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Heterointerface engineering in hierarchical assembly of the Co/Co(OH)_(2)@carbon nanosheets composites for wideband microwave absorption

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Nano Research 2023年第2期16卷 2611-2621页

作者： Yuhan Wu Guodong Wang Xixi Yuan Gang Fang Peng Li Guangbin Ji College of Materials Science and Technology Nanjing University of Aeronautics and AstronauticsNanjing 210016China Aerospace Research Institute of Material&Processing Technology Beijing 100076China

Heterogeneous interface engineering strategy is an effective method to optimize electromagnetic functional ***,the mechanism of heterogeneous interfaces on microwave absorption is still *** this study,abundant heterointerfaces were customized in hierarchical structures via a collaborative strategy of lyophilization and hard *** impressive electromagnetic heterostructures and strong interfacial polarization were realized on the zero-dimensional(0D)hexagonal close-packed(hcp)-face-centered cubic(fcc)Co/two-dimensional(2D)Co(OH)_(2)nanosheets@three-dimensional(3D)porous carbon nanosheets(Co/Co(OH)_(2)@PCN).By controlling the carbonization temperature,the electromagnetic parameters were further adjusted to broaden the effective absorption bandwidth(EAB).Accordingly,the EAB of these absorbers were almost greater than 6 GHz(covering the entire Ku-band)in the thickness range of 2.0–2.2 mm except the sample *** far as to the S-0.8-700 achieved an EAB up to 7.1 GHz at 2.2 mm and the minimum reflection loss(RLmin)value was−25.8 ***,in the far-field condition,the radar cross section(RCS)of S-0.8-700 can be reduced to 19.6 dB·m^(2).We believe that this work will stimulate interest in interface engineering and provide a direction for achieving efficient absorbing materials.

关键词： microwave absorption wide bandwidth interface engineering hierarchical porous structure absorption mechanism

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Effect of densification process on mechanical enhancement of graphene laminates

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Nano materials Science 2025年第2期7卷 240-248页

作者： Zhu, Yue Liao, Yalong Wang, Meng Dai, Jingxin Lei, Chaoshuai Liu, Xiaobo Mu, Pengyu Li, Wenjing Zhang, Hao Aerospace Institute of Advanced Material & Processing Technology Beijing100074 China Academy of Deep Earth Sciences China Coal Research Institute Beijing100013 China

Graphene nanosheets have attracted great attention in the field of nanotechnology applications due to their extraordinary mechanical properties. While the structural defects such as gaps will occur during the preparation of graphene laminates, which will greatly damage the performance of the macroscopic material. Hence, a simple and promising mechanical compression method is used to improve the mechanical properties of graphene laminates. However, the roles of the densification process in the mechanical enhancement mechanism of graphene laminates are not clear. In our work, the mechanical enhancement of the compressed graphene (PG) laminates was investigated by the coarse-grained molecular dynamics simulation method. The tensile strength of PG model could be increased by increasing the graphene nanosheet size and the degree of compression in the system. And the model has the stronger van der Waals effect between graphene sheets due to the larger graphene size as well as the higher overlap ratio. Furthermore, two kinds of PG laminates were prepared by densification method, and the tensile strength was consistent with the upward trend of the PG model. This work provides an in-depth understanding on the mechanical enhancement of the densification process and lays a foundation for the future practical application of graphene laminates. © 2024 Chongqing University

关键词： Structural design

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advanced nanofabrication for elastic inorganic aerogels

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Nano Research 2024年第10期17卷 8842-8862页

作者： Xiaota Cheng Xinyi Chang Fan Wu Yalong Liao Kai Pan Hao Fong Jianyong Yu Yi-Tao Liu Bin Ding Innovation Center for Textile Science and Technology College of TextilesDonghua UniversityShanghai 201620China Aerospace Institute of Advanced Material and Processing Technology Beijing 100074China College of Materials Science and Engineering Beijing University of Chemical TechnologyBeijing 100029China

Inorganic aerogels with low density,high porosity,large specific surface area,and superior mechanical properties are excellent candidate materials in fields such as thermal management,energy,catalysis,and biomedical applications.A comprehensive overview of existing elastic inorganic aerogels is provided,covering their structural units,preparation methods,mechanical performances,and ***,based on the constituent building blocks and microstructures,a detailed analysis of the mechanical properties and guidelines for elastic design of aerogels is *** with a succinct summary of prospective developmental direction,this review deliberates on the challenges and potential opportunities of elastic inorganic aerogels,with the intent of providing a versatile platform for designing new types of elastic inorganic aerogels for various applications.

