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Tailoring Catalysis of Encapsulated Platinum Nanoparticles by Pore Wall Engineering of Covalent Organic Frameworks

Angewandte Chemie 2024年第39期136卷

作者： Mingchun Guo Dr. Xinyu Guan Dr. Qiangqiang Meng Dr. Ming-Liang Gao Prof. Dr. Qunxiang Li Prof. Dr. Hai-Long Jiang Hefei National Research Center for Physical Sciences at the Microscale Department of Chemistry University of Science and Technology of China Hefei Anhui 230026 P. R. China Hangzhou Institute of Advanced Studies Zhejiang Normal University Hangzhou Zhejiang 310000 P. R. China Department of Chemical Physics University of Science and Technology of China Hefei Anhui 230026 P. R. China

While supported metal nanoparticles (NPs) have shown significant promise in heterogeneous catalysis, precise control over their interaction with the support, which profoundly impacts their catalytic performance, remains a significant challenge. In this study, Pt NPs are incorporated into thioether-functionalized covalent organic frameworks (denoted COF-S x ), enabling precise control over the size and electronic state of Pt NPs by adjusting the thioether density dangling on the COF pore walls. Notably, the resulting Pt@COF-S x demonstrate exceptional selectivity (> 99 %) in catalytic hydrogenation of p -chloronitrobenzene to p -chloroaniline, in sharp contrast to the poor selectivity of Pt NPs embedded in thioether-free COFs. Furthermore, the conversion over Pt@COF-S x exhibits a volcano-type curve as the thioether density increases, due to the corresponding change of accessible Pt sites. This work provides an effective approach to regulating the catalysis of metal NPs via their microenvironment modulation, with the aid of rational design and precise tailoring of support structure.

关键词： Covalent Organic Framework Heterogeneous Catalysis Selective Hydrogenation Metal Nanoparticles Microenvironment Modulation

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Deep-learning-driven event reconstruction applied to simulated data from a single Large-Sized Telescope of CTA 37

Deep-learning-driven event reconstruction applied to simulat...

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37th International Cosmic Ray Conference, ICRC 2021

作者： Abe, H. Aguasca, A. Agudo, I. Antonelli, L.A. Aramo, C. Armstrong, T. Artero, M. Asano, K. Ashkar, H. Aubert, P. Baktash, A. Bamba, A. Baquero Larriva, A. Baroncelli, L. Barres de Almeida, U. Barrio, J.A. Batkovic, I. Becerra González, J. Bernardos, M.I. Berti, A. Biederbeck, N. Bigongiari, C. Blanch, O. Bonnoli, G. Bordas, P. Bose, D. Bulgarelli, A. Burelli, I. Buscemi, M. Cardillo, M. Caroff, S. Carosi, A. Cassol, F. Cerruti, M. Chai, Y. Cheng, K. Chikawa, M. Chytka, L. Contreras, J.L. Cortina, J. Costantini, H. Dalchenko, M. De Angelis, A. de Bony de Lavergne, M. Deleglise, G. Delgado, C. Delgado Mengual, J. della Volpe, D. Depaoli, D. Di Pierro, F. Di Venere, L. Díaz, C. Dominik, R.M. Dominis Prester, D. Donini, A. Dorner, D. Doro, M. Elsässer, D. Emery, G. Escudero, J. Fiasson, A. Foffano, L. Fonseca, M.V. Freixas Coromina, L. Fukami, S. Fukazawa, Y. Garcia, E. Garcia López, R. Giglietto, N. Giordano, F. Gliwny, P. Godinovic, N. Green, D. Grespan, P. Gunji, S. Hackfeld, J. Hadasch, D. Hahn, A. Hassan, T. Hayashi, K. Heckmann, L. Heller, M. Herrera Llorente, J. Hirotani, K. Hoffmann, D. Horns, D. Houles, J. Hrabovsky, M. Hrupec, D. Hui, D. Hütten, M. Inada, T. Inome, Y. Iori, M. Ishio, K. Iwamura, Y. Jacquemont, M. Jimenez Martinez, I. Jouvin, L. Jurysek, J. Kagaya, M. Karas, V. Katagiri, H. Kataoka, J. Kerszberg, D. Kobayashi, Y. Kong, A. Kubo, H. Kushida, J. Lamanna, G. Lamastra, A. Le Flour, T. Longo, F. López-Coto, R. López-Moya, M. López-Oramas, A. Luque-Escamilla, P.L. Majumdar, P. Makariev, M. Mandat, D. Manganaro, M. Mannheim, K. Mariotti, M. Marquez, P. Marsella, G. Martí, J. Martinez, O. Martínez, G. Martínez, M. Marusevec, P. Mas, A. Maurin, G. Mazin, D. Mestre Guillen, E. Micanovic, S. Miceli, D. Miener, T. Miranda, J.M. Miranda, L.D.M. Mirzoyan, R. Mizuno, T. Molina, E. Montaruli, T. Monteiro, I. Moralejo, A. Morcuende, D. Moretti, E. Morselli, A. Mrakovcic, K. Murase, K. Nagai, A. Nakamori, T. Nickel, L. LISTIC Université Savoie Mont-Blanc Polytech Annecy-Chambéry 5 chemin de bellevue Annecy74940 France Institute for Cosmic Ray Research University of Tokyo Japan Departament de Física Quàntica i Astrofísica Institut de Ciències del Cosmos Universitat de Barcelona IEEC-UB Spain Instituto de Astrofísica de Andalucía-CSIC Italy INAF Osservatorio Astronomico di Roma Italy INFN Sezione di Napoli Italy Aix Marseille Univ CNRS IN2P3 CPPM France The Barcelona Institute of Science and Technology Spain IRFU CEA Université Paris-Saclay France Laboratoire d'Annecy de Physique des Particules Univ. Grenoble Alpes Univ. Savoie Mont Blanc CNRS LAPP 9 chemin de bellevue Annecy74940 France Universität Hamburg Institut für Experimentalphysik Germany Graduate School of Science University of Tokyo Japan Instituto de Física de Partículas y del Cosmos Departamento de EMFTEL Universidad Complutense de Madrid Madrid Spain INAF Osservatorio di Astrofisica e Scienza Spazio di Bologna Italy Centro Brasileiro de Pesquisas Físicas Brazil INFN Istituto Nazionale di Fisica Nucleare Sezione di Padova PadovaI-35131 Italy Università degli Studi di Padova Italy Instituto de Astrofísica de Canarias Departamento de Astrofísica Universidad de La Laguna Spain Max-Planck-Institut für Physik Germany Department of Physics TU Dortmund University Germany Saha Institute of Nuclear Physics INFN Sezione di Trieste Università degli Studi di Udine Italy INFN Sezione di Catania Italy Italy University of Geneva Département de Physique Nucléaire et Corpusculaire Switzerland Palacky University Olomouc Faculty of Science Czech Republic CIEMAT Port d'Informació Científica INFN Sezione di Torino Italy Dipartimento di Fisica Universitá degli Studi di Torino Italy INFN Sezione di Bari Università di Bari Italy University of Rijeka Department of Physics Croatia Institute for Theoretical Physics and Astrophysics Universität Würzburg Germany Physics Program Graduate School of Advanced Science and Engin

