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Lifetime-tunable circularly polarized luminescent system based on triplet-to-singlet Förster resonance energy transfer

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science China Chemistry 2024年第9期67卷 2918-2922页

作者： Zhenyi He Zizhao Huang Xiang Ma Key Laboratory for Advanced Materials and Feringa Nobel Prize Scientist Joint Research Center Institute of Fine ChemicalsSchool of Chemistry and Molecular EngineeringEast China University of Science and TechnologyShanghai 200237China

Circularly polarized luminescence(CPL)materials have received widespread attention due to their remarkable performance and broad ***,current CPL material research primarily focuses on tunable color,intensity,and *** CPL with adjustable lifetime remains a significant ***,a series of CPL polymeric materials with tunable lifetime were obtained by employing phosphorescent terephthalic acid and chiral organic small molecule R/S-BNAF(a luminescent binaphthol derivative)to copolymerize with acrylamide in different *** was verified that this performance results from the different energy transfer efficiency between luminophores with varying ratios of the monomers for *** strategy to realize CPL with tunable lifetime by modulating the energy transfer efficiency will provide a new perspective to broaden the applications of CPL materials.

关键词： circularly polarized luminescence tunable lifetime Förster resonance energy transfer room temperature phosphorescence

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Scalable graphene foam with ultrahigh conductivity for stabilizing Pt towards efficient hydrogen evolution

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Nano research 2024年第8期17卷 6968-6976页

作者： Ming Zhao Meng Huang Huihui Jin Dayin He Wei Qian Zixin Zhang Daping He State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China Hubei Engineering Research Center of RF-Microwave Technology and Application Wuhan University of TechnologyWuhan 430070China School of Information Engineering Wuhan University of TechnologyWuhan 430070China School of Chemistry and Materials Science University of Science and Technology of ChinaHefei 230026China Sanya Science and Education Innovation Park of Wuhan University of Technology Sanya 572000China

For the carbon-based catalyst to be active and stable,especially in harsh electrochemical environments,the key is to decrease the concentration of defects and raise the degree of graphitization of the carbon ***,we develop a highly graphitized graphene foam with multiplicated structure to fabricate self-supporting Pt-based catalysts for efficient and stable hydrogen evolution reaction(HER)*** foam(GO-2850)is obtained through an ultra-high temperature treatment at 2850℃,with perfect graphene structure and extremely low defect,ensuring high electrical conductivity and corrosion ***,its multiplicated structure provides an inherently favorable environment for the dispersion of Pt nanoparticles(Pt NPs)and offers abundant channels for electrolyte infiltration during the catalytic *** a result,the as-prepared Pt/GO-2850 is far active and stable than the Pt NPs supported on commercial carbon paper(Pt/CP)counterpart toward catalyzing HER,exhibiting an outstanding activity and long-term durability(300 h@10 mA·cm^(−2))in acidic/alkaline/seawater *** can be attributed to the stronger interaction between the lower-defect GO-2850 substrate and Pt,as evidenced by characterization and theoretical *** work extends further insight into the design self-supporting catalysts of high activity and stability with promising prominent application toward green energy devices.

关键词： graphene foam high graphitization Pt nanoparticles hydrogen evolution reaction long-term stability

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Acid-stable antimonate based catalysts for the electrocatalytic oxygen evolution reaction

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Nano research 2023年第4期16卷 4691-4697页

作者： Xiaoping Gao Huang Zhou Zhe Wang Gang Zhou Jin Wang Yuen Wu College of Materials Science and Engineering Shenzhen UniversityShenzhen 518071China School of Chemistry and Materials Science University of Science and Technology of ChinaHefei 230026China Preservation Technology Advanced Research CenterHefei Hualing Co.LtdHefei 230000China School of Science Hubei University of TechnologyWuhan 430068China

