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The Future of environmental Engineering Technology:A Disruptive Innovation Perspective

Engineering 2024年第10期41卷 153-160页

作者： Hui Huang Junjie Lu Lili Jin Hongqiang Ren State Key Laboratory of Pollution Control and Resource Reuse School of the EnvironmentNanjing UniversityNanjing 210023China

Scientific and technological revolutions and industrial transformations have accelerated the rate of innovation in environmental engineering ***,few researchers have evaluated the current status and future trends of *** paper summarizes the current research status in eight major subfields of environmental engineering—water treatment,air pollution control,soil/solid waste management,environmental biotechnology,environmental engineering equipment,emerging contaminants,synergistic reduction of pollution and carbon emissions,and environmental risk and intelligent management—based on bibliometric analysis and future trends in greenization,low carbonization,and *** technologies are further identified based on discontinuous transformation,and ten such technologies are proposed,covering general and specific fields,technical links,and value ***,the background and key innovations in disruptive technologies are elucidated in *** study not only provides a scientific basis for strategic decision-making,planning,and implementation in the environmental engineering field but also offers methodological guidance for the research and determination of breakthrough technologies in other areas.

关键词： environmental engineering technology Disruptive innovation Bibliometric analysis Discontinuous transformation

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Nitrogen-removed organic matters from cyanobacterial decomposition promote the release of nitrogen from lake sediment

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environmental Science and pollution Research 2025年第13期32卷 8219-8230页

作者： Wang, Mengmeng Zhan, Yixuan Wang, Chenyu Song, Xiaohua Gan, Lin Lu, Hao Yang, Liuyan Key Laboratory of Taihu Basin Water Resources Management Ministry of Water Resources Nanjing210012 China State Key Laboratory of Pollution Control and Resource Reuse Key Laboratory of Aquatic Ecosystem Health in the Middle and Lower Reaches of Yangtze River School of Environment Nanjing University Nanjing210023 China

Cyanobacterial blooms, which carry a lot of nitrogen (N) and phosphorus (P), have emerged as one of the most severe environmental issues in freshwater ecosystems. However, there are few studies on the effect of organic matters released during cyanobacterial decomposition in promoting N release from lake sediments that remain underexplored. An essential step is to eliminate the impact of the N contributions from cyanobacteria when evaluating sedimentary N release. The response surface methodology (RSM) was developed to optimize the struvite precipitation model, and the results indicated that 1.3 of Mg/N, 1.0 of P/N, and pH 9.5 were the optimum conditions for N removal from cyanobacterial pyrolysis liquid. Following this, calcium phosphate crystallization (at pH 10 and Ca/P = 4.98) removed residual P, and zeolite adsorption (at pH 8 and 10 g/L zeolite dosage) eliminated the remaining N. Ultimately, 99.3% of N was removed with the two methods in cyanobacterial pyrolysis liquid. The cyanobacterial pyrolysis liquid, stripped of N, was found to significantly enhance the release of N from lake sediment under anaerobic conditions, which can then be reutilized by cyanobacteria. These findings reveal that organic matter derived from cyanobacterial decomposition promotes sedimentary N release, creating a feedback loop that sustains cyanobacterial blooms in freshwater ecosystems. © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2025.

关键词： Blooms (metal)

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Occurrence, partition behavior, source and ecological risk assessment of nitro-PAHs in the sediment and water of Taige Canal, China

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Journal of environmental Sciences 2023年第2期124卷 782-793页

作者： Jijie Kong Tao Ma Xiaoyu Cao Weidi Li Fengxiao Zhu Huan He Cheng Sun Shaogui Yang Shiyin Li Qiming Xian School of Environment Nanjing Normal UniversityNanjing 210023China School of Geography Nanjing Normal UniversityNanjing 210023China The State Key Laboratory of Pollution Control and Resource Reuse School of the EnvironmentNanjing UniversityNanjing 210023China Fujian Provincial Key laboratory of Eco-Industrial Green Technology College of Ecological and Resource EngineeringWuyi UniversityWuyishan 354300China Nanjing Institute of Environmental Sciences Ministry of Ecology and EnvironmentNanjing 210042China

