end of the 21st century[5].China is bolstering its efforts to achieve the climate change mitigation goals and has announced a plan for achieving carbon neutrality by 2060[6].The carbon neutrality goal poses a challenge to the current policies promoting rapid urbanisation across China.

关键词： jointly carbon goals

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Thin Film Composite Reverse Osmosis Membranes with Metal-Organic Coordination Complexes Stabilized Cnts Interlayer for Enhanced Removal of Trace Organic Contaminants

SSRN

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SSRN 2023年

作者： Liu, Lin Mei, Ying Lin, Xiaocheng Li, Weiyi Liu, Xin Fan, Fuqiang Yang, Yi Research and Development Center for Watershed Environmental Eco-Engineering Advanced Institute of Natural Sciences Beijing Normal University Zhuhai Campus Zhuhai519087 China State Key Laboratory of Water Environment Simulation School of Environment Beijing Normal University Beijing100875 China College of Chemical Engineering Fuzhou University Fujian Fuzhou350116 China School of Environmental Science and Engineering Southern University of Science and Technology Shenzhen518005 China Center for Water Research Advanced Institute of Natural Sciences Beijing Normal University Zhuhai519087 China College of Education for the Future Faculty of Arts and Sciences Beijing Normal University Zhuhai519087 China

Reverse osmosis (RO) has been recognized as a reliable technique for wastewater reclamation. To enhance its rejection of trace organic contaminants (TrOCs), a novel strategy was proposed to improve reverse osmosis (RO) membranes by fabricating thin-film nanocomposite membrane (TFNi) with a TA-Fe3+/CNTs interlayer. The TFNi-30 membrane was obtained by optimizing the loading capacity. This optimized membrane gave rise to an enhanced water permeance of 3.2 ± 0.2 L m-2 h-1 bar-1, which was two times higher than that of the control membrane (1.1 ± 0.2 L m-2 h-1 bar-1), while achieving a considerably higher rejection of inorganic salts and trace organic contaminants (TrOCs) thanks to the formation of a denser polyamide rejection layer. In addition, the specific roles of the interlayer structure in determining the separation performance of RO membranes were investigated by tailoring the support-free RO membranes and comparing them with the conventional membranes. This study would provide a peer reference for designing high performance RO membranes for wastewater reclamation via the TFNi strategy. © 2023, The Authors. All rights reserved.

关键词： Reverse osmosis

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Coupled Pacific Rim megadroughts contributed to the fall of the MingDynasty’s capital in 1644 CE

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science Bulletin 2024年第19期69卷 3106-3114页

作者： Feng Chen Tao Wang Xiaoen Zhao Jan Esper Fredrik Charpentier Ljungqvist Ulf Büntgen Hans W.Linderholm David Meko Hongna Xu Weipeng Yue Shijie Wang Yujiang Yuan Jingyun Zheng Wei Pan Fidel Roig Martín Hadad Mao Hu Jiachang Wei Fahu Chen Yunnan Key Laboratory of International Rivers and Transboundary Eco-Security Institute of International Rivers and Eco-SecurityYunnan UniversityKunming 650504China Southwest United Graduate School Kunming 650504China Climate Change Research Center and Nansen-Zhu International Research Centre Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China Department of Geography Johannes Gutenberg UniversityMainz 55099Germany Global Change Research Institute(CzechGlobe) Czech Academy of SciencesBrno 60300Czech Republic Department of History Stockholm UniversityStockholm 10691Sweden Bolin Centre for Climate Research Stockholm UniversityStockholm 10691Sweden Swedish Collegium for Advanced Study LinneanumUppsala 75238Sweden Department of Geography University of CambridgeCambridge CB23ENUK Department of Geography Faculty of ScienceMasaryk UniversityBrno 61137Czech Republic Swiss Federal Research Institute(WSL) Birmensdorf 8903Switzerland Regional Climate Group Department of Earth SciencesUniversity of GothenburgGothenburg 40530Sweden Laboratory of Tree-Ring Research University of ArizonaTucson AZ 85721USA Collaborative Innovation Center on Forecast and Evaluation of Meteorological Disasters(CIC FEMD) Nanjing University of Information Science and TechnologyNanjing 210044China Key Laboratory of Tree-ring Physical and Chemical Research Institute of Desert MeteorologyChina Meteorological AdministrationUrumqi 830002China Key Laboratory of Land Surface Pattern and Simulation Institute of Geographical Sciences and Natural Resources ResearchChinese Academy of SciencesBeijing 100101China Key Laboratory of Digital Human Technology R&D and Application of Yunnan Provincial Department of Education Yunnan UniversityKunming 650504China Laboratorio de Dendrocronología e Historia Ambiental IANIGLA-CCT CONICET-Universidad Nacional de CuyoMendoza 5500Argentina Hémera Centro de Observación de La Tierra Escuela de Ingeniería ForestalFacultad de CienciasUniversidad MayorHuechuraba 85

