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第十九次中国暨国际生物物理大会

作者： Zhenzhen Min Lu Yu Ao Kun Liu Yueyong Xin Junjie Qi Fei Sun Changlin Tian Xiaoling Xu Hangzhou Normal University High Magnetic Field Laboratory Chinese Academy of Science Hefei National Laboratory of Physical Sciences at Microscale and School of Life Sciences University of Science and Technology of China National Laboratory of Biomacromolecules CAS Center for Excellence in BiomacromoleculesInstitute of BiophysicsChinese Academy of Sciences

Roseiflexus castenholzii is an anoxygenic photosynthetic bacterium that acquired a unique light harvesting,transformation and electron transport system during *** from higher plants and other photosynthetic bacteria,it doesn't contain the antenna complexes,the only light harvesting complex(LH) is assembled by several LHαβ subunits to form a ring like structure,having the L,M and cytochrome c subunits composed reaction center(RC) tightly bound in middle.

关键词： Molecular mechanisms of the electron transport chains in a photosynthetic bacteria Roseiflexus castenholzii

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Charging quantum batteries via Otto machines: Influence of monitoring

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physical Review A 2022年第5期106卷 052202-052202页

作者： Jeongrak Son Peter Talkner Juzar Thingna Center for Theoretical Physics of Complex Systems Institute for Basic Science (IBS) Daejeon 34126 Republic of Korea Department of Physics and Astronomy Seoul National University Seoul 08826 Republic of Korea School of Physical and Mathematical Sciences Nanyang Technological University 637371 Singapore Institut für Physik Universität Augsburg Universitätsstraße 1 D-86135 Augsburg Germany Basic Science Program Korea University of Science and Technology Daejeon 34113 Republic of Korea Department of Physics and Applied Physics University of Massachusetts Lowell Massachusetts 01854 USA

The charging of a quantum battery by a four-stroke quantum machine that works either as an engine or a refrigerator is investigated. The presented analysis provides the energetic behavior of the combined system in terms of the heat- and workflows of the machine, the average, the variance of the battery's energy, as well as the coherent and incoherent parts of its ergotropy. To monitor the battery state, its energy is measured either after the completion of any cycle or after a prescribed number of cycles is carried out. The resulting battery performances greatly differ for those two cases. During the first charging epoch with an engine, the regular measurements speed up the charging, whereas the gain of ergotropy is more pronounced in the absence of measurements. In a later stage, the engine fails to work as such, while it still continues charging the battery that eventually reaches the maximally charged state in the absence of intermediate measurements and a suboptimally charged state for a periodically measured battery. For a refrigerator, the charging of the measured battery also proceeds faster during the first epoch. Only during the second stage, when the machine fails to extract heat from the cold bath, the influence of the measurements becomes less pronounced, leading to rather similar asymptotic states for the two measurement scenarios.

关键词： Quantum thermodynamics Nonequilibrium systems Quantum heat engines & refrigerators Density matrix methods Master equation

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A class III ligand oscillates between internal and terminal binding modes as it engages with the Dishevelled PDZ domain

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Structure 2025年

作者： Jitender Kumar Miroslav Micka Jan Komárek Tomáš Klumpler Vojtěch Bystrý Remco Sprangers Cyril Bařinka Vítězslav Bryja Konstantinos Tripsianes CEITEC – Central European Institute of Technology Masaryk University Brno Czech Republic Department of Experimental Biology Faculty of Science Masaryk University Brno Czech Republic Institute of Biotechnology of the Czech Academy of Sciences Vestec Czech Republic Institute of Biophysics and Physical Biochemistry Regensburg Center for Biochemistry University of Regensburg Regensburg Germany

One of the largest domain-motif interactomes in human involves PSD-95/Discs-large/ZO-1 (PDZ) domains. The framework for understanding the PDZ interactome is well established; however the functional dynamics associated with PDZ-ligand interactions are poorly understood. Here, we report a dual PDZ-binding mode that ascribes unique dynamic features to class III ligand recognition. The crystal structure revealed that the PDZ domain can recognize either of the carboxylate moieties (terminal or internal) present in the class III ligand and laid out the register rules responsible for the dual recognition. Variants of the ligand designed to retain one or the other carboxylate of the native sequence were sufficient for PDZ binding. The conformational dynamics of PDZ probed by NMR relaxation dispersion experiments demonstrated that the class III ligand is shuffling binding modes as it engages with the PDZ domain. Our mechanistic findings reveal yet another aspect of PDZ binding plasticity specific to class III ligands.