When very-high-energy gamma rays interact high in the Earth's atmosphere, they produce cascades of particles that induce flashes of Cherenkov light. Imaging Atmospheric Cherenkov Telescopes (IACTs) detect these flashes and convert them into shower images that can be analyzed to extract the properties of the primary gamma ray. The dominant background for IACTs is comprised of air shower images produced by cosmic hadrons, with typical noise-to-signal ratios of several orders of magnitude. The standard technique adopted to differentiate between images initiated by gamma rays and those initiated by hadrons is based on classical machine learning algorithms, such as Random Forests, that operate on a set of handcrafted parameters extracted from the images. Likewise, the inference of the energy and the arrival direction of the primary gamma ray is performed using those parameters. State-of-the-art deep learning techniques based on convolutional neural networks (CNNs) have the potential to enhance the event reconstruction performance, since they are able to autonomously extract features from raw images, exploiting the pixel-wise information washed out during the parametrization process. Here we present the results obtained by applying deep learning techniques to the reconstruction of Monte Carlo simulated events from a single, next-generation IACT, the Large-Sized Telescope (LST) of the Cherenkov Telescope Array (CTA). We use CNNs to separate the gamma-ray-induced events from hadronic events and to reconstruct the properties of the former, comparing their performance to the standard reconstruction technique. Three independent implementations of CNN-based event reconstruction models have been utilized in this work, producing consistent results. © Copyright owned by the author(s) under the terms of the Creative Commons Attribution-NonCommercial-NoDerivatives 4.0 International License (CC BY-NC-ND 4.0)

关键词： Hadrons

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Investigation of a novel biocide material for biocorrosion in simulated seawater: A case study on Tinospora cordifolia extract

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Case Studies in chemical and Environmental Engineering 2024年 10卷

作者： Royani, Ahmad Hanafi, Muhammad Aigbodion, Victor Sunday Prastya, Muhammad Eka Verma, Chandrabhan Mubarak, Nabisab Mujawar Alfantazi, Akram Manaf, Azwar Research Center for Metallurgy National Research and Innovation Agency – BRIN Kawasan Puspiptek Banten Tangerang Selatan 15314 Indonesia Postgraduate Program of Materials Science Study Department of Physics Faculty of Mathematics and Natural Sciences Universitas Indonesia Depok 16424 Indonesia Research Center for Pharmaceutical Ingredients and Traditional Medicine National Research and Innovation Agency – BRIN Kawasan Puspiptek Banten Tangerang Selatan 15314 Indonesia Department of Metallurgical and Materials Engineering University of Nigeria Nsukka 410001 Nigeria Department of Chemical and Petroleum Engineering Khalifa University of Science and Technology P.O. Box 127788 Abu Dhabi United Arab Emirates Petroleum and Chemical Engineering Faculty of Engineering Universiti Teknologi Brunei Bandar Seri Begawan BE1410 Brunei Darussalam Department of Biosciences Saveetha School of Engineering Saveetha Institute of Medical and Technical Sciences Chennai India

