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Degradation of carbamazepine by the UVA-LED_(365)/ClO_(2)/NaClO process:Kinetics,mechanisms and DBPs yield

Journal of Environmental Sciences 2025年第2期148卷 399-408页

作者： Chenyan Hu Yihui Wu Zhengyu Dong Ziyi Dong Shengjie Ji Lili Hu Xinyu Yang Hao Liu College of Environmental and Chemical Engineering Shanghai Engineering Research Center of EnergySaving in Heat Exchange SystemsShanghai University of Electric PowerShanghai 200090China Shanghai Institute of Pollution Control and Ecological Security Shanghai 200092China

A mixed oxidant of chlorine dioxide(ClO_(2))and NaClO was often used in water treatment.A novel UVA-LED(_(365) nm)-activated mixed ClO_(2)/NaClO process was proposed for the degradation of micropollutants in this ***(CBZ)was selected as the target *** with the UVA_(365)/ClO_(2) process,the UVA_(365)/ClO_(2)/NaClO process can improve the degradation of CBZ,with the rate constant increasing from 2.11×10^(−4) sec^(−1) to 2.74×10^(−4) sec^(−1).In addition,the consumption of oxidants in the UVA_(365)/ClO_(2)/NaClO process(73.67%)can also be lower than that of UVA_(365)/NaClO(86.42%).When the NaClO ratio increased,both the degradation efficiency of CBZ and the consumption of oxidants can increase in the UVA_(365)/ClO_(2)/NaClO *** solution pH can affect the contribution of NaClO in the total oxidant *** the pH range of 6.0-8.0,the combination process can generate more active species to promote the degradation of *** change of active species with oxidant molar ratio was investigated in the UVA_(365)/ClO_(2)/NaClO *** ClO_(2) acted as the main oxidant,HO·and Cl·were the main active species,while when NaClO was the main oxidant,ClO·played a role in the *** chloride ion(Cl^(-)),bicarbonate ion(HCO_(3)^(-)),and nitrate ion(NO_(3)^(-))can promote the reaction *** the concentration of NaClO in the reaction solution increased,the generation of chlorates will *** UVA_(365)/ClO_(2)/NaClO process can effectively control the formation of volatile disinfection by-products(DBPs),and with the increase of ClO_(2) dosage,the formation of DBPs can also decrease.

关键词： UVA Chlorine dioxide(ClO_(2)) NaClO Carbamazepine(CBZ) Disinfection by-products

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Time-Varying Formation Tracking control of Heterogeneous Multi-Agent systems With Intermittent Communications and Directed Switching Networks

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IEEE/CAA Journal of Automatica Sinica 2025年第1期12卷 294-296页

作者： Yuhan Wang Zhuping Wang Hao Zhang Huaicheng Yan the Shanghai Research Institute for Intelligent Autonomous Systems Tongji University the National Key Laboratory of Autonomous Intelligent Unmanned Systems the Frontiers Science Center for Intelligent Autonomous System of Ministry of Education the College of Electronic and Information Engineering the Department of Control Science and Engineering Tongji University the Key Laboratory of Advanced Control and Optimization for Chemical Processes of Ministry of Education the School of Information Science and Engineering East China University of Science and Technology

Dear Editor,This letter is concerned with the problem of time-varying formation tracking for heterogeneous multi-agent systems(MASs) under directed switching networks. For this purpose, our first step is to present so... 详细信息

关键词： Switches Topology Observers Formation control Event detection Switched systems Multi-agent systems control theory Autonomous systems Stability

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Observer-based stabilization for discrete nonlinear semi-Markov jump singularly perturbed models with mode-switching delay

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Science China(Information Sciences) 2025年第4期68卷 389-390页

作者： Wenhai QI Runkun LI Ju H.PARK Zheng-Guang WU Huaicheng YAN School of Engineering Qufu Normal University Department of Electrical Engineering Yeungnam University Institute of Cyber-Systems and Control Zhejiang University Key Laboratory of Smart Manufacturing in Energy Chemical Process of Ministry of Education East China University of Science and Technology

Semi-Markov jump systems(S-MJMs) not only characterize hybrid systems but also address the limitations of Markov jump systems(MJMs) [1–3]. Due to their ability to exhibit multi-time-scale features, singularly perturbed models(SPMs) effectively model practical systems influenced by multiple time-scale phenomena [4]. In this study, the observer-based output feedback controller is asynchronous with the original system due to the time delay in the controller mode switching. A nonlinear plant with singularly perturbed parameters(SPPs) is represented using an interval type-2(IT2) fuzzy model [5].