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Room-temperature multiple ligands-tailored SnO_(2) quantum dots endow in situ dual-interface binding for upscaling efficient perovskite photovoltaics with high V_(OC)

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Light(science & Applications) 2021年第12期10卷 2467-2481页

作者： Zhiwei Ren Kuan Liu Hanlin Hu Xuyun Guo Yajun Gao Patrick W.K.Fong Qiong Liang Hua Tang Jiaming Huang Hengkai Zhang Minchao Qin Li Cui Hrisheekesh Thachoth Chandran Dong Shen Ming-Fai Lo Annie Ng Charles Surya Minhua Shao Chun-Sing Lee Xinhui Lu Frédéric Laquai Ye Zhu Gang Li Department of Electronic and Information Engineering Research Institute for Smart Energy(RISE)Guangdong-Hong Kong-Macao(GHM)Joint Laboratory for Photonic-Thermal-Electrical Energy Materials and DevicesThe Hong Kong Polytechnic UniversityHung HomKowloonHong KongChina Department of Electrical and Computer Engineering Nazarbayev UniversityNur-SultanKazakhstan The Hong Kong Polytechnic University Shenzhen Research Institute Shenzhen 518057China Hoffmann Institute of Advanced Materials Shenzhen Polytechnic7098 Liuxian BoulevardShenzhen 518055China Department of Applied Physics The Hong Kong Polytechnic UniversityHung HomKowloonHong KongChina Department of Chemical and Biological Engineering The Hong Kong University of Science and TechnologyClear Water BayKowloonHong KongChina King Abdullah University of Science and Technology(KAUST) KAUST Solar Center(KSC)Physical Sciences and Engineering Division(PSE)Material Science and Engineering Program(MSE)Thuwal 23955-6900Kingdom of Saudi Arabia Department of Physics The Chinese University of Hong KongShatin 999077 Hong KongChina Center of Super-Diamond and Advanced Films(COSDAF) Department of ChemistryCity University of Hong KongHong KongChina

The benchmark tin oxide(SnO_(2))electron transporting layers(ETLs)have enabled remarkable progress in planar perovskite solar cell(PSCs).However,the energy loss is still a challenge due to the lack of“hidden interface”*** report a novel ligand-tailored ultrafine SnO_(2) quantum dots(QDs)via a facile rapid room temperature ***,the ligand-tailored SnO_(2) QDs ETL with multi-functional terminal groups in situ refines the buried interfaces with both the perovskite and transparent electrode via enhanced interface binding and perovskite *** novel ETLs induce synergistic effects of physical and chemical interfacial modulation and preferred perovskite crystallization-directing,delivering reduced interface defects,suppressed non-radiative recombination and elongated charge carrier *** conversion efficiency(PCE)of 23.02%(0.04 cm^(2))and 21.6%(0.98 cm^(2),V_(OC) loss:0.336 V)have been achieved for the blade-coated PSCs(1.54 eV E_(g))with our new ETLs,representing a record for SnO_(2) based blade-coated ***,a substantially enhanced PCE(V_(OC))from 20.4%(1.15 V)to 22.8%(1.24 V,90 mV higher V_(OC),0.04 cm^(2) device)in the blade-coated 1.61 eV PSCs system,via replacing the benchmark commercial colloidal SnO_(2) with our new ETLs.

关键词： perovskite interface quantum

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Topological control of magnetic textures

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physical Review B 2021年第6期103卷 L060407-L060407页

作者： H. Arava F. Barrows M. D. Stiles A. K. Petford-Long Northwestern-Argonne Institute of Science and Engineering (NAISE) Northwestern University Evanston Illinois 60208 USA Materials Sciences Division (MSD) Argonne National Laboratory Argonne Illinois 60439 USA Applied Physics Program Northwestern University Evanston Illinois 60208 USA Physical Measurement Laboratory National Institute of Standards and Technology Gaithersburg Maryland 20899 USA

A micromagnetic study is carried out on the role of using topology to stabilize different magnetic textures, such as a vortex or an antivortex state, in a magnetic heterostructure consisting of a permalloy disk coupled to a set of nanomagnetic bars. The topological boundary condition is set by the stray field contributions of the nanomagnet bars and thus by their magnetization configuration, and can be described by a discretized winding number that will be matched by the winding number of the topological state set in the disk. The lowest number of nanomagnets that defines a suitable boundary is 4, and we identify a critical internanomagnet angle of 225 ° between two nanomagnets, at which the boundary fails because the winding number of the nanomagnet configuration no longer controls that of the disk magnetization. The boundary also fails when the disk-nanomagnets separation is >50 nm and for disk diameters >480 nm. Finally, we provide preliminary experimental evidence from magnetic force microscopy studies in which we demonstrate that an energetically unstable, antivortex-like structure can indeed be stabilized in a permalloy disk, provided that the appropriate topological conditions are set.