This case report investigates the preventive effect of Tinospora cordifolia extract on biocorrosion induced by Pseudomonas aeruginosa on mild steel API 5L in the simulated seawater medium. Electrochemical techniques, spectroscopic techniques, and surface analysis were employed to investigate biocide performance and corrosion behavior. P. aeruginosa has been shown to enhance iron dissolution in seawater medium. These findings point to the role of P. aeruginosa bacteria in forming differential oxygen, which causes corrosion. Morphology results from atomic Fourier microscopy (AFM) highlight the presence of P. aeruginosa in biotic environments, where the surface is rougher than in abiotic conditions. On the other hand, adding T. cordifolia to the biotic medium resulted in a smoother and more homogeneous surface without any significant deterioration. Electrochemical findings reveal that adding 300 mg L⁻¹ of T. cordifolia extract prevents the microbiologically influenced corrosion (MIC) of steel API 5L, with an optimum effectiveness value of 74.50 % after 21 days of incubation. This protective effect is caused by forming a more compact iron oxide surface layer and the adsorption of phenolic active compounds such as Moupinamide and others on the surface of mild steel API 5L, as detected by liquid chromatography-mass/spectrometry-mass spectrometry (LCMS-MS), Fourier-transform infrared spectroscopy (FTIR) and field emission scanning electron microscopy (FE-SEM) techniques. © 2024 The Authors

关键词： Bio-corrosion Biofilm Green biocide Plant extract Pseudomonas aeruginosa Tinospora cordifolia

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Measurement of Two-Particle Correlations of Hadrons in e+e− Collisions at Belle

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physical Review Letters 2022年第14期128卷 142005-142005页

作者： Y.-C. Chen Y.-J. Lee P. Chang I. Adachi H. Aihara S. Al Said D. M. Asner T. Aushev R. Ayad V. Babu P. Behera K. Belous J. Bennett M. Bessner T. Bilka D. Bodrov J. Borah M. Bračko P. Branchini T. E. Browder A. Budano M. Campajola D. Červenkov M.-C. Chang V. Chekelian B. G. Cheon K. Chilikin H. E. Cho K. Cho S.-J. Cho S.-K. Choi Y. Choi D. Cinabro S. Das G. De Nardo G. De Pietro R. Dhamija F. Di Capua J. Dingfelder T. V. Dong D. Dossett D. Epifanov T. Ferber B. G. Fulsom R. Garg V. Gaur A. Giri P. Goldenzweig T. Gu K. Gudkova C. Hadjivasiliou O. Hartbrich K. Hayasaka H. Hayashii W.-S. Hou C.-L. Hsu T. Iijima K. Inami A. Ishikawa R. Itoh M. Iwasaki Y. Iwasaki W. W. Jacobs S. Jia Y. Jin A. B. Kaliyar C. H. Kim D. Y. Kim K.-H. Kim Y.-K. Kim P. Kodyš T. Konno A. Korobov S. Korpar E. Kovalenko P. Križan R. Kroeger P. Krokovny M. Kumar R. Kumar K. Kumara A. Kuzmin Y.-J. Kwon Y.-T. Lai T. Lam J. S. Lange M. Laurenza S. C. Lee J. Li Y. Li Y. B. Li L. Li Gioi J. Libby K. Lieret C.-W. Lin D. Liventsev A. Martini M. Masuda T. Matsuda D. Matvienko F. Meier M. Merola F. Metzner K. Miyabayashi G. B. Mohanty T. J. Moon R. Mussa M. Nakao A. Natochii L. Nayak N. K. Nisar S. Nishida K. Nishimura S. Ogawa H. Ono G. Pakhlova T. Pang S. Pardi S.-H. Park S. Patra S. Paul T. K. Pedlar L. E. Piilonen T. Podobnik E. Prencipe M. T. Prim N. Rout G. Russo D. Sahoo S. Sandilya A. Sangal L. Santelj T. Sanuki V. Savinov G. Schnell C. Schwanda R. Seidl Y. Seino M. E. Sevior M. Shapkin J.-G. Shiu J. B. Singh A. Sokolov E. Solovieva M. Starič Z. S. Stottler M. Sumihama K. Sumisawa W. Sutcliffe M. Takizawa U. Tamponi K. Tanida F. Tenchini M. Uchida T. Uglov Y. Unno K. Uno S. Uno R. Van Tonder G. Varner A. Vinokurova A. Vossen E. Waheed C. H. Wang D. Wang E. Wang X. L. Wang S. Watanuki E. Won W. Yan S. B. Yang H. Ye J. Yelton Y. Zhai Z. P. Zhang V. Zhilich V. Zhukova Department of Physics National Taiwan University Taipei 10617 High Energy Accelerator Research Organization (KEK) Tsukuba 305-0801 SOKENDAI (The Graduate University for Advanced Studies) Hayama 240-0193 Department of Physics University of Tokyo Tokyo 113-0033 Department of Physics Faculty of Science University of Tabuk Tabuk 71451 Department of Physics Faculty of Science King Abdulaziz University Jeddah 21589 Brookhaven National Laboratory Upton New York 11973 National Research University Higher School of Economics Moscow 101000 Deutsches Elektronen–Synchrotron 22607 Hamburg Indian Institute of Technology Madras Chennai 600036 Institute for High Energy Physics Protvino 142281 University of Mississippi University Mississippi 38677 University of Hawaii Honolulu Hawaii 96822 Faculty of Mathematics and Physics Charles University 121 16 Prague P.N. Lebedev Physical Institute of the Russian Academy of Sciences Moscow 119991 Indian Institute of Technology Guwahati Assam 781039 Faculty of Chemistry and Chemical Engineering University of Maribor 2000 Maribor J. Stefan Institute 1000 Ljubljana INFN - Sezione di Roma Tre I-00146 Roma INFN - Sezione di Napoli I-80126 Napoli Università di Napoli Federico II I-80126 Napoli Department of Physics Fu Jen Catholic University Taipei 24205 Max-Planck-Institut für Physik 80805 München Department of Physics and Institute of Natural Sciences Hanyang University Seoul 04763 Korea Institute of Science and Technology Information Daejeon 34141 Yonsei University Seoul 03722 Chung-Ang University Seoul 06974 Sungkyunkwan University Suwon 16419 Wayne State University Detroit Michigan 48202 Malaviya National Institute of Technology Jaipur Jaipur 302017 Indian Institute of Technology Hyderabad Telangana 502285 University of Bonn 53115 Bonn Institute of Theoretical and Applied Research (ITAR) Duy Tan University Hanoi 100000 School of Physics University of Melbourne Victoria 3010 Budker Institute of Nuclear Physics SB RAS Novosibirsk 630090 Novosib

