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Nanoscale 2024年第9期16卷 4919页

作者： Michael A Casasanta G M Jonaid Liam Kaylor William Y Luqiu Maria J Solares Mariah L Schroen William J Dearnaley Jarad Wilson Madeline J Dukes Deborah F Kelly Department of Biomedical Engineering Pennsylvania State University University Park PA 16802 USA. Debkelly@psu.edu. Materials Research Institute Pennsylvania State University University Park PA 16802 USA. Bioinformatics and Genomics Graduate Program Huck Institutes of the Life Sciences Pennsylvania State University University Park PA 16802 USA. Molecular Cellular and Integrative Biosciences Graduate Program Huck Institutes of the Life Sciences Pennsylvania State University University Park PA 16802 USA. Department of Electrical and Computer Engineering Duke University Durham NC 27708 USA. RayBiotech Life Peachtree Corners GA 30092 USA. Applications Science Protochips Inc. Morrisville NC 27560 USA.

Expression of concern for 'Microchip-based structure determination of low-molecular weight proteins using cryo-electron microscopy' by Michael A. Casasanta , , 2021, , 7285-7293, https://***/10.1039/D1NR00388G.

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ZnO/BiOI heterojunction catalyst: Efficient photocatalytic decomposition of perfluorooctanoic acid (PFOA) and mixed dye pollutants in wastewater

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Separation and Purification Technology 2025年

作者： Kareem Mazen Gopal Venkatesh Fatin Samara Sofian Kanan Department of Biology Chemistry & Environmental Sciences College of Arts and Sciences American University of Sharjah Sharjah P.O. Box 26666 United Arab Emirates Sharjah Environmental Hazards Assessment and Remediation (SEHAR) American University of Sharjah Sharjah P.O. Box 26666 United Arab Emirates Energy Water and Sustainable Environment Research Center (EWSERC) American University of Sharjah PO Box 26666 United Arab Emirates Materials Science and Engineering Program College of Arts and Sciences American University of Sharjah PO Box 26666 United Arab Emirates

ZnO/BiOI binary composites were synthesized via facile hydrothermal method for visible light active photocatalyst. The physiochemical properties of the photocatalysts were characterized using XRD, SEM, EDX, FTIR, Raman, XPS, UV–vis. and PL techniques. The synthesized material’s photocatalytic activity was assessed against mixed textile dyes including MB and Rh B, and a class of emerging contaminants labelled as “forever chemicals,” specifically Perfluorooctanoic acid (PFOA). The integration of BiOI with ZnO creates a ZB binary heterostructure, which significantly enhances the photocatalytic efficiency by combining the strengths of both materials. ZnO is active in the UV region, while BiOI broadens the light absorption into the visible spectrum. The formation of this heterojunction effectively inhibited charge carrier recombination, enhancing photocatalytic performance through a Z-scheme charge transfer mechanism. The results showed that the synthesized photocatalyst achieved an efficient elimination rate of MB and Rh B by 97% and 84%, respectively. Moreover, a complete degradation and defluorination of PFOA was confirmed via liquid gas chromatography coupled with mass spectrometry. This study highlights the significant potential of the synthesized BiOI incorporated ZnO as a photocatalyst for the effective removal of mixed dyes and the defluorination of PFOA compounds in environmental wastewater treatment.

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Three-dimensional bioprinting of gelatin methacryloyl (GelMA)

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Bio-Design and Manufacturing 2018年第4期1卷 215-224页

作者： Guoliang Ying Nan Jiang Cunjiang Yu Yu Shrike Zhang Division of Engineering in Medicine Department of MedicineBrigham and Women's HospitalHarvard Medical SchoolCambridgeMA 02139USA School of Materials Science and Engineering Wuhan Institute of TechnologyWuhan 430205People's Republic of China School of Engineering and Applied Sciences Harvard UniversityCambridgeMA 02139USA Departments of Mechanical Engineering Electrical and Computer EngineeringBiomedical EngineeringMaterials Science and Engineering ProgramThe Texas Center for SuperconductivityUniversity of HoustonHoustonTX 77204USA