关键词： inorganic aerogels compressive stretchable fabrication mechanical performances applications

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Regulating the concentration of silica sol to prepare high thermal insulation ceramic nanofiber aerogel composites 5

Regulating the concentration of silica sol to prepare high t...

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2024 5th International Conference on advanced material and Clean Energy, ICAMCE 2024

作者： Xu, Yuanyuan Zhang, Hao He, Lijuan Li, Wenjing Liu, Yitao Innovation Center for Textile Science and Technology College of Textiles Donghua University Shanghai201620 China Aerospace Institute of Advanced Material and Processing Technology Beijing100074 China

Ceramic aerogels can maintain excellent thermal insulation performance under extreme conditions due to their outstanding pore structure and specific surface area. However, the current application of ceramic aerogels is limited by their brittleness, easy collapse of the structure under external forces, and insufficient mechanical properties. In this study, ceramic nanofiber aerogels prepared by PEO as a polymer were used as building blocks, and silica sol was selected as a high-temperature binder. Through the sol impregnation-atmospheric pressure drying method and calcination treatment, we obtained ceramic nanofiber composites with excellent performance. It is found that when the impregnation concentration is 0.4wt%, the thermal conductivity at room temperature is as low as 27 m W·m-1·K-1, the cold surface temperature at 800°C is as low as 255°C, the tensile strength at 20% tensile strain is as high as 400 kPa, and the compressive strength at 80% compressive strain is as high as 32 kPa. Compared with the traditional ceramic fiber aerogel material, the material exhibits excellent high-temperature insulation performance and mechanical properties, which greatly broadens the application scene of ceramic aerogel. © Published under licence by IOP Publishing Ltd.

关键词： Aerogels

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Tightened1D/3Dcarbonheterostructure infiltratingphase change materials for solar-thermoelectric energy harvesting:Faster and better

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Carbon Energy 2023年第6期5卷 104-117页

作者： Zhaodi Tang Piao Cheng Panpan Liu Yan Gao Xiao Chen Ge Wang Beijing Advanced Innovation Center for Materials Genome Engineering Beijing Key Laboratory of Function Materials for Molecule&Structure ConstructionSchool of Materials Science and EngineeringUniversity of Science and Technology BeijingBeijingPR China Institute of Advanced Materials Beijing Normal UniversityBeijingPR China Aerospace Institute of Advanced Material and Processing Technology BeijingPR China Shunde Graduate School University of Science and Technology BeijingShundePR China

Extensive use of thermal energy in daily life is ideal for reducing carbon emissions to achieve carbon neutrality;however,the effective collection of thermal energy is a major ***(TE)conversion technology based on the Seebeck effect and thermal energy storage technology based on phase change materials(PCMs)represent smart,feasible,and research-worthy approaches to overcome this ***,the integration of multiple thermal energy sources freely existing in the environment for storage and output of thermal and electrical energy simultaneously still remains a huge ***,three-dimensional(3D)nanostructured metal-organic frameworks(MOFs)are in situ nucleated and grown onto carbon nanotubes(CNTs)via coordination *** calcination,the prepared core-shell structural CNTs@MOFs are transformed into tightened 1D/3D carbon heterostructure loading Co nanoparticles for efficient solar-thermoelectric energy ***,the corresponding composite PCMs show a record-breaking solar-thermal conversion efficiency of 98.1%due to the tightened carbon heterostructure and the local surface plasmon resonance effect of Co ***,our designed all-in-one composite PCMs are also capable of creating an electrical potential of 0.5 mV based on the Seebeck effect without a TE *** promising approach can store thermal and electrical energy simultaneously,providing a new direction in the design of advanced all-in-one multifunctional PCMs for thermal energy storage and utilization.