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Two-tier control structure design methodology applied to heat exchanger networks

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Chinese Journal of chemical engineering 2022年第7期35卷 231-244页

作者： Siwen Gu Lei Zhang Yu Zhuang Weida Li Jian Du Cheng Shao Institute of Chemical Process Systems Engineering School of Chemical EngineeringDalian University of TechnologyDalian 116024China Jiangsu Collaborative Innovation Center for Cultural Creativity School of Photoelectric EngineeringChangzhou Institute of TechnologyChangzhou 213032China Institute of Advanced Control Technology School of Control Science and EngineeringDalian University of TechnologyDalian 116024China

Because of its paramount importance in the successful industrial control strategy of a given heat exchanger network(HEN),the control structure designs for providing appropriate manipulated variable(MV)and controlled variable pairings have received considerable ***,quite frequently HENs with such control structures face the problem of hard constraints,typically holding the HENs at less controlled operating *** both the MV pairings and the above control pairings should be considered to design a control *** paper investigates the systematic incorporation of the two pairings,and presents a methodology for designing such two-tier control *** is developed based on the sequential strategy,coupling an indirect-tier with direct-tier control structure design,wherein the intention is realized in the former stage and the latter is implemented for further *** MV identification and pairing are achieved through variations in heat load of heat exchangers to design the indirect-tier control *** the direct-tier control structure is followed the relative gain array pairing *** the proposed methodology,on the one hand,it generates an explicit connection between the MV pairings and the HEN configuration,and the quantitative interaction measure is improved to avoid the multiple solutions to break the relationship among all the control pairings into individuals;on the other hand,a two-tier control structure reveals control potentials and control system design requirements,this may avoid complex and economically unfavourable control and HEN *** application of proposed framework is illustrated with two cases involving the dynamic simulation analysis,the quantitative assessment and the random test.

关键词： Heat exchanger networks(HENs) controllability Two-tier control structure Manipulated variable pairing control pairing

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Stability and Performance Analysis of Model Predictive control of Uncertain Linear systems 63

Stability and Performance Analysis of Model Predictive Contr...

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63rd IEEE Conference on Decision and control, CDC 2024

作者： Liu, Changrui Shi, Shengling De Schutter, Bart Delft University of Technology Delft Center for Systems and Control Delft Netherlands Massachusetts Institute of Technology Department of Chemical Engineering Cambridge United States

ISBN: (纸本)9798350316339

Model mismatch often presents significant challenges in model-based controller design. This paper investigates model predictive control (MPC) for uncertain linear systems with input constraints, where the uncertainty is characterized by a parametric mismatch between the true system and its estimated model. The main contributions of this work are twofold. First, a theoretical performance bound is derived using relaxed dynamic programming. This bound provides a novel insight into how the prediction horizon and modeling errors affect the suboptimality of the MPC controller to the oracle infinite-horizon optimal controller, which has complete knowledge of the true system. Second, sufficient conditions are established under which the nominal MPC controller, which relies solely on the estimated system model, can stabilize the true system despite model mismatch. Numerical simulations are presented to validate these theoretical results, demonstrating the practical applicability of the derived conditions and bounds. These findings offer practical guidelines for achieving desired modeling accuracy and selecting an appropriate prediction horizon in designing certainty-equivalence MPC controllers for uncertain linear systems. © 2024 IEEE.

关键词： Predictive control systems

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Imitation Learning of MPC with Neural Networks: Error Guarantees and Sparsification 63

Imitation Learning of MPC with Neural Networks: Error Guaran...