The three-dimensional (3D)bioprinting technology has progressed tremendously over the past *** controlling the size, shape,and architecture of the bioprinted constructs,3D bioprinting allows for the fabrication of tissue/organ-like constructs with strong structural-functional similarity with their in vivo counterparts at high *** bioink,a blend of biomaterials and living cells possessing both high biocompatibility and printability,is a critical component of *** particular, gelatin methacryloyl (GelMA)has shown its potential as a viable bioink material due to its suitable biocompatibility and readily tunable physicochemical *** GelMA-based bioinks and relevant bioprinting strategies for GelMA bioprinting are briefly reviewed.

关键词： Bioprinting Bioink Gelatin methacryloyl (GelMA) Biofabrication -Tissue engineering Tissue model

Terahertz Inverse Spin Hall Effect in Spintronic Nanostructures

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SSRN

SSRN 2023年

作者： Cheng, Jing Komissarov, Ivan Chen, Genyu Adam, Roman Chaktraborty, Debamitra Bürgler, Daniel E. Heidtfeld, Sarah Cao, Derang Büscher, Markus Hardtdegen, Hilde Mikulics, Martin Schneider, Claus Michael Gladczuk, Leszek Przyslupski, Piotr Sobolewski, Roman Materials Science Program University of Rochester RochesterNY14627-1299 United States Laboratory for Laser Energetics University of Rochester RochesterNY14623 United States Department of Electrical and Computer Engineering University of Rochester RochesterNY14627-0231 United States Research Centre Jülich Peter Grünberg Institute Jülich52425 Germany Faculty of Physics University Duisburg-Essen Duisburg47048 Germany College of Physics Center for Marine Observation and Communications National Demonstration Center for Experimental Applied Physics Education Qingdao University Qingdao266071 China Research Centre Jülich Ernst Ruska Centre for Microscopy and Spectroscopy With Electrons Jülich52425 Germany Department of Physics University of California Davis DavisCA95616-5270 United States Institute of Physics Polish Academy of Sciences WarszawaPL-02668 Poland Department of Physics and Astronomy University of Rochester RochesterNY14627-0171 United States

Bilayers of ferromagnetic and heavy metal nanolayers excited with femtosecond laser pulses emit subpicosecond bursts of electromagnetic radiation with spectral frequencies up to several THz. We fabricated such spintronic THz emitters containing various ferromagnetic materials with vastly different magnetic remanence, saturation magnetization, and coercive field. In all cases, the THz amplitude versus magnetic field dependence follows the independently measured magnetization hysteresis loops and the THz polarization direction is perpendicular to the sample’s magnetization M, both consistent with the inverse spin Hall effect as physical origin. The M(T) variation governs the temperature dependence of the THz generation. Emitters with weakly remanent ferromagnets are field-tunable, while moderately and strongly remanent ferromagnets, once magnetized, allow intense THz generation even without an external field, nevertheless exhibiting low susceptibility to magnetic perturbations, if the hysteresis loop is square. Hence, exploiting the magnetic properties of the ferromagnetic layer enables tailoring of weakly temperature-dependent spintronic THz emitters. Finally, we explored the applicability of perovskite oxide materials such as La-Sr-Mn-O (LSMO) for THz transient generation. Although we detected THz emissions from, e.g., LSMO/Au nanobilayers, the signal was attributed to the ultrafast transient demagnetization and not the inverse spin Hall effect. © 2023, The Authors. All rights reserved.