Nitrated polycyclic aromatic hydrocarbons(NPAHs)are widespread organic pollutants that possess carcinogenic and mutagenic properties,so they may pose a risk to the environment and human *** this study,the concentrations of 15 NPAHs and 16 polycyclic aromatic hydrocarbons(PAHs)in 30 surface water samples and 26 sediment samples were measured in 2018 from the Taige Canal,one of the main rivers flowing into Taihu Lake,*** total NPAH concentrations in water and sediment ranged from 14.7 to 235 ng/L and 22.9 to 96.5 ng/g dw,respectively.9-nitrophenanthrene(nd–76.3 ng/L)was the dominant compound in surface water,while 2+3-nitrofluoranthene(1.73–18.1 ng/g dw)dominated in *** PAHs,concentration ranging from 1,097 to 2,981 ng/L and 1,089 to 4,489 ng/g dw in surface water and sediment,*** was a strong positive correlation between the log octanol-water partition coefficient(Kow)and log sediment-water partition coefficient due to hydrophobic *** fugacity fraction value increased with the decrease of log Kow,and chrysene was transferred from water into *** residual NPAHs in surface water and sediment of the Taige Canal have partial *** engine and coal combustion emissions were probably the principal sources of NPAHs in surface water and *** results of ecological risk assessment showed that some NPAHs inwater(e.g,1-nitropyrene and 6-nitrochrysene)and sediment(e.g.,2-nitrobiphenyl,5-nitroacenaphthene,9-nitrophenanthrene and 2+3-nitrofluoranthene)had moderate ecological risks,which should be of concern.

关键词： Nitrated polycyclic aromatic hydrocarbons(NPAHs) Occurrence Partition behavior Source apportionment Ecological risk assessment

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A study on singlet oxygen generation for tetracycline degradation via modulating the size ofα-Fe_(2)O_(3)nanoparticle anchored on g-C_(3)N_(4) nanotube photocatalyst

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Nano Research 2023年第2期16卷 2236-2244页

作者： Hongjie Zhu Minghui Li Luning Zou Youyou Hu Hongguo Hao Jianmin Dou Junjie Mao Shandong Provincial Key Laboratory of Chemical Energy Storage and Novel Cell Technology School of Chemistry and Chemical EngineeringLiaocheng UniversityLiaocheng 252059China Key Laboratory of Functional Molecular Solids Ministry of EducationCollege of Chemistry and Materials ScienceAnhui Normal UniversityWuhu 241002China State Key Laboratory of Pollution Control and Resource Reuse School of the EnvironmentNanjing UniversityNanjing 210023China Gaotang liguo chemical plant Liaocheng 252059China

Photocatalysis is considered as an effective technique for mitigating ecological risks posed by residual tetracycline(TC).To improve the efficiency of this technique,it is necessary to enable photocatalysts to produce highly reactive species,such as singlet oxygen(1O2).However,due to the high activation energy of 1O2,photocatalysts can hardly produce 1O2 without assistance from external ***,we find that the size-reducedα-Fe_(2)O_(3)nanoparticles(~4 nm)that anchored on g-C_(3)N_(4)nanotube(α-Fe_(2)O_(3)@CNNT)can spontaneously generate ^(1)O_(2) for degradation of *** comparison,only hydroxyl radical(·OH)can be produced by g-C_(3)N_(4)nanotube loaded with~14 nmα-Fe_(2)O_(3)nanoparticles(α-Fe_(2)O_(3)/CNNT).Owing to the high reactivity of the ^(1)O_(2) species,the photocatalytic degradation rate(Kapp)of TC withα-Fe_(2)O_(3)@CNNT(0.056 min^(−1))was 1.8 times higher than that ofα-Fe_(2)O_(3)/*** experimental results and theoretical calculations suggested that reducing the size ofα-Fe_(2)O_(3)nanoparticles anchored on g-C_(3)N_(4)nanotube decreased the surface electron density ofα-Fe_(2)O_(3),which induces the generation of high-valent Fe(IV)active sites overα-Fe_(2)O_(3)@CNNT and turns the degradation pathway into a unique ^(1)O_(2) dominated *** study provides a new insight on the generation of ^(1)O_(2) for effective degradation of environmental pollutant.

关键词： singlet oxygen degradation pathway high-valent Fe(IV) tetracycline degradation

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Research on Flood control of Urban River Network in Northern anhui Plain Based on MIKE Model 24

Research on Flood Control of Urban River Network in Northern...