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63rd IEEE Conference on Decision and control, CDC 2024

作者： Alsmeier, Hendrik Theiner, Lukas Savchenko, Anton Mesbah, Ali Findeisen, Rolf Technical University of Darmstadt Control and Cyber-Physical Systems Laboratory Germany University of California Dept of Chemical & Biomolecular Engineering Berkeley United States

ISBN: (纸本)9798350316339

This paper presents a framework for bounding the approximation error in imitation model predictive controllers utilizing neural networks. Leveraging the Lipschitz properties of these neural networks, we derive a bound that guides dataset design to ensure the approximation error remains at chosen limits. We discuss how this method can be used to design a stable neural network controller with performance guarantees employing existing robust model predictive control approaches for data generation. Additionally, we introduce a training adjustment, which is based on the sensitivities of the optimization problem and reduces dataset density requirements based on the derived bounds. We verify that the proposed augmentation results in improvements to the network's predictive capabilities and a reduction of the Lipschitz constant. Moreover, on a simulated inverted pendulum problem, we show that the approach results in a closer match of the closed-loop behavior between the imitation and the original model predictive controller. © 2024 IEEE.

关键词： Predictive control systems

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Degradation kinetics and disinfection by-products formation of benzophenone-4 during UV/persulfate process

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Environmental Technology (United Kingdom) 2024年第26期45卷 5618-5629页

作者： Hu, Chen-Yan Xiong, Cun Lin, Yi-Li Zhang, Tian-Yang College of Environmental and Chemical Engineering Shanghai Engineering Research Center of Energy-Saving in Heat Exchange Systems Shanghai University of Electric Power Shanghai China Shanghai Institute of Pollution Control and Ecological Security Shanghai China Department of Safety Health and Environmental Engineering National Kaohsiung University of Science and Technology Kaohsiung Taiwan State Key Laboratory of Pollution Control and Resources Reuse Key Laboratory of Yangtze Water Environment Ministry of Education College of Environmental Science and Engineering Tongji University Shanghai China

The degradation kinetics, reaction pathways, and disinfection by-products formation of an organic UV filter, benzophenone-4 (BP4) during UV/persulfate oxidation were investigated. BP4 can hardly be degraded by UV alone, but can be effectively decomposed by UV/persulfate following pseudo-first order kinetics. BP4 degradation rate was enhanced with increasing persulfate dosage and decreasing pH from 8 to 5. However, the degradation rate of BP4 at pH 9 was higher than that at pH 8 because of the presence of phenolic group in BP4 structure. and (Formula presented.) were confirmed as the major contributors to BP4 decomposition in radical scavenging experiments, and the second-order rate constants between (Formula presented.) and BP4 as well as those between (Formula presented.) and BP4 were estimated by establishing and solving a kinetic model. The presence of (Formula presented.) and humic acid inhibited the decomposition of BP4, while (Formula presented.) promoted it. The mineralisation of BP4 was only 9.1% at the persulfate concentration of 50 μM. Six degradation intermediates were identified for the promulgation of the reaction pathways of BP4 during UV/persulfate oxidation were proposed as a result. In addition, the formation of DBP in the sequential chlorination was evaluated at different persulfate dosages, pH values, and water matrix. The results of this study can provide essential knowledge for the effective control of DBP formation with reducing potential hazard to provide safe drinking water to the public. © 2023 Informa UK Limited, trading as Taylor & Francis Group.

关键词： Rate constants

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MATD3-Based End-Edge Collaborative Resource Optimization for NOMA-Assisted Industrial Wireless Networks

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Computers, Materials & Continua 2025年第2期82卷 3203-3222页

作者： Ru Hao Chi Xu Jing Liu College of Information Engineering Shenyang University of Chemical TechnologyShenyang110142China State Key Laboratory of Robotics Shenyang Institute of AutomationChinese Academy of SciencesShenyang110016China Key Laboratory of Networked Control Systems Chinese Academy of SciencesShenyang110016China

Non-orthogonal multiple access (NOMA) technology has recently been widely integrated into multi-access edge computing (MEC) to support task offloading in industrial wireless networks (IWNs) with limited radio resources. This paper minimizes the system overhead regarding task processing delay and energy consumption for the IWN with hybrid NOMA and orthogonal multiple access (OMA) schemes. Specifically, we formulate the system overhead minimization (SOM) problem by considering the limited computation and communication resources and NOMA efficiency. To solve the complex mixed-integer nonconvex problem, we combine the multi-agent twin delayed deep deterministic policy gradient (MATD3) and convex optimization, namely MATD3-CO, for iterative optimization. Specifically, we first decouple SOM into two sub-problems, i.e., joint sub-channel allocation and task offloading sub-problem, and computation resource allocation sub-problem. Then, we propose MATD3 to optimize the sub-channel allocation and task offloading ratio, and employ the convex optimization to allocate the computation resource with a closed-form expression derived by the Karush-Kuhn-Tucker (KKT) conditions. The solution is obtained by iteratively solving these two sub-problems. The experimental results indicate that the MATD3-CO scheme, when compared to the benchmark schemes, significantly decreases system overhead with respect to both delay and energy consumption.