关键词： Nanostructures

Revealing the Origin of Transition-Metal Migration in Layered Sodium-Ion Battery Cathodes: Random Na Extraction and Na-Free Layer Formation

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Angewandte Chemie 2023年第12期135卷

作者： Dr. Shiyong Chu Prof. Duho Kim Gwanghyeon Choi Chunchen Zhang Haoyu Li Prof. Wei Kong Pang Yameng Fan Anita M. D'Angelo Prof. Shaohua Guo Prof. Haoshen Zhou College of Engineering and Applied Sciences Jiangsu Key Laboratory of Artificial Functional Materials National Laboratory of Solid State Microstructures Collaborative Innovation Center of Advanced Microstructures Frontiers Science Center for Critical Earth Material Cycling Nanjing University Nanjing 210023 China Shenzhen Research Institute of Nanjing University Shenzhen 518000 China Department of Mechanical Engineering (Integrated Engineering Program) Kyung Hee University 1732 Deogyeong-daero Giheung-gu Yongin-si Gyeonggi-do 17104 (Republic of Korea Institute for Superconducting & Electronic Materials University of Wollongong Wollongong NSW-2522 Australia Australian Synchrotron Australian Nuclear Science and Technology Organization 800 Blackburn Road Clayton Victoria 3168 Australia

Cation migration often occurs in layered oxide cathodes of lithium-ion batteries due to the similar ion radius of Li and transition metals (TMs). Although Na and TM show a big difference of ion radius, TMs in layered cathodes of sodium-ion batteries (SIBs) can still migrate to Na layer, leading to serious electrochemical degeneration. To elucidate the origin of TM migration in layered SIB cathodes, we choose NaCrO 2 , a typical layered cathode suffering from serious TM migration, as a model material and find that the TM migration is derived from the random desodiation and subsequent formation of Na-free layer at high charge potential. A Ru/Ti co-doping strategy is developed to address the issue, where the doped active Ru is first oxidized to create a selective desodiation and the doped inactive Ti can function as a pillar to avoid complete desodiation in Ru-contained TM layers, leading to the suppression of the Na-free layer formation and subsequent enhanced electrochemical performance.

关键词： Layered Sodium-Ion Battery Cathodes Na-Free Layer Random Na Extraction Selective Na Extraction Transition-Metal Migration

How to verify the precision of density-functional-theory implementations via reproducible and universal workflows

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arXiv 2023年

作者： Bosoni, Emanuele Beal, Louis Bercx, Marnik Blaha, Peter Blügel, Stefan Bröder, Jens Callsen, Martin Cottenier, Stefaan Degomme, Augustin Dikan, Vladimir Eimre, Kristjan Flage-Larsen, Espen Fornari, Marco Garcia, Alberto Genovese, Luigi Giantomassi, Matteo Huber, Sebastiaan P. Janssen, Henning Kastlunger, Georg Krack, Matthias Kresse, Georg Kühne, Thomas D. Lejaeghere, Kurt Madsen, Georg K.H. Marsman, Martijn Marzari, Nicola Michalicek, Gregor Mirhosseini, Hossein Müller, Tiziano M.A. Petretto, Guido Pickard, Chris J. Poncé, Samuel Rignanese, Gian-Marco Rubel, Oleg Ruh, Thomas Sluydts, Michael Vanpoucke, Danny E.P. Vijay, Sudarshan Wolloch, Michael Wortmann, Daniel Yakutovich, Aliaksandr V. Yu, Jusong Zadoks, Austin Zhu, Bonan Pizzi, Giovanni Institut de Ciència de Materials de Barcelona ICMAB-CSIC Campus UAB Bellaterra08193 Spain Univ. Grenoble-Alpes CEA IRIG-MEM-L Sim Grenoble38000 France LausanneCH-1015 Switzerland Institute for Materials Chemistry Technical University of Vienna Getreidemarkt 9/165-TC ViennaA-1060 Austria Peter Grünberg Institut Institute for Advanced Simulation Forschungszentrum Jülich JARA JülichD-52425 Germany Forschungszentrum Jülich JülichD-52425 Germany Department of Electromechanical Systems and Metal Engineering Ghent University Belgium Ghent University Belgium Institute of Atomic and Molecular Sciences Academia Sinica Taipei10617 Taiwan Norwegian EuroHPC Competence Center Sigma2 AS Norway SINTEF Industry Materials Physics Oslo Norway Department of Physics Science of Advanced Materials Program Central Michigan University Mount PleasantMI48859 United States Université catholique de Louvain Chemin des Étoiles 8 Louvain-la-Neuve1348 Belgium LausanneCH-1015 Switzerland Kongens Lyngby2800 Denmark VilligenCH-5232 Switzerland University of Vienna Faculty of Physics Center for Computational Materials Science Kolingasse 14-16 ViennaA-1090 Austria VASP Software GmbH Sensengasse 8 ViennaA-1090 Austria Helmholtz-Zentrum Dresden-Rossendorf GörlitzD-02826 Germany Center for Sustainable Systems Design University of Paderborn PaderbornD-33098 Germany OCAS NV ArcelorMittal Global R&D Gent Pres. J. F. Kennedylaan 3 ZelzateB-9060 Belgium Dynamics of Condensed Matter Theoretical Chemistry University of Paderborn PaderbornD-33098 Germany HPE HPC EMEA Research Lab BaselCH-4051 Switzerland Department of Materials Science & Metallurgy University of Cambridge 27 Charles Babbage Road CambridgeCB3 0FS United Kingdom Advanced Institute for Materials Research Tohoku University 2-1-1 Katahira Aoba Sendai980-8577 Japan Department of Materials Science and Engineering McMaster University 1280 Main Street West HamiltonONL8S 4L8 Canada ePot