Acid-stable and highly active catalysts for the electrocatalytic oxygen evolution reaction(OER)are paramount to the advancement of electrochemical technologies for clean energy conversion and *** this work,based on the density functional theory(DFT)calculations,we systematically investigated the MSb_(2)O_(6)(M=Fe,Co,and Ni)and transition metal(TM)doped MSb_(2)O_(6)(TM-MSb_(2)O_(6),TM=Mn,Fe,Co,Ni,Cu,Zn,Ru,Rh,Pd,Ir,and Pt)as potential antimonate-based electrocatalysts for the *** stability and OER activity of these considered electrocatalysts were systematically studied under acidic *** was found that Rh-NiSb_(2)O_(6),Pt-CoSb_(2)O_(6),Rh-FeSbO4,and Co-NiSb_(2)O_(6)can serve as efficient and stable OER electrocatalysts,and their OER catalytic activities are better than that of the current state-of-the-art OER catalyst(IrO2).Our findings highlight a family of promising antimonate-based OER electrocatalysts for future experimental verification.

关键词： oxygen evolution reaction antimonates acid-stable oxides electrocatalysis density functional theory

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Controlling molecular assembly on time scale:Time-dependent multicolor fluorescence for information encryption

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Chinese Chemical Letters 2024年第7期35卷 336-340页

作者： Zixi Zou Jingyuan Wang Yian Sun Qian Wang Da-Hui Qu Key Laboratory for Advanced Materials and Feringa Nobel Prize Scientist Joint Research Center School of Chemistry and Molecular EngineeringEast China University of Science and TechnologyShanghai 200237China

Dynamic assembly on time scale is common in biological systems but rare for artificial materials,especially for smart luminescent *** molecular assembly in a spatio-temporal manner and resulting in white-light-including multicolor fluorescence with time-dynamic features remains ***,controlling molecular assembly on time scale is achieved by integrating a pH-responsive motif to a transient alkaline solution which is fabricated by activators(NaOH)and deactivators(esters),leading to automatic assembly on time scale and time-dependent multicolor fluorescence changing from blue to white and *** kinetics of the assembly process is dependent on the ester hydrolysis process,which can be controlled by varying ester concentrations,temperature,initial pH,stirring rate and ester *** dynamic fluorescent system can be further developed for intelligent fluorescent materials such as fluorescent ink,three-dimension(3D)codes and even four-dimension(4D)codes,exhibiting a promising potential for information encryption.

关键词： Supramolecular chemistry Multicolor fluorescence White light emission Time-dependent fluorescence Information encryption

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Controlled vapour growth and phase engineering of large-area bilayer WSe2 for optoelectronic applications

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Progress in Natural science:Materials International 2023年第6期33卷 947-953页

作者： Zhikang Ao Xiangdong Yang Xiang Lan Fen Zhang Yang Du Le Gao Xuyang Zhang Baihui Zhang Shunhui Zhang Tian Zhang Yinghao Chen Jianing Xie Wenkui Wen Chenyang Zha Huifang Ma Zhengwei Zhang College of Physics and Electronics Central South University School of Flexible Electronics(Future Technologies) & Institute of Advanced Materials(IAM) Jiangsu National Synergetic Innovation Center for Advanced MaterialsNanjing Tech University Institute of Micro/Nano Materials and Devices Ningbo University of Technology College of Materials Science and Engineering Hunan University College of Energy and Power Engineering Changsha University of Science and Technology Institute of Applied Physics and Materials Engineering(IAPME) Zhuhai UM Science & Technology Research Institute(ZUMRI) University of Macau

