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Correction to: Environmental consequences of interacting effects of changes in stratospheric ozone, ultraviolet radiation, and climate: UNEP Environmental Effects Assessment Panel, Update 2024 (Photochemical & Photobiological sciences, (2025), 24, 3, (357-392), 10.1007/s43630-025-00687-x)

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Photochemical and Photobiological sciences 2025年第5期24卷 863-865页

作者： Neale, Patrick J. Hylander, Samuel Banaszak, Anastazia T. Häder, Donat-P. Rose, Kevin C. Vione, Davide Wängberg, Sten-Åke Jansen, Marcel A. K. Busquets, Rosa Andersen, Mads P. Sulbæk Madronich, Sasha Hanson, Mark L. Schikowski, Tamara Solomon, Keith R. Sulzberger, Barbara Wallington, Timothy J. Heikkilä, Anu M. Pandey, Krishna K. Andrady, Anthony L. Bruckman, Laura S. White, Christopher C. Zhu, Liping Bernhard, Germar H. Bais, Alkiviadis Aucamp, Pieter J. Chiodo, Gabriel Cordero, Raúl R. Petropavlovskikh, Irina Neale, Rachel E. Olsen, Catherine M. Hales, Simon Lal, Aparna Lingham, Gareth Rhodes, Lesley E. Young, Antony R. Robson, T. Matthew Robinson, Sharon A. Barnes, Paul W. Bornman, Janet F. Harper, Anna B. Lee, Hanna Calderón, Roy Mackenzie Ossola, Rachele Paul, Nigel D. Revell, Laura E. Wang, Qing-Wei Zepp, Richard G. Environmental Research Center Smithsonian Institution EdgewaterMD United States Centre for Ecology and Evolution in Microbial Model Systems Linnaeus University Kalmar Sweden Unidad Académica de Sistemas Arrecifales Universidad Nacional Autónoma de México Puerto Morelos Mexico Erlangen Germany Department of Biological Sciences and Department of Civil and Environmental Engineering Rensselaer Polytechnic Institute TroyNY United States Department of Chemistry University of Turin Turin Italy Department of Marine Sciences University of Gothenburg Gotheburg Sweden School of Biological Earth and Environmental Sciences Environmental Research Institute University College Cork Cork Ireland Chemical and Pharmaceutical Sciences Kingston University London Kingston Upon Thames United Kingdom Civil Environmental & Geomatic Engineering University College London London United Kingdom Department of Chemistry and Biochemistry California State University NorthridgeCA United States Atmospheric Chemistry Observations and Modeling National Center for Atmospheric Research BoulderCO United States USDA UV-B Monitoring and Research Program Colorado State University Fort. CollinsCO United States Department of Environment and Geography University of Manitoba WinnipegMB Canada Working Group Environmental Epidemiology IUF-Leibniz Research Institute for Environmental Medicine Düsseldorf Germany Department of Environment and Health School of Public Health University of Bielefeld Bielefeld Germany School of Environmental Sciences University of Guelph GuelphON Canada Retired From Eawag Swiss Federal Institute of Aquatic Science and Technology Dübendorf Switzerland Center for Sustainable Systems School for Environment and Sustainability University of Michigan Ann ArborMI United States Climate Research Finnish Meteorological Institute Helsinki Finland Indian Academy of Wood Science Bengaluru India Chemical and Biomolecular Engineering North Carolina State University RaleighN

This work is not a product of the U.S. Government or the U.S. Environmental Protection Agency, and the author is not doing this work in any governmental capacity. This research was not performed or funded by EPA and was not subject to EPA’s quality system requirements. The views expressed in this journal article are those of the author(s) and do not necessarily represent the views or the policies of the U.S. Environmental Protection Agency. The original article has been corrected. © The Author(s), under exclusive licence to the European Photochemistry Association, European Society for Photobiology 2025.