Historical documents provide evidence for regional droughts preceding the political turmoil and fall of Beijing in 1644 CE,when more than 20 million people died in northern China during the late Ming famine ***,the role climate and environmental changes may have played in this pivotal event in Chinese history remains ***,we provide tree-ring evidence of persistent megadroughts from1576 to 1593 CE and from 1628 to 1644 CE in northern China,which coincided with exceptionally cold summers just before the fall of *** analysis reveals that these regional hydroclimatic extremes are part of a series of megadroughts along the Pacific Rim,which not only impacted the ecology and society of monsoonal northern China,but likely also exacerbated external geopolitical and economic *** finding is corroborated by last millennium reanalysis data and numerical climate model simulations revealing internally driven Pacific sea surface temperature variations and the predominance of decadal scale La Ni?a-like conditions to be responsible for precipitation decreases over northern China,as well as extensive monsoon regions in the *** teleconnection patterns provide a mechanistic explanation for reoccurring drought spells during the late Ming Dynasty and the environmental framework fostering the fall of Beijing in 1644 CE,and the subsequent demise of the Ming Dynasty.

关键词： Paleoclimate Beijing Precipitation reconstruction Climate-society interactions Tree rings Ming Dynasty

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Ternary quasifission in collisions of actinide nuclei

arXiv

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arXiv 2023年

作者： Zhang, D.D. Li, B. Vretenar, D. Nikšić, T. Ren, Z.X. Zhao, P.W. Meng, J. State Key Laboratory of Nuclear Physics and Technology School of Physics Peking University Beijing100871 China Physics Department Faculty of Science University of Zagreb Zagreb10000 Croatia Institut für Kernphysik Institute for Advanced Simulation Jülich Center for Hadron Physics Forschungszentrum Jülich JülichD-52425 Germany Helmholtz-Institut für Strahlen- und Kernphysik Bethe Center for Theoretical Physics Universität Bonn BonnD-53115 Germany

The microscopic framework of time-dependent covariant density functional theory is applied to a systematic study of ternary quasifission in collisions of pairs of 238U nuclei. It is shown that the inclusion of octupole degree of freedom in the case of head-to-head collisions, extends the energy window in which ternary quasifission occurs, and greatly enhances the number of nucleons contained in a middle fragment. Dynamical pairing correlations, included here in the time-dependent BCS approximation, prevent the occurrence of ternary quasifission in head-to-head collisions, and have an effect on the location of the energy window in which a middle fragment is formed in tail-to-tail collisions. In the latter case, as well as for tail-to-side collisions, the formation of very heavy neutron-rich systems in certain energy intervals is predicted. Copyright © 2023, The Authors. All rights reserved.

