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arXiv 2022年

作者： Huang, Jianwei Yu, Rong Xu, Zhijun Zhu, Jian-Xin Oh, Ji Seop Jiang, Qianni Wang, Meng Wu, Han Chen, Tong Denlinger, Jonathan D. Mo, Sung-Kwan Hashimoto, Makoto Michiardi, Matteo Pedersen, Tor M. Gorovikov, Sergey Zhdanovich, Sergey Damascelli, Andrea Gu, Genda Dai, Pengcheng Chu, Jiun-Haw Lu, Donghui Si, Qimiao Birgeneau, Robert J. Yi, Ming Department of Physics and Astronomy Rice Center for Quantum Materials Rice University HoustonTX77005 United States Department of Physics Renmin University of China Beijing100872 China NIST Center for Neutron Research National Institute of Standards and Technology GaithersburgMD20899 United States Department of Materials Science and Engineering University of Maryland College ParkMD20742 United States Department of Physics University of California Berkeley BerkeleyCA94720 United States Theoretical Division Los Alamos National Laboratory Los AlamosNM87545 United States Center for Integrated Nanotechnologies Los Alamos National Laboratory Los AlamosNM87545 United States Department of Physics University of Washington SeattleWA98195 United States School of Physics Sun Yat-Sen University Guangdong Guangzhou510275 China Advanced Light Source Lawrence Berkeley National Lab BerkeleyCA94720 United States Stanford Synchrotron Radiation Lightsource SLAC National Accelerator Laboratory Menlo ParkCA94025 United States Department of Physics & Astronomy University of British Columbia VancouverBCV6T 1Z1 Canada Quantum Matter Institute University of British Columbia VancouverBCV6T 1Z4 Canada Max Planck Institute for Chemical Physics of Solids Nöthnitzer Straße 40 Dresden01187 Germany Canadian Light Source Inc. 44 Innovation Boulevard SaskatoonSKS7N 2V3 Canada Condensed Matter Physics and Materials Science Department Brookhaven National Laboratory UptonNY11973 United States Materials Sciences Division Lawrence Berkeley National Laboratory BerkeleyCA94720 United States Department of Materials Science and Engineering University of California Berkeley BerkeleyCA94720 United States

Electronic correlation is of fundamental importance to high temperature superconductivity. While the low energy electronic states in cuprates are dominantly affected by correlation effects across the phase diagram, observation of correlation-driven changes in fermiology amongst the iron-based superconductors remains rare. Here we present experimental evidence for a correlation-driven reconstruction of the Fermi surface tuned independently by two orthogonal axes of temperature and Se/Te ratio in the iron chalcogenide family FeTe1−xSex. We demonstrate that this reconstruction is driven by the de-hybridization of a strongly renormalized dxy orbital with the remaining itinerant iron 3d orbitals in the emergence of an orbital-selective Mott phase. Our observations are further supported by our theoretical calculations to be salient spectroscopic signatures of such a non-thermal evolution from a strongly correlated metallic phase into an orbital-selective Mott phase in dxy as Se concentration is reduced. Copyright © 2022, The Authors. All rights reserved.

关键词： Copper compounds

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Ofatumumab and Granzyme B as immunotoxin against CD20 antigen

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In silico pharmacology 2022年第1期10卷 6页

作者： Fateme Sefid Armina Alagheband Bahrami Zahra Payandeh Saeed Khalili Ghasem Azamirad Seyed Mehdy Kalantar Maryam Touhidinia Department of Medical Genetics Shahid Sadoughi University of Medical Science Yazd Iran. Department of Biology Science and Art University Yazd Iran. Department of Biotechnology School of Advanced Technologies in Medicine Shahid Beheshti University of Medical Sciences Tehran Iran. Department Medical Biochemistry and Biophysics Division Medical Inflammation Research Karolinska Institute Stockholm Sweden. Department of Biology Sciences Shahid Rajaee Teacher Training University Tehran Iran. School of Mechanical Engineering Yazd University Yazd Iran. Reproductive & Genetic Unit Research and Clinical Center for Infertility Yazd Reproduction Sciences Institute Shahid Sadoughi University of Medical Sciences Yazd Iran. Department of Biology Faculty of Science Yazd University Yazd Iran.