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Lattice Induced Short-Range Attraction between Like-Charged Colloidal Particles

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physical Review Letters 2022年第1期129卷 018002-018002页

作者： Peng Liu Luhui Ning Yiwu Zong Fangfu Ye Mingcheng Yang Ke Chen Beijing National Laboratory for Condensed Matter Physics and Laboratory of Soft Matter Physics Institute of Physics Chinese Academy of Sciences Beijing 100190 China School of Physical Sciences University of Chinese Academy of Sciences Beijing 100049 China Wenzhou Institute University of Chinese Academy of Sciences Wenzhou Zhejiang 325001 China Frontiers Science Center for Synthetic Biology and Key Laboratory of Systems Bioengineering (Ministry of Education) School of Chemical Engineering and Technology Tianjin University Tianjin 300072 China Songshan Lake Materials Laboratory Dongguan Guangdong 523808 China

We perform experiments and computer simulations to study the effective interactions between like-charged colloidal tracers moving in a two-dimensional fluctuating background of colloidal crystal. By a counting method that properly accounts for the configurational degeneracy of tracer pairs, we extract the relative probability of finding a tracer pair in neighboring triangular cells formed by background particles. We find that this probability at the nearest neighbor cell is remarkably greater than those at cells with larger separations, implying an effective attraction between the tracers. This effective attraction weakens sharply as the background lattice constant increases. Furthermore, we clarify that the lattice-mediated effective attraction originates from the minimization of free energy increase from deformation of the crystalline background due to the presence of diffusing tracers.

关键词： Depletion interactions Diffusion Fluctuation mediated interactions Charged colloids Colloidal crystal Brownian dynamics Optical microscopy

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Influence of preparation techniques on the structural and electrical properties of PVdF-HFP/P123 blend polymer membranes for energy storage applications

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Applied Surface science Advances 2024年 20卷

作者： S, Pavithra Moorthy, Sasikumar S, Pauline Sheeba A, Brusly Solomon P, Senthil Kumar A, Sakunthala Solid State Ionics Lab Division of Physical Sciences Karunya Institute of Technology and Sciences Tamil Nadu Coimbatore 641114 India PG & Research Department of Physics Bishop Heber College (Affiliated to Bharathidasan University) Tamil Nadu Tiruchirapalli 620017 India Department of Mechanical Engineering Centre for Research in Material Science and Thermal Management Karunya Institute of Technology and Sciences Tamil Nadu Coimbatore 641114 India Department of Chemical Engineering National Taiwan University Taipei 10617 Taiwan

Exploration of blend polymer membrane with desire performances is a highly essential research topic because it makes them as key component of the battery technologies. However, the blend membrane cannot simultaneously meet out the high electrical insulation and ion conductivity. Here, we report porous PVdF-HFP based polymer membrane blended with P123 polymer which is prepared by phase inversion technique and along with solution casting technique for comparison. Especially, the major improvements can be claimed with porous PVdF-HFP blend with P123 matrix by phase inversion process that could be mainly due to increasing the disorganize crystallinity of the PVdF-HFP, thereby enhancing the ionic conductivity of PVdF-HFP/P123 than the same prepared by traditional solution casting. More importantly, our studies reveals that, besides having an effect of crystallinity and high ionic conduction PVdF-HFP/P123 blend matrix yield homogeneous pores with higher pore density when prepared by phase inversion approach. We attribute this to remarkable enhancement in higher electrolyte uptake and higher cation transport in the blend membrane. This facilitates high ionic conductivity of 7.06 × 10⁻⁵ S/cm and electrochemical stability of 2.8 V,while the solution casting approach display low ionic conductivity of 1.63 × 10⁻⁶ S/cm and electrochemical stability of 2.2 V, respectively. A symmetric supercapacitor device is fabricated with the membrane prepared by phase inversion process, resulting in a high specific capacitance of 80 F/g at the current density of 0.25 A/g with 90.51% specific capacitance retention at 0.5 A/g. The energy density of 90.9 W/kg can be achieved at the power density of 0.375 W/kg. © 2024 The Authors

关键词： P123 Phase inversion Polymer blend membranes PVdF-HFP Solution casting

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Hydrogen-Bond Induced Enhanced Emission Ratiometric Fluorescent Handy Pen for Visualization Assay of Amoxicillin

SSRN

引用

SSRN 2022年

作者： Jiang, Changlong Li, Lingfei Yang, Liang Lin, Dan Xu, Shihao Mei, Chunsheng Yu, Shaoming School of Chemistry and Chemical Engineering Hefei University of Technology Anhui Hefei230009 China Institute of Solid State Physics Hefei Institutes of Physical Science Chinese Academy of Sciences Anhui Hefei230031 China State Key Laboratory of Transducer Technology Chinese Academy of Sciences Anhui Hefei230031 China