The measurement of two-particle angular correlation functions in high-multiplicity e+e− collisions at s=10.52 GeV is reported. In this study, the 89.5 fb−1 of hadronic e+e− annihilation data collected by the Belle detector at KEKB are used. Two-particle angular correlation functions are measured in the full relative azimuthal angle (Δϕ) and three units of pseudorapidity (Δη), defined by either the electron beam axis or the event-shape thrust axis, and are studied as a function of charged-particle multiplicity. The measurement in the thrust axis analysis, with mostly outgoing quark pairs determining the reference axis, is sensitive to the region of additional soft gluon emissions. No significant anisotropic collective behavior is observed with either coordinate analyses. Near-side jet correlations appear to be absent in the thrust axis analysis. The measurements are compared to predictions from various event generators and are expected to provide new constraints to the phenomenological models in the low-energy regime.

关键词： Particle & resonance production Quark & gluon jets Quark-gluon plasma

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A deep potential model with long-range electrostatic interactions

arXiv

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arXiv 2021年

作者： Zhang, Linfeng Wang, Han Muniz, Maria Carolina Panagiotopoulos, Athanassios Z. Car, Roberto Weinan, E. DP Technology Beijing China Laboratory of Computational Physics Institute of Applied Physics and Computational Mathematics Fenghao East Road 2 Beijing100094 China HEDPS CAPT College of Engineering Peking University Beijing100871 China Department of Chemical and Biological Engineering Princeton University PrincetonNJ08544 United States Department of Chemistry Department of Physics Program in Applied and Computational Mathematics Princeton Institute for the Science and Technology of Materials Princeton University PrincetonNJ08544 United States School of Mathematical Sciences Peking University Beijing100871 China AI for Science Institute Beijing China Department of Mathematics and Program in Applied and Computational Mathematics Princeton University PrincetonNJ08544 United States

Machine learning models for the potential energy of multi-atomic systems, such as the deep potential (DP) model, make possible molecular simulations with the accuracy of quantum mechanical density functional theory, at a cost only moderately higher than that of empirical force fields. However, the majority of these models lack explicit long-range interactions and fail to describe properties that derive from the Coulombic tail of the forces. To overcome this limitation we extend the DP model by approximating the long-range electrostatic interaction between ions (nuclei+core electrons) and valence electrons with that of distributions of spherical Gaussian charges located at ionic and electronic sites. The latter are rigorously defined in terms of the centers of the maximally localized Wannier distributions, whose dependence on the local atomic environment is modeled accurately by a deep neural network. In the deep potential long-range (DPLR) model, the electrostatic energy of the Gaussian charge system is added to short-range interactions that are represented as in the standard DP model. The resulting potential energy surface is smooth and possesses analytical forces and virial. Missing effects in the standard DP scheme are recovered, improving on accuracy and predictive power. By including long-range electrostatics, DPLR correctly extrapolates to large systems the potential energy surface learned from quantum mechanical calculations on smaller systems. We illustrate the approach with three examples, the potential energy profile of the water dimer, the free energy of interaction of a water molecule with a liquid water slab, and the phonon dispersion curves of the NaCl crystal. © 2021, CC BY.

关键词： Electrostatics

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First test of lepton flavor universality in the charmed baryon decays Ωc0→Ω−ℓ+νℓ using data of the Belle experiment

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physical Review D 2022年第9期105卷 L091101-L091101页