In the past decades many density-functional theory methods and codes adopting periodic boundary conditions have been developed and are now extensively used in condensed matter physics and materials science research. Only in 2016, however, their precision (i.e., to which extent properties computed with different codes agree among each other) was systematically assessed on elemental crystals: a first crucial step to evaluate the reliability of such computations. We discuss here general recommendations for verification studies aiming at further testing precision and transferability of density-functional-theory computational approaches and codes. We illustrate such recommendations using a greatly expanded protocol covering the whole periodic table from Z=1 to 96 and characterizing 10 prototypical cubic compounds for each element: 4 unaries and 6 oxides, spanning a wide range of coordination numbers and oxidation states. The primary outcome is a reference dataset of 960 equations of state cross-checked between two all-electron codes, then used to verify and improve nine pseudopotential-based approaches. Such effort is facilitated by deploying AiiDA common workflows that perform automatic input parameter selection, provide identical input/output interfaces across codes, and ensure full reproducibility. Finally, we discuss the extent to which the current results for total energies can be reused for different goals (e.g., obtaining formation energies). © 2023, CC BY.

关键词： Density functional theory

The bulk van der Waals layered magnet CrSBr is a quasi-1D material

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arXiv 2022年

作者： Klein, Julian Pingault, Benjamin Florian, Matthias Heißenbüttel, Marie-Christin Steinhoff, Alexander Song, Zhigang Torres, Kierstin Dirnberger, Florian Curtis, Jonathan B. Weile, Mads Penn, Aubrey Deilmann, Thorsten Dana, Rami Bushati, Rezlind Quan, Jiamin Luxa, Jan Sofer, Zdenek Alù, Andrea Menon, Vinod M. Wurstbauer, Ursula Rohlfing, Michael Narang, Prineha Lončar, Marko Ross, Frances M. Department of Materials Science and Engineering Massachusetts Institute of Technology CambridgeMA02139 United States John A. Paulson School of Engineering and Applied Sciences Harvard University CambridgeMA02138 United States QuTech Delft University of Technology Delft2600 GA Netherlands Department of Electrical and Computer Engineering Department of Physics University of Michigan Ann ArborMI48109 United States Institut für Festkörpertheorie Westfälische Wilhelms-Universität Münster Münster48149 Germany Institut für Theoretische Physik Universität Bremen P.O. Box 330 440 Bremen28334 Germany Bremen Center for Computational Materials Science University of Bremen Bremen28359 Germany Department of Physics City College of New York New YorkNY10031 United States College of Letters and Science UCLA Los AngelesCA90095 United States Department of Physics Technical University of Denmark Kgs. LyngbyDK-2800 Denmark MIT.nano Massachusetts Institute of Technology CambridgeMA02139 United States Department of Physics The Graduate Center City University of New York New YorkNY10016 United States Photonics Initiative CUNY Advanced Science Research Center New YorkNY10031 United States Physics Program Graduate Center City University of New York New YorkNY10026 United States Department of Inorganic Chemistry University of Chemistry and Technology Prague Technická 5 Prague 6166 28 Czech Republic Institute of Physics Center for Nanotechnology University of Münster Münster48149 Germany