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2024 International Conference on Smart City and Information System, ICSCIS 2024

作者： Yang, Jianguo Wang, Zhong Zhu, Yulong Sheng, Lin Wu, Houfan Zhu, Shuguang Wei, Wei Anhui shui'An Construction Group Co. Ltd. Hefei Anhui230601 China Anhui Provincial Key Laboratory of Environmental Pollution Control and Resource Reuse Anhui Jianzhu University Hefei Anhui230601 China Anhui Urban Construction Design Institute Corp. Ltd. Hefei Anhui230051 China

ISBN: (纸本)9798400710155

This paper explores the flood control characteristics of a study area in the Guo River Basin, situated in the Northern anhui Plain, under ten-year and twenty-year rainfall conditions. The MIKE 11 model within the DHI MIKE software, developed by the Danish Hydraulic Institute (DHI), is employed for this investigation. By integrating the rainfall-runoff module and hydraulic module, various water flow scenarios are simulated, considering different rainfall and operating conditions. The model calculates changes in water level, flow rate, and flow velocity in each river channel. These data are then used to analyze water dynamic conditions and flood control safety. The study demonstrates that the MIKE11 model effectively simulates rainfall runoff and river network flow in the Guo River Basin. By appropriately configuring and scheduling hydraulic structures, the model proves successful in preventing flooding even under twenty-year heavy rainfall conditions. © 2024 ACM.

关键词： Flood control

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Degradation and detoxification of ribavirin by UV/chlorine/Fe(II) process in water treatment system

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environmental Science and pollution Research 2024年第35期31卷 48164-48174页

作者： Jiang, Yayin He, Zhenle Zhang, Tao Yang, Jing Fan, Yongjie Lu, Zhilei Cai, Kaicong Sun, Qiyuan Wang, Feifeng College of Environmental and Resource Sciences College of Carbon Neutral Modern Industry Fujian Normal University Fujian Fuzhou350117 China Fujian Key Laboratory of Pollution Control & amp Resource Reuse Fujian Fuzhou350117 China College of Chemistry and Materials Science Fujian Provincial Key Laboratory of Advanced Materials Oriented Chemical Engineering Fujian Normal University Fuzhou350117 China Fujian Provincial Key Laboratory of Theoretical and Computational Chemistry Xiamen361005 China

Ribavirin (RBV), which is extensively used to treat viral diseases such as COVID-19, is considered one of the major emerging contaminants due to its long-term existence and health risk in the aqueous environmental system. However, research on effective removal of RBV still remains insufficient. In this study, we investigated the RBV degradation kinetics and mechanism in UV/chlorine/Fe(II) process. The degradation rate constant kobs-RBV of RBV was 2.52 × 10−4 s−1 in UV/chlorine/Fe(II) process, which increased by 1.6 times and 1.3 times than that in chlorine alone and UV/chlorine process, respectively. Notably, trace amount Fe(II) promoted RBV degradation in UV/chlorine system through Fe2+/Fe3+ cycles, enhancing the yield of reactive species such as HO· and certain species reactive chlorine radicals (RCS). The contributions of HO· and RCS toward RBV degradation were 53.91% and 16.11%, respectively. Specifically, Cl·, ClO·, and Cl2·− were responsible for 8.59%, 2.69%, and 4.83% of RBV removal. The RBV degradation pathway indicated that the reactive species preferentially attacked the amide moiety of RBV, which cleaved the ether bond and the hydroxyl group. The toxicity evaluation of RBV degradation products elucidated that UV/chlorine/Fe(II) process was beneficial for RBV detoxification. Graphical abstract: (Figure presented.) © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2024.