关键词： carbon neutrality metal-organic framework phase change materials solar-thermoelectric conversion thermal energy storage

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A novel medium-entropy(TiVNb)_(2)AlC MAX phase:Fabrication,microstructure,and properties

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Journal of materials Science & technology 2023年第6期137卷 91-99页

作者： Guangqi He Yi Zhang Pei Yao Xingchao Li Ke Ma Jun Zuo Meishuan Li Changsheng Liu Jingjun Xu School of Materials Science and Engineering Northeastern UniversityShenyang 110819China Shenyang National Laboratory for Materials Science Institute of Metal ResearchChinese Academy of SciencesShenyang 110016China School of Materials Science and Engineering University of Science and Technology of ChinaShenyang 110016China Science and Technology on Advanced Functional Composites Laboratory Aerospace Research Institute of Material and Processing TechnologyBeijing 100076China

Medium-or high-entropy materials have great potential for applications due to their diverse compo-sitions and unexpected physicochemical ***,a novel medium-entropy(TiVNb)_(2)AlC was synthesized via hot pressing at 1400℃from three individual M_(2)AlC(M=Ti,V,Nb)MAX *** microstructure of(TiVNb)_(2)AlC was characterized from the microscale to the atomic scale by scanning electron microscope microscopy(SEM),scanning transmission electron microscopy(STEM),and energy dispersive spectroscopy(EDS).The results showed that Ti,V,and Nb atoms were fully solid-soluble in the M-sites of the M_(2)AlC MAX *** with three individual MAX phases,the thermal conduc-tivity of(TiVNb)_(2)AlC was reduced greatly in the temperature range of 293-1473 K,and its mechanical properties(including Young’s modulus,Vickers hardness,and bending strength)were all increased due to the solid solution strengthening and electronic mechanism.

关键词： Medium-entropy ceramics MAX phases Microstructure Thermal properties Mechanical properties

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Ultrabroadband chiral metasurface for linear polarization conversion and asymmetric transmission based on enhanced interference theory

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Chinese Optics Letters 2023年第11期21卷 147-154页

作者：赵京城李南程用志 School of Electronics Information Engineering Beihang UniversityBeijing 100191China Aerospace Institute of Advanced Material&Processing Technology Beijing 100074China School of Information Science and Engineering Wuhan University of Science and TechnologyWuhan 430081China Hubei Longzhong Laboratory Xiangyang 441000China

In this paper,we propose an ultrabroadband chiral metasurface(CMS)composed of S-shaped resonator structures situated between two twisted subwavelength gratings and dielectric *** innovative structure enables ultrabroadband and high-efficiency linear polarization(LP)conversion,as well as asymmetric transmission(AT)effect in the microwave *** enhanced interference effect of the Fabry-Perot-like resonance cavity greatly expands the bandwidth and efficiency of LP conversion and AT *** numerical simulations,it has been revealed that the cross-polarization transmission coefficients for normal forward(-z)and backward(+z)incidence exceed 0.8 in the frequency range of 4.13 to 17.34 GHz,accompanied by a polarization conversion ratio of over 99%.Furthermore,our microwave experimental results validate the consistency among simulation,theory,and ***,we elucidate the distinct characteristics of ultrabroadband LP conversion and significant AT effect through analysis of polarization azimuth rotation and ellipticity angles,total transmittance,AT coefficient,and electric field *** proposed CMS structure shows excellent polarization conversion properties via AT effect and has potential applications in areas such as radar,remote sensing,and satellite communication.

关键词： chiral metasurface linear polarization conversion asymmetric transmission Fabry-Perot-like resonance electromagnetic interference model

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Application of high-throughput first-principles calculations in ceramic innovation

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Journal of materials Science & technology 2021年第29期88卷 143-157页

作者： Bin Liu Juanli Zhao Yuchen Liu Jianqi Xi Qian Li Huimin Xiang Yanchun Zhou School of Materials Science and Engineering Shanghai UniversityShanghai200444China Department of Materials Science and Engineering University of WisconsinMadisonWI53706USA Science and Technology on Advanced Functional Composite Laboratory Aerospace Research Institute of Material&Processing TechnologyBeijing100076China

Recent technical progress in the industry has led to an urgent requirement on new materials with enhanced *** meet this multi-property requirement,the materials consisting of three and more elements have attracted increasing ***,facing to the nearly unknown huge multi-component materials system,the traditional trial and error method cannot provide sufficient data ***,an efficient material innovation strategy is *** first-principles calculation based on the density functional theory is a powerful tool for both the accurate prediction of material properties and the identification of its underlying thermodynamics and *** the same time,the advances of computational methods and computer calculation abilities that are orders of magnitude faster than before make the high throughput first-principles calculations *** present,the simulation-assisted material design has become a main branch in the material research field and a great many successes have been *** this article,the advances of the high throughput first-principles calculations are reviewed to show the achievements of the first-principles calculations and guide the future directions of its applications in ceramics.