Correlated quantum phenomena in one-dimensional (1D) systems that exhibit competing electronic and magnetic order are of strong interest for studying fundamental interactions and excitations, such as Tomonaga-Luttinger liquids and topological orders and defects with properties completely different from the quasiparticles expected in their higher-dimensional counterparts. However, clean 1D electronic systems are difficult to realize experimentally, particularly magnetically ordered systems. Here, we show that the van der Waals layered magnetic semiconductor CrSBr behaves like a quasi-1D material embedded in a magnetically ordered environment. The strong 1D electronic character originates from the Cr-S chains and the combination of weak interlayer hybridization and anisotropy in effective mass and dielectric screening with an effective electron mass ratio of meX/meY ∼ 50. This extreme anisotropy experimentally manifests in strong electron-phonon and exciton-phonon interactions, a Peierls-like structural instability and a Fano resonance from a van Hove singularity of similar strength of metallic carbon nanotubes. Moreover, due to the reduced dimensionality and interlayer coupling, CrSBr hosts spectrally narrow (1 meV) excitons of high binding energy and oscillator strength that inherit the 1D character. Overall, CrSBr is best understood as a stack of weakly hybridized monolayers and appears to be an experimentally attractive candidate for the study of exotic exciton and 1D correlated many-body physics in the presence of magnetic order. Copyright © 2022, The Authors. All rights reserved.

关键词： Excitons

Three-dimensional dynamics of magnetic hopfion driven by spin transfer torque

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arXiv 2020年

作者： Liu, Yizhou Hou, Wentao Han, Xiufeng Zang, Jiadong Beijing National Laboratory for Condensed Matter Physics Institute of Physics Chinese Academy of Sciences Beijing100190 China Department of Physics and Astronomy University of New Hampshire DurhamNH03824 United States Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of Sciences Beijing100049 China Songshan Lake Materials Laboratory Dongguan Guangdong523808 China Materials Science Program University of New Hampshire DurhamNH03824 United States

Magnetic hopfion is three-dimensional (3D) topological soliton with novel spin structure that would enable exotic dynamics. Here we study the current driven 3D dynamics of a magnetic hopfion with unit Hopf index in a frustrated magnet. Attributed to spin Berry phase and symmetry of the hopfion, the phase space entangles multiple collective coordinates, thus the hopfion exhibits rich dynamics including longitudinal motion along the current direction, transverse motion perpendicular to the current direction, rotational motion and dilation. Furthermore, the characteristics of hopfion dynamics is determined by the ratio between the non-adiabatic spin transfer torque parameter and the damping parameter. Such peculiar 3D dynamics of magnetic hopfion could shed light on understanding the universal physics of hopfions in different systems and boost the prosperous development of 3D spintronics. Copyright © 2020, The Authors. All rights reserved.

关键词： Magnetism

Anharmonicity and Universal Response of Linear Carbon Chain Mechanical Properties under Hydrostatic Pressure

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Physical Review Letters 2020年第10期125卷 105501-105501页

作者： Keshav Sharma Nathalia L. Costa Yoong Ahm Kim Hiroyuki Muramatsu Newton M. Barbosa Neto Luiz G. P. Martins Jing Kong Alexandre Rocha Paschoal Paulo T. Araujo Department of Physics and Astronomy University of Alabama Tuscaloosa Alabama 35487 USA Department of Physics Federal University of Ceara 60455-760 Fortaleza Ceara Brazil Department of Polymer Engineering School of Polymer Science and Engineering and Alan G. MacDiarmid Energy Research Institute Chonnam National University 77 Yongbong-ro Buk-gu Gwangju 61186 Republic of Korea Research Institute for Supra-Materials Shinshu University 4-17-1 Wakasato Nagano Japan Institute of Natural Sciences Graduate Program in Physics Federal University of Para 66075-110 Belem PA Brazil Department of Physics Massachusetts Institute of Technology Cambridge Massachusetts 02139 USA Department of Electrical Engineering and Computer Science Massachusetts Institute of Technology Cambridge Massachusetts 02139 USA

