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Effect of electrolyte anions on the cycle life of a polymer electrode in aqueous batteries

escience 2022年第1期2卷 110-115页

作者： Ye Zhang Lihong Zhao Yanliang Liang Xiaojun Wang Yan Yao Department of Electrical and Computer Engineering Materials Science and Engineering ProgramUniversity of HoustonHoustonTX77204USA Texas Center for Superconductivity at the University of Houston HoustonTX77204USA

Redox polymers are a class of high-capacity, low-cost electrode materials for electrochemical energy storage, butthe mechanisms governing their cycling stability are not well understood. Here we investigate the effect of anionson the longevity of a p-dopable polymer through comparing two aqueous zinc-based electrolytes. Galvanostaticcycling studies reveal the polymer has better capacity retention in the presence of triflate anions than that withsulfate anions. Based on electrode microstructural analysis and evolution profiles of the cell stacking pressure, theorigin of capacity decay is ascribed to mechanical fractures induced by volume change of the polymer activematerials during repeated cycling. The volume change of the polymer with the triflate anion is 61% less than thatwith the sulfate anion, resulting in fewer cracks in the electrodes. The difference is related to the different anionsolvation structures—the triflate anion has fewer solvated water molecules compared with the sulfate anion,leading to smaller volume expansion. This work highlights that anions with low solvation degree are preferablefor long-term cycling.

关键词： Aqueous batteries Polymer electrode Anions Volume chang

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Promoting effect of d-band center and in-situ precipitation strategy on sulfur evolution reaction

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Journal of Energy Chemistry 2025年第5期104卷 740-748页

作者： Jun Pu Yun Tan Jiasen Yin Zihan Shen Shoujie Liu Kai Zhang Lei Zhou Yagang Yao Key Laboratory of Functional Molecular Solids Ministry of Education Anhui Provincial Engineering Laboratory for New-Energy Vehicle Battery Energy-Storage Materials College of Chemistry and Materials Science Anhui Normal University National Laboratory of Solid State Microstructures College of Engineering and Applied Sciences Jiangsu Key Laboratory of Artificial Functional Materials Collaborative Innovation Center of Advanced Microstructures Nanjing University State Key Laboratory of Multiphase Complex Systems Institute of Process Engineering Chinese Academy of Sciences School of Materials Science and Engineering Anhui University School of Energy and Power Engineering Jiangsu University Department of Electrical Engineering Eindhoven University of Technology

The slow conversion of polyphase in lithium-sulfur （Li-S） batteries not only intensifies the shuttle effect of lithium polysulfides （LiPSs）,but also causes the continuous accumulation of inactive sulfur species,resulting in rapid capacity attenuation and sluggish dynamic ***,the promoting effect of atomic interface stress on sulfur reaction was investigated via CoFe-CoFe2O4heterogeneous nanosheets with a cavity *** strain force induced by the in-situ precipitation of Co Fe bimetallic alloy in oxide matrix increased the d-band center,which was conducive to the interaction between catalyst and Li *** sulfur cathode based on this two-dimensional （2D） nanosheet design showed an extremely high capacity of 751 mAh g-1at 4 *** with a sulfur loading of 5.55 mg cm-2,its area capacity was still as high as 7.15 mAh ***,the enhanced stability greatly improved the practical potential of Li-S batteries.

关键词： 2D nanosheets D-band center In-situ precipitation Li-S batteries Strain effect

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Identification and Monitoring Strategies for Multiphase Batch Processes based on Dissimilarity Analysis 43

Identification and Monitoring Strategies for Multiphase Batc...

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43rd Chinese Control Conference, CCC 2024

作者： Guo, Qingxiu Liu, Jianchang Tan, Shubin Wang, Honghai Zhang, Xinnan Zhang, Lijie Northeastern University The College of Information Science and Engineering Shenyang110819 China Northeastern University The National Frontiers Science Center for Industrial Intelligence and Systems Optimization Shenyang110819 China Ningxia Institute of Science and Technology The College of Electrical Information Engineering Ningxia753000 China

ISBN: (纸本)9789887581581

Batch processes often have multiphase characteristics, and the dynamic transition between phases cannot be ignored. Therefore, this paper proposes identification and monitoring strategies for multiphase batch processes based on dissimilarity analysis(DAIM). In the identification section, dissimilarity analysis is introduced, which can divide the transitions between different phases from the perspective of similarity. The average difference vector is proposed in the monitoring section. It could be used to evaluate the test sample deviation and provide new statistics to monitor the state of the test samples, which improves the fault detection rate. The method proposed in this paper was applied to the benchmark penicillin fermentation process, and the experimental results verified the effectiveness of the DAIM. © 2024 Technical Committee on Control Theory, Chinese Association of Automation.

