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Highly Tunable Perpendicular Magnetic Anisotropy and Anisotropic Magnetoresistance in Ru-Doped La_(0.67)Sr_(0.33)MnO_(3)Epitaxial Films

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Chinese Physics Letters 2023年第7期40卷 74-79页

作者：华恩达戴坤杰王庆叶欢刘宽章金凤鲁京迪刘楷金锋王凌飞吴文彬 Hefei National Research Center for Physical Sciences at Microscale University of Science and Technology of ChinaHefei 230026China Collaborative Innovation Center of Advanced Microstructures Nanjing UniversityNanjing 210093China

As a prototypical half-metallic ferromagnet,La_(0.67)Sr_(0.33)MnO_(3)(LSMO)has been extensively studied due to its versatile physical properties and great potential in spintronic ***,the weak perpendicular magnetic anisotropy(PMA)limits the controllability and detection of magnetism in LSMO,thus hindering the realization of oxide-based spintronic devices with low energy consumption and high integration *** by this challenge,we develop an experimental approach to enhance the PMA of LSMO epitaxial *** cooperatively introducing 4d Ru doping and a moderate compressive strain,the maximum uniaxial magnetic anisotropy in Ru-doped LSMO can reach 3.0×10^(5)J/m^(3)at 10 ***,we find a significant anisotropic magnetoresistance effect in these Ru-doped LSMO films,which is dominated by the strong *** findings offer an effective pathway to harness and detect the orientations of magnetic moments in LSMO films,thus promoting the feasibility of oxide-based spintronic devices,such as spin valves and magnetic tunnel junctions.

关键词： anisotropy Highly realization

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Ultrasonic scalpel based on fusiform phononic crystal structure

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Chinese Physics B 2024年第10期33卷 302-310页

作者： Sha Wang Junjie Shan Shuyu Lin Ocean College Jiangsu University of Science and TechnologyZhenjiang 212100China Shaanxi Key Laboratory of Ultrasonics School of Physics and Information TechnologyShaanxi Normal UniversityXi’an 710119China National Laboratory of Solid State Microstructures School of PhysicsCollaborative Innovation Center of Advanced MicrostructuresNanjing UniversityNanjing 210093China

In response to the ultrasonic scalpels with the vibrational modal coupling which leads to a decrease in efficiency,an ultrasonic scalpel based on fusiform phononic crystals(PnCs)is *** accurate theoretical model is constructed,which is mainly composed of electromechanical equivalent circuit models to analyze the frequency response function and the frequency response curves of the *** band gaps exist in the fusiform PnCs owing to the periodic constraint,which can suppress the corresponding vibrational *** vibration characteristics(vibration mode,frequency,and displacement distribution)of the ultrasonic scalpel are analyzed,and the validity of the electromechanical equivalent circuit method is *** results indicate that other vibration modes near the working frequency can be *** addition,blades based on fusiform PnCs have a function akin to that of the horn,which enables displacement amplification.

关键词： phononic crystals ultrasonic scalpel bandgap vibration characteristics

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Enhanced Coupling of Superconductivity and Evolution of the Gap Structure in CsV_(3)Sb_(5)via Ta Doping

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Chinese Physics Letters 2024年第12期41卷 121-128页

作者： Yiwen Li Zhengyan Zhu Qing Li Yongze Ye Zhiwei Wang Yugui Yao Hai-Hu Wen National Laboratory of Solid State Microstructures and Department of Physics Collaborative Innovation Center of Advanced MicrostructuresNanjing UniversityNanjing 210093China Key Laboratory of Advanced Optoelectronic Quantum Architecture and Measurement Ministry of EducationSchool of PhysicsBeijing Institute of TechnologyBeijing 100081China Micronano Center Beijing Key Lab of Nanophotonics and Ultrafine Optoelectronic SystemsBeijing Institute of TechnologyBeijing 100081China Material Science Center Yangtze Delta Region Academy of Beijing Institute of TechnologyJiaxing 314011China

In this study,Kagome superconductors,i.e.,CsV_(3)Sb_(5)single crystals and its Ta-doped variant,Cs(V_(0.86)Ta_(0.14))_(3)Sb_(5),were studied in detail via specific heat *** revealed that the charge density wave(CDW)was suppressed and the superconducting transition temperature(Tc)considerably increased from 2.8 to 4.6K upon Ta *** electronic specific heat of CsV_(3)Sb_(5)was fitted with a model comprising an s-wave gap and a highly anisotropic extended s-wave gap,where 2Δ/kBTc was smaller than the weak coupling limit of ***(V_(0.86)Ta_(0.14))_(3)Sb_(5) exhibited two isotropic s-wave gaps and yielded a larger gap of 2Δ/kBTc=5.04,indicating a significant enhancement in superconducting *** evolution was attributed to the increased density of states near the Fermi level released by CDW gap *** findings demonstrated that Ta doping enhanced superconducting coupling and variation of gap structure in CsV_(3)Sb_(5).