Amoxicillin (AMO) is one of the most used antibiotics, and its abuse in animal husbandry or clinical therapy can cause unpredictable hazard to human. Therefore, it is crucial to develop a real-time and rapid method to give accurate content of AMO. Here, we designed a fluorescent nanoprobe for qualitative and quantitative AMO by using as-synthesized green safe material of nontoxic red carbon dots (RCDs) and blue carbon dots (BCDs). In the presence of AMO, the hydrogen bond enhancement reaction occurred immediately, resulting in instant intensity increasement of the blue fluorescence of BCDs, accompanied with a marked color changed from red to blue. Considering the practical application, we further design a non-toxic sensing fluorescent handy pen that can intuitively and quantitatively detect AMO in real sample. The portable and easy-to-use device can be demonstrated on a smartphone platform based on 3D printing technology, with the advantages of simple production, excellent visualization, fast response, and instant quantitative performance. Meanwhile, the detection time is extremely short with a sensitive detection limit of 2.39 nM. The method presented here enables real-time assessment of food safety as well as on-site detection under field conditions to track various trace substances for timely health checks. © 2022, The Authors. All rights reserved.

关键词： Smartphones

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Ratiometric Fluorescent Sensor for Shutter-Speedy and Ultra-Sensitive Monitoring of Antibiotic Utilizing Multiple Fluorescent Devices

SSRN

引用

SSRN 2022年

作者： Li, Lingfei Lin, Dan Xu, Shihao Yang, Liang Yu, Shaoming Jiang, Changlong Institute of Solid State Physics Hefei Institutes of Physical Science Chinese Academy of Sciences Anhui Hefei230031 China School of Chemistry and Chemical Engineering Hefei University of Technology Anhui Hefei230009 China State Key Laboratory of Transducer Technology Chinese Academy of Sciences Anhui Hefei230031 China

Sensitive and rapid sensing is extremely vital to in-situ monitor trace chemicals, herein, multiple visual devices have been developed to ultra-sensitively screen antibiotic oxytetracyline (OTC) with shutter-speed. The calcium ion fixed on the nanoprobe sensitively and rapidly coordinates to the hydroxyl group of OTC due to its special electronic orbital structure, resulting in evolutive visual distinct color change from red to bright green within a shutter pressing ( © 2022, The Authors. All rights reserved.

关键词： Fluorescence

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Model-Free Measurement of Local Entropy Production and Extractable Work in Active Matter

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physical Review Letters 2022年第22期129卷 220601-220601页

作者： Sunghan Ro Buming Guo Aaron Shih Trung V. Phan Robert H. Austin Dov Levine Paul M. Chaikin Stefano Martiniani Department of Physics Technion-Israel Institute of Technology Haifa 3200003 Israel Center for Soft Matter Research Department of Physics New York University New York 10003 USA Courant Institute of Mathematical Sciences New York University New York 10003 USA Department of Chemical Engineering and Materials Science University of Minnesota Minneapolis Minnesota 55455 USA Department of Physics Princeton University Princeton 08544 New Jersey USA Simons Center for Computational Physical Chemistry Department of Chemistry New York University New York 10003 USA

Time-reversal symmetry breaking and entropy production are universal features of nonequilibrium phenomena. Despite its importance in the physics of active and living systems, the entropy production of systems with many degrees of freedom has remained of little practical significance because the high dimensionality of their state space makes it difficult to measure. Here we introduce a local measure of entropy production and a numerical protocol to estimate it. We establish a connection between the entropy production and extractability of work in a given region of the system and show how this quantity depends crucially on the degrees of freedom being tracked. We validate our approach in theory, simulation, and experiments by considering systems of active Brownian particles undergoing motility-induced phase separation, as well as active Brownian particles and *** in a rectifying device in which the time-reversal asymmetry of the particle dynamics couples to spatial asymmetry to reveal its effects on a macroscopic scale.