Isolated linear carbon chains (LCCs) encapsulated by multiwalled carbon nanotubes are studied under hydrostatic pressure (P) via resonance Raman scattering. The LCCs’ spectroscopic signature C band around 1850 cm−1 softens linearly with increasing P. A simple anharmonic force-constant model not only describes such softening but also shows that the LCCs’ Young’s modulus (E), Grüneisen parameter (γ), and strain (ϵ) follow universal P−1 and P2 laws, respectively. In particular, γ also presents a unified behavior for all LCCs. To the best of our knowledge, these are the first results reported on such isolated systems and the first work to explore universal P-dependent responses for LCCs’ E, ϵ, and γ.

关键词： Anharmonic lattice dynamics Compressive strength Elasticity Mechanical & acoustical properties Pressure effects Stress 1-dimensional systems Lattice models in condensed matter Pressure techniques Raman spectroscopy

Human brain mapping with multi-thousand channel PtNRGrids resolves novel spatiotemporal dynamics

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arXiv 2021年

作者： Tchoe, Youngbin Bourhis, Andrew M. Cleary, Daniel R. Stedelin, Brittany Lee, Jihwan Tonsfeldt, Karen J. Brown, Erik C. Siler, Dominic Paulk, Angelique C. Yang, Jimmy C. Oh, Hongseok Ro, Yun Goo Choi, Woojin Lee, Keundong Russman, Samantha Ganji, Mehran Galton, Ian Ben-Haim, Sharona Raslan, Ahmed M. Dayeh, Shadi A. Integrated Electronics and Biointerfaces Laboratory Department of Electrical and Computer Engineering University of California San Diego San DiegoCA92093 United States Department of Neurological Surgery University of California San Diego San DiegoCA92093 United States Department of Neurological Surgery Oregon Health & Science University Mail Code CH8N 3303 SW Bond Avenue PortlandOR97239-3098 United States Department of Obstetrics Gynecology and Reproductive Sciences Center for Reproductive Science and Medicine University of California San Diego San DiegoCA92093 United States Department of Neurology Massachusetts General Hospital BostonMA02114 United States Department of Neurosurgery Massachusetts General Hospital BostonMA02114 United States Graduate Program of Materials Science and Engineering University of California San Diego San DiegoCA92093 United States

Electrophysiological devices are critical for mapping eloquent and diseased brain regions and for therapeutic neuromodulation in clinical settings and are extensively utilized for research in brain-machine interfaces. However, the existing devices are often limited in either spatial resolution or cortical coverage, even including those with thousands of channels used in animal experiments. Here, we developed scalable manufacturing processes and dense connectorization to achieve reconfigurable thin-film, multi-thousand channel neurophysiological recording grids using platinum-nanorods (PtNRGrids). With PtNRGrids, we have achieved a multi-thousand channel array of small (30 μm) contacts with low impedance, providing unparalleled spatial and temporal resolution over a large cortical area. We demonstrate that PtNRGrids can resolve sub-millimeter functional organization of the barrel cortex in anesthetized rats that captured the histochemically-demonstrated structure. In the clinical setting, PtNRGrids resolved fine, complex temporal dynamics from the cortical surface in an awake human patient performing grasping tasks. Additionally, the PtNRGrids identified the spatial spread and dynamics of epileptic discharges in a patient undergoing epilepsy surgery at 1 mm spatial resolution, including activity induced by direct electrical stimulation. Collectively, these findings demonstrate the power of the PtNRGrids to transform clinical mapping and research with brain-machine interfaces and highlights a path toward novel therapeutics. Copyright © 2021, The Authors. All rights reserved.

关键词： Mapping