作者： Y. B. Li C. P. Shen I. Adachi H. Aihara S. Al Said D. M. Asner H. Atmacan T. Aushev R. Ayad V. Babu S. Bahinipati P. Behera K. Belous J. Bennett F. Bernlochner M. Bessner B. Bhuyan T. Bilka A. Bobrov D. Bodrov J. Borah A. Bozek M. Bračko P. Branchini T. E. Browder A. Budano M. Campajola D. Červenkov M.-C. Chang P. Chang V. Chekelian A. Chen B. G. Cheon K. Chilikin H. E. Cho K. Cho S.-J. Cho S.-K. Choi Y. Choi S. Choudhury D. Cinabro S. Cunliffe N. Dash G. De Nardo G. De Pietro R. Dhamija F. Di Capua J. Dingfelder Z. Doležal T. V. Dong T. Ferber D. Ferlewicz B. G. Fulsom R. Garg V. Gaur N. Gabyshev A. Giri P. Goldenzweig B. Golob E. Graziani K. Gudkova C. Hadjivasiliou T. Hara K. Hayasaka H. Hayashii M. T. Hedges W.-S. Hou K. Inami G. Inguglia A. Ishikawa R. Itoh M. Iwasaki Y. Iwasaki W. W. Jacobs E.-J. Jang S. Jia Y. Jin K. K. Joo J. Kahn K. H. Kang T. Kawasaki H. Kichimi C. Kiesling C. H. Kim D. Y. Kim K.-H. Kim K. T. Kim Y.-K. Kim K. Kinoshita P. Kodyš T. Konno A. Korobov S. Korpar E. Kovalenko P. Križan R. Kroeger P. Krokovny M. Kumar R. Kumar K. Kumara A. Kuzmin Y.-J. Kwon K. Lalwani T. Lam M. Laurenza S. C. Lee J. Li L. K. Li Y. Li L. Li Gioi J. Libby K. Lieret D. Liventsev A. Martini M. Masuda D. Matvienko S. K. Maurya M. Merola K. Miyabayashi R. Mizuk G. B. Mohanty M. Nakao D. Narwal A. Natochii L. Nayak M. Nayak N. K. Nisar S. Nishida K. Ogawa S. Ogawa H. Ono P. Oskin P. Pakhlov G. Pakhlova T. Pang S. Pardi S.-H. Park S. Patra S. Paul T. K. Pedlar R. Pestotnik L. E. Piilonen T. Podobnik E. Prencipe M. T. Prim M. Röhrken A. Rostomyan N. Rout G. Russo D. Sahoo S. Sandilya A. Sangal L. Santelj V. Savinov G. Schnell J. Schueler C. Schwanda Y. Seino K. Senyo M. E. Sevior M. Shapkin C. Sharma V. Shebalin J.-G. Shiu B. Shwartz J. B. Singh A. Sokolov E. Solovieva M. Starič Z. S. Stottler M. Sumihama T. Sumiyoshi M. Takizawa U. Tamponi K. Tanida F. Tenchini M. Uchida T. Uglov Y. Unno K. Uno S. Uno P. Urquijo S. E. Vahsen R. Van Tonder G. Varner A. Vinokurova E. Waheed D. Wang E. Wang M.-Z. Wang S. Watanuki E. Won Key Laboratory of Nuclear Physics and Ion-beam Application (MOE) and Institute of Modern Physics Fudan University Shanghai 200443 High Energy Accelerator Research Organization (KEK) Tsukuba 305-0801 SOKENDAI (The Graduate University for Advanced Studies) Hayama 240-0193 Department of Physics University of Tokyo Tokyo 113-0033 Department of Physics Faculty of Science University of Tabuk Tabuk 71451 Department of Physics Faculty of Science King Abdulaziz University Jeddah 21589 Brookhaven National Laboratory Upton New York 11973 University of Cincinnati Cincinnati Ohio 45221 National Research University Higher School of Economics Moscow 101000 Deutsches Elektronen–Synchrotron 22607 Hamburg Indian Institute of Technology Bhubaneswar Satya Nagar 751007 Indian Institute of Technology Madras Chennai 600036 Institute for High Energy Physics Protvino 142281 University of Mississippi University Mississippi 38677 University of Bonn 53115 Bonn University of Hawaii Honolulu Hawaii 96822 Indian Institute of Technology Guwahati Assam 781039 Faculty of Mathematics and Physics Charles University 121 16 Prague Budker Institute of Nuclear Physics SB RAS Novosibirsk 630090 Novosibirsk State University Novosibirsk 630090 P.N. Lebedev Physical Institute of the Russian Academy of Sciences Moscow 119991 H. Niewodniczanski Institute of Nuclear Physics Krakow 31-342 Faculty of Chemistry and Chemical Engineering University of Maribor 2000 Maribor J. Stefan Institute 1000 Ljubljana INFN—Sezione di Roma Tre I-00146 Roma INFN—Sezione di Napoli I-80126 Napoli Università di Napoli Federico II I-80126 Napoli Department of Physics Fu Jen Catholic University Taipei 24205 Department of Physics National Taiwan University Taipei 10617 Max-Planck-Institut für Physik 80805 München National Central University Chung-li 32054 Department of Physics and Institute of Natural Sciences Hanyang University Seoul 04763 Korea Institute of Science and Technology Information Daejeon 34141 Yonsei University Seoul 0372

We present the first observation of the Ωc0→Ω−μ+νμ decay and present measurements of the branching fraction ratios of the Ωc0→Ω−ℓ+νℓ decays compared to the reference mode Ωc0→Ω−π+, (ℓ=e or μ). This analysis is based on 89.5 fb−1, 711 fb−1, and 121.1 fb−1 data samples collected with the Belle detector at the KEKB asymmetric-energy e+e− collider at the center-of-mass energies of 10.52 GeV, 10.58 GeV, and 10.86 GeV, respectively. The Ωc0 signal yields are extracted by fitting MΩℓ and MΩπ spectra. The branching fraction ratios B(Ωc0→Ω−e+νe)/B(Ωc0→Ω−π+) and B(Ωc0→Ω−μ+νμ)/B(Ωc0→Ω−π+) are measured to be 1.98±0.13(stat)±0.08(syst) and 1.94±0.18(stat)±0.10(syst), respectively. The ratio of B(Ωc0→Ω−e+νe)/B(Ωc0→Ω−μ+νμ) is measured to be 1.02±0.10(stat)±0.02(syst), which is consistent with the expectation of lepton flavor universality.

