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CLEO: Applications and Technology in CLEO 2024, CLEO: A and T 2024 - Part of Conference on Lasers and Electro-Optics

作者： Walden, D. Chakraborty, D. Cheng, J. Straksys, A. Stirke, A. Melo, W.C.M.A. Jukna, A. Komissarov, I. Sobolewski, Roman Department of Physics and Astronomy University of Rochester RochesterNY14627 United States Laboratory for Laser Energetics University of Rochester RochesterNY14623-1299 United States Materials Science Graduate Program University of Rochester RochesterNY14627 United States State Research Institute Center for Physical Sciences & Technology Vilnius Lithuania Department of Physics Vilnius Gediminas Technical University Vilnius Lithuania Department of Electrical and Computer Engineering University of Rochester RochesterNY14627 United States

A novel method has been developed to evaluate the water diffusion dynamics in gelatin-based gels, based on transient terahertz time-domain spectroscopy measurements. Such gels are widely used models for human skin. &#... 详细信息

关键词： Terahertz spectroscopy

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Recent advance in synthesis and application of heteroatom zeolites

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Chinese Chemical Letters 2021年第1期32卷 328-338页

作者： Tingting Pang Xuanyu Yang Chenyi Yuan Ahmed A.Elzatahry Abdulaziz Alghamdi Xing He Xiaowei Cheng Yonghui Deng School of Materials Science and Engineering University of Shanghai for Science and TechnologyShanghai 200093China Department of Chemistry Shanghai Key Laboratory of Molecular Catalysis and Innovative MaterialsFudan UniversityShanghai 200433China Materials Science and Technology Program College of Arts and SciencesQatar UniversityP.O.Box 2713DohaQatar Department of Chemistry College of ScienceKing Saud UniversityP.O.Box 2455Riyadh 11451Saudi Arabia State Key Lab of Transducer Technology Shanghai Institute of Microsystem and Information TechnologyChinese Academy of SciencesShanghai 200050China

Incorporation of heteroatoms into the framewo rk of zeolites has become a significant strategy to improve their performance in catalysis and adsorption,because the obtained heteroatom zeolites exhibit quite different properties from the conventional aluminosilicate zeolites in aspects of surface acidity,pore structures,particle size and so *** this review,the progress on the heteroatom zeolites including their synthesis and application is ***,the recent advance on the design and synthesis of different heteroatom zeolites is *** emphasis is placed on the introduction and comparison of three typical methods,including the direct synthesis,post synthesis and improved direct synthesis,for the traditional heteroatom zeolites(such as TS-1,Sn-MFI,Sn-β) and newly-reported heteroatom zeolites(such as W-MFI,Mo-MFI).According to their intrinsic characteristics,the application of heteroatom zeolites in diverse fields,such as production of fine chemicals,air pollution control and biomass conversion is then ***,the challenges and perspective on the future development of heteroatom zeolites in low-cost preparation and practical application are proposed.

关键词： Heteroatom zeolite Incorporation Tetrahedral coordination Research status Synthesis Application Prospective

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Multistate Control of Nonlinear Photocurrents in Optoferroelectrics via phase manipulation of light field

arXiv

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arXiv 2025年

作者： Kazempour, Ali Sisakht, Esmaeil Taghizadeh Okyay, Mahmut Sait Jiang, Xiao Sato, Shunsuke Park, Noejung Department of physics Payame Noor University PO BOX Tehran119395-3697 Iran Department of Physics Ulsan National Institute of Science and Technology Ulsan689-798 Korea Republic of Materials Science and Engineering Program Department of Chemical and Environmental Engineering University of California-Riverside RiversideCA92521 United States Center for Computational Sciences University of Tsukuba Tsukuba305-8577 Japan

Ultrafast optical control of ferroelectricity based on short and intense light can be utilized to achieve accurate manipulations of ferroelectric materials, which may pave a basis for future breakthrough in nonvolatile memories. Here, we demonstrate that phase manipulation of electric field in the strong field sub-cycle regime induces a nonlinear injection current, efficiently coupling with the topology of band structure and enabling dynamic reversal of both current and polarization. Our time-dependent first-principles calculations reveal that tuning the phase of linearly or circularly polarized light through time-varying chirp, or constant carrier envelop phases within sub-laser-cycle dynamics effectively breaks the time-reversal symmetry, allowing the control over current and electronic polarization reversal over multi-ferroelectric states. Our time- and momentum-resolved transverse current analysis reveal the significance of Berry curvature higher order poles in the apparent association between the odd (even) orders of Berry curvature multipoles to odd (even) pseudo-harmonics in driving polarization dynamics reversal. We suggest that these phase manipulations of short pulse waveform may lead to unprecedented accurate control of nonlinear photocurrents and polarization states, which facilitate the development of precise ultrafast opto-ferroelectric devices. © 2025, CC BY.

关键词： Ferroelectricity

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3D printed bioabsorbable composite scaffolds of poly (lactic acid)-tricalcium phosphate-ceria with osteogenic property for bone regeneration

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Biomaterials and Biosystems 2024年 13卷 100086页

作者： Harb, Samarah V. Kolanthai, Elayaraja Pugazhendhi, Abinaya S. Beatrice, Cesar A.G. Pinto, Leonardo A. Neal, Craig J. Backes, Eduardo H. Nunes, Ana C.C. Selistre-de-Araújo, Heloisa S. Costa, Lidiane C. Coathup, Melanie J. Seal, Sudipta Pessan, Luiz A. Department of Materials Engineering (DEMa) Federal University of Sao Carlos (UFSCar) SP São Carlos Brazil Advanced Materials Processing and Analysis Center Department of Materials Science and Engineering University of Central Florida Orlando FL United States Biionix Cluster College of Medicine University of Central Florida Orlando FL United States Graduate Program in Materials Science and Engineering Department of Materials Engineering (DEMa) Federal University of São Carlos (UFSCar) SP São Carlos Brazil Department of Physiological Sciences Federal University of São Carlos (UFSCar) SP São Carlos Brazil

The fabrication of customized implants by additive manufacturing has allowed continued development of the personalized medicine field. Herein, a 3D-printed bioabsorbable poly (lactic acid) (PLA)- β-tricalcium phosphate (TCP) (10 wt %) composite has been modified with CeO₂ nanoparticles (CeNPs) (1, 5 and 10 wt %) for bone repair. The filaments were prepared by melt extrusion and used to print porous scaffolds. The nanocomposite scaffolds possessed precise structure with fine print resolution, a homogenous distribution of TCP and CeNP components, and mechanical properties appropriate for bone tissue engineering applications. Cell proliferation assays using osteoblast cultures confirmed the cytocompatibility of the composites. In addition, the presence of CeNPs enhanced the proliferation and differentiation of mesenchymal stem cells;thereby, increasing alkaline phosphatase (ALP) activity, calcium deposition and bone-related gene expression. Results from this study have shown that the 3D printed PLA-TCP-10%CeO₂ composite scaffold could be used as an alternative polymeric implant for bone tissue engineering applications: avoiding additional/revision surgeries and accelerating the regenerative process. © 2023

关键词： Additive manufacturing Biomaterial Bone tissue engineering Ceria nanoparticle Polymer-matrix composites

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Developments in the utilization of heterogeneous catalysts for biodiesel generation: An update on recent advancements

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Journal of the Taiwan Institute of Chemical Engineers 2024年

作者： Parameshwar, Sai Agnihotri, Mayank Bhan, Uday Nangan, Senthilkumar Verma, Deepak Rajendran, Saravanan Jain, Siddharth Department of Petroleum Engineering and Earth Sciences UPES Dehradun248007 India Metallurgy and Materials Science Research Institute Chulalongkorn University Bangkok10330 Thailand International Graduate Program of Nanoscience and Technology Chulalongkorn University Bangkok10330 Thailand Instituto de Alta Investigacion Universidad de Tarapacá Arica1000000 Chile Department of Mechanical Engineering UPES Dehradun248007 India

Background: Biodiesel is one of the ecofriendly energy sources that can be generated from edible, non-edible, waste, and algae feedstocks. Over time, the utilization of different kinds of heterogeneous catalysts has been proven critical in the manufacture of biodiesel from diverse feedstocks. They exhibit better reusability and easier separation compared to the homogenous catalysts. Methods: In this work, the advances in the use of heterogeneous catalysts for biodiesel production from 2018 to 2024 have been evaluated. The process parameters like alcohol to oil molar ratio (M/O), catalyst concentration (%), reaction time and reaction temperature (RT), reusability of the catalyst, etc. are evaluated. The catalysts derived from waste materials through the calcination process are an efficient and cost-effective substitute for conventional catalysts. Nanomaterials, due to their small size and higher aspect ratio, provide very high efficiency and reusability in catalytic reactions. Significant findings: The heterogeneous catalysts are also found to be highly reusable for multiple cycles and the leaching of active sites, clogging of pore spaces of catalyst, etc. are the major causes of catalyst deactivation. Magnetic heterogeneous catalysts have shown good biodiesel yields and high reusability. Also, naturally occurring calcium oxide and potassium compounds present in waste derived catalysts helped to give high biodiesel yields. The future direction in the path of development of heterogeneous catalysts from cheap, abundant, and environmentally benign materials. The synthesis of heterogeneous catalysts from waste materials addresses the issue of waste disposal and converting solid waste to value-added catalysts. The life cycle assessment studies, encompassing heterogeneous catalyst synthesis, feedstock oil extraction, biodiesel production, and fuel combustion may give valuable input on the environmental impact of the entire process. © 2024

关键词： Potassium compounds

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Charge-Carrier Dynamics and Relaxation in Cs2SnI6 Perovskite for Energy Storage: Existence of Anharmonic Rattling-Assisted Polaron Dynamics

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Physical Review Applied 2023年第5期20卷 054032-054032页

作者： Moumita Ghosh Pulak Pal Tufan Paul Soumen Maiti Souvik Bhattacharjee Kausik Sardar Aditi Sahoo Aswini Ghosh Kalyan Kumar Chattopadhyay Departments of Physics Jadavpur University Kolkata 700032 India School of Materials Science and Nanotechnology Jadavpur University Kolkata 700032 India Department of Physics St. Thomas College of Engineering & Technology Kolkata 700023 India Advanced Mechanical and Materials Characterization Division CSIR-Central Glass & Ceramic Research Institute Kolkata 700032 India School of Physical Sciences Indian Association for the Cultivation of Science Jadavpur Kolkata 700032 India

We have explored different aspects of charge-carrier dynamics and relaxation in lead-free Cs2SnI6 double perovskite using dielectric spectroscopy and assessed its electrochemical response. The cubic phase (Fm3¯m) with a lattice constant of 11.644 Å is confirmed for synthesized perovskite. The phonon dispersion illustrated by density-functional theory indicates the existence of soft optical modes triggered by anharmonic rattling of Cs atoms and dynamical rotation of SnI6 octahedra. Complex impedance spectra have provided details of the contributions of grain boundaries, grains, and anharmonic rattling to charge-carrier dynamics. The Cs2SnI6 exhibits electrical conductivity of 3.77×10−5Scm−1 at ambient conditions. The values of the power-law exponent for all temperatures suggest superlinear power-law (SPL) behavior of the ac conductivity. The relaxation time and the stretched exponent in the Kohlrausch-Williams-Watts (KWW) function of the electric modulus are caused by charge-carrier short-range mobility and the hopping of rattling-assisted polarons. The supercapacitor fabricated with Cs2SnI6 as the electrode has delivered a specific capacitance of 3830 F g−1 at a current density of 2 A g−1. A quasi-solid-state asymmetric supercapacitor device was also fabricated, which delivered an energy density of 51 Wh kg−1 and a power density as high as 852 W kg−1 at a current density of 1 A g−1. We believe this work will open up the avenue to another generation of lead-free, perovskite-based, sustainable energy-storage systems.

关键词： Carrier dynamics Dielectric properties Impedance Polarons Supercapacitors Energy materials Perovskites Semiconductor compounds

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Ultra-high sensitive 2D photonic crystal for gas and chemical sensing applications

Ultra-high sensitive 2D photonic crystal for gas and chemica...

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Optical Sensors 2023

作者： Salama, Norhan A. Swillam, Mohamed A. Hameed, Mohamed Farhat O. Alexeree, Shaimaa M. Obayya, Salah S.A. Laser Applications in Metrology Photochemistry and Agriculture National Institute of Laser Enhanced Sciences Cairo University Giza Egypt Department of Physics The American University in Cairo Cairo11835 Egypt Centre for Photonics and Smart Materials Zewail City of Science Technology and Innovation October Gardens 6th of October City Giza12578 Egypt Nanotechnology and Nanoelectronics Engineering Program Zewail City of Science Technology and Innovation October Gardens 6th of October City Giza12578 Egypt Faculty of Engineering University of Mansoura Mansoura Egypt

ISBN: (数字)9781510662650

ISBN: (纸本)9781510662643

Mid infrared (MID-IR) band of electromagnetic radiation plays the key role for gas and chemical sensing application because it provides molecular fingerprints for most trace gases and molecules. Photonic crystal cavity coupled waveguide (PC-CWG) based sensors is a remarkable platform for sensing applications due to its capability to confine light modes on small volume displaying high sensitivity and high quality factors. In this work, we report a novel design of (PC-CWG) based on square lattice of silicon pillars in air with radius of 0.2μm and lattice constant of 1 μm. A waveguide is introduced by removing three columns of silicon pillars, and a microcavity is created by removing a number of silicon pillars forming curved shapes on both sides of the waveguide. The proposed design demonstrates multiple resonances covering a broad spectral range in MID-IR ranging from 2.4 μm to 4.2 μm that represents the bandgap region. Remarkable resonances are observed at operating wavelengths 2.67 μm, 2.88 μm, 3.03 μm, 3.2 μm and 3.5 μm. Moreover, the reported design shows ultra-high sensitivity reaching 2680 nm/RIU with a significant quality factor of Q=6475 giving rise to a figure-of-merit of 5.7 × 106 at the operating wavelength of (λ=3.03μm). The suggested photonic crystal design offers simple fabrication and broad applicability for refractive index sensing applications. © 2023 SPIE.

关键词： Photonic crystals

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Magnetochiral Tunneling in Paramagnetic Co1/3NbS2

arXiv

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arXiv 2024年

作者： Lim, Seongjoon Singh, Sobhit Huang, Fei-Ting Pan, Shangke Wang, Kefeng Kim, Jaewook Kim, Jinwoong Vanderbilt, David Cheong, Sang-Wook Rutgers Center for Emergent Materials Department of Physics and Astronomy PiscatawayNJ08854 United States Department of Mechanical Engineering University of Rochester RochesterNY14627 United States Materials Science Program University of Rochester RochesterNY14627 United States State Key Laboratory Base of Novel Function Materials and Preparation Science School of Material Sciences and Chemical Engineering Ningbo University Zhejiang Ningbo315211 China Department of Physics and Astronomy Rutgers University PiscatawayNJ08854 United States

Electric currents have the intriguing ability to induce magnetization in nonmagnetic crystals with sufficiently low crystallographic symmetry. Some associated phenomena include the non-linear anomalous Hall effect in polar crystals and the nonreciprocal directional dichroism in chiral crystals when magnetic fields are applied. In this work, we demonstrate that the same underlying physics is also manifested in the electronic tunneling process between the surface of a nonmagnetic chiral material and a magnetized scanning probe. In the paramagnetic but chiral metallic compound Co1/3NbS2, the magnetization induced by the tunneling current is shown to become detectable by its coupling to the magnetization of the tip itself. This results in a contrast across different chiral domains, achieving atomic-scale spatial resolution of structural chirality. To support the proposed mechanism, we used first-principles theory to compute the chirality-dependent current-induced magnetization and Berry curvature in the bulk of the material. Our demonstration of this magnetochiral tunneling effect opens up a new avenue for investigating atomic-scale variations in the local crystallographic symmetry and electronic structure across the structural domain boundaries of low-symmetry nonmagnetic crystals. © 2024, CC BY.

关键词： Magnetization

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Meta-optic accelerators for object classifier

Meta-optic accelerators for object classifier

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Conference on Lasers and Electro-Optics (CLEO)

作者： Hanyu Zheng Quan Liu You Zhou Ivan I. Kravchenko Yuankai Huo Jason Valentine Department of Electrical and Computer Engineering Vanderbilt University Nashville TN USA Department of Computer Science Vanderbilt University Nashville TN USA Interdisciplinary Materials Science Program Vanderbilt University Nashville TN USA Center for Nanophase Materials Sciences Oak Ridge National Laboratory Oak Ridge TN USA Department of Mechanical Engineering Vanderbilt University Nashville TN USA

A meta-optic platform for accelerating object classification is demonstrated. End-to-end design is used to co-optimize the optical and digital systems resulting in a high-speed and robust classifier with 93.1% accurac... 详细信息

ISBN: (纸本)9781957171258

关键词： Image analysis Image resolution Machine vision Neural networks Optical systems Signal processing

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Effect of pyrolysis temperature on characteristics of tunable magnetic biochar synthesized from watermelon rind and its tetracycline adsorption performance

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Journal of the Taiwan Institute of Chemical Engineers 2024年 160卷

作者： Thairattananon, Phisit Le, Giang T.T. Matsumura, Yukihiko Wu, Kevin C.W. Charinpanitkul, Tawatchai Department of Chemical Engineering Faculty of Engineering Center of Excellence in Particle and Material Processing Technology Chulalongkorn University Bangkok10330 Thailand Institute of Fundamental and Applied Sciences Duy Tan University Ho Chi Minh700000 Viet Nam Faculty of Environmental and Chemical Engineering Duy Tan University Da Nang550000 Viet Nam Mechanical Engineering Program Graduate School of Advanced Science and Engineering Kagamiyama Hiroshima Higashi-Hiroshima739-8527 Japan Department of Chemical Engineering National Taiwan University Taipei10617 Taiwan Department of Chemical Engineering and Materials Science Yuan Ze University Chung-Li Taoyuan Taiwan Research Network of NANOTEC-KU on Nanocatalyst and Nanomaterials for Sustainable Energy and Environment Bangkok10900 Thailand

Background: Tetracycline is an emerging contaminant in water reservoirs, causing undesirable influences on human society. The promising usage of magnetic biochar (MBC) derived from watermelon rind has been explored in the adsorption of various contaminants owing to its high specific surface area and separability;however, the temperature-dependent changes of MBC and its sorption ability toward antibiotics have not been widely examined. Method: Tunable MBCs could be synthesized via simple pyrolysis of watermelon rind impregnated with FeCl3 at different temperatures (700–900 °C). The as-synthesized MBCs were characterized using scanning electron microscopy (SEM), an elemental analyzer, N2 adsorption/desorption, Fourier-transform infrared spectroscopy (FTIR), Raman spectroscopy, X-ray diffractometry (XRD), and vibrating sample magnetometry (VSM). Then Tetracycline, an emerging contaminant in water reservoirs, was employed as the target contaminant, while adsorption kinetics, isotherm, the effect of pH, and reusability were investigated. Significant findings: The tunability of as-synthesized MBCs could be observed by their distinct changes in structural characteristics when varying pyrolysis temperature. MBC synthesized at 900 °C (MBC900) possessed a high-specific surface area (401 m2.g−1) and saturation magnetization (55.29 emu.g−1), resulting in a greater amount of sorption sites. Tetracycline adsorption by MBCs followed a pseudo-second-order kinetic model and fitted well with the Freundlich model. MBC900 is an excellent adsorbent with a maximum adsorption capacity of 77.6 mg.g−1 and could be used for at least five cycles with an insignificant decrease in the adsorption capacity. © 2024 Taiwan Institute of Chemical Engineers

关键词： Adsorption

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