关键词： Density functional theory

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Improved atmospheric mercury simulation using updated gas-particle partition and organic aerosol concentrations

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Journal of environmental Sciences 2022年第9期34卷 106-118页

作者： Kaiyun Liu Qingru Wu Shuxiao Wang Xing Chang Yi Tang Long Wang Tonghao Liu Lei Zhang Yu Zhao Qin’geng Wang Jinsheng Chen State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing 100084China Institute of Atmospheric Environment Guangdong provincial academy of environmental scienceGuangzhou 510045China China National Environmental Monitoring Centre Beijing 100012China State Key Laboratory of Pollution Control and Resource Reuse School of the EnvironmentNanjing UniversityNanjing210023China Center for Excellence in Regional Atmos.Environ. Institute of Urban EnvironmentChinese Academy of SciencesXiamen 361021China

The gaseous or particulate forms of divalent mercury(HgⅡ) significantly impact the spatial distribution of atmospheric mercury concentration and deposition flux(FLX). In the new nested-grid GEOS-Chem model, we try to modify the HgⅡ gas-particle partitioning relationship with synchronous and hourly observations at four sites in China. Observations of gaseous oxidized Hg(GOM), particulate-bound Hg(PBM), and PM 2.5 were used to derive an empirical gas-particle partitioning coefficient as a function of temperature( T) and organic aerosol(OA) concentrations under different relative humidity(RH). Results showed that with increasing RH, the dominant process of HgⅡ gas-particle partitioning changed from physical adsorption to chemical desorption. And the dominant factor of HgⅡ gas-particle partitioning changed from T to OA concentrations. We thus improved the simulated OA concentration field by introducing intermediate-volatility and semi-volatile organic compounds(I/SVOCs) emission inventory into the model framework and refining the volatile distributions of I/SVOCs according to new filed tests in the recent literatures. Finally, normalized mean biases(NMBs) of monthly gaseous element mercury(GEM), GOM, PBM, WFLX were reduced from-33%–29%, 95%–300%, 64%–261%, 117%–122% to-13%–0%,-20%–80%,-31%–50%,-17%–23%. The improved model explains 69%–98% of the observed atmospheric Hg decrease during 2013–2020 and can serve as a useful tool to evaluate the effectiveness of the Minamata Convention on Mercury.

关键词： Nested GEOS-Chem model HgⅡgas-particle partitioning Organic aerosol Atmospheric mercury Mercury deposition flux

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Metal-free diatomaceous carbon-based catalyst for ultrafast and anti-interference Fenton-like oxidation

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Chinese Chemical Letters 2024年第12期35卷 351-355页

作者： Kexin Yin Jingren Yang Yanwei Li Qian Li Xing Xu Shandong Key Laboratory of Water Pollution Control and Resource Reuse School of Environmental Science and EngineeringShandong UniversityQingdao 266237China Environment Research Institute Shandong UniversityQingdao 266237China State Environmental Protection Key Laboratory of Environmental Health Impact Assessment of Emerging Contaminants Shanghai Academy of Environmental SciencesShanghai 200233China

Herein,a diatomite biomorphic Si-O doped carbon-based catalyst(DB-SiOC)was prepared using natura mineral diatomite as the silicon source and porous *** results showed that the metal-free DB SiOC catalyst exhibited ultrafast oxidation towards chlorophenol(CP)via peroxymonosulfate(PMS)activa tion,which was almost one order of magnitudes than most of carbon-based *** DB-SiOC/PMS system also showed the high ability to resist the interference of environmental *** radicals(^(·)OH and SO_(4)^(·–))exhibited a very small contribution to the CP oxidation while the electron transfer processe(ETP)played the major role in the DB-SiOC/PMS *** electron shuttles from the electron-donating CP molecules to the adjacent DB-SiOC/PMS^(*)could be efficiently triggered via Si-O bonds as bridges,mak ing it possible for ultrafast oxidation of *** addition,the hollow-disc shaped DB-Si OC provided the biomorphic DE structures with abundant pores for enriching the PMS and pollutants,thus further ac celerating the oxidation *** work provided a new routine for the fabrication of Si-O doped carbon-based catalysts with excellent Fenton-like catalytic activity,which would greatly promote thei application prospects in Fenton-like systems.

