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Issues and challenges of water purification membranes

International Journal of Energy and Water Resources 2025年 1-25页

作者： Amin, M. Shah, H.H. Khalid, S. Sharif, S. Butt, A.S. Fareed, A.G. Shah, S.M.H. Khan, I.A. Interdisciplinary Research Center for Hydrogen Technologies and Carbon Management (IRC-HTCM) King Fahd University of Petroleum and Minerals (KFUPM) Dhahran 31261 Saudi Arabia Department of Engineering University of Sannio Piazza Roma 21 Benevento 82100 Italy Department of Chemical Engineering Wah Engineering College University of Wah Wah Cantt Pakistan Department of Polymer and Process Engineering UET Lahore Lahore Pakistan Department of Chemical Engineering University of Engineering and Technology Lahore Lahore Pakistan Department of Engineering University of Naples Parthenope Italy Interdisciplinary Research Center for Membranes and Water Security King Fahd University of Petroleum and Minerals Dhahran 31261 Saudi Arabia Tsinghua Shenzhen International Graduate School Tsinghua University Shenzhen China

With increasing risks of climate change, the water resources have also been declining, and to address this many water treatment and water separation technologies has emerged. Water-based microfiltration membranes (MF) offer numerous benefits over other types of membranes, such as energy efficiency, high flux, and ease of operation. The ultrafiltration membrane (UM) technology has the potential to contribute to this water separation process at the greater level, with its features such as small land occupation, lower energy consumption, easy to handle and customize operation allow this technology to widely used. The most promising technique for purifying water is nanofiltration (NF) membranes, which provide several benefits, such as minimal maintenance costs, high penetration flux, low operating pressure, and high retention of multivalent ions. Among different process the polymeric RO membranes are the dominant stream due to their low cost, ease to mold according requirements and ability to modify their structure by different methods (surface modification and filler incorporation). This review article summarizes the issue and challenges of water purification membranes. © The Author(s), under exclusive licence to Iranian Society of Environmentalists (IRSEN) and Science and research Branch, Islamic Azad University 2025.

关键词： Nanofiltration membranes Reverse osmosis Ultrafiltration membrane Water separation

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Liquefied dimethyl ether as alternative extraction solvent for high γ-oryzanol rice bran oil:Systematic HSP theory and experimental evaluation

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Journal of Bioresources and Bioproducts 2024年第4期9卷 577-591页

作者： Phannipha Daisuk Seiichi Takami Masaki Honda Motonobu Goto Chonlatep Usaku Artiwan Shotipruk Bio-Circular-Green-economy Technology&Engineering Center BCGeTECDepartment of Chemical EngineeringFaculty of EngineeringChulalongkorn UniversityBangkok 10330Thailand Department of Materials Process Engineering Graduate School of EngineeringNagoya UniversityFuro-choChikusa-kuNagoya 464-8603Japan Department of Chemistry Faculty of Science&TechnologyMeijo UniversityShiogamaguchiTempaku-kuNagoyaAichi 468-8502Japan Super Critical Technology Centre Co.Ltd. Kuwan1Mie 511-0838Japan Research Unit on Sustainable Algal Cultivation and Applications Faculty of EngineeringChulalongkorn UniversityBangkok 10330Thailand

This study aimed to systematically find an alternative solvent to replace hexane for the extraction of bio-oil with high𝛾-oryzanol content from rice bran(RB).The selection involved predicting solubility through Hansen solubility theory,experimental validation,determination of suitable extraction conditions,and comparison of oil quality with that of conventional hexane.A wide variety of solvents:subcritical water(SCW),supercritical carbon dioxide(SCCO_(2)),bio-based sol-vents(alcohols and terpenes),and liquefied dimethyl ether(LDME),were initially assessed for rice bran oil(RBO)and𝛾-oryzanol solubility using Hansen solubility *** demon-strating high solubility for both RBO and𝛾-oryzanol,including LDME,ethyl acetate,acetone,and others(alcohols and SCCO_(2))known for effective vegetable oil extraction,were selected/identified for experimental extraction *** these,LDME performed better overall,affording greater solubility and requiring less solvent,shorter duration,lower pressure,and no additional