关键词： Dynamical phase transitions Nonequilibrium statistical mechanics Stochastic thermodynamics Active brownian particles Active matter Bacteria Information theory

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Reconstructing Anode/Electrolyte Interface Towards High Stable Zinc Anode

SSRN

引用

SSRN 2022年

作者： Wei, Tingting Zhang, Xianxi Ren, Yingke Wang, Yifan Li, Zhaoqian Zhang, Hong Hu, Linhua Key Laboratory of Photovoltaic and Energy Conservation Materials CAS Institute of Solid State Physics Hefei Institutes of Physical Science Chinese Academy of Sciences Anhui Hefei230031 China Shandong Provincial Key Laboratory Collaborative Innovation Center of Chemical Energy Storage & Novel Cell Technology School of Chemistry and Chemical Engineering Liaocheng University Liaocheng252000 China College of Science Hebei University of Science and Technology Shijiazhuang050018 China School of Mathematics and Physics Science and Engineering Hebei University of Engineering Handan Hebei056038 China University of Science and Technology of China Anhui Hefei230026 China

The dendrite growth and side-reactions at unstable anode/electrolyte interface severely impair the electrochemical performance of aqueous zinc-ion battery. Herein, guided by the metal-coordination chemistry, a multifunctional electrolyte additive, sulfolane (SL), is introduced into aqueous ZnSO4 electrolyte to achieve uniform Zn deposition for highly stable and reversible zinc-ion batteries. Experimental results and theoretical calculations prove that the SL molecules can simultanously modulate Zn2+ solvation structure and anode/electrolyte interface. The electrolyte engineering is capable of modulating the primary solvation structure through expelling some active water to mitigate common parasitic reaction. Concomitantly, SL molecules are inclined to adsorb on the Zn metal surface, forming H2O-poor electrical double layer and regulating the nucleation and growth of Zn, leading to the alleviated side-reactions induced by water and uniform Zn deposition. Benefiting from this versatility, the batteries exhibit high reversibility with 99.64% coulombic efficiency and outstanding stability (over 600 h at 10 mA·cm-2/10 mAh·cm-2). Even cycled at harsh conditions of 20 mA·cm-2/20 mAh·cm-2, the remarkable stability of 100 h is obtained. The Zn//V2O5 full battery delivers high specific capacity of 249 mAh g-1 with capacity retention of 87.1% after 5000 cycles. © 2022, The Authors. All rights reserved.

关键词： Electrolytes

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Performance of joint gamma-ray observations with MAGIC and LST-1 telescopes 38

Performance of joint gamma-ray observations with MAGIC and L...

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38th International Cosmic Ray Conference, ICRC 2023

