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CoS_(2)/N,S co-doped mesoporous carbon with 3D micro-nano crosslinked structure as efficient bifunctional oxygen electrocatalysts for zinc-air batteries

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Chinese Chemical Letters 2023年第5期34卷 604-609页

作者： Wei Wang Liqin Li Jie Ouyang Jialin Gong Jie Tian Liang Chen Junlin Huang Binhong He Zhaohui Hou Key Laboratory of Hunan Province for Advanced Carbon-based Functional Materials School of Chemistry and Chemical EngineeringHunan Institute of Science and TechnologyYueyang 414006China Guangxi Key Laboratory of Low Energy Material Guangxi Normal UniversityGuilin 541004China Hubei Key Laboratory of Pollutant Analysis&Reuse Technology Hubei Normal UniversityHuangshi 435002China Hunan Province Key Laboratory of Materials Surface&Interface Science and Technology Material Science and Engineering SchoolCentral South University of Forestry and TechnologyChangsha 410004China

This work describes a bifunctional oxygen catalyst made of cobalt disulfide encapsulated in N,S codoped mesoporous carbon with a novel three-dimensional micro-nano crosslinking *** proposed composite materials exhibit promising oxygen electrocatalytic activity and *** composite assembled rechargeable zinc-air battery can achieve a high power density of 208.9 m W/cm^(2),and can be stably cycled for more than 160 ***,the all-solid zinc-air battery assembled with the electrocatalyst also performs *** micro-nano crosslinking and high porosity structure,as well as the large number of active sites generated by the synergy of N,S doping and the close interface between carbon matrix and CoS_(2),contribute to the composite's exceptional electrochemical *** study's rational strategy lays the path for the development of other high-performance bifunctional electrocatalysts.

关键词： Micro-nano crosslinked CoS_2 ORR OER Zn-air battery

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Self-assembled CoOOH on TiO_(2) for enhanced photoelectrochemical water oxidation

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Journal of Energy Chemistry 2021年第9期30卷 512-521页

作者： Xiangrong Ren Yujin Ji Yiyue Zhai Ningyi Yuan Jianning Ding Youyong Li Junqing Yan Shengzhong Frank Liu Key Laboratory of Applied Surface and Colloid Chemistry Ministry of EducationShaanxi Key Laboratory for Advanced Energy DevicesShaanxi Engineering Lab for Advanced Energy TechnologySchool of Materials Science and EngineeringShaanxi Normal UniversityXi’an 710119ShaanxiChina Institute of Functional Nano&Soft Materials(FUNSOM) Jiangsu Key Laboratory for Carbon-Based Functional Materials&DevicesSoochow UniversitySuzhou 215123JiangsuChina iChEM Dalian Institute of Chemical PhysicsUniversity of Chinese Academy of SciencesChinese Academy of SciencesDalian 116023LiaoningChina School of Materials Science and Engineering Jiangsu Collaborative Innovation Center of Photovoltaic Science and EngineeringJiangsu Cultivation Base for State Key Laboratory of Photovoltaic Science and TechnologyChangzhou UniversityChangzhou 213164JiangsuChina

Providing efficient charge transfer through the interface between the semiconductor and co-catalyst is greatly desired in photoelectrocatalytic (PEC) energy ***,we excogitate a novel and facile means,via electrochemical activation,to successfully load the amorphous CoOOH layer architecture onto the surface of TiO_(2).Intriguingly,the as-obtained 6%CoOOH-TiO_(2)photoelectrode manifests optimal PEC performance with a high photocurrent density of 1.3 mA/cm~2,3.5 times higher than that of pristine TiO_(2).Electrochemical impedance spectroscopy (EIS),Tafel analysis and cyclic voltammetry (CV) methods show that the carrier transfer barrier within the electrode and the transition of Co^(3+)OOH to Co^(4+)OOH have the dominating effects on the PEC *** calculation reveals that the interface between the CoOOH and TiO_(2)improves the homogeneity of effective d-orbital electronic-transfer ability among Co *** research sheds light on the water oxidation reaction and the design of more favorable PEC cocatalysts.