关键词： Domains Magnetic coupling Magnetic interactions Magnetic order Magnetic texture Ferromagnets Magnetic systems Nanostructures Atomic force microscopy Film deposition Landau-Lifschitz-Gilbert equation Lithography Magnetic force microscopy Micromagnetic modeling

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Effect of polyvinylidene fluoride concentration in PVDF-TiO₂-PVP composite membranes properties and its performance in bovine serum albumin rejection

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Case Studies in Chemical and Environmental Engineering 2024年 9卷

作者： Gayatri, Rianyza Fizal, Ahmad Noor Syimir Yuliwati, Erna Zailani, Muhamad Zulhilmi Jaafar, Juhana Hossain, Md Sohrab Zulkifli, Muzafar Taweepreda, Wirach Ahmad Yahaya, Ahmad Naim Polymer Science Program Division of Physical Science Faculty of Science Prince of Songkla University Hat-Yai Songkhla 90110 Thailand Universiti Kuala Lumpur Malaysian Institute of Chemical and Bioengineering Technology Alor Gajah Melaka 78000 Malaysia Centre for Sustainability of Ecosystem & Earth Resources (Pusat ALAM) Universiti Malaysia Pahang Lebuh Persiaran Tun Khalil Yaakob Pahang Gambang 26300 Malaysia Program Study of Chemical Engineering Faculty of Engineering Universitas Muhammadiyah Palembang Jalan A.Yani 13 Ulu Kota Palembang 30263 Indonesia Advanced Membrane Technology Research Centre (AMTEC) Faculty of Chemical and Energy Engineering Universiti Teknologi Malaysia Johor Skudai 81310 Malaysia HICoE-Centre for Biofuel and Biochemical Research Institute of Self-Sustainable Building Department of Fundamental and Applied Sciences Universiti Teknologi PETRONAS Perak Darul Ridzuan Seri Iskandar 32610 Malaysia Green Chemistry and Sustainability Cluster Universiti Kuala Lumpur Branch Campus Malaysian Institute of Chemical and BioEngineering Technology Alor Gajah Melaka 78000 Malaysia

In the present study, the polyvinylidene fluoride (PVDF) was incorporated with polyvinylpyrrolidone (PVP) and titanium dioxide (TiO2) nanoparticles to prepare PVDF-TiO2-PVP composite membrane for Bovine Serum Albumin ... 详细信息

In the present study, the polyvinylidene fluoride (PVDF) was incorporated with polyvinylpyrrolidone (PVP) and titanium dioxide (TiO₂) nanoparticles to prepare PVDF-TiO₂-PVP composite membrane for Bovine Serum Albumin (BSA) rejection from protein contaminated wastewater. The preparation of PVDF-TiO₂-PVP composite membrane was conducted by a non-solvent phase inversion (NIPS) process with varying PVDF weight percentages ranging from 16 to 19 wt%. The polymer concentration plays a critical role in the formation of composite membranes that is commonly overlooked. The primary goal of this study is to examine how the concentration of polymers affects the process of membrane creation, the ensuing structure, and the properties of these membranes. Presently, there is a restricted comprehension concerning the impact of PVDF polymer concentration in the fabrication of membranes using the NIPS approach, particularly for PVDF-TiO₂-PVP composite membranes. FE-SEM analysis revealed the lowest skin layer thickness and the number of macro-void formations in a PVDF composite membrane were at 16 wt% PVDF, compared to composite membranes over higher PVDF concentrations from 17 to 19 wt%. There were only slight variations in the percentages of individual elements across all PVDF-TiO₂-PVP membranes, yet the values were identical for C, O, F, and Ti. The viscosity was lowest at 16 wt percent PVDF (576.5 MPa s) and greatest at 19 wt percent PVDF (2054.3 MPa s). It showed that 19%wt PVDF viscosity increased fourfold higher than 16%wt. As the concentration of PVDF was increased, a related decrease in the surface porosity of the membrane was observed. The highest hydrophobicity with the contact angle of 79.62° of the composite membranes were detected at 19 wt% of PVDF loading. The maximum water flux (265.43 L/m²h) and BSA flux (250.31 L/m²h) were obtained at 19 wt% of PVDF loading. The lowest PVDF concentration of 16

