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A review of whole-process control of industrial volatile organic compounds in China

Journal of Environmental Sciences 2023年第1期123卷 127-139页

作者： Hailin Wang Shumei Sun Lei Nie Zhongshen Zhang Wenpeng Li Zhengping Hao Beijing Key Laboratory for Urban Atmospheric VOCs Pollution Control and Technology Application Beijing Municipal Research Institute of Environmental ProtectionBeijing 100037China College of Resources Environment and Tourism Capital Normal UniversityBeijing 100048China National Engineering Laboratory for VOCs Pollution Control Material&Technology Research Center for Environmental Material and Pollution Control TechnologyUniversity of Chinese Academy of SciencesBeijing 101408China

Volatile organic compounds(vocs)play an important role in the formation of ground-level ozone and secondary organic aerosol(SOA),and they have been key issues in current air pollution prevention and control in *** attention has been paid to industrial activities due to their large and relatively complex vocs *** present research aims to provide a comprehensive review on whole-process control of industrial vocs,which mainly includes source reduction,collection enhancement and end-pipe *** vocs materials including water-borne ones are the keys to source substitution in industries related to coating and solvent usage,leak detection and repair(LDAR)should be regarded as an efficient means of source reduction in refining,petrochemical and other chemical *** types of vocs collection methods such as gas-collecting hoods,airtight partitions and others are discussed,and airtight collection at negative pressure yields the best collection *** end-pipe treatments like UV oxidation,low-temperature plasma,activated carbon adsorption,combustion,biodegradation,and adsorption-combustion are discussed in ***,several recommendations are made for future advanced treatment and policy development in industrial vocs emission control.

关键词： Volatile organic compounds Materials substitution Collection enhancement End-pipe treatments

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Aerosol-radiation interaction and its variation in North China within 2015–2019 period under continuous PM_(2.5)improvements

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Journal of Environmental Sciences 2024年第2期136卷 81-94页

作者： Zhe Lv Xiaoqi Wang Wei Wei Huahua Bai Xiaoyu Liu Guohao Li Shuiyuan Cheng Department of Environmental Science and Engineering Beijing University of TechnologyBeijing 100124China Key Laboratory of Beijing on Regional Air Pollution Control Beijing 100124China Beijing Municipal Research Institute of Eco-Environmental Protection Beijing 100037China Beijing Key Laboratory of Urban Atmospheric Volatile Organic Compounds Pollution Control and Application Beijing 100037China

A study was conducted on aerosol-radiation interactions over six cities in this region within the 2015–2019 ***-Chem simulations on 2017 showed that based on the six-city average,the aerosol load(PM_(2.5)concentrations)of 121.9,49.6,43.3,and 66.3μg/m^(3)in January,April,July,and October,mainly lowered the level of downward shortwave radiation by 38.9,24.0,59.1,and 24.4 W/m~2and reduced the boundary layer height by 79.9,40.8,87.4,and 31.0 m,via scattering and absorbing solar *** sensitivity of meteorological changes to identical aerosol loads varied in the order July>January>October and ***,the cooling and stabilizing effects of aerosols further led to increases in PM_(2.5),by23.0,3.4,4.6,and 7.3μg/m^(3)respectively in the four *** sensitivity of the effect of aerosols on PM_(2.5)was greatest in January rather than in July,contrary to the effect on ***,a negative linear relation was observed between daily BLH reductions and aerosol loads in fall and winter,and between PM_(2.5)increases and aerosol loads in all *** the PM_(2.5)pollution improvements in this region,the aerosol radiative forcing was effectively *** should result in daily BLH increases of 10–24 m in fall and winter,and the estimates in beijing agreed well with the corresponding results based on AMDAR ***,the reduction in aerosol radiation effects brought about daily PM_(2.5)decreases of 1.6-2.8μg/m^(3),accounting for 7.0%–17.7%in PM_(2.5)improvements.

关键词： Radiative forcing Aerosol PM_(2.5) Boundary layer height(BLH) North China

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Adsorption of typical gasoline vapor emitted from service stations by commercial activated carbon:static/dynamic adsorption and kinetics simulation

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Frontiers of Environmental Science & Engineering 2025年第3期19卷 87-98页

作者： Wei Hu Quanming Liang Dan Lu Beibei Li Biqi Ren Qingye Luan Jia Liu Wenjun Liang Yuhu Huang National Engineering Research Center of Urban Environmental Pollution Control Beijing Key Laboratory of Urban Atmospheric Volatile Organic Compounds Control Technology and ApplicationsBeijing Municipal Research Institute of Eco-Environmental ProtectionBeijing 100037China Key Laboratory of Beijing on Regional Air Pollution Control Faculty of Environment and LifeBeijing University of TechnologyBeijing 100124China Institute of Urban Safety and Environmental Science Beijing Academy of Science and TechnologyBeijing 100054China

Gasoline vapor emissions from service stations significantly affect urban *** the research on the mechanisms and effectiveness of gasoline vapor removal is limited,this study innovatively investigates the static and dynamic adsorption of xylene—a typical gasoline vapor and one of the most active secondary organic aerosol(SOA)species—by commercial activated carbon(AC).The results showed that the saturation static adsorption capacity(Q_(e))of 12 ACs varied from 0.9 to 870.7 mg/g,which correlated with the specific surface area(SSA)and pore *** them,11#and 12#ACs were identified as the most effective adsorbents for typical gasoline vapor *** maximum dynamic Q_(e) increased from 301.5 to 414.3 mg/g when the initial xylene concentration rose from 918 to 2008 mg/m^(3) for 11#AC,and from 201.4 to 406.2 mg/g when the initial xylene concentration increased from 589 to 2120 mg/m^(3) for 12#*** findings implied a direct correlation between higher initial xylene concentrations and greater dynamic Q_(e) values,with static Q_(e) values surpassing dynamic *** adsorption kinetics simulation were analyzed by the pseudo-first-order(PFO)and pseudo-second-order(PSO)*** kinetics results demonstrated that the PFO was more effective in characterizing the adsorption of xylene onto ACs(R2>0.989),indicating that the adsorption of typical gasoline vapor by ACs primarily involves physical *** findings of static/dynamic adsorption and kinetics provide valuable guidance for practical applications of gasoline vapor removal in service stations.

关键词： Activated carbon Gasoline vapor Xylene Dynamic adsorption Breakthrough curve

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Chemical characterization of volatile organic compounds (vocs) emitted from multiple cooking cuisines and purification efficiency assessments

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Journal of Environmental Sciences 2023年第8期130卷 163-173页

作者： Hanyu Zhang XuejunWang Xianbao Shen Xin Li BoboWu Guohao Li Huahua Bai Xinyue Cao Xuewei Hao Qi Zhou Zhiliang Yao School of Ecology and Environment Beijing Technology and Business UniversityBeijing 100048China State Environmental Protection Key Laboratory of Food Chain Pollution Control Beijing Technology and Business UniversityBeijing 100048China Beijing Municipal Research Institute of Environmental Protection Beijing Key Laboratory of Urban Atmospheric Volatile Organic Compounds Pollution Control and ApplicationNational Urban Environmental Pollution Control Engineering Research CenterBeijing 100037China

Cooking process can produce abundant volatile organic compounds(vocs),which are harmful to environment and human ***,we conducted a comprehensive analysis in which vocs emissions from multiple cuisines have been sampled based on the simulation and acquisition platform,involving concentration characteristics,ozone formation potential(OFP)and purification efficiency *** emissions varied from 1828.5 to 14,355.1μg/m^(3),with the maximumand minimumvalues fromBarbecue and Family cuisine,*** and alcohol had higher contributions to vocs from Sichuan and Hunan cuisine(64.1%),Family cuisine(66.3%),Shandong cuisine(69.1%)and Cantonese cuisine(69.8%),with the dominant vocs species of ethanol,isobutane and *** comparison,alcohols(79.5%)were abundant for Huaiyang cuisine,while alkanes(19.7%),alkenes(35.9%)and haloalkanes(22.9%)accounted for higher proportions from ***,carbon tetrachloride,n-hexylene and 1-butene were the most abundant vocs species for Barbecue,ranging from 8.8%to 14.6%.The highest OFP occurred in *** sensitive species of OFP for Huaiyang cuisine were alcohols,while other cuisines were *** efficiency assessments shed light on the removal differences of individual and synergistic control *** emissions exhibited a strong dependence on the photocatalytic oxidation,with the removal efficiencies of 29.0%–54.4%.However,the high voltage electrostatic,wet purification and mechanical separation techniques played a mediocre or even counterproductive role in the vocs reduction,meanwhile collaborative control technologies could not significantly improve the removal *** results identifiedmore effective control technologies,which were conductive to alleviating air pollution from cooking emissions.

关键词： Cooking emissions Volatile organic compounds(vocs) vocs categories Ozone formation potential(OFP) Purification efficiency

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Advanced modeling of the absorption enhancement of black carbon particles in chamber experiments by considering the morphology and coating thickness

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Frontiers of Environmental Science & Engineering 2024年第9期18卷 129-142页

作者： Xiaodong Wei Jianlin Hu Chao Liu Xiaodong Xie Junjie Yin Song Guo Min Hu Jianfei Peng Huijun Wang Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control Collaborative Innovation Center of Atmospheric Environment and Equipment TechnologySchool of Environmental Science and EngineeringNanjing University of Information Science&TechnologyNanjing 210044China Collaborative Innovation Center on Forecast and Evaluation of Meteorological Disasters Key Laboratory of Meteorological Disaster(Ministry of Education)Nanjing University of Information Science and TechnologyNanjing 210044China Nansen−Zhu International Research Centre Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China East China Air Traffic Management Bureau CAAC Shanghai 200335China State Key Joint Laboratory of Environmental Simulation and Pollution Control International Joint Laboratory for Regional Pollution Control(IJRC)(Ministry of Education)College of Environmental Sciences and EngineeringPeking UniversityBeijing 100871China Tianjin Key Laboratory of Urban Transport Emission Research&State Environmental Protection Key Laboratory of Urban Ambient Air Particulate Matter Pollution Prevention and Control College of Environmental Science and EngineeringNankai UniversityTianjin 300071China

Measurements studies have shown that the absorption of radiation by black carbon(BC)increases as the particles ***,there are significant discrepancies between the measured and modeled absorption enhancement(E_(abs)),largely due to the simplifications used in modeling the mixing states and shape *** took advantage of chamber experiments on BC aging and developed an efficient method to resolve the particle shape based on the relationship between the coating fraction(ΔD_(ve)/D_(ve),0)and fractal dimension(D_(f)),which can also reflect the variations of D_(f)during the whole BC aging *** with externally and partly mixed states(0≤ΔD_(ve)/D_(ve),0≤0.5)can be considered to be uniformly distributed with the D_(f)values of 1.8–2.1,whereas the Df values are constrained in the range 2.2–2.8 for fully mixed states(ΔD_(ve)/D_(ve),0>0.5).The morphological parameters(i.e.,the effective density and the dynamic shape factor)were compared with the measured values to verify the simulated *** simulated mean deviations of morphological parameters were smaller than 8%for the method resolving the particle *** applying a realistic shape and refractive index,the mass absorption cross for fully mixed states can be improved by 11%compared with a simplified core–shell *** on our understanding of the influence of D_(f)andΔD_(ve)/D_(ve),0 on E_(abs),we propose a two-stage calibration equation to correct the E_(abs)values estimated by the core–shell model,which reduces the simulation error in the Mie calculation by 6%–14%.

关键词： Black carbon Mixing states Fractal dimension Dynamic shape factor Absorption enhancement

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Emission characteristics and influences assessment of volatile organic compounds from a typical petrochemical park in the beijing-Tianjin-Hebei Region

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Zhongguo Huanjing Kexue/China Environmental Science 2025年第5期45卷 2423-2433页

作者： Zhang, Xiang-Rui Wei, Wei Li, Guo-Hao Bai, Hua-Hua Liu, Xiao-Yu Lyu, Zhe Key Laboratory of Beijing on Regional Air Pollution Control College of Environment Sciences and Technology Beijing University of Technology Beijing100124 China Beijing Key Laboratory of Urban Atmospheric Volatile Organic Compounds Pollution Control and Application Beijing100037 China National Engineering Research Center of Urban Environmental Pollution Control Beijing Municipal Research Institute of Eco-Environmental Protection Beijing100037 China

We chose a petrochemical park in beijing-Tianjin-Hebei as the research target, and five representative sites were selected for sampling and analysis. 85 volatile organic compounds (vocs) were detected and their impacts on the environment and health were evaluated. The results showed that the concentration of total volatile organic compounds (Tvocs) were 546.0~4472.2µg/m3, in which alkanes and alkenes were the dominant group, followed by aromatics and halocarbons. Compared with the diurnal variation of vocs components at each site, the time of peak and valley values appearing were different, and the typical species were different. Additionally, OFP in the synthetic rubber area was the richest (13239.8µg/m3). The contribution of alkenes to OFP was the highest (62.8%~90.5%), followed by alkanes (3.8%~34.8%) and aromatics (2.2%~22.1%). Otherwise, only the synthetic rubber area was polluted by odor, 1,3-butadiene (0.68) and n-hexane (0.30) were the main vocs species that produced odor. Moreover, the health risk associated with each site was assessed by the US EPA method, indicating that the non-cancer risk of synthetic rubber and cancer risk of oil refining were higher than those of other sites. © 2025 Chinese Society for Environmental Sciences. All rights reserved.

关键词： Diseases

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Ten-year emission characteristics of atmospheric pollutants from incineration of sacrificial offerings in China

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Journal of Environmental Sciences 2022年第4期34卷 391-400页

作者： Yangyang Cui Gen Zhang Wei Wang Yan Shen Xiaoman Zhai Xuefang Wu Renfei Li Bobo Wu Yifeng Xue National Engineering Research Center of Urban Environmental Pollution Control Beijing Municipal Research Institute of Environmental ProtectionBeijing 100037China State Key Laboratory of Severe Weather&Key Laboratory for Atmospheric Chemistry of CMA Institute of Atmospheric CompositionChinese Academy of Meteorological SciencesBeijing 100081China Key Laboratory of Pollution Control of Ministry of Civil Affairs 101 Institute of Ministry of Civil AffairsBeijing 100070China Beijing Technology and Business University Beijing 100048China

The incineration of sacrificial offerings is a significant widely practiced custom that is also a kind of neglected air pollution source in *** results showed that the emission factors of particulate matter,SO_(2),CO,NO_(x),and vocs emitted from the incineration of sacrificial offerings with purification systems were reduced by 95%,19%,9%,82%,and 42%,respectively,compared with those without a purification system,revealing a significant effect of the flue gas purification system on reducing particulate matter and gaseous *** emission level of air pollutants from the incineration of sacrificial offerings remained stable before 2013 and then showed a remarkable decrease after the implementation of China′s Air pollution Prevention Action Plan in *** emissions of TSP(total suspended particulate),PM_(10),PM_(2.5),and NO_(x)in 2009 were 8222,6106,5656 and 15,878 ton,respectively,obviously higher than 3434,2551,2305 and 8579 ton in *** trend was affected by both the quantity of incineration and the installation rate of purification systems after the Emission Standard of Air Pollutants for Crematory(GB 13801-2015)issued in *** spatial distribution of atmospheric pollutants from incineration of sacrificial offerings was found with higher in the east and south of China than the west and north of China,which is proportional to the regional economy and *** maximum ground-level concentration typically occurred at 0.12-0.2 km from the pollution source,posing potential health risks to people entering and exiting funeral and burial sites and nearby residents.

关键词： Incineration of sacrificial offerings atmospheric pollutants Purification system Emission inventory

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atmospheric environment monitoring technology and equipment in China:A review and outlook

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Journal of Environmental Sciences 2023年第1期123卷 41-53页

作者： Youwen Sun Ting Yang Huaqiao Gui Xin Li Weigang Wang Jun Duan Shushuai Mao Hao Yin Bin Zhou Jianlei Lang Haijin Zhou Cheng Liu Pinhua Xie Key Laboratory of Environmental Optics and Technology Anhui Institute of Optics and Fine MechanicsHFIPSChinese Academy of SciencesHefei 230031China Department of Precision Machinery and Precision Instrumentation University of Science and Technology of ChinaHefei 230026China State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China State Key Joint Laboratory of Environmental Simulation and Pollution Control College of Environmental Sciences and EngineeringPeking UniversityBeijing 100871China State Key Laboratory for Structural Chemistry of Unstable and Stable Species Institute of ChemistryChinese Academy of SciencesBeijing 100190China Key Laboratory of Beijing on Regional Air Pollution Control College of Environmental&Energy EngineeringBeijing University of TechnologyBeijing 100124China Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention(LAP3) Department of Environmental Science and EngineeringFudan UniversityShanghai 200438China Center for Excellence in Regional Atmospheric Environment Institute of Urban EnvironmentChinese Academy of SciencesXiamen 361021China Key Laboratory of Precision Scientific Instrumentation of Anhui Higher Education Institutes University of Science and Technology of ChinaHefei 230026China Anhui Province Key Laboratory of Polar Environment and Global Change University of Science and Technology of ChinaHefei 230026China

Accurate monitoring of the atmospheric environment and its evolution are important for understanding the sources,chemical mechanisms,and transport processes of air pollution and carbon emissions in China,and for regulatory and control *** study gives an overview of atmospheric environment monitoring technology and equipment in China and summarizes the major achievements obtained in recent *** has made great progress in the development of atmospheric environment monitoring technology and equipment with decades of *** manufacturing level of atmospheric environment monitoring equipment and the quality of products have steadily improved,and a technical&production system that can meet the requirements of routine monitoring activities has been *** is expected that domestic atmospheric environment monitoring technology and equipment will be able to meet future demands for routine monitoring activities in China and provide scientific assistance for addressing air pollution problems.

关键词： atmospheric pollution atmospheric environment atmospheric monitoring Environmental instrument

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Low-condensation diesel use contributes to winter haze in cold regions of China

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Environmental Science and Ecotechnology 2024年第6期22卷 226-232页

作者： Weiwei Song Mengying Wang Yixuan Zhao Yu Bo Wanying Yao Ruihan Chen Xianshi Wang Xiaoyan Wang Chunhui Li Kebin He State Key Laboratory of Urban Water Resource and Environment School of EnvironmentHarbin Institute of TechnologyHarbin150090China State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing100084China Institute of Atmospheric Physics Chinese Academy of SciencesBeijing100029China Harbin Ecological and Environmental Monitoring Center Harbin150076China Collaborative Innovation Center for Regional Environmental Quality Beijing100084China State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing100084China

The application of low-condensation diesel in cold regions with extremely low ambient temperatures(−14 to−29℃)has enabled the operation of diesel ***,it may contribute to heavy haze pollution in cold regions during *** we examine pollutant emissions from low-condensation diesel in *** measure the emissions of elemental carbon(EC),organic carbon(OC),and elements,including heavy metals such as arsenic(As).Our results show that low-condensation diesel increased EC and OC emissions by 2.5 and 2.6 times compared to normal diesel fuel,*** of vehicular sources,including EC,As,lead(Pb),cadmium(Cd),chromium(Cr),nickel(Ni),and manganese(Mn),increased by approximately 20.2-162.5%when using low-condensation *** variation of vehicular source indicators,observed at road site ambient environments revealed the enhancement of PM2.5 pollution by the application of low-condensation diesel in *** findings suggest that−35#diesel,a low-cetane index diesel,may enhance air pollution in winter,according to a dynamometer test conducted in *** raises questions about whether higher emissions are released if−35#diesel is applied to running vehicles in real-world cold ambient environments.

关键词： Low condensation diesel Carbonaceous matterHeavy metal Dynamometer Cold regions

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Tuning SMSI to stabilize metallic Pd species:A case study on Pd/TiO_(2) for HCHO oxidation

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Chinese Chemical Letters 2024年第3期35卷 162-166页

作者： Chunying Wang Xiaofeng Liu Jingyi Wang Yaobin Li Shaohua Xie Fudong Liu Changbin Zhang Yuming Zheng Wenpo Shan Hong He Center for Excellence in Regional Atmospheric Environment Key Laboratory of Urban Pollutant ConversionInstitute of Urban EnvironmentChinese Academy of SciencesXiamen 361021China Zhejiang Key Laboratory of Urban Environmental Processes and Pollution Control Ningbo Urban Environment Observation and Research StationChinese Academy of SciencesNingbo 315800China Department of Civil Environmentaland Construction Engineering(CECE)Catalysis Cluster for Renewable Energy and Chemical Transformations(REACT)Nano Science Technology Center(NSTC)University of Central FloridaOrlandoFL 32816USA State Key Joint Laboratory of Environment Simulation and Pollution Control Research Center for Eco-environmental SciencesChinese Academy of SciencesBeijing 100085China

Pretreatment of the carrier for supported catalysts can effectively improve the strong metal-support interaction(SMSI)and increase the dispersion of precious metals,which are critical to many important catalytic *** this work,we tuned SMSI on Pd/TiO_(2)catalysts through inducing surface defects of TiO_(2)by pretreated with different atmospheres(H_(2)/N_(2),N_(2),O_(2)/N_(2))at the high temperature(800℃).Multiple characterization results illustrated that surface defects anchored Pd species and thus enhanced their *** reduction,Ti^(3+)species formed and transferred onto the metallic Pd species and then induced SMSI,which effectively stabilize Pd species in the metallic *** stronger MSI,the more stability of Pd *** a case,Pd/TiO_(2)–800H_(2),with strongest MSI,displayed the best HCHO oxidation performance at low temperature(10℃).

关键词： Pd/TiO_(2) Surface defects SMSI Formaldehyde Stability of Pd species

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