Anti‐CD20 antibodies such as ofatumumab has demonstrated efficacy in relapsed/refractory chronic lymphocytic leukemia, are among the most successful therapies to date. In this study, we have designed an immunotoxin composed of Granzyme B and the high affinity variant of Ofatumumab. Different simulation software applied to explore the structure of Granzyme B, a serine protease in cytotoxic lymphocytes granules as an apoptosis mediator was attached to its specific antibody structure (Ofatumumab) via an adaptor sequence. The accuracy, energy minimization and characterization of biological properties of the final structure were evaluated. Our computational outcomes indicated that the employed method for structure prediction has been successfully managed to design the immunotoxin structure. The precise and accurate design of the immune-therapeutic agents against cancer cells can be confirmed by employment of in-silico approaches. Consequently, based on this approach we could introduce a capable immunotoxin which specifically targeting CD20 in an accurate orientation and initiates cancer cell destruction by its toxin domain.

关键词： Bioinformatics CD20 Granzyme B Immunotoxin Ofatumumab

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Reflections on the ERN ITHACA 2024 Patient Workshop in Bucharest

Rare

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Rare 2025年 3卷 100072-100072页

作者： Tanja Zdolšek Draksler Anne Hugon Dorica Dan ERN ITHACA-European Reference Network for Rare Malformation Syndromes and Rare Intellectual and Neurodevelopmental Disorders IDefine Europe Foundation for the Advanced Treatment of Rare Genetic Diseases Slovenia International Research Centre on Artificial Intelligence (IRCAI) under the Auspices of UNESCO Jožef Stefan Institute Ljubljana Slovenia Faculty of Electrical Engineering and Computer Science University of Maribor Maribor Slovenia European Reference Network for Rare Malformation Syndromes and Rare Intellectual and Neurodevelopmental Disorders Clinical Genetics Department Robert Debré University Hospital Paris France Romanian Prader Willi Association Romania Romanian National Alliance for Rare Diseases Romania NoRo Center Zalău Romania EURORDIS-Rare Diseases Europe Paris France

The ERN ITHACA (European reference network for rare malformation syndromes and rare intellectual and neurodevelopmental disorders) Patient Workshop 2024, held on December 12th in Bucharest, Romania, brought together over 70 participants (healthcare providers and patient advocates), to enhance support for individuals with rare genetic diseases. The workshop featured two key segments: Best Practice Sharing, highlighting innovative projects and success stories within the ERN ITHACA patient network, and The Patient Journey, which explored the emotional and psychological challenges faced by patients and families. Breakout discussions focused on building family resilience and addressing grief. Participant feedback was overwhelmingly positive, with a 4.68/5 satisfaction rating, and suggestions for improvement included more interactive exercises and extended workshop duration. The event underscored the importance of collaboration in advancing patient-centred care and will serve as a foundation for the next Patient workshop within ERN ITHACA in December 2025 in Bergen, Norway.

关键词： ERN ITHACA European reference network for rare malformation syndromes and rare intellectual and neurodevelopmental disorders Rare diseases Patient-centred Learning Training ERN ITHACA

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Excited-state lifetimes in In131, Sn131, and Te136 measured with the HiCARI γ-ray spectrometer at RIBF at RIKEN

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Physical Review C 2025年第6期111卷 064316-064316页