关键词： Amorphous Co-catalyst Water oxidation Mechanism TiO_(2)

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Sandwiching Sulfur into the Dents Between N,O Co-Doped Graphene Layered Blocks with Strong Physicochemical Confinements for Stable and High-Rate Li-S Batteries

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Nano-Micro Letters 2020年第11期12卷 13-24页

作者： Mengjiao Shi Su Zhang Yuting Jiang Zimu Jiang Longhai Zhang Jin Chang Tong Wei Zhuangjun Fan Key Laboratory of Superlight Materials and Surface Technology Ministry of EducationCollege of Material Science and Chemical EngineeringHarbin Engineering UniversityHarbin 150001People’s Republic of China Key Laboratory of Energy Materials Chemistry Ministry of EducationKey Laboratory of Advanced Functional MaterialsAutonomous RegionInstitute of Applied ChemistryXinjiang UniversityUrumqi 830046People’s Republic of China State Key Laboratory of Heavy Oil Processing School of Materials Science and EngineeringChina University of PetroleumQingdao 266580People’s Republic of China

The development of lithium-sulfur batteries(LSBs)is restricted by their poor cycle stability and rate performance due to the low conductivity of sulfur and severe shuttle ***,an N,O co-doped graphene layered block(NOGB)with many dents on the graphene sheets is designed as effective sulfur host for high-performance LSB *** sulfur platelets are physically confined into the dents and closely contacted with the graphene scaffold,ensuring structural stability and high *** highly doped N and O atoms can prevent the shuttle effect of sulfur species by strong chemical ***,the micropores on the graphene sheets enable fast Li^+transport through the *** a result,the obtained NOGB/S composite with 76 wt%sulfur content shows a high capacity of 1413 mAh g^-1 at 0.1 C,good rate performance of 433 mAh g^-1 at 10 C,and remarkable stability with 526 mAh g^-1 at after 1000 cycles at 1 C(average decay rate:0.038%per cycle).Our design provides a comprehensive route for simultaneously improving the conductivity,ion transport kinetics,and preventing the shuttle effect in LSBs.

关键词： Graphene Physicochemical confinement Cycle stability Shuttle effect Li-S batteries

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Ductile and high strength Cu fabricated by solid-state cold spray additive manufacturing

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Journal of Materials science & technology 2023年第3期134卷 234-243页

作者： Chaoyue Chen Yingchun Xie Shuo Yin Wenya Li Xiaotao Luo Xinliang Xie Ruixin Zhao Chunming Deng Jiang Wang Hanlin Liao Min Liu Zhongming Ren State Key Laboratory of Advanced Special Steels School of Materials Science and EngineeringShanghai UniversityShanghai 200444China Institute of New Materials Guangdong Academy of SciencesNational Engineering Laboratory of Modern Materials Surface Engineering TechnologyGuangdong Provincial Key Laboratory of Modern Surface Engineering TechnologyGuangzhou 510651China Trinity College Dublin The University of DublinDepartment of Mechanical and Manufacturing EngineeringParsons BuildingDublin 2Ireland State Key Laboratory of Solidification Processing Shaanxi Key Laboratory of Friction Welding TechnologiesSchool of Materials Science and EngineeringNorthwestern Polytechnical UniversityXi’an 710072China State Key Laboratory for Mechanical Behavior of Materials School of Materials Science and EngineeringXi’an Jiaotong UniversityXi’an 710049China Key laboratory for Light-weight Materials Nanjing Techchnology UniversityNanjing 211816China ICB UMR 6303 CNRSUniv.Bourgogne Franche-ComtéUTBMF-90010 BelfortFrance

In this work,pure Cu with excellent strength and ductility(UTS of 271 MPa,elongation to fracture of 43.5%,uniform elongation of 30%)was prepared using cold spray additive manufacturing(CSAM),realizing a breakthrough in the *** in-depth investigation was conducted to reveal the microstructure evolution,strengthening and ductilization mechanisms of the CSAM Cu,as well as the single *** results show that the CSAM Cu possesses a unique heterogeneous microstructure with a bimodal grain structure and extensive infinitely circulating ring-mounted distribution of *** on the single splat observation,the entire copper particle forms a gradient nano-grained(GNG)structure after high-speed impact *** GNG-structured single splat serves as a unit to build the heterogeneous microstructure with bimodal grain distribution during the successive deposition in *** results also show that CSAM can achieve synergistic strengthening and ductilization by controlling the grain refinement and dislocation *** work provides potential for CSAM technique in manufacturing various metallic parts with the desired combination of high strength and good ductility without additional post-treatments.

关键词： Cold spray additive manufacturing Copper Heterogeneous microstructure Strength Ductility

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Effect of homogenization annealing on internal residual stress distribution and texture in ME21 magnesium alloy extruded plates

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Journal of Magnesium and Alloys 2019年第1期7卷 186-192页

作者： Yong Lian Pengfei Ji Jin Zhang Xiaomin Yuan Weisheng Xu Yongle Zhao Jiahao Mo Lin Zheng Shitao Dou Institute for Advanced Materials and Technology University of Science and Technology BeijingBeijing 100083China Beijing Key Laboratory of Corrosion Erosion and Surface TechnologyBeijing 100083China Capital Aerospace Machinery Company Beijing 10076China Institute of Southwest Technology and Engineering Chongqing 400039China

The distribution of residual stresses through thickness of 5 mm-thick ME21 magnesium alloy extruded plates was analyzed non-destructively using short-wavelength X-ray diffraction(SWXRD),and the effect of homogenization annealing before extrusion on the residual stress was *** classic d 0 method with an annealed stress-free reference specimen was employed to determine the residual stress of the extruded *** residual stress results showed that the gradient of residual stress in the transverse direction was larger than that of the extrusion *** homogenization process prior to extrusion weaken the formed sample’s *** maximum residual stress of the as-extruded plate was reduced,and the residual stress distribution was homogenized.

关键词： ME21 magnesium alloy Homogenization annealing Residual stress Short-wavelength X-ray diffraction

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High-rate sodium-ion storage of vanadium nitride via surface-redox pseudocapacitance

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Interdisciplinary Materials 2023年第3期2卷 434-442页

作者： Qiulong Wei Tingyi Huang Xiaojuan Huang Binhao Wang Yalong Jiang Dafu Tang Dong-Liang Peng Bruce Dunn Liqiang Mai Department of Materials Science and Engineering Fujian Key Laboratory of Surface and Interface Engineering for High Performance MaterialsCollege of MaterialsXiamen UniversityXiamenChina State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhanChina Department of Materials Science and Engineering University of California Los AngelesLos AngelesCaliforniaUSA

Vanadium nitride(VN)electrode displays high-rate,pseudocapacitive responses in aqueous electrolytes,however,it remains largely unclear in nonaqueous,Na+-based *** traditional view supposes a conversion-type mechanism for Na+storage in VN anodes but does not explain the phenomena of their size-dependent specific capacities and underlying causes of pseudocapacitive charge storage ***,we insightfully reveal the VN anode exhibits a surface-redox pseudocapacitive mechanism in nonaqueous,Na+-based electrolytes,as demonstrated by kinetics analysis,experimental observations,and first-principles *** ex situ X-ray photoelectron spectroscopy and semiquantitative analyses,the Na+storage is characterized by redox reactions occurring with the V5+/V4+to V3+at the surface of VN particles,which is different from the well-known conversion reaction *** pseudocapacitive performance is enhanced through nanoarchitecture design via oxidized vanadium states at the *** optimized VN-10 nm anode delivers a sodium-ion storage capability of 106 mAh g−1 at the high specific current of 20 A g−1,and excellent cycling performance of 5000 cycles with negligible capacity *** work demonstrates the emerging opportunities of utilizing pseudocapacitive charge storage for realizing high-rate sodium-ion storage applications.

关键词： high-rate capability pseudocapacitance sodium-ion storage vanadium nitride

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Recent advances in resistive random access memory based on lead halide perovskite

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InfoMat 2021年第3期3卷 293-315页

作者： Jiayu Di Jianhui Du Zhenhua Lin Shengzhong(Frank)Liu Jianyong Ouyang Jingjing Chang State Key Discipline Laboratory of Wide Band Gap Semiconductor Technology Shaanxi Joint Key Laboratory of GrapheneSchool of MicroelectronicsXidian UniversityXi'anChina Advanced Interdisciplinary Research Center for Flexible Electronics Xidian UniversityXi'anChina Key Laboratory of Applied Surface and Colloid Chemistry Ministry of EducationShaanxi Key Laboratory for Advanced Energy DevicesShaanxi Engineering Lab for Advanced Energy TechnologyInstitute for Advanced Energy MaterialsSchool of Materials Science and EngineeringShaanxi Normal UniversityXi'anChina Department of Materials Science and Engineering National University of SingaporeSingaporeSingapore

Lead halide perovskites have attracted increasing attention in photovoltaic devices,light-emitting diodes,photodetectors,and other fields due to their excellent *** optoelectronic devices,growing numbers of studies have focused on the perovskite-based electrical devices in the past few years,such as transistors and resistive random access memories(RRAMs).Here,this article summarizes the recent progress the researchers have made of RRAM ***,the working mechanism and the key parameters of RRAM are ***,the working principles,including the conductive filament model(containing the types of the model of the metal cationsinduced filament and the model of the ions migration in bulk),the interface effect,and the electronic effect are the origins of the RRAM behaviors,and hence,various factors that affect the device performance are ***,RRAMs based on organolead halide perovskite and all-inorganic perovskite are discussed in terms of different structures,different compositions,and different fabrication ***,a brief conclusion and a broad outlook are given on the progress and challenges in the field of perovskite-based RRAMs.

关键词： all-inorganic perovskites conductive filament models organolead halide perovskites resistive random access memories resistive switching

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Powder injection molding of Ti6Al4V alloy

Powder injection molding of Ti6Al4V alloy

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5th International Conference on Processing and Manufacturing of advanced Materials, THERMEC 2006

作者： Qu, Xuan Hui Guo, Shi Bo Tang, Chun Feng Qin, Ming Li He, Xin Bo Islam, Syed Humail School of Materials Science and Engineering State Key Laboratory for Advanced Metals and Materials University of Science and Technology Beijing Beijing100083 China Jiangxi Key Laboratory of Surface Engineering Jiangxi Science and Technology Normal University Nanchang China

ISBN: (纸本)9780878494286

An improved wax-based binder was developed for powder injection molding of Ti6Al4V alloy. The molding behavior, debinding kinetics and sintering process were studied. Components with relative density of 96.5% were produced with PIM process. The density of the components was increased up to 99% by HIP treatment. The tensile properties of the alloy were as follows: tensile strength 1060MPa, yield stress 960MPa, elongation 9.5%, which are equivalent to those of the same alloy made with traditional press-sintering process. The dimension deviation of the sintered samples could be controlled in the range of ±0.03mm with the optimized processing parameters. © (2007) Trans Tech Publications, Switzerland.

关键词： Aluminum alloys

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Al-modification for PS-PVD 7YSZ TBCs to improve particle erosion and thermal cycle performances

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Journal of advanced Ceramics 2022年第7期11卷 1093-1103页

作者： Xiaofeng ZHANG Ming LI Ao ZHANG Shuangquan GUO Jie MAO Chunming DENG Panpan WANG Changguang DENG Junli FENG Min LIU Kesong ZHOU Cheng LAI National Engineering Laboratory for Modern Materials Surface Engineering Technology&the Key Lab of Guangdong for Modern Surface Engineering Technology Institute of New MaterialsGuangdong Academy of ScienceGuangzhou 510650China PERA Guangzhou Information Technology Co. Ltd.Guangzhou 510650China Chengdu Holy(Group)Industry Co. Ltd.Chengdou 610000China School of Aviation and Mechanical Engineering Changzhou Institute of TechnologyChangzhou 213032China Shenzhen Customs Industrial Products Inspection Technology Center Shenzhen 518067China

Plasma spray-physical vapor deposition(PS-PVD)as a novel process was used to prepare feather-like columnar thermal barrier coatings(TBCs).This special microstructure shows good strain tolerance and non-line-of-sight(NLOS)deposition,giving great potential application in ***,due to serious service environment of aero-engine,particle erosion performance is a weakness for PS-PVD 7YSZ *** a solution,an Al-modification approach was proposed in this *** in-situ reaction of Al and ZrO2,anα-Al2O3 overlay can be formed on the surface of 7YSZ columnar *** results demonstrate that this approach can improve particle erosion resistance since hardness improvement of Al-modified ***,as another important performance of thermal cycle,it has a better optimization with 350-cycle water-quenching,compared with the as-sprayed TBCs.

关键词： plasma spray-physical vapor deposition(PS-PVD) thermal barrier coatings(TBCs) Al-modification particle erosion resistance thermal cycle performance

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Shining light on transition metal tungstate-based nanomaterials for electrochemical applications:Structures,progress,and perspectives

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Nano Research 2022年第8期15卷 6924-6960页

作者： Kaijia Feng Zhefei Sun Yong Liu Feng Tao Junqing Ma Han Qian Renhong Yu Kunming Pan Guangxin Wang Shizhong Wei Qiaobao Zhang National Joint Engineering Research Center for Abrasion Control and Molding of Metal Materials Henan Key Laboratory of Non–Ferrous Materials Science&Processing TechnologySchool of Materials Science and EngineeringHenan University of Science and TechnologyLuoyang 471023China Provincial and Ministerial Co–construction of Collaborative Innovation Center for Non-ferrous Metal New Materials and Advanced Processing Technology Henan Key Laboratory of High-temperature Structural and Functional MaterialsHenan University of Science and TechnologyLuoyang 471023China Department of Materials Science and Engineering College of MaterialsXiamen UniversityXiamen 361005China Fujian Key Laboratory of Surface and Interface Engineering for High Performance Materials Xiamen UniversityXiamen 361005China

Transition metal tungstate-based nanomaterials have become one of the research hotspots in electrochemistry due to their abundant natural resources,low costs,and environmental *** studies have demonstrated their significant potentials for electrochemical applications,such as supercapacitors,Li-ion batteries,Na-ion batteries,electrochemical sensing,and *** the rapidly growing research enthusiasm for this topic over the last several years,herein,a critical review of recent progress on the application of transition metal tungstates and their composites for electrochemical applications is *** relationships between synthetic methods,nano/micro structures and electrochemical properties are systematically ***,their promising prospects for future development are also *** is anticipated that this review will inspire ongoing interest in rational designing and fabricating novel transition metal tungstate-based nanomaterials for high-performance electrochemical devices.

关键词： transition metal tungstates supercapacitors lithium-ion batteries sodium-ion batteries electrochemical sensing electrocatalysis

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