关键词： Bovine serum albumin rejection Composite membrane Flat sheet Membrane separation Polymeric composite

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Strain-programmable van der Waals magnetic tunnel junctions

arXiv

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arXiv 2023年

作者： Cenker, John Ovchinnikov, Dmitry Yang, Harvey Chica, Daniel G. Zhu, Catherine Cai, Jiaqi Diederich, Geoffrey Liu, Zhaoyu Zhu, Xiaoyang Roy, Xavier Cao, Ting Daniels, Matthew W. Chu, Jiun-Haw Xiao, Di Xu, Xiaodong Department of Physics University of Washington SeattleWA98195 United States Department of Chemistry Columbia University New YorkNY10027 United States Intelligence Community Postdoctoral Research Fellowship Program University of Washington SeattleWA United States Department of Materials Science and Engineering University of Washington SeattleWA98195 United States Physical Measurement Laboratory National Institute of Standards and Technology GaithersburgMD20899 United States

The magnetic tunnel junction (MTJ) is a backbone device for spintronics. Realizing next generation energy efficient MTJs will require operating mechanisms beyond the standard means of applying magnetic fields or large electrical currents. Here, we demonstrate a new concept for programmable MTJ operation via strain control of the magnetic states of CrSBr, a layered antiferromagnetic semiconductor used as the tunnel barrier. Switching the CrSBr from antiferromagnetic to ferromagnetic order generates a giant tunneling magnetoresistance ratio without external magnetic field at temperatures up to ≈ 140 K. When the static strain is set near the phase transition, applying small strain pulses leads to active flipping of layer magnetization with controlled layer number and thus magnetoresistance states. Further, finely adjusting the static strain to a critical value turns on stochastic switching between metastable states, with a strain-tunable sigmoidal response curve akin to the stochastic binary neuron. Our results highlight the potential of strain-programmable van der Waals MTJs towards spintronic applications, such as magnetic memory, random number generation, and probabilistic and neuromorphic computing. Copyright © 2023, The Authors. All rights reserved.

关键词： Tunnel junctions

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Diamine Surface Passivation and Post-Annealing Enhance Performance of Silicon-Perovskite Tandem Solar Cells

arXiv

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arXiv 2024年

作者： Taddei, Margherita Contreras, Hannah Doan, Hai-Nam McCarthy, Declan P. Seo, Seongrok Westbrook, Robert J.E. Graham, Daniel J. Datta, Kunal Carroy, Perrine Muñoz, Delfina Correa-Baena, Juan-Pablo Barlow, Stephen Marder, Seth R. Smith, Joel A. Snaith, Henry J. Ginger, David S. Department of Chemistry University of Washington SeattleWA98195 United States Department of Physics University of Oxford OxfordOX1 3PU United Kingdom Institute of Materials Science Technical University of Munich München85748 Germany Department of Chemistry University of Colorado-Boulder BoulderCO80309 United States Department of Bioengineering University of Washington SeattleWA98195 United States School of Materials Science and Engineering Georgia Institute of Technology North Ave NW AtlantaGA30332 United States Université Grenoble Alpes CEA Liten Campus Ines Le Bourget du Lac73375 France Renewable and Sustainable Energy Institute University of Colorado-Boulder BoulderCO80309 United States Department of Chemical and Biological Engineering and Materials Science Program University of Colorado-Boulder BoulderCO80309 United States Physical Sciences Division Physical and Computational Sciences Directorate Pacific Northwest National Laboratory RichlandWA99352 United States

We show that the use of 1,3-diaminopropane (DAP) as a chemical modifier at the perovskite/electron-transport layer (ETL) interface enhances the power conversion efficiency (PCE) of 1.7 eV bandgap FACs mixed-halide perovskite single-junction cells, primarily by boosting the open-circuit voltage (VOC) from 1.06 V to 1.15 V. Adding a post-processing annealing step after C60 evaporation, further improves the fill factor (FF) by 20% from the control to the DAP + post-annealing devices. Using hyperspectral photoluminescence microscopy, we demonstrate that annealing helps improve compositional homogeneity at the top and bottom interfaces of the solar cell, which prevents detrimental bandgap pinning in the devices and improves C60 adhesion. Using time-of-flight secondary ion mass spectrometry, we show that DAP reacts with formamidinium present near the surface of the perovskite lattice to form a larger molecular cation, 1,4,5,6-tetrahydropyrimidinium (THP) that remains at the interface. Combining the use of DAP and the annealing of C60 interface, we fabricate Si-perovskite tandems with PCE of 25.29%, compared to 23.26% for control devices. Our study underscores the critical role of chemical reactivity and thermal post-processing of the C60/Lewis-base passivator interface in minimizing device losses and advancing solar-cell performance of wide-bandgap mixed-cation mixed-halide perovskite for tandem application. © 2024, CC BY.