关键词： doping coupling fitted

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Effects of carrier density and interactions on pairing symmetry in a t_(2g) model

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Chinese Physics B 2024年第1期33卷 223-230页

作者：李云霄西文翰董召阳姚子健于顺利李建新 National Laboratory of Solid State Microstructures and Department of Physics Nanjing UniversityNanjing 210093China Nanjing University of Science and Technology Nanjing 210094China Department of Physics Nanjing Normal UniversityNanjing 210023China Collaborative Innovation Center of Advanced Microstructures Nanjing UniversityNanjing 210093China

By utilizing the fluctuation exchange approximation method,we perform a study on the superconducting pairing symmetry in a t_(2g) three-orbital model on the square *** the tight-binding parameters of the model are based on Sr_(2)RuO_(4),we have systematically studied the evolution of superconducting pairing symmetry with the carrier density and interactions,making our findings relevant to a broader range of material *** a moderate Hund’s coupling,we find that spin fluctuations dominate the superconducting pairing,leading to a prevalent spin-singlet pairing with a d_(x^(2)-y^(2))-wave symmetry for the carrier density within the range of n=1.5-4 per *** reducing the Hund’s coupling,the charge fluctuations are enhanced and play a crucial role in determining the pairing symmetry,leading to a transition of the pairing symmetry from the spin-singlet d_(x^(2)-y^(2))-wave to the spin-triplet ***,we find that the superconducting pairings are orbital *** the carrier density changes from n=4 to n=1.5,the active orbitals for superconducting pairing shift from the quasi-two-dimensional orbital dxy to the quasi-one-dimensional orbitals d_(xz) and d_(yz).

关键词： unconventional superconductivity pairing mechanism Fermi surface three-orbital model

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2D materials for intelligent devices

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science China(Physics,Mechanics & Astronomy) 2023年第11期66卷 44-54页

作者： Xuan Pan Yixiang Li Bin Cheng Shi-Jun Liang Feng Miao Institute of Brain-Inspired Intelligence National Laboratory of Solid State MicrostructuresCollaborative Innovation Center of Advanced MicrostructuresSchool of PhysicsNanjing UniversityNanjing210093China Institute of Interdisciplinary Physical Sciences School of ScienceNanjing University of Science and TechnologyNanjing210094China

Neuromorphic intelligent hardware technologies have undergone rapid advancement during the past decade,with the goal of building intelligent devices and systems capable of overcoming challenges associated with conventional *** of neuromorphic intelligent hardware depends on major advances in materials science,condensed matter physics,device physics and *** a revolutionary discovery,two-dimensional(2D)materials with atomically-thin thickness and exceptionally high tunability introduce a new physical paradigm and show great promise in the development of intelligent ***,we give prominence to three categories of tunable properties(i.e.,charge carrier,band structure,lattice structure)that are inherent for 2D materials and review their superiorities in constructing intelligent devices particularly in electronics and ***,we provide insight into how the unique physical mechanisms emerging in 2D materials offer a fertile ground for the design of diverse intelligence devices.

关键词： tunability 2D materials intelligent devices

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In situ resource utilization of lunar soil for highly efficient extraterrestrial fuel and oxygen supply

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National science Review 2023年第2期10卷 224-231页

作者： Yuan Zhong Jingxiang Low Qing Zhu Yawen Jiang Xiwen Yu Xinyu Wang Fei Zhang Weiwei Shang Ran Long Yingfang Yao Wei Yao Jun Jiang Yi Luo Weihua Wang Jinlong Yang Zhigang Zou Yujie Xiong Hefei National Research Center for Physical Sciences at the Microscale School of Chemistry and Materials Science National Synchrotron Radiation Laboratory School of Information Science and TechnologyUniversity of Science and Technology of China Eco-Materials and Renewable Energy Research Center (ERERC) Jiangsu Key Laboratory for Nano Technology National Laboratory of Solid State MicrostructuresSchool of PhysicsCollaborative Innovation Center of Advanced MicrostructuresCollege of Engineering and Applied SciencesNanjing University Qian Xuesen Laboratory of Space Technology China Academy of Space Technology