关键词： Branching fraction Leptonic, semileptonic & radiative decays Charmed baryons Lepton colliders

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JWST Discovery of a High-Redshift Tidal Disruption Event Candidate in COSMOS-Web

arXiv

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arXiv 2025年

作者： Karmen, Mitchell Gezari, Suvi Lambrides, Erini Akins, Hollis B. Norman, Colin Casey, Caitlin M. Pierel, Justin Coulter, David Rest, Armin Fox, Ori Dr. Ajay, Yukta Allen, Natalie Drakos, Nicole E. Fujimoto, Seiji Gomez, Sebastian Gozaliasl, Ghassem Ilbert, Olivier Kartaltepe, Jeyhan S. Koekemoer, Anton M. Lane, Zachary G. McCracken, Henry Joy Paquereau, Louise Rhodes, Jason Robertson, Brant E. Shuntov, Marko Siebert, Matthew R. Toft, Sune Wevers, Thomas Zenati, Yossef Department of Physics and Astronomy Johns Hopkins University 3400 N. Charles Street BaltimoreMD21218 United States Space Telescope Science Institute BaltimoreMD21218 United States NASA-Goddard Space Flight Center Code 662 GreenbeltMD20771 United States The University of Texas at Austin 2515 Speedway Blvd Stop C1400 AustinTX78712 United States Department of Physics University of California Santa Barbara Santa BarbaraCA93109 United States Denmark Niels Bohr Institute University of Copenhagen Jagtvej 128 CopenhagenDK-2200 Denmark Department of Physics and Astronomy University of Hawaii Hilo 200 W Kawili St HiloHI96720 United States Center for Astrophysics | Harvard & Smithsonian 60 Garden Street CambridgeMA02138-1516 United States Department of Computer Science Aalto University P.O. Box 15400 EspooFI-00076 Finland Department of Physics P.O. Box 64 HelsinkiFI-00014 Finland Aix Marseille Univ CNRS CNES LAM Marseille France Laboratory for Multiwavelength Astrophysics School of Physics and Astronomy Rochester Institute of Technology 84 Lomb Memorial Drive RochesterNY14623 United States School of Physical and Chemical Sciences — Te Kura Matū University of Canterbury Private Bag 4800 Christchurch8140 New Zealand Institut d’Astrophysique de Paris UMR 7095 CNRS Sorbonne Université 98 bis boulevard Arago ParisF-75014 France Jet Propulsion Laboratory California Institute of Technology 4800 Oak Grove Drive PasadenaCA91001 United States Department of Astronomy and Astrophysics University of California Santa Cruz 1156 High Street Santa CruzCA95064 United States Astrophysics & Space Institute Schmidt Sciences New YorkNY10011 United States

The rates and properties of tidal disruption events (TDEs) provide valuable insights into their host galaxy central stellar densities and the demographics of their central supermassive black holes (SMBHs). TDEs have been observed only at low redshifts (z 1), due to the difficulty in conducting deep time-domain surveys. In this work, we present the discovery of a high-redshift TDE candidate, HZTDE-1, in the COSMOS-Web survey with JWST’s NIRCam, using a novel selection technique based on color and morphology. We first outline a methodology for identifying high-z TDEs in deep infrared imaging surveys, leveraging their unique spectral energy distributions (SEDs) and morphologies of these transients. We apply this technique to COSMOS-Web in filters F115W, F150W, F277W, and F444W, and identify HZTDE-1, a transient point source relative to archival UltraVISTA infrared observations. If we assume it is a TDE, we estimate its photometric redshift to be z = 5.02+1−1.3211. HZTDE-1 cannot be explained by reasonable supernova or AGN models. However, we cannot rule out a superluminous supernova at z 3. If confirmed with follow-up observations, HZTDE-1 would represent the highest-redshift TDE discovery to date, and would suggest an enhancement of the TDE rate in the high-redshift universe. Our method, which can be applied to future deep surveys with JWST and Roman, offers a pathway to identify TDEs at z > 4 and probe black hole demographics at early cosmic times. © 2025, CC BY.