作者： J. Acosta A. Jungclaus M. Armstrong M. Górska T. Parry Zs. Podolyák P. Doornenbal K. Wimmer A. Gargano N. Aoi H. Baba F. Browne C. Campbell H. Crawford H. de Witte F. Flavigny C. Fransen H. Hess E. Ideguchi S. Iwazaki J. Kim A. Kohda T. Koiwai B. Mauss R. Mizuno B. Moon M. Niikura R. Orlandi L. Plagnol P. Reiter H. Sakurai D. Suzuki R. Taniuchi S. Thiel Y. Yamamoto Instituto de Estructura de la Materia CSIC E-28006 Madrid Spain GSI Helmholtzzentrum für Schwerionenforschung D-64291 Darmstadt Germany Department of Physics University of Surrey Guildford GU2 7XH United Kingdom RIKEN Nishina Center 2-1 Hirosawa Wako Saitama 351-0198 Japan Department of Physics University of Tokyo 7-3-1 Hongo Bunkyo Tokyo 113-0033 Japan Istituto Nazionale di Fisica Nucleare Complesso Universitario di Monte S. Angelo I-80126 Napoli Italy Research Center for Nuclear Physics (RCNP) Osaka University Mihogakoa Ibaraki Osaka 567-0047 Japan Nuclear Science Division Lawrence Berkeley National Laboratory Berkeley California 94720 USA Institute for Nuclear and Radiation Physics KU Leuven Leuven B-3001 Belgium LPC Caen ENSICAEN Université de Caen CNRS/IN2P3 F-14050 Caen France Institut für Kernphysik Universität zu Köln D-50937 Cologne Germany Department of Physics Korea University Seoul 02841 Republic of Korea Center for Exotic Nuclear Studies Institute for Basic Science Daejeon 34126 Republic of Korea Advanced Science Research Center Japan Atomic Energy Agency Tokai Ibaraki 319-1195 Japan School of Physics Engineering and Technology University of York Heslington York YO10 5DD United Kingdom

In the years 2020 to 2021, a high resolution in-beam γ-ray spectroscopy campaign took place at the Radio Isotope Beam Factory within the frame of the HiCARI project. An array composed of 12 composite Ge detectors of different types was put together by an international collaboration in order to address a variety of physics cases of interest, in many cases by measuring excited-state half-lives using Doppler-shift techniques. The analysis of the Doppler-shifted lineshapes observed for the 988-keV, 3/2−→1/2− and 1655-keV, 5/2+→3/2+ spin-flip M1 transitions in In131 and Sn131, respectively, the 332-keV, 1/2+→3/2+l-forbidden M1 transition in Sn131, as well as the 607-keV, 21+→01+ decay in Te136 allowed to characterize this new detector array and to establish a valid analysis procedure. The extracted half-lives are compared to previously reported results as well as theoretical calculations.

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Inside Back Cover: Atomically Local Electric Field Induced Interface Water Reorientation for Alkaline Hydrogen Evolution Reaction (Angew. Chem. Int. Ed. 26/2023)

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Angewandte Chemie International Edition 2023年第26期62卷

作者： Chao Cai Kang Liu Long Zhang Fangbiao Li Yao Tan Pengcheng Li Yanqiu Wang Maoyu Wang Zhenxing Feng Debora Motta Meira Wenqiang Qu Andrei Stefancu Wenzhang Li Hongmei Li Junwei Fu Hui Wang Dengsong Zhang Emiliano Cortés Min Liu Hunan Joint International Research Center for Carbon Dioxide Resource Utilization School of Physics and Electronics Central South University Changsha 410083 Hunan P. R. China School of Chemistry and Chemical Engineering Central South University Changsha 410083 Hunan P. R. China School of Chemical Biological and Environmental Engineering Oregon State University Corvallis OR 97331 USA X-ray Science Division Advanced Photon Source Argonne National Laboratory Argonne IL 60439 USA International Joint Laboratory of Catalytic Chemistry Department of Chemistry Research Center of Nanoscience and Technology College of Sciences Shanghai University Shanghai 200444 P. R. China Nanoinstitut München Fakultät für Physik Ludwig-Maximilians-Universität München 80539 München Germany

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Atomically Local Electric Field Induced Interface Water Reorientation for Alkaline Hydrogen Evolution Reaction

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Angewandte Chemie 2023年第26期135卷

The slow water dissociation process in alkaline electrolyte severely limits the kinetics of HER. The orientation of H 2 O is well known to affect the dissociation process, but H 2 O orientation is hard to control because of its random distribution. Herein, an atomically asymmetric local electric field was designed by IrRu dizygotic single-atom sites (IrRu DSACs) to tune the H 2 O adsorption configuration and orientation, thus optimizing its dissociation process. The electric field intensity of IrRu DSACs is over 4.00×10 10 N/C. The ab initio molecular dynamics simulations combined with in situ Raman spectroscopy analysis on the adsorption behavior of H 2 O show that the M−H bond length (M=active site) is shortened at the interface due to the strong local electric field gradient and the optimized water orientation promotes the dissociation process of interfacial water. This work provides a new way to explore the role of single atomic sites in alkaline hydrogen evolution reaction.