关键词： Density functional theory

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Burning products of TA15 titanium alloy by friction oxygen concentration method

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Rare Metals 2018年第11期37卷 952-960页

作者： Nan Sui Guang-Bao Mi Meng-Qi Yan Jing-Xia Cao Xu Huang Aviation Key Laboratory of Science and Technology on Advanced Titanium Alloys AECC Beijing Institute of Aeronautical Materials

The microstructural characteristics, elemental distribution law and microscopic formation mechanism of the burning products of TA15 titanium alloy were investigated by friction oxygen concentration method, associated with in situ observation, X-ray diffraction(XRD),scanning electron microscopy(SEM) and energy-dispersive spectroscopy(EDS) analyses, providing the thoughts to improve fireproof property. The results show that, when the friction contact pressure(p) is 0.20 MPa and oxygen concentration of premixed air flow(c) is 60 vol%, TA15 titanium alloy produces violent sparks and presents dazzling white light during combustion. The generated products after burning are mainly TiOand small amount of AlOoxides. Four distinct zones form from the combustion surface to the alloy matrix, and they are in the sequence of combustion zone, fusion zone, heat-affected zone and transition zone. Further, combustion zone is composed of TiOand A1203 compounds, containing obvious cracks. In the fusion zone, discontinuous oxygenrich Al-based solid solution forms, and the elemental distribution has strong volatility. In the heat-affected zone,there are abundant of Ti-based solid solution and small amount of Al-and Mo-based solid solution. Transition zone is made of lamellar structure. Two technical approaches are given to prevent oxygen diffusion inside the reaction zone and reaction-affected zone. On the one hand,the content of Al is designed as the upper limit of alloy composition; on the other hand, fireproof coatings are deposited on the surface of the alloy.

关键词： Friction oxygen concentration method TA15 titanium alloy Burning products Microstructure Titanium fire

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Formation Mechanisms and Atmospheric Implications of Summertime Nitrous Acid (HONO) During Clean, Ozone Pollution and Double High Pollution Periods in Beijing

SSRN

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SSRN 2022年

作者： Xuan, Huiying Zhao, Yaqi Ma, Qingxin Chen, Tianzeng Liu, Jun Wang, Yonghong Liu, Chang Wang, Yafei Liu, Yongchun Mu, Yujing He, Hong State Key Joint Laboratory of Environment Simulation and Pollution Control Research Center for Eco-Environmental Sciences Chinese Academy of Sciences Beijing100085 China College of Resources and Environment University of Chinese Academy of Sciences Beijing100049 China Center for Excellence in Regional Atmospheric Environment Institute of Urban Environment Chinese Academy of Sciences Xiamen361021 China State Key Laboratory of Severe Weather Key Laboratory of Atmospheric Chemistry of China Meteorological Administration Chinese Academy of Meteorological Sciences Beijing100081 China Beijing Institute of Petrochemical Technology Beijing102617 China Aerosol and Haze Laboratory Beijing Advanced Innovation Center for Soft Matter Science and Engineering Beijing University of Chemical Technology Beijing100029 China

Nitrous acid (HONO) is a key precursor of the hydroxyl radicals (OH) and has a significant impact on air quality. Nowadays, the source of HONO is still controversial due to its complex formation mechanisms, which is widely explored in extensive field and laboratory studies. In this study, the pollution characteristics and source contribution of HONO under different air quality conditions in summer in Beijing were analyzed. The observation periods were classified as three typical periods: clean, ozone pollution, and double high pollution (co-occurrence of high PM2.5 and O3 concentrations). The average concentrations of observed HONO were 0.38 ± 0.35 ppb, 0.21 ± 0.18 ppb, 0.26 ± 0.20 ppb and 0.54 ± 0.45 ppb during the whole, clean, ozone and double high periods, respectively. The elevated HONO levels at night were attributed to vehicle emissions and the RH-dependent heterogeneous conversion of NO2 to HONO. The average emission ratio (HONO/NOx) was 0.85 ± 0.38%, and the mean value of calculated nocturnal NO2 to HONO conversion frequency was 0.0076 ± 0.0031 h-1. Based on daytime HONO budget analysis, the largest potential source of HONO was the homogeneous reaction of NO and OH (0.33 and 0.34 ppb h-1), followed by the unknown source (0.11 and 0.21 ppb h-1) during clean and ozone periods, while the unknown source (0.49 ppb h-1) played the predominant role during double high period. The unknown sources of HONO could be attributed to the photo-enhanced heterogeneous conversion of NO2 and the photolysis of particulate nitrate. Furthermore, the photolysis of ozone (0.17, 0.34 and 0.44 ppb h-1) was the major contributor to primary OH during three typical periods. HONO photolysis contributed considerable amounts of primary OH (0.32 ppb h-1) during double high period. These results are helpful to further understand the linkage between HONO and air quality variation. © 2022, The Authors. All rights reserved.