作者： Di Pierro, F. Berti, A. de Menezes, R. Jobst, E. Ohtani, Y. Sitarek, J. Suda, Y. Visentin, E. Abe, H. Abe, K. Abe, S. Abhir, J. Acciari, V.A. Aguasca-Cabot, A. Agudo, I. Alvarez Crespo, N. Aniello, T. Ansoldi, S. Antonelli, L.A. Aramo, C. Arbet-Engels, A. Cornelia, A. Artero, M. Asano, K. Aubert, P. Baack, D. Babić, A. Baktash, A. Bamba, A. Baquero Larriva, A. Baroncelli, L. Barres de Almeida, U. Barrio, J.A. Batkovic, I. Baxter, J. Becerra González, J. Bednarek, W. Bernardini, E. Bernardos, M.I. Bernete Medrano, J. Besenrieder, J. Bhattacharjee, P. Biederbeck, N. Bigongiari, C. Biland, A. Bissaldi, E. Blanch, O. Bonnoli, G. Bordas, P. Bošnjak, Ž. Bulgarelli, A. Burelli, I. Burmistrov, L. Buscemi, M. Busetto, G. Campoy-Ordaz, A. Cardillo, M. Caroff, S. Carosi, A. Carosi, R. Carrasco, M.S. Carretero-Castrillo, M. Cassol, F. Castro-Tirado, A.J. Cauz, D. Cerasole, D. Ceribella, G. Chai, Y. Cheng, K. Chiavassa, A. Chikawa, M. Chilingarian, A. Chytka, L. Cifuentes, A. Cikota, S. Colombo, E. Contreras, J.L. Cortina, J. Costantini, H. Covino, S. D’Amico, G. Dalchenko, M. D’Elia, V. Da Vela, P. Dazzi, F. De Angelis, A. de Bony de Lavergne, M. De Lotto, B. De Lucia, M. de Menezes, R. Del Peral, L. Deleglise, G. Delfino, M. Delgado, C. Delgado Mengual, J. della Volpe, D. Dellaiera, M. Del Popolo, A. Depaoli, D. Di Piano, A. Di Pierro, F. Di Pilato, A. Di Tria, R. Di Venere, L. Díaz, C. Dominik, R.M. Dominis Prester, D. Donini, A. Dorner, D. Doro, M. Eisenberger, L. Elsässer, D. Emery, G. Escudero, J. Fallah Ramazani, V. Fariña, L. Fattorini, A. Ferrara, G. Ferrarotto, F. Fiasson, A. Foffano, L. Font, L. Freixas Coromina, L. Fröse, S. Fukami, S. Fukazawa, Y. Garcia, E. Garcia López, R. Garczarczyk, M. Gasbarra, C. Gasparrini, D. Gasparyan, S. Gaug, M. Geyer, D. Giesbrecht Paiva, J. Giglietto, N. Giordano, F. Gliwny, P. Godinovic, N. Grau, R. Green, J. Green, D. Gunji, S. Günther, P. Hackfeld, J. Hadasch, D. Hahn, A. Hashiyama, K. Hassan, T. Hayashi, K. INFN Torino Via P. Giuria 1 Torino Italy Max-Planck-Institut für Physik Föhringer Ring 6 München Germany Università degli Studi di Torino Dipartimento di Fisica Via P. Giuria 1 Torino Italy University of Tokyo Institute for Cosmic Ray Research 5-1-5 Kashiwa-no-ha Chiba Kashiwa277-8582 Japan University of Lodz Faculty of Physics and Applied Informatics ul. Pomorska 149-153 Lodz Poland Hiroshima University Physics Program Graduate School of Advanced Science and Engineering Hiroshima739-8526 Japan Department of Physics Tokai University Japan ETH Zürich Switzerland Instituto de Astrofísica de Canarias Departamento de Astrofísica Universidad de La Laguna Spain Departament de Física Quàntica i Astrofísica Institut de Ciències del Cosmos Universitat de Barcelona IEEC-UB Spain Instituto de Astrofísica de Andalucía-CSIC Spain EMFTEL department IPARCOS Universidad Complutense de Madrid Spain Italy INFN Sezione di Trieste Università degli Studi di Udine Italy Italy INAF - Osservatorio Astronomico di Roma Italy INFN Sezione di Napoli Italy INFN Sezione di Padova Università degli Studi di Padova Italy The Barcelona Institute of Science and Technology Spain LAPP Univ. Grenoble Alpes Univ. Savoie Mont Blanc CNRS-IN2P3 Annecy France Department of Physics TU Dortmund University Germany Croatia Universität Hamburg Institut für Experimentalphysik Germany Graduate School of Science University of Tokyo Japan Universidad del Azuay Ecuador INAF - Osservatorio di Astrofisica e Scienza dello spazio di Bologna Italy Centro Brasileiro de Pesquisas Físicas Brazil CIEMAT Spain INFN Sezione di Bari Politecnico di Bari Italy INAF - Osservatorio Astronomico di Brera Italy University of Geneva Département de physique nucléaire et corpusculaire Switzerland INFN Sezione di Catania Italy Departament de Física CERES-IEEC Universitat Autónoma de Barcelona Spain Italy Università di Pisa INFN Pisa Italy Aix Marseille Univ CNRS IN2P3 CPPM France INFN Sezione di Bari

The prototype Large-Sized Telescope (LST-1) of the Cherenkov Telescope Array Observatory (CTAO) is in commissioning phase at the Observatorio del Roque de Los Muchachos at 2200 m a.s.l. in La Palma (Canary Islands, Spain). LST-1 is a 23-m diameter telescope and is the first of four that will compose the LST part of the CTAO Northern array. The LST subarray is optimized to provide the best sensitivity for gamma rays in the 20 GeV - 200 GeV energy range. The MAGIC telescopes, which are located approximately 100 m from the LST-1, is operating as a two 17-m telescope stereoscopic system for more than 14 years. LST-1 and MAGIC routinely perform joint observations of gamma-ray sources to exploit the potential of the three-telescope system. This contribution describes the analysis pipeline and evaluates the performance of the system using Monte Carlo simulations and data on the Crab Nebula. The sensitivity achieved during joint observations with MAGIC and LST-1 is about 30% higher than that of MAGIC alone. © Copyright owned by the author(s) under the terms of the Creative Commons.