关键词： Industrial wireless networks(IWNs) multi-access edge computing(MEC) non-orthogonal multiple access(NOMA) task offloading resource allocation

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Efficient and Safe Learning-based control of Piecewise Affine systems Using Optimization-Free Safety Filters 63

Efficient and Safe Learning-based Control of Piecewise Affin...

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63rd IEEE Conference on Decision and control, CDC 2024

作者： He, Kanghui Shi, Shengling Van Den Boom, Ton De Schutter, Bart Delft University of Technology Delft Center for Systems and Control Delft Netherlands Massachusetts Institute of Technology Department of Chemical Engineering CambridgeMA United States

ISBN: (纸本)9798350316339

control of piecewise affine (PWA) systems under complex constraints faces challenges in guaranteeing both safety and online computational efficiency. Learning-based methods can rapidly generate control signals with good performance, but rarely provide safety guarantees. A safety filter is a modular method to improve safety for any controller. When applied to PWA systems, a traditional safety filter usually need to solve a mixed-integer convex program, which reduces the computational benefit of learning-based controllers. We propose a novel optimization-free safety filter designed to handle state constraints that involve a combination of polyhedra and ellipsoids. The proposed safety filter only utilizes algebraic and min-max operations to determine safe control inputs. This offers a notable advantage compared with traditional safety filters by allowing for significantly more efficient computation of control signals. The proposed safety filter can be integrated into various function approximators, such as neural networks, enabling safe learning throughout the learning process. Simulation results on a bicycle model with PWA approximation validate the proposed method regarding constraint satisfaction, CPU time, and the preservation of sub-optimality. © 2024 IEEE.

关键词： Integer programming

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Progresses on two-phase modeling of proton exchange membrane water electrolyzer

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Energy Reviews 2024年第3期3卷 30-57页

作者： Boshi Xu Tao Ouyang Yang Wang Yang Yang Jun Li Liangliang Jiang Chaozhong Qin Dingding Ye Rong Chen Xun Zhu Qiang Liao Key Laboratory of Low-grade Energy Utilization Technologies and Systems Ministry of EducationChongqing UniversityChongqing400030China Institute of Engineering Thermophysics School of Energy and Powering EngineeringChongqing UniversityChongqing400030China Department of Chemical and Petroleum Engineering The University of CalgaryCalgaryAlbertaCanada State Key Laboratory of Coal Mine Disaster Dynamics and Control Chongqing UniversityChongqing400044China

The Proton Exchange Membrane(PEM)water electrolyzer is considered one of the promising energy storing means for harnessing variable renewable energy sources to produce *** the internal fluid dynamics,which are often challenging to directly observe experimentally,has prompted the use of numerical models to investigate two-phase flow within PEM water *** this study,we provide a comprehensive review of prior research focusing on two-phase modeling of PEM electrolyzers,encompassing both components at mesoscopic scales and the full electrolyzer at the macroscopic *** delve into the specifics of various modeling approaches for two-phase flow at different scales and summarize and discuss the current state of the art in the ***,two-phase models for the full electrolyzer predominantly employ a macroscopic homogeneous ***,mesoscopic and microscopic models capable of tracking phase interfaces are limited to *** persist in integrating various modeling scales into a comprehensive electrolyzer model,particularly in coupling two-phase flow between the channels and porous *** efforts should focus on developing multi-scale models and simulating two-phase flow under fluctuating input ***,given the structural similarities between PEM water electrolyzers and PEM fuel cells,we compare and discuss differences in two-phase modeling between the two *** work offers the insights for researchers in the field of modeling of PEM water electrolyzers and even fuel cells.

关键词： Proton exchange membrane(PEM)water electrolyzer Two-phase model Multiscale modeling Water management Numerical simulation

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