The engineering of stacking order plays an important role in regulations of electronic and optical properties of layered van der Waals ***,we demonstrate a developed physical vapour deposition approach to grow WSe2 atomic layers with controllable 3R and 2H *** 3R WSe2bilayer tends to form at a lower deposition temperature（830℃）,and the 2H WSe2bilayer prefers to grow at a higher deposition temperature（930℃）.Efficient phase engineering was demonstrated by simply controlling the deposition ***,by photoluminescence,Raman,selected area electron diffraction and so on,it was determined that the AA'-stacking corresponds to the 2H phase,and the AB-stacking corresponds to the 3R ***,different layer stacking and interlayer coupling result in differences in the optical and optoelectronic properties of the two *** responsivity of 3R bilayer WSe2is ～195 times higher than 2H phase exhibiting dramatically improved photoelectric detection performance by phase engineering(R3R=2.54 A/W vs R2H=0.013 A/W at 780 nm,82.7 mW cm-2).Hence,the findings of this study not only contribute to the controllable synthesis of two-dimensional materials with diverse stacking phases but also hold promise for advancing the design and fabrication of future optoelectronic devices.

关键词： Transition metal dichalcogenides Phase engineering WSe2 3R stacking Optoelectronics

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Recent advances in photopolymerization 3D printing of alumina-ceramic

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Progress in Natural science:Materials International 2025年第1期35卷 1-30页

作者： M.Irfan Hussain Min Xia XiaoNa Ren Zhen Shen Muhammad Jamil Changchun Ge Institute of Powder Metallurgy and Advanced Ceramics School of Material Science and Engineering University of Science and Technology Beijing State Key Laboratory of Multimodal Artificial Intelligence Systems Beijing Engineering Research Center of Intelligent Systems and Technology Institute of AutomationChinese Academy of Sciences College of Mechanical and Electrical Engineering Nanjing University of Aeronautics and Astronautics

Digital light processing(DLP) 3D printing has a huge potential for manufacturing intricate and customized ceramic parts with high precision and cost-effectiveness. research in this field contributes to material innovation,opening the avenues for new process designs in both scientific and industrial sectors. However, the implementation of DLP 3D printing technology in ceramic research has not yet reached the maturity level as that in polymer and tissue engineering. Necessarily, a holistic in-depth literature reporting the successful integration of alumina ceramics within DLP 3D printing technology is urgently needed. This review, systematic examines recent progress in DLP technology, focusing on photopolymer resins that incorporate UV-sensitive monomers, photoinitiators, and dispersants, as well as their synergistic effects on achieving high-quality printing, desirable material properties, and enhanced performance. Further, the review discusses key factors including post-processing characteristics such as debinding and sintering, which influence microstructure, and defect formation including microcracks, porosity and voids. Finally, the challenges associated with printing and sintering are highlighted,aiming to identify focused focused development pathways and potential solution to optimize outcomes. This analysis clarifies existing challenges and also propsoes future applications for DLP technology in the aluminaceramic field.

关键词： Al2O3 ceramics Applications Digital light processing (DLP) Post-processing Resin

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Phase-coherence dynamics of frequency-comb emission via high-order harmonic generation in few-cycle pulse trains

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Chinese Physics B 2023年第3期32卷 205-211页

作者：梁畅通张晶晶李鹏程 Research Center for Advanced Optics and Photoelectronics Department of PhysicsCollege of ScienceShantou UniversityShantou 515063China Key Laboratory of Intelligent Manufacturing Technology of the Ministry of Education Shantou UniversityShantou 515063China Institute of Applied Physics and Computational Mathematics Beijing 100088China

Frequency-comb emission via high-order harmonic generation(HHG)provides an alternative method for the coherent vacuum ultraviolet(VUV)and extreme ultraviolet(XUV)radiation at ultrahigh repetition *** particular,the temporal and spectral features of the HHG were shown to carry profound insight into frequency-comb emission *** we present an ab initio investigation of the temporal and spectral coherence of the frequency comb emitted in HHG of He atom driven by few-cycle pulse *** find that the emission of frequency combs features a destructive and constructive coherences caused by the phase interference of HHG,leading to suppression and enhancement of frequency-comb *** results reveal intriguing and substantially different nonlinear optical response behaviors for frequency-comb emission via *** dynamical origin of frequency-comb emission is clarified by analyzing the phase coherence in HHG processes in *** results provide fresh insight into the experimental realization of selective enhancement of frequency comb in the VUV–XUV regimes.