关键词： Space telescopes

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First Measurement of A=4 Hypernuclei and Antihypernuclei at the LHC

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physical Review Letters 2025年第16期134卷 162301-162301页

作者： S. Acharya A. Agarwal G. Aglieri Rinella L. Aglietta M. Agnello N. Agrawal Z. Ahammed S. Ahmad S. U. Ahn I. Ahuja A. Akindinov V. Akishina M. Al-Turany D. Aleksandrov B. Alessandro H. M. Alfanda R. Alfaro Molina B. Ali A. Alici N. Alizadehvandchali A. Alkin J. Alme G. Alocco T. Alt A. R. Altamura I. Altsybeev J. R. Alvarado C. O. R. Alvarez M. N. Anaam C. Andrei N. Andreou A. Andronic E. Andronov V. Anguelov F. Antinori P. Antonioli N. Apadula L. Aphecetche H. Appelshäuser C. Arata S. Arcelli R. Arnaldi J. G. M. C. A. Arneiro I. C. Arsene M. Arslandok A. Augustinus R. Averbeck D. Averyanov M. D. Azmi H. Baba A. Badalà J. Bae Y. W. Baek X. Bai R. Bailhache Y. Bailung R. Bala A. Balbino A. Baldisseri B. Balis Z. Banoo V. Barbasova F. Barile L. Barioglio M. Barlou B. Barman G. G. Barnaföldi L. S. Barnby E. Barreau V. Barret L. Barreto C. Bartels K. Barth E. Bartsch N. Bastid S. Basu G. Batigne D. Battistini B. Batyunya D. Bauri J. L. Bazo Alba I. G. Bearden C. Beattie P. Becht D. Behera I. Belikov A. D. C. Bell Hechavarria F. Bellini R. Bellwied S. Belokurova L. G. E. Beltran Y. A. V. Beltran G. Bencedi A. Bensaoula S. Beole Y. Berdnikov A. Berdnikova L. Bergmann M. G. Besoiu L. Betev P. P. Bhaduri A. Bhasin B. Bhattacharjee L. Bianchi J. Bielčík J. Bielčíková A. P. Bigot A. Bilandzic G. Biro S. Biswas N. Bize J. T. Blair D. Blau M. B. Blidaru N. Bluhme C. Blume G. Boca F. Bock T. Bodova J. Bok L. Boldizsár M. Bombara P. M. Bond G. Bonomi H. Borel A. Borissov A. G. Borquez Carcamo E. Botta Y. E. M. Bouziani L. Bratrud P. Braun-Munzinger M. Bregant M. Broz G. E. Bruno V. D. Buchakchiev M. D. Buckland D. Budnikov H. Buesching S. Bufalino P. Buhler N. Burmasov Z. Buthelezi A. Bylinkin S. A. Bysiak J. C. Cabanillas Noris M. F. T. Cabrera M. Cai H. Caines A. Caliva E. Calvo Villar J. M. M. Camacho P. Camerini F. D. M. Canedo S. L. Cantway M. Carabas A. A. Carballo F. Carnesecchi R. Caron L. A. D. Carvalho J. Castillo Castellanos M. Castoldi F. Catalano S. Cattaruzzi R. Cerri I. Chakaberia P. Chakraborty S. Chandra S. Cha Université Clermont Auvergne CNRS/IN2P3 LPC Clermont-Ferrand France Variable Energy Cyclotron Centre Homi Bhabha National Institute Kolkata India European Organization for Nuclear Research (CERN) Geneva Switzerland Dipartimento di Fisica dell’Università and Sezione INFN Turin Italy Dipartimento DISAT del Politecnico and Sezione INFN Turin Italy Dipartimento di Fisica e Astronomia dell’Università and Sezione INFN Bologna Italy Department of Physics Aligarh Muslim University Aligarh India Korea Institute of Science and Technology Information Daejeon Republic of Korea Faculty of Science P.J. Šafárik University Košice Slovak Republic Affiliated with an institute covered by a cooperation agreement with CERN Frankfurt Institute for Advanced Studies Johann Wolfgang Goethe-Universität Frankfurt Frankfurt Germany Research Division and ExtreMe Matter Institute EMMI GSI Helmholtzzentrum für Schwerionenforschung GmbH Darmstadt Germany INFN Sezione di Torino Turin Italy Central China Normal University Wuhan China Instituto de Física Universidad Nacional Autónoma de México Mexico City Mexico University of Houston Houston Texas USA Sungkyunkwan University Suwon City Republic of Korea Department of Physics and Technology University of Bergen Bergen Norway INFN Sezione di Cagliari Cagliari Italy Institut für Kernphysik Johann Wolfgang Goethe-Universität Frankfurt Frankfurt Germany INFN Sezione di Bari Bari Italy Physik Department Technische Universität München Munich Germany High Energy Physics Group Universidad Autónoma de Puebla Puebla Mexico Horia Hulubei National Institute of Physics and Nuclear Engineering Bucharest Romania University of Derby Derby United Kingdom Universität Münster Institut für Kernphysik Münster Germany Physikalisches Institut Ruprecht-Karls-Universität Heidelberg Heidelberg Germany INFN Sezione di Padova Padova Italy INFN Sezione di Bologna Bologna Italy Lawrence Berkeley National Laboratory Berkeley California USA SUBATECH I