关键词： Alkaline HER Atomic Charge Distribution Interfacial Water Orientation Single-Atom Site Water Dissociation

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Ultrafast ferromagnetic fluctuations preceding magnetoelastic first-order transitions

arXiv

引用

arXiv 2020年

作者： Zhang, Zhao Chen, Yanna Yu, Dehong Mole, Richard Yu, Chenyang Zhang, Zhe Zhou, Houbo Yan, Xuexi Zhao, Xinguo Ren, Weijun Chen, Chunlin Owada, Shigeki Tono, Kensuke Sugahara, Michihiro Cao, Yue Sakata, Osami Bedzyk, Michael J. Li, Bing Hu, Fengxia Shen, Baogen Zhang, Zhidong Shenyang National Laboratory for Materials Science Institute of Metal Research Chinese Academy of Sciences 72 Wenhua Road Shenyang Liaoning110016 China School of Materials Science and Engineering University of Science and Technology of China 72 Wenhua Road Shenyang Liaoning110016 China Department of Materials Science and Engineering Northwestern University EvanstonIL60208 United States Synchrotron X-ray Group Research Center for Advanced Measurement and Characterization National Institute for Materials Science 1-1-1 Kouto Sayo-choHyogo679-5148 Japan Australian Nuclear Science and Technology Organisation Locked Bag 2001 Kirrawee DCNSW2232 Australia Beijing National Laboratory for Condensed Matter Physics State Key Laboratory of Magnetism Institute of Physics Chinese Academy of Sciences Beijing100190 China School of Physical Sciences University of Chinese Academy of Sciences Beijing100049 China Japan Synchrotron Radiation Research Institute 1-1-1 Kouto Sayo-cho Sayo-gunHyogo679-5198 Japan RIKEN SPring-8 Center 1-1-1 Kouto Sayo-cho Sayo-gunHyogo679-5198 Japan Materials Science Division Argonne National Laboratory LemontIL60439 United States

First-order magnetic transitions are of both fundamental and technological interest given that a number of emergent phases and functionalities are thereby created1-5. Of particular interest are giant magnetocaloric effects, which are attributed to first-order magnetic transitions and have attracted broad attention for solid-state refrigeration applications6. While the conventional wisdom is that atomic lattices play an important role in first-order magnetic transitions7,8, a coherent microscopic description of the lattice and spin degrees of freedom is still lacking. Here, we study the magnetic phase transition dynamics on the intermetallic LaFe13-xSix, which is one of the most classical giant magnetocaloric systems, in both frequency and time domains utilizing neutron scattering and ultrafast X-ray diffraction. We have observed a strong magnetic diffuse scattering in the paramagnetic state preceding the first-order magnetic transition, corresponding to picosecond ferromagnetic fluctuations. Upon photon-excitation, the ferromagnetic state is completely suppressed in 0.9 ps and recovered in 20 ps. The ultrafast dynamics suggest that the magnetic degree of freedom dominates this magnetoelastic transition and ferromagnetic fluctuations might be universally relevant for this kind of compounds. Copyright © 2020, The Authors. All rights reserved.

关键词： Neutron scattering

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Evidence-Based Health Informatics as the Foundation for the COVID-19 Response: A Joint Call for Action

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Methods of Information in Medicine 2021年第6期59卷 183-192页