关键词： high-order harmonic generation frequency comb time-dependent Schro¨dinger equation intense laser field systems

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Phase Equilibria of the Binary Ag-In System

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Journal of Phase Equilibria and Diffusion 2024年第4期45卷 790-803页

作者： Chang, Chih-Chia Bill Kao, C.R. Department of Materials Science and Engineering National Taiwan University Taipei Taiwan Advanced Research Center for Green Materials Science & amp Technology National Taiwan University Taipei Taiwan

In this work, the phase equilibria of the binary Ag-In system were determined using electron probe microanalysis and differential scanning calorimetry on equilibrated alloys and diffusion couples. The compositions of the phase boundaries of solid phases that are highly scattered in the literature have been precisely determined. The temperatures of the invariant reaction ζ γ + L and the polymorphic transformation ζ γ are substantially lower than previously reported values. In addition, it was found that the In-rich ζ phase phase-separates after months of room-temperature aging. © ASM International 2024.

关键词： Differential scanning calorimetry

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Single-Valued Neutrosophic Graph with Heptapartitioend Structure

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Neutrosophic Sets and Systems 2025年 80卷 728-748页

作者： Fathi, Hanaa Myvizhi, M. Abdelhafeez, Ahmed Abdellah, Mohamed Refaat Eassa, Mohamed Sawah, Mohamed S. Elbehiery, Hussam College of Information Technology Amman Arab University Amman Jordan KPR Institute of Engineering and Technology Tamilnadu Coimbatore India Computer Science Department Faculty of Information System and Computer Science October 6 University Giza12585 Egypt Applied Science Research Center Applied Science Private University Amman Jordan The Department of Computer Science College of Information Technology Misr University for Science and Technology Cairo Egypt Department of Computer Science Faculty of Information Technology Ajloun National University P.O.43 Ajloun26810 Jordan

This study applies single-valued neutrosophic sets, which extend the frameworks of fuzzy and intuitionistic fuzzy sets, to graph theory. We introduce a new category of graphs called Single-Valued Heptapartitioned Neutrosophic Graphs (SVHNG) and investigate their characteristics through comprehensive proofs and illustrative examples. © 2025, University of New Mexico. All rights reserved.

关键词： Heptapartitioend Neutrosophic Set Neutrosophic Graph Neutrosophic Sets SVHN-Graph

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Enhanced MADM Strategy with Heptapartitioned Neutrosophic Distance Metrics

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Neutrosophic Sets and Systems 2025年 78卷 74-96页

作者： Eassa, Mohamed Myvizhi, M. Elkholy, Mohamed Abdelhafeez, Ahmed Elbehiery, Hussam Computer Science Department Faculty of Information System and Computer Science October 6 University Giza12585 Egypt Applied Science Research Center Applied Science Private University Amman Jordan Department of Mathematics KPR Institute of Engineering and Technology Tamilnadu Coimbatore India Faculty of Computer Science& Engineering Alamein International University Egypt

In this work, a novel methodological approach to multi-attribute decision-making problems is developed and the notion of Heptapartitioned Neutrosophic Set Distance Measures (HNSDM) is introduced. By averaging the Penta-Partitioned Neutrosophic Distance Measures under particular conditional criteria, the suggested technique ranks the options. Additionally, we explore the fundamental characteristics of HNSDM and provide several illustrative theorems. The Heptapartitioned Neutrosophic Set Distance Measures are formulated based on the Hepta Neutrosophic Set. Lastly, a practical numerical example is provided to illustrate the efficacy of the suggested methodology. © 2025, University of New Mexico. All rights reserved.

关键词： Heptapartitioned Neutrosophic set Heptapartitioned Neutrosophic set and MADM strategy Heptapartitioned set Neutrosophic sine distance measure

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