Building up a lunar settlement is the ultimate aim of lunar ***, limited fuel and oxygen supplies restrict human survival on the ***,we demonstrate the in situ resource utilization of lunar soil for extraterrestrial fuel and oxygen production,which may power up our solely natural satellite and supply respiratory ***,the lunar soil is loaded with Cu species and employed for electro catalytic CO2conversion,demonstrating significant production of *** addition,the selected component in lunar soil（***3） loaded with Cu can reach a CH4F aradaic efficiency of 72.05% with a CH4production rate of 0.8 mL/min at 600 mA/***,an O2production rate of 2.3 mL/min can be ***,we demonstrate that our developed process starting from catalyst preparation to electrocatalytic CO2conversion is so accessible that it can be operated in an unmmaned manner via a robotic *** a highly efficient extraterrestrial fuel and oxygen production system is expected to push forward the development of mankind's civilization toward an extraterrestrial settlement.

关键词： Chang’E-5 lunar soil fuel production CO2 conversion extraterrestrial settlement in situ resource utilization

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Ultrasensitive Mechanical Sensor Using Tunable Ordered Array of Metallic and Insulating States in Vanadium Dioxide

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Chinese Physics Letters 2024年第7期41卷 74-86页

作者：马泽成闫胜楠陈繁强戴玉頔刘增霖徐康徐涛童湛钦陈墨雨王利铮王鹏飞孙立涛程斌梁世军缪峰 Institute of Brain-Inspired Intelligence National Laboratory of Solid State MicrostructuresSchool of PhysicsCollaborative Innovation Center of Advanced MicrostructuresNanjing UniversityNanjing 210093China SEU-FEI Nano-Pico Center Key Laboratory of MEMS of Ministry of EducationSoutheast UniversityNanjing 210096China Institute of Interdisciplinary of Physical Sciences School of ScienceNanjing University of Science and TechnologyNanjing 210094China

Detecting tiny deformations or vibrations, particularly those associated with strains below 1%, is essential in various technological applications. Traditional intrinsic materials, including metals and semiconductors, face challenges in simultaneously achieving initial metallic state and strain-induced insulating state, hindering the development of highly sensitive mechanical sensors. Here we report an ultrasensitive mechanical sensor based on a strain-induced tunable ordered array of metallic and insulating states in the single-crystal bronze-phase vanadium dioxide [VO_(2)(B)] quantum material. It is shown that the initial metallic state in the VO_(2)(B) flake can be tuned to the insulating state by applying a weak uniaxial tensile strain. Such a unique property gives rise to a record-high gauge factor of above 607970, surpassing previous values by an order of magnitude, with excellent linearity and mechanical resilience as well as durability. As a proof-of-concept application, we use our proposed mechanical sensor to demonstrate precise sensing of the micro piece, gentle airflows and water droplets. We attribute the superior performance of the sensor to the strain-induced continuous metal-insulator transition in the single-crystal VO_(2)(B) flake, evidenced by experimental and simulation results. Our findings highlight the potential of exploiting correlated quantum materials for next-generation ultrasensitive flexible mechanical sensors, addressing critical limitations in traditional materials.

关键词： metallic durability hinder

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Enhanced conductivity and weakened magnetism in Pb-doped Sr_(2)IrO_(4)

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Chinese Physics B 2024年第1期33卷 680-685页

作者：岳智来甄伟立牛瑞焦珂珂朱文卡皮雳张昌锦 High Magnetic Field Laboratory Hefei Institutes of Physical ScienceChinese Academy of SciencesHefei 230031China Science Island Branch of Graduate School University of Science and Technology of ChinaHefei 230026China Collaborative Innovation Center of Advanced Microstructures Nanjing UniversityNanjing 210093China

Group IV element Pb has been selected as the dopant to dope at the Sr site of Sr_(2)IrO_(4). It is exciting to find that the single-phase crystal structure could be maintained with a high Pb doping level of up to x=0.3 in Sr_(2-x)Pb_(x)IrO_(4). The mapping data obtained from energy-dispersive x-ray spectroscopy analyses give solid evidence that the Pb ions are uniformly distributed in the Sr_(2)IrO_(4) matrix. The incorporation of Pb leads to a moderate depression of the canted antiferromagnetic ordering state. The electrical conductivity could be greatly enhanced when the Pb doping content is higher than x=*** present results give a fresh material base to explore new physics in doped Sr_(2)IrO_(4) systems.