关键词： Ozone

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Feasibility study of NiCoCrFeAl0 .8 Si 0.1 (NbMoTaW) 0.1 denary alloy as a bond coat for thermal barrier coatings: from structural stability to high-temperature oxidation behavior

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Surface and Coatings technology 2025年 512卷

作者： Zhuo Chen Yongzhi Jing Chao Zhang Xiufang Cui Wei Xu Xiang Wang Yongchao Fang Dechang Ma Guo Jin Institute of Surface/Interface Science and Technology Key Laboratory of Superlight Material and Surface Technology of Ministry of Education College of Material Science and Chemical Engineering Harbin Engineering University Harbin 150001 China Northwest Institute for Nonferrous Metal Research Xi an 710016 China No.703 Research Institute China State Shipbuilding Co. Ltd. Harbin 150078 China The Military Industry Program Evaluation Center of Costind of SASTIND Beijing 100048 China Aviation Key Laboratory of Science and Technology on Advanced Corrosion and Protection for Aviation Material Beijing Beijing Institute of Aeronautical Materials Beijing 100095 China

In this study, the feasibility of NiCoCrFeAl 0.8 Si 0.1 (NbMoTaW) 0.1 complex concentrated alloy as a bond coat for thermal barrier coatings (TBCs) was investigated. The alloy bond coat was prepared using plasma spraying technology and compared with the conventional NiCoCrAlY bond coat. The phase composition and microstructural changes of the NiCoCrFeAl 0.8 Si 0.1 (NbMoTaW) 0.1 alloy before and after plasma deposition were analyzed, and the thermal expansion coefficients, microhardness, and oxidation resistance of the two coatings were evaluated. Additionally, a Yttria-Stabilized Zirconia (YSZ) ceramic layer was deposited on the surfaces of both bond coats, forming a complete TBC system, and the evolution of the thermally grown oxide (TGO) layer was studied under different oxidation stages. Results indicate that after plasma spraying, the denary alloy bond coat maintains a single-phase BCC structure with slight compositional segregation, dense microstructure, and effective suppression of segregation of refractory elements due to its high aluminum content. The thermal expansion coefficient of the alloy is comparable to that of NiCoCrAlY, but its microhardness is nearly double that of NiCoCrAlY, with a more uniform hardness distribution. Oxidation testing at 1100 °C revealed that the TGO growth rate of the NiCoCrFeAl-based bond coat TBC is 36 % lower than that of the NiCoCrAlY-based system, demonstrating superior oxidation resistance. This improvement is attributed to the active elements such as Si, Nb, and Mo, which promote the formation of a protective Cr/Al dual-layer oxide film, effectively slowing down further oxidation, internal stress, and the formation of spinel. These findings suggest that the NiCoCrFeAl 0.8 Si 0.1 (NbMoTaW) 0.1 complex concentrated alloy has the potential to serve as a high-performance bond coat in TBC systems, providing superior oxidation resistance, thermal expansion matching, and mechanical integrity at high temperatures.

关键词：

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A hyperelastic model for hollow fiber-reinforced composites at finite deformation

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Mechanics of Materials 2025年 207卷

作者： Wang, Jialin Chen, Liangbin Hao, Meirong Chen, Yang Guo, Zaoyang Liang, Jun School of Science Harbin Institute of Technology Guangdong Shenzhen518055 China School of Civil Aviation Northwestern Polytechnical University Shaanxi Xi'an710072 China Research & Development Institute of Northwestern Polytechnical University in Shenzhen Northwestern Polytechnical University Guangdong Shenzhen518063 China Division of Atmosphere and Aerospace Information Technology Beijing Institute of Technology Guangdong Zhuhai519088 China Institute of Advanced Structure Technology Beijing Institute of Technology Beijing100081 China Beijing Key Laboratory of Lightweight Multi-functional Composite Materials and Structures Beijing Institute of Technology Beijing100081 China State Key Laboratory of Explosion Science and Technology Beijing Institute of Technology Beijing100081 China