关键词： Peroxymonosulfate Diatomite Si-O doping Fenton-like reaction Electron transfer process(ETP)

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Retrofitting low-performance units to abate sewer overflow pollution based on mathematical model and Sobol algorithm

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Journal of Hydrodynamics 2023年第4期35卷 770-781页

作者： Zhi-chao Zhao Xiao-min Huang Hai-long Yin Jun-bo Wen Xiao-wei Fu Changjiang Institute of Survey PlanningDesign and ResearchWuhan430010China Key Laboratory of Yangtze River Water Environment Ministry of EducationTongji UniversityShanghai200092China State Key Laboratory of Pollution Control and Resource Reuse College of Environmental Science and EngineeringTongji UniversityShanghai200092China Hubei Provincial Engineering Research Center for Comprehensive Water Environment Treatment in the Yangtze River Basin Wuhan430010China Key Laboratory of Urban Water Supply Water Saving and Water Environment Governance in the Yangtze River Delta of Ministry of Water ResourcesShanghai200092China

Optimal retrofit of low-performance units(LPUs)is promising to abate overflow pollutant mass loading of sewer systems during *** study presents a combination of mathematical model and Sobol algorithm to help identify LPUs of sewer systems and design retrofitting ***,the solution to minimize the overflow pollutant mass loading from sewers systems can be efficiently *** developed method was demonstrated at a catchment served by one wastewater treatment plant in the Chaohu City,anhui Province of China,with five pumping stations and a total sewer length of 58.3 *** the catchment,there are three rivers and a small lake to receive overflows from the sewer *** them,one river that was mostly polluted was selected as the object of overflow pollution abatement during wet weather *** identifying the LPUs of the sewer system and developing retrofitting strategies using Sobol sequence,the mitigation of overflow pollution during wet weather period was *** show that the mass loading of chemical oxygen demand(COD)discharged into the target river could be reduced by 40.6%,by implementing optimal retrofit strategy of LPUs,i.e.,increasing the conveyance capacities of two pumping stations by 2.5–3.2 times and augmenting the diameters of 12 sewers by 1.25–1.29 *** further coordinate the abatement of overflow pollution and retrofit investment,Sobol sensitivity analysis was conducted to screen the dominant LPUs to update the optimal retrofit *** applying the updated strategy,the overflow COD mass loading per overflow event was close to that of non-updated strategy,while the retrofitting length of sewers was reduced by 40%.Therefore,on the basis of the presented method,decision-makers can flexibly develop retrofitting strategies of sewer system to abate overflow pollution during wet weathers in a cost-effective way.

关键词： Urban sewer system low-performance units Sobol sensitivity analysis sewer overflow optimal retrofit strategy

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Transformation and drive mechanism of nitrogen functional genes at estuaries in dry and wet seasons

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Chemosphere 2024年 363卷 142938页

作者： Huang, Jian Jin, Changzhou Zhang, Hua Zhao, Bingbing Man, Yacan Zhang, Jiamei Shuai, Zichen School of Environmental and Energy Engineering Anhui Jianzhu University Hefei230601 China Anhui Provincial Key Laboratory of Environmental Pollution Control and Resource Reuse Hefei230601 China Pollution Control and Resource Utilization in Industrial Parks Joint Laboratory of Anhui Province Hefei230601 China

The nitrogen cycle plays a vital role in maintaining ecological health and biodiversity. In aquatic systems, nitrogen transformation genes significantly contribute to biological nitrogen cycling. Although the function of these genes is known to be influenced by environmental factors, there is limited research exploring the relationship between nitrogen transformation genes and environmental factors. Therefore, the correlations, between nitrogen transformation genes and environmental factors, were investigated at the estuaries of Chaohu lake (China) in different seasons. The results showed that the values of temperature, pH, organic compounds, nitrogen, and dissolved oxygen were higher in dry season, whereas the abundance of the genes was lower in dry season. In addition, the abundance of the anaerobic ammoxidation gene was much lower than the nitrification gene and denitrification gene. The results indicated that biological nitrification and denitrification were the primary mechanisms for nitrogen removal at estuaries in different seasons, and the reduction of nitric oxide may be a limiting step in the denitrification process. The Co-occurrence Network and Mantel test indicated that, during the dry season, the temperature was the primary driver of ammonification and nitrification functions, the NO3− and NO2− were the primary drivers of denitrification, and the total nitrogen (TN) and NH4+ were the main drivers of anaerobic ammonia oxidation. During the wet season, the dissolved oxygen was the primary driver of ammonification and nitrification functions, the chemical oxygen demand was the primary driver of denitrification, and the TN was the main driver of anaerobic ammonia oxidation. This study provides valuable insights into nitrogen cycling in surface water, contributing to a better understanding of this important process. © 2024 Elsevier Ltd

关键词： Genes

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