关键词： iridates doping conductivity magnetism

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Selective substitution induced anomalous phonon stiffening within quasi-one-dimensional P–P chains in SiP2

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Nano Research 2023年第1期16卷 1107-1114页

作者： Xueting Dai Feng Qin Caiyu Qiu Ling Zhou Junwei Huang Fanghua Cheng Xiangyu Bi Caorong Zhang Zeya Li Ming Tang Shengqiang Wu Xiaoxu Zhao Yangfan Lu Huiyang Gou Hongtao Yuan National Laboratory of Solid State Microstructures Jiangsu Key Laboratory of Artificial Functional MaterialsCollege of Engineering and Applied Sciencesand Collaborative Innovation Center of Advanced MicrostructuresNanjing UniversityNanjing 210000China School of Materials Science and Engineering Peking UniversityBeijing 100871China College of Materials Science and Engineering National Engineering Research Center for Magnesium AlloysChongqing UniversityChongqing 400030China Center for High Pressure Science and Technology Advanced Research Beijing 100094China

Light-matter interactions in low-dimensional quantum-confined structures can dominate the optical properties of the materials and lead to optoelectronic *** anisotropic layered silicon diphosphide(SiP2)crystal,the embedded quasi-onedimensional(1D)phosphorus–phosphorus(P–P)chains directly result in an unconventional quasi-1D excitonic state,and a special phonon mode vibrating along the P–P chains,establishing a unique 1D quantum-confined *** SiP2 with the homologous element serves as an effective way to study the properties of these excitons and phonons associated with the quasi-1D P–P chains,as well as the strong interaction between these ***,the experimental observation and the related optical spectral understanding of SiP2 with isoelectronic dopants remain ***,with the photoluminescence and Raman spectroscopy measurements,we demonstrate the redshift of the confined excitonic peak and the stiffening of the phonon vibration mode■of a series of Si(P1−xAsx)2 alloys with increasing arsenic(As)*** anomalous stiffening of■is attributed to the selective substitution of As atoms for P atoms within the P–P chains,which is confirmed via our scanning transmission electron microscopy *** optical spectra evolutions with selective substitution pave a new way to understand the 1D quantum confinement in semiconductors,offering opportunities to explore quasi-1D characteristics in SiP2 and the resulting photonic device application.

关键词： SiP2 quasi-one-dimensional structure Raman photoluminescence phosphide

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Highly crystalline and water-wettable benzobisthiazole-based covalent organic frameworks for enhanced photocatalytic hydrogen production

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National science Review 2023年第1期10卷 268-276页

作者： Wei Huang Yongpan Hu Zhengyuan Qin Yujin Ji Xuan Zhao Yunling Wu Qing He Youyong Li Chunfeng Zhang Jun Lu Yanguang Li Institute of Functional Nano and Soft Materials(FUNSOM) Soochow University Jiangsu Key Laboratory for Advanced Negative Carbon Technologies Soochow University National Laboratory of Solid State Microstructures School of Physics and Collaborative Innovation Center for Advanced MicrostructuresNanjing University Macao Institute of Materials Science and Engineering (MIMSE) MUST-SUDA Joint Research Center for Advanced Functional Materials Macau University of Science and Technology College of Chemical and Biological Engineering Zhejiang University

Two-dimensional covalent organic frameworks are promising for photocatalysis by virtue of their structural and functional diversity,but generally suffer from low activities relative to their inorganic *** fulfill their full potential re quires a rational tailoring of their structures at different scales as well as their surface ***,we demonstrate benzobisthiazole-based covalent organic frameworks as a superior photocatalyst for hydrogen *** product features high crystallinity with ordered 2.5-nm-wide cylindrical mesopores and great water *** structural advantages afford our polymeric photo catalyst with fast charge carrier dynamics as evidenced by a range of spectroscopic characterizations and excellent catalytic performances when suspended in solution or supported on melamine *** visible-light irradiation,it enables efficient and stable hydrogen evolution with a production rate of 487 μmol h-1(or a mass-specific rate of 48.7 mmol g-1h-1)—far superior to the previous state of the *** also demonstrate that hydrogen production can be stoichiometrically coupled with the oxidation conversion of biomass as exemplified by the conversion of furfuryl alcohol to 2-furaldehyde.

关键词： covalent organic frameworks photocatalysis hydrogen evolution benzobisthiazole water-wettable

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