This study introduces a micromechanics-based constitutive model to describe the effective hyperelastic behaviors of hollow fiber-reinforced composites under finite deformation. The multiplicative decomposition approach is employed to decompose a general deformation into three fundamental deformations: isochoric uniaxial deformation along the fiber direction, equi-biaxial deformation on the transverse plane, and pure shear deformation. Based on this multiplicative decomposition, the free energy density function of the composites is thus additively decomposed into the three corresponding components. Subsequently, the effective free energy density functions of the composite for triaxial deformation (composed of the isochoric uniaxial deformation along the fiber direction and equi-biaxial deformation on the transverse plane), along-fiber shear, and transverse shear are derived using a cylindrical composite element model. The total free energy density function of the composite is then obtained by summing the contributions of these decomposed deformations. To validate the proposed model, finite element simulations based on representative volume elements are conducted. The effects of fiber volume fraction, fiber/matrix stiffness ratio, and wall thickness of hollow fiber on the effective mechanical behaviors of the composites are explored. The theoretical predictions show excellent agreement with numerical results for all considered cases, demonstrating that the proposed model reliably predicts the effective mechanical response of hollow fiber-reinforced composites under finite deformation. Finally, to further validate the prediction accuracy and computational efficiency of the developed model, it is applied to the structural analysis of a cantilever beam, with results compared to those obtained using the FE2 method. This comparative analysis demonstrates again the accuracy and efficiency of the proposed approach in practical structural analysis. © 2025

关键词： Fiber reinforced plastics

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Observation of the Orbital Rashba-Edelstein Magnetoresistance

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Physical Review Letters 2022年第6期128卷 067201-067201页

作者： Shilei Ding Zhongyu Liang Dongwook Go Chao Yun Mingzhu Xue Zhou Liu Sven Becker Wenyun Yang Honglin Du Changsheng Wang Yingchang Yang Gerhard Jakob Mathias Kläui Yuriy Mokrousov Jinbo Yang State Key Laboratory for Mesoscopic Physics School of Physics Peking University Beijing 100871 People’s Republic of China Peter Grünberg Institut and Institute for Advanced Simulation Forschungszentrum Jülich and JARA 52425 Jülich Germany Institute of Physics Johannes Gutenberg-University Mainz Staudingerweg 7 55128 Mainz Germany Graduate School of Excellence Materials Science in Mainz 55128 Mainz Germany Center for Quantum Spintronics Department of Physics Norwegian University of Science and Technology NO-7491 Trondheim Norway Collaborative Innovation Center of Quantum Matter Beijing 100871 People’s Republic of China Beijing Key Laboratory for Magnetoelectric Materials and Devices Beijing 100871 People’s Republic of China

We report the observation of magnetoresistance (MR) that could originate from the orbital angular momentum (OAM) transport in a permalloy (Py)/oxidized Cu (Cu*) heterostructure: the orbital Rashba-Edelstein magnetoresistance. The angular dependence of the MR depends on the relative angle between the induced OAM and the magnetization in a similar fashion as the spin Hall magnetoresistance. Despite the absence of elements with large spin-orbit coupling, we find a sizable MR ratio, which is in contrast to the conventional spin Hall magnetoresistance which requires heavy elements. Through Py thickness-dependence studies, we conclude another mechanism beyond the conventional spin-based scenario is responsible for the MR observed in Py/Cu* structures—originated in a sizable transport of OAM. Our findings not only suggest the current-induced torques without using any heavy elements via the OAM channel but also provide an important clue towards the microscopic understanding of the role that OAM transport can play for magnetization dynamics.

关键词： Magnetoresistance Spin coherence Spin current Spin diffusion Spin torque Spin-orbit coupling

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