关键词： Stereo image processing

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Imaging interstitial atoms with multislice electron ptychography

arXiv

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arXiv 2024年

作者： Chen, Zhen Shao, Yu-Tsun Zeltmann, Steven E. Harikrishnan, K.P. Rosenberg, Ethan R. Ross, Caroline A. Jiang, Yi Muller, David A. Beijing National Laboratory for Condensed Matter Physics Institute of Physics Chinese Academy of Sciences Beijing100190 China School of Physical Sciences University of Chinese Academy of Sciences Beijing100049 China Mork Family Department of Chemical Engineering and Materials Science University of Southern California Los AngelesCA90089 United States Platform for the Accelerated Realization Analysis and Discovery of Interface Materials Cornell University IthacaNY14853 United States School of Applied and Engineering Physics Cornell University IthacaNY14853 United States Department of Materials Science and Engineering Massachusetts Institute of Technology CambridgeMA02139 United States Advanced Photon Source Argonne National Laboratory LemontIL60439 United States Kavli Institute Cornell for Nanoscale Science IthacaNY14853 United States

Doping impurity atoms is a strategy commonly used to tune the functionality of materials including catalysts, semiconductors, and quantum emitters. The location of dopants and their interaction with surrounding atoms could significantly modulate the transport, optical, or magnetic properties of materials. However, directly imaging individual impurity atoms inside materials remains a generally unaddressed need. Here, we demonstrate how single atoms can be detected and located in three dimensions via multislice electron ptychography. Interstitial atoms in a complex garnet oxide heterostructure are resolved with a depth resolution better than 2.7 nm, together with a deep-sub-Ångstrom lateral resolution. Single-scan atomic-layer depth resolution should be possible using strongly divergent electron probe illumination. Our results provide a new approach to detecting individual atomic defects and open doors to characterize the local environments and spatial distributions that underlie a broad range of systems such as single-atom catalysts, nitrogen-vacancy centers, and other atomic-scale quantum sensors. © 2024, CC BY.

关键词： Catalysts

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Preferential bond formation and interstitial/vacancy annihilation rate drive atomic clustering in gallium ion sputtered compound materials

arXiv

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arXiv 2023年

作者： Ma, Zhenyu Zhang, Xin Liu, Pu Deng, Yong Hu, Wenyu Chen, Longqing Zhu, Jun Chen, Sen Wang, Zhengshang Shi, Yuechun Ma, Jian Wang, Xiaoyi Qiu, Yang Zhang, Kun Cui, Xudong Walther, Thomas Southwest Minzu University State Ethnic Affairs Commission Chengdu610041 China NCS Testing Technology Co. Ltd Chengdu610041 China Pico center SUSTech Core Research Facilities Southern University of Science and Technology Shenzhen518055 China Key Laboratory of Radiation Physics and Technology of Ministry of Education Institute of Nuclear Science and Technology Sichuan University Chengdu610064 China College of Physical Science and Technology Sichuan University Chengdu610064 China Laboratory for Shock Wave and Detonation Physics Institute of Fluid Physics China Academy of Engineering Physics Sichuan Mianyang621900 China Sichuan Research Center of New Materials 596 Yinhe Road Shuangliu Chengdu610200 China Yongjiang Laboratory Ningbo315000 China Institute of Chemical Materials China Academy of Engineering Physics Mianyang621900 China Dept. Electronic & Electrical Eng. University of Sheffield Mappin St. SheffieldS1 3JD United Kingdom

The investigation of chemical reactions during the ion irradiation is a frontier for the study of the ion-material interaction. In order to derive the contribution of bond formation to chemistry of ion produced nanoclusters, the valence electron energy loss spectroscopy (VEELS) was exploited to investigate the Ga+ ion damage in Al2O3, InP and InGaAs, where each target material has been shown to yield different process for altering the clustering of recoil atoms: metallic Ga, metallic In and InGaP clusters in Al2O3, InP and InGaAs *** simulations based on Monte Carlo and crystal orbital Hamiltonianindicate that the chemical constitution of cascade induced nano-precipitates is a result of a competition between interstitial/vacancy consumption rate and preferential bond formation. Copyright © 2023, The Authors. All rights reserved.

关键词： Indium phosphide

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