作者： Luis Fernandez-Luque Andre W. Kushniruk Andrew Georgiou Arindam Basu Carolyn Petersen Charlene Ronquillo Chris Paton Christian Nøhr Craig E. Kuziemsky Dari Alhuwail Diane Skiba Elaine Huesing Elia Gabarron Elizabeth M. Borycki Farah Magrabi Kerstin Denecke Linda W. P. Peute Max Topaz Najeeb Al-Shorbaji Paulette Lacroix Romaric Marcilly Ronald Cornet Shashi B. Gogia Shinji Kobayashi Sriram Iyengar Thomas M. Deserno Tobias Mettler Vivian Vimarlund Xinxin Zhu Adhera Health Inc. Palo Alto California United States School of Health Information Science University of Victoria Victoria Canada Australian Institute of Health Innovation Macquarie University Macquarie New South Wales Australia School of Health Sciences University of Canterbury Christchurch New Zealand Division of Biomedical Statistics and Informatics Mayo Clinic Rochester Minnesota United States Daphne Cockwell School of Nursing Ryerson University Ryerson Toronto Canada Department of Information Science University of Otago Dunedin New Zealand Nuffield Department of Medicine University of Oxford Oxford United Kingdom Centre for Health Informatics and Technology Maersk McKinney Moller Institute University of Southern Denmark Denmark Office of Research Services MacEwan University Edmonton AB Canada Department of Information Science Kuwait University Kuwait Health Informatics Unit Dasman Diabetes Institute Kuwait University of Colorado Denver Colorado United States IMIA CEO Norwegian Centre for E-health Research University Hospital of North Norway Tromsø Norway Institute for Medical Informatics Bern University of Applied Sciences Bern Switzerland Medical Informatics Amsterdam UMC University of Amsterdam Amsterdam The Netherlands Columbia University Medical Center Data Science Institute Columbia University Columbia United States Amman Jordan University of Victoria Victoria Canada Univ. Lille Inserm CHU Lille ULR 2694 - METRICS: Évaluation des technologies de santé et des pratiques médicales F-59000 Lille France Society for Administration of Telemedicine and Healthcare Informatics New Delhi India National Institute of Public Health Japan The University of Arizona Arizona United States Peter L. Reichertz Institute for Medical Informatics of TU Braunschweig and Hannover Medical School Braunschweig Germany Swiss Graduate School of Public Administration University of Lausanne Lausanne Switzerland Department of Computer and Information Science (IDA)

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Broadband delay lines and nonreciprocal resonances in unidirectional waveguides

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Physical Review B 2019年第2期100卷 020303(R)-020303(R)页

作者： Sander A. Mann Dimitrios L. Sounas Andrea Alù Photonics Initiative Advanced Science Research Center City University of New York New York 10031 USA Department of Electrical and Computer Engineering The University of Texas at Austin Austin Texas 78712 USA Department of Electrical and Computer Engineering Wayne State University Detroit Michigan 48202 USA Physics Program Graduate Center City University of New York New York 10016 USA Department of Electrical Engineering City College of The City University of New York New York 10031 USA

Slow-light waveguides play an important role in optical pulse delay lines, but are practically limited by disorder-induced attenuation. Topological edge states, unidirectional and robust against disorder, have been proposed as a way to address this issue. Here, we study the transmission phase and pulse propagation dynamics through unidirectional systems in the presence of strong discontinuities. We first investigate a magnetically biased slow-light channel, demonstrating broadband pulse delays in small footprints. We uncover a nonreciprocal etalonlike resonance, sustained by propagating forward and evanescent backward modes, affecting pulse propagation and delay. We then show the existence of these features in topologically protected edge states, highlighting their universality. These exotic resonances provide a new degree of freedom in unidirectional waveguides to engineer their response, and they may therefore prove highly useful in various nanophotonic applications.

关键词： Plasmonics Topological effects in photonic systems Topological insulators Topological materials Waveguides Lorentz symmetry

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Measurement of the iron spectrum in cosmic rays from 10 GeV/n to 2.0 TeV/n with the calorimetric electron telescope on the international space station

arXiv

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arXiv 2021年

作者： Adriani, O. Akaike, Y. Asano, K. Asaoka, Y. Berti, E. Bigongiari, G. Binns, W.R. Bongi, M. Brogi, P. Bruno, A. Buckley, J.H. Cannady, N. Castellini, G. Checchia, Caterina Cherry, M.L. Collazuol, G. Ebisawa, K. Fuke, H. Gonzi, S. Guzik, T.G. Hams, T. Hibino, K. Ichimura, M. Ioka, K. Ishizaki, W. Israel, M.H. Kasahara, K. Kataoka, J. Kataoka, R. Katayose, Y. Kato, C. Kawanaka, N. Kawakubo, Y. Kobayashi, K. Kohri, K. Krawczynski, H.S. Krizmanic, J.F. Link, J. Maestro, P. Marrocchesi, P.S. Messineo, A.M. Mitchell, J.W. Miyake, S. Moiseev, A.A. Mori, M. Mori, N. Motz, H.M. Munakata, K. Nakahira, S. Nishimura, J. de Nolfo, G.A. Okuno, S. Ormes, J.F. Ospina, N. Ozawa, S. Pacini, L. Papini, P. Rauch, B.F. Ricciarini, S.B. Sakai, K. Sakamoto, T. Sasaki, M. Shimizu, Y. Shiomi, A. Spillantini, P. Stolzi, F. Sugita, S. Sulaj, A. Takita, M. Tamura, T. Terasawa, T. Torii, S. Tsunesada, Y. Uchihori, Y. Vannuccini, E. Wefel, J.P. Yamaoka, K. Yanagita, S. Yoshida, A. Yoshida, K. Department of Physics University of Florence Via Sansone 1 Sesto Fiorentino50019 Italy INFN Sezione di Florence Via Sansone 1 Sesto Fiorentino50019 Italy Waseda Research Institute for Science and Engineering Waseda University 17 Kikuicho Shinjuku Tokyo162-0044 Japan JEM Utilization Center Human Spaceflight Technology Directorate Japan Aerospace Exploration Agency 2-1-1 Sengen Ibaraki Tsukuba305-8505 Japan Institute for Cosmic Ray Research University of Tokyo 5-1-5 Kashiwa-no-Ha Chiba Kashiwa277-8582 Japan Department of Physical Sciences Earth and Environment University of Siena via Roma 56 Siena53100 Italy INFN Sezione di Pisa Polo Fibonacci Largo B. Pontecorvo Pisa3-56127 Italy Department of Physics McDonnell Center for the Space Sciences Washington University One Brookings Drive St. LouisMO63130-4899 United States Heliospheric Physics Laboratory NASA GSFC GreenbeltMD20771 United States Center for Space Sciences and Technology University of Maryland Baltimore County 1000 Hilltop Circle BaltimoreMD21250 United States Astroparticle Physics Laboratory NASA GSFC GreenbeltMD20771 United States Center for Research and Exploration in Space Sciences and Technology NASA GSFC GreenbeltMD20771 United States Via Madonna del Piano 10 Sesto Fiorentino50019 Italy Department of Physics and Astronomy Louisiana State University 202 Nicholson Hall Baton RougeLA70803 United States Department of Physics and Astronomy University of Padova Via Marzolo 8 Padova35131 Italy INFN Sezione di Padova Via Marzolo 8 Padova35131 Italy Institute of Space and Astronautical Science Japan Aerospace Exploration Agency 3-1-1 Yoshinodai Chuo Kanagawa Sagamihara252-5210 Japan Kanagawa University 3-27-1 Rokkakubashi Kanagawa Yokohama Kanagawa221-8686 Japan Faculty of Science and Technology Graduate School of Science and Technology Hirosaki University 3 Bunkyo Hirosaki Aomori036-8561 Japan Yukawa Institute for Theoretical Physics Kyoto

The Calorimetric Electron Telescope (CALET), in operation on the International Space Station since 2015, collected a large sample of cosmic-ray iron over a wide energy interval. In this Letter a measurement of the iron spectrum is presented in the range of kinetic energy per nucleon from 10 GeV/n to 2.0 TeV/n allowing the inclusion of iron in the list of elements studied with unprecedented precision by space-borne instruments. The measurement is based on observations carried out from January 2016 to May 2020. The CALET instrument can identify individual nuclear species via a measurement of their electric charge with a dynamic range extending far beyond iron (up to atomic number Z = 40). The energy is measured by a homogeneous calorimeter with a total equivalent thickness of 1.2 proton interaction lengths preceded by a thin (3 radiation lengths) imaging section providing tracking and energy sampling. The analysis of the data and the detailed assessment of systematic uncertainties are described and results are compared with the findings of previous experiments. The observed differential spectrum is consistent within the errors with previous experiments. In the region from 50 GeV/n to 2 TeV/n our present data are compatible with a single power law with spectral index −2.60 ± 0.03. Copyright © 2021, The Authors. All rights reserved.

关键词： Iron

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