关键词： Perovskite

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Comparison of volume transport in the Halmahera Sea between la Nina 2011 and El Nino 2015 events based on numerical model 2

Comparison of volume transport in the Halmahera Sea between ...

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2nd Maritime science and Advanced technology: Marine science and technology in Framework of The Sustainable Development Goals, MSAT 2019

作者： Riza, Muhammad Putri, Mutiara R. Mandang, Idris Department of Earth Science Faculty of Earth Science and Technology Bandung Institute of Technology Jalan Ganesha No 10 Bandung40132 Indonesia Hydro-Atmosphere Environment Research Group Physical Oceanography and Computational Modeling Laboratory Program Study of Physics Faculty of Mathematics and Natural Sciences Mulawarman University Jalan Barong Tongkok No 04 Samarinda75123 Indonesia

Variations of volume transport in the Halmahera Sea are strongly influenced by the El Nino Southern Oscillation (ENSO). Based on the Southern Oscillation Index (SOI), in 2011 La Nina event took place with a strength of 3.02, while in 2015 El Nino occurred with a strength of -2.6. This paper discusses the variation of transport volume caused by the ENSO phenomenon based on the results of the Regional Ocean Model System (ROMS). On the Halmahera Sea at a latitude of 0.3°S with a width of 67 km and a depth of down to 200 m, net volume transport always moves southward. The largest volume transport in La Nina 2011 occurred in September-October, which was -8.9 Sv. Meanwhile, in El Nino 2015 the largest volume transport occurred in July-August, which was equal to -4.9 Sv. The cross correlation coefficient between volume transport and SOI in 2011 and 2015 was r = 0.55 and r = 0.61 respectively, where these results indicate a strong relationship. © Published under licence by IOP Publishing Ltd.

关键词： Numerical models

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Numerical Modeling of Currents Circulation in Balikpapan Bay during Oil Spill Event on March 31, 2018 2

Numerical Modeling of Currents Circulation in Balikpapan Bay...

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2nd Maritime science and Advanced technology: Marine science and technology in Framework of The Sustainable Development Goals, MSAT 2019

作者： Nur, A.A. Radjawane, I.M. Suprijo, T. Mandang, I. Department of Earth Science Faculty of Earth Science and Technology Bandung Institute of Technology Jalan Ganesha No 10 Bandung40132 Indonesia Hydro-Atmosphere Environment Research Group Physical Oceanography and Computational Modeling Laboratory Program Study of Physics Faculty of Mathematics and Natural Sciences Mulawarman University Jalan Barong Tongkok No 04 Samarinda75123 Indonesia

The coastal area in Balikpapan Bay and its surrounding area has been devastated after the burst of an underwater oil pipe at the bay on March 31st, 2018, and the crude oil still continues spreading for a few days later. A three-dimensional hydrodynamic model is used to simulate the currents dynamic and investigate the influence of the current circulation on the spreading of the oil spill in Balikpapan Bay from March 31th to April 15th, 2018, to cover the event i.e. several weeks after the oil spill incident. Model results are validated by calculating the RMSE, MAPE and model skill using water level between available observation data at Semayang Port, Balikpapan station and numerical model from October 1st, 2012 to January 1st, 2013. Verification result of tidal elevation data from observation and model prediction shows a good agreement with RMSE = 7.8 cm, MAPE = 14.3% and model skill = 0.995. Surface currents circulation in Balikpapan Bay can be distinguished by the currents pattern on the spring tide and neap tide condition. During the spring tide condition, the surface currents mostly move to the east after coming out from the bay. However, the surface currents are strongly going southward after come out from the bay on the neap tide condition. Based on the satellite images captured for the next days after the event, the spreading pattern of the oil spill seems to be matched to the pattern of surface currents circulation on the spring tide condition. From the analysis of the model result, it shows that the currents circulation playing the main role to disperse the oil spill in Balikpapan Bay towards the Makassar Strait. © Published under licence by IOP Publishing Ltd.

关键词： Oil spills

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