关键词： Batch data processing

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Coupling Mobile Brain Imaging and Virtual Reality Omnidirectional Treadmill to Explore Attenuated Situational Awareness during Distracted Walking

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IEEE Transactions on Cognitive and Developmental systems 2024年第3期16卷 1063-1076页

作者： Chuang, Chun-Hsiang Chiu, Tsai-Feng Hsu, Hao-Che Lin, Shih-Syun National Tsing Hua University Research Center for Education and Mind Sciences College of Education The Institute of Information Systems and Applications College of Electrical Engineering and Computer Science Hsinchu300 Taiwan National Tsing Hua University Research Center for Education and Mind Sciences Hsinchu300 Taiwan National Yang Ming Chiao Tung University Department of Computer Science Hsinchu300193 Taiwan National Taiwan Ocean University Department of Computer Science and Engineering Keelung20224 Taiwan

Walking while engaging in distracting activities affects our perception of changes happening on the road, leading to exposure to hazardous conditions. This study aimed to evidence that pedestrians who become distracted when absorbed in their smartphones fail to maintain situational awareness. Thirty-six recruited participants performed a psychomotor vigilance task and a wayfinding task designed to simulate a multitasking scenario;meanwhile, an auditory oddball paradigm presented to participants tested their situational awareness of an external stimulus. The experiment was conducted in virtual reality (VR) environment with an omnidirectional treadmill. Participant's behavioral and electroencephalographic (EEG) responses were measured and analyzed using a newly proposed brain network measure, phase locking distance (PLD), to capture multitasking-associated couplings between brain regions. The current study supports the notion that multitasking can lead to diminished behavioral performance and changes in walking patterns. Despite the increased interregional brain connectivity, which may be an adaptive response to heightened cognitive demands, the associated reduction in event-related EEG activity suggests competition for neural resources during multitasking. Moreover, the observed EEG activities could indicate additional information processing capacity limitations and provide evidence of decreased situational awareness during multitasking, thereby increasing susceptibility to potentially hazardous situations. © 2016 IEEE.

关键词： Electroencephalography

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A flexible capacitive photoreceptor for the biomimetic retina

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Light(science & Applications) 2022年第1期11卷 38-49页

作者： Mani Teja Vijjapu Mohammed E.Fouda Agamyrat Agambayev Chun Hong Kang Chun-Ho Lin Boon S.Ooi Jr-Hau He Ahmed M.Eltawil Khaled N.Salama Sensors lab Advanced Membranes and Porous Materials CenterComputerElectrical and Mathematical Science and Engineering DivisionKing Abdullah University of Science and Technology(KAUST)Thuwal 23955-6900Kingdom of Saudi Arabia Communication and Computing Systems Lab ComputerElectrical and Mathematical Science and Engineering DivisionKing Abdullah University of Science and Technology(KAUST)Thuwal 23955-6900Kingdom of Saudi Arabia Department of Electrical Engineering and Computer Science University of California-IrvineIrvineCA 92612USA Department of Electrical Computer and Energy EngineeringArizona State UniversityTempeAZUSA Computer Electrical and Mathematical Science and Engineering DivisionKing Abdullah University of Science and Technology(KAUST)Thuwal 23955-6900Kingdom of Saudi Arabia Department of Materials Science and Engineering City University of Hong KongHong Kong SARChina

Neuromorphic vision sensors have been extremely beneficial in developing energy-efficient intelligent systems for robotics and privacy-preserving security *** is a dire need for devices to mimic the retina's photoreceptors that encode the light illumination into a sequence of spikes to develop such ***,we develop a hybrid perovskite-based flexible photoreceptor whose capacitance changes proportionally to the light intensity mimicking the retina's rod cells,paving the way for developing an efficient artificial retina *** proposed device constitutes a hybrid nanocomposite of perovskites(methyl-ammonium lead bromide)and the ferroelectric terpolymer(polyvinylidene fluoride trifluoroethylene-chlorofluoroethylene).A metal-insulator-metal type capacitor with the prepared composite exhibits the unique and photosensitive capacitive behavior at various light intensities in the visible light *** proposed photoreceptor mimics the spectral sensitivity curve of human photopic *** hybrid nanocomposite is stable in ambient air for 129 weeks,with no observable degradation of the composite due to the encapsulation of hybrid perovskites in the hydrophobic *** functionality of the proposed photoreceptor to recognize handwritten digits(MNIST)dataset using an unsupervised trained spiking neural network with 72.05%recognition accuracy is *** demonstration proves the potential of the proposed sensor for neuromorphic vision applications.

关键词： perovskite illumination preserving

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Optimized photonic integrated circuit components for optical coherence tomography at 1060 nm

Optimized photonic integrated circuit components for optical...

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CLEO: Applications and Technology in CLEO 2024, CLEO: A and T 2024 - Part of Conference on Lasers and Electro-Optics

作者： Hao, Senyue Adkins, Aaron J. Zhang, Yitian Zhou, Chao Department of Electrical & Systems Engineering Washington University Saint Louis United States Imaging Science PhD Program Washington University Saint Louis United States Department of Biomedical Engineering Washington University Saint Louis United States

To implement optical coherence tomography on photonic chips, we developed optimized and experimentally validated silicon nitride-based components for photonic integrated circuits in order to achieve high sensitivity a... 详细信息

关键词： Photonic integrated circuits

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XDEVS: A hybrid system modeling framework

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International Journal of Modeling, Simulation, and Scientific Computing 2022年第2期13卷 233-249页

作者： Kunyu Xie Lin Zhang Yuanjun Laili Xiaohan Wang School of Automation Science and Electrical Engineering Engineering Research Center of Complex Product Advanced Manufacturing Systems Ministry of Education Beihang University No.37Xueyuan RoadBeijingChina

When Discrete Event System Specification(DEVS)is used as a modeling tool,there is a semantic gap between a DEVS model and the mathematical representation,which may result in understanding *** provide a more intuitive form of modeling,XDEVS expands the concept of states in *** continuous state is introduced in XDEVS,which enhances the ability to model hybrid *** on the DEVS simulation framework,a simulation engine is developed to drive the XDEVS model safely and efficiently and avoid the wrong location of state events during the simulation of the continuous model.A hybrid model is constructed and simulated using XDEVS.A comparison between the XDEVS model and models described by DEV&DESS and GDEVS shows that XDEVS can clearly express the structure of the model and reduce the burden on modelers.

关键词： DEVS XDEVS hybrid model modeling framework

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Optimized photonic integrated circuit components for optical coherence tomography at 1060 nm

Optimized photonic integrated circuit components for optical...

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2024 Conference on Lasers and Electro-Optics, CLEO 2024

ISBN: (纸本)9781957171395

关键词： Photonic integrated circuits

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Optimal Placement of Electric Vehicle Charging Stations: A Case Study in Jordan

Optimal Placement of Electric Vehicle Charging Stations: A C...

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2023 IEEE Texas Power and Energy Conference, TPEC 2023

作者： Bashaireh, Ahmad Obeidat, Duaa Almehizia, Abdullah A. Shalalfeh, Laith Jordan University of Science and Technology Electrical Engineering Department Irbid Jordan National Center for Electrical Systems and Cooling King Abdulaziz City for Science and Technology Riyadh Saudi Arabia German Jordanian University Energy Engineering Department Amman Jordan

ISBN: (纸本)9781665490719

Several economic factors have contributed to an increased adoption of electric vehicles (EVs) in Jordan. Charging EVs constitutes a considerable electrical load, and hence, the rise in the number of EVs has a major effect on the electric distribution network. To address this, the charging infrastructure should be carefully studied, and an optimal implementation that minimizes the negative impact is crucial. In this paper, we develop a framework for optimal placement of EV charging stations using Particle Swarm optimization (PSO). The optimization problem maximizes the total EV charging capacity while minimizing transmission line and transformer loading and total power losses. This framework is implemented in MATLAB and DIgSILENT PowerFactory and applied to two cases in Jordan's distribution network: an industrial area and a small town. © 2023 IEEE.

关键词： Electric power distribution

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In situ calibrated angle between the quantization axis and the propagating direction of the light field for trapping neutral atoms

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Chinese Physics B 2024年第2期33卷 318-323页

作者：郭瑞军何晓东盛诚王坤鹏许鹏刘敏王谨孙晓红曾勇詹明生 Henan Key Laboratory of Laser and Optoelectronic Information National Center for International Joint Research of Electronic Materials and SystemsSchool of Electrical and Information EngineeringZhengzhou UniversityZhengzhou 450001China State Key Laboratory of Magnetic Resonance and Atomic and Molecular Physics Innovation Academy for Precision Measurement Science and TechnologyChinese Academy of SciencesWuhan 430071China

The recently developed magic-intensity trapping technique of neutral atoms efficiently mitigates the detrimental effect of light shifts on atomic qubits and substantially enhances the coherence time. This technique relies on applying a bias magnetic field precisely parallel to the wave vector of a circularly polarized trapping laser field. However, due to the presence of the vector light shift experienced by the trapped atoms, it is challenging to precisely define a parallel magnetic field, especially at a low bias magnetic field strength, for the magic-intensity trapping of85Rb qubits. In this work, we present a method to calibrate the angle between the bias magnetic field and the trapping laser field with the compensating magnetic fields in the other two directions orthogonal to the bias magnetic field direction. Experimentally, with a constantdepth trap and a fixed bias magnetic field, we measure the respective resonant frequencies of the atomic qubits in a linearly polarized trap and a circularly polarized one via the conventional microwave Rabi spectra with different compensating magnetic fields and obtain the corresponding total magnetic fields via the respective resonant frequencies using the Breit–Rabi formula. With known total magnetic fields, the angle is a function of the other two compensating magnetic ***, the projection value of the angle on either of the directions orthogonal to the bias magnetic field direction can be reduced to 0(4)° by applying specific compensating magnetic fields. The measurement error is mainly attributed to the fluctuation of atomic temperature. Moreover, it also demonstrates that, even for a small angle, the effect is strong enough to cause large decoherence of Rabi oscillation in a magic-intensity trap. Although the compensation method demonstrated here is explored for the magic-intensity trapping technique, it can be applied to a variety of similar precision measurements with trapped neutral atoms.

关键词： quantization axis trapping laser angle compensating magnetic fields

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