关键词： First-principles calculations Ceramics Defect Dynamics Structure-property relationship

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Achieving ultra-broadband electromagnetic wave absorption in high-entropy transition metal carbides (HE TMCs)

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Journal of advanced Ceramics 2022年第4期11卷 545-555页

作者： Weiming ZHANG Huimin XIANG Fu-Zhi DAI Biao ZHAO Shijiang WU Yanchun ZHOU Science and Technology on Advanced Functional Composite Laboratory Aerospace Research Institute of Materials&Processing TechnologyBeijing 100076China Henan Key Laboratory of Aeronautical Materials and Application Technology School of Material Science and EngineeringZhengzhou University of AeronauticsZhengzhou 450046China Zibo Firststar New Material Incorporated Co. Ltd.Zibo 255000China

Electronic devices pervade everyday life,which has triggered severe electromagnetic(EM)wave *** face this challenge,developing EM wave absorbers with ultra-broadband absorption capacity is critically ***,nano-composite construction has been widely utilized to realize impedance match and broadband ***,complex experimental procedures,limited thermal stability,and interior oxidation resistance are still unneglectable ***,it is appealing to realize ultra-broadband EM wave absorption in single-phase materials with good *** at this target,two high-entropy transition metal carbides(HE TMCs)including(Zr,Hf,Nb,Ta)C(HE TMC-2)and(Cr,Zr,Hf,Nb,Ta)C(HE TMC-3)are designed and synthesized,of which the microwave absorption performance is investigated in comparison with previously reported(Ti,Zr,Hf,Nb,Ta)C(HE TMC-1).Due to the synergistic effects of dielectric and magnetic losses,HE TMC-2 and HE TMC-3 exhibit better impedance match and wider effective absorption bandwidth(EAB).In specific,the exclusion of Ti element in HE TMC-2 endows it optimal minimum reflection loss(RL_(min))and EAB of−41.7 dB(2.11 mm,10.52 GHz)and 3.5 GHz(at 3.0 mm),***,the incorporation of Cr element in HE TMC-3 significantly improves the impedance match,thus realizing EAB of 10.5,9.2,and 13.9 GHz at 2,3,and 4 mm,*** significance of this study lays on realizing ultra-broadband capacity in HE TMC-3(Cr,Zr,Hf,Nb,Ta),demonstrating the effectiveness of high-entropy component design in tailoring the impedance match.

关键词： transition metal carbide(TMC) high-entropy ceramics electromagnetic(EM)wave absorption dielectric and magnetic loss coupling ultra-broadband absorption

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Cobalt doping boosted electrocatalytic activity of CaMn3O6 for hydrogen evolution reaction

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Nano Research 2022年第4期15卷 2870-2876页

作者： Qun Li Kaisi Liu Siwei Gui Jiabin Wu Xiaogang Li Zaifang Li Hongrun Jin Hui Yang Zhimi Hu Wenxi Liang Liang Huang Wuhan National Laboratory for Optoelectronics Huazhong University of Science and TechnologyWuhan 430074China China-Australia Institute for Advanced Materials and Manufacturing Jiaxing UniversityJiaxing 314001China State Key Laboratory of Material Processing and Die&Mold Technology Department of MechanicsSchool of Aerospace EngineeringHuazhong University of Science and TechnologyWuhan 430074China

The development of earth-abundant-metal-based electrocatalysts with high efficiency and long-term stability for hydrogen evolution reaction(HER)is crucial for the clean and renewable energy ***,we report a molten-salt method to synthesize Co-doped CaMn_(3)O_(6)(CMO)nanowires(NWs)as effective electrocatalyst for *** as-obtained CaMn_(3-x)Co_(x)O_(6)(CMCO)exhibits a small onset overpotential of 70 mV,a required overpotential of 140 mV at a current density of 10 mA·cm^(-2),a Tafel slope of 39 mV·dec^(-1)in 0.1 M HClO_(4),and a satisfying long-term *** characterizations combined with density functional theory(DFT)calculations demonstrate that the obtained HER performance can be attributed to the Co-doping which altered CMO’s surface electronic structures and *** the simplicity of synthesis route and the abundance of the pertinent elements,the synthesized CMCO shows a promising prospect as a candidate for the development of earth-abundant,metal-based,and cost-effective electrocatalyst with superior HER *** results also establish a strategy of rational design and construction of novel electrocatalyst toward HER by tailoring band structures of transition metal oxides(TMOs).

关键词： CMCO nanowires hydrogen evolution reaction electronic structure dopant

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