In this Letter, the first evidence of the He¯Λ¯4 antihypernucleus is presented, along with the first measurement at the LHC of the production of (anti)hypernuclei with mass number A=4, specifically (anti)HΛ4 and (anti)HeΛ4. In addition, the antiparticle-to-particle ratios for both hypernuclei (H¯Λ¯4/HΛ4 and He¯Λ¯4/HeΛ4) are shown, which are sensitive to the baryochemical potential of the strongly interacting matter created in heavy-ion collisions. The results are obtained from a data sample of central Pb-Pb collisions, collected during the 2018 LHC data taking at a center-of-mass energy per nucleon pair of sNN=5.02 TeV. The yields measured for the average of the charge-conjugated states are found to be [0.78±0.19(stat)±0.17(syst)]×10−6 for the (anti)HΛ4 and [1.08±0.34(stat)±0.20(syst)]×10−6 for the (anti)HeΛ4, and the measured antiparticle-to-particle ratios are in agreement with unity. The presence of (anti)HΛ4 and (anti)HeΛ4 excited states is expected to strongly enhance the production yield of these hypernuclei. The yield values exhibit a combined deviation of 3.3σ from the theoretical ground-state-only expectation, while the inclusion of the excited states in the calculations leads to an agreement within 0.6σ with the present measurements. Additionally, the measured (anti)HΛ4 and (anti)HeΛ4 masses are compatible with the world-average values within the uncertainties.

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Effect of Zn doped on electronic and optical properties of HfO2: A DFT study

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AIP Conference Proceedings 2023年第1期2800卷

作者： Ramesh Sharma Jisha Annie Abraham Sajad Ahmad Dar Vipul Srivastava Departmentof Applied Science Feroze Gandhi Institute of Engineering and Technology Raebareli-229001(India) Department of Physics National Defence Academy Pune-Maharashtra (India) Department of Physics Govt. Maulana Azad Memorial PG College Jammu-180006 India Department of Physics School of Chemical Engineering and Physical Sciences Lovely Professional University Phagwara - 144411 Punjab India

In the present work,the structural, electronic, and optical properties of cubic Hf(1-x)ZnxO2(x=0, 0.25) have been studied by using self-consistent full potential linearized augmented plane wave (FP-LAPW) method with PBE-sol and mBJ potentials. The lattice parameter of un-doped cubic HfO2 was found to be in good agreement with the previous experimental work. A decrease in the lattice parameter and band gap as well, found on the doping of Zn impurities to the cubic HfO2, which has been reflected in the band structure and density of states diagrams. The band structure diagram revealed insulating nature of c-HfO2 with band gap of 5.81 eV, nevertheless metallic nature has been observed in Hf0.75Zn0.25O2. We also presented the optical properties such as the real and imaginary part of dielectric function the refractive index and the absorption coefficient etc. The computed results show that Zn doped Hafnia are perfectly suited for optoelectronic devices operating in the deep blue and near-ultraviolet (UV) region. The origin of dielectric function from the change in hybridization of the Hf-5d, Zn-3d, O-2porbital and the Hf-6s, Zn-4s,O-2s orbital, which are responsible for engineering energy positions and shapesof the valence-band (VB) top and the conduction band (CB) bottom, respectively.

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Direct Synthesis of High Silica Ssz-16 Zeolite with Extraordinarily Superior Performance in Nh3-Scr Reaction

SSRN

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SSRN 2023年

作者： Han, Shichao Rao, Wei Hu, Junyi Tang, Xiaomin Ma, Ye Du, Jinpeng Liu, Zhongqi Wu, Qinming Ma, Yanhang Meng, Xiangju Shan, Wenpo Xiao, Feng-Shou He, Hong Center for Excellence in Regional Atmospheric Environment Institute of Urban Environment Chinese Academy of Sciences Xiamen361021 China Zhejiang Key Laboratory of Urban Environmental Processes and Pollution Control Ningbo Urban Environment Observation and Research Station Institute of Urban Environment Chinese Academy of Sciences Ningbo315800 China State Key Laboratory of Magnetic Resonance and Atomic and Molecular Physics National Center for Magnetic Resonance in Wuhan Key Laboratory of Magnetic Resonance in Biological Systems Wuhan Institute of Physics and Mathematics Innovation Academy for Precision Measurement Science and Technology Chinese Academy of Sciences Wuhan430071 China School of Physical Science and Technology Shanghai Key Laboratory of High-resolution Electron Microscopy ShanghaiTech University Shanghai201210 China State Key Joint Laboratory of Environment Simulation and Pollution Control Research Center for Eco-Environmental Sciences Chinese Academy of Sciences Beijing100085 China College of Chemical and Biological Engineering Zhejiang University Hangzhou310027 China Key Lab of Applied Chemistry of Zhejiang Province Department of Chemistry Zhejiang University Hangzhou310007 China

The development of Cu ion-exchanged small-pore zeolites with excellent performance and high hydrothermal stability in NH3-SCR reaction is of great importance. However, many frameworks of the small-pore zeolites are Al-rich, for instance, Cu-SSZ-16 zeolite with Si/Al ratio always no more than 5, showing relatively low hydrothermal stability. In this work, inspired by theoretical calculation for the interaction between organic structural directing agents (OSDAs) and zeolite framework, high silica SSZ-16 zeolite with Si/Al ratio at 6.7 was directly synthesized using an economical diquaternary alkylammonium cation as an OSDA. After exchanged with Cu ion, the Cu-SSZ-16 catalyst shows extraordinarily superior performance in NH3-SCR reaction even after hydrothermal aging at 900 °C. The designed synthesis combined with excellent performance as well as high hydrothermal stability of the high silica SSZ-16 zeolite might provide an attractive alternative candidate for NH3-SCR catalyst on diesel vehicles and non-road mobile machinery in the future. © 2023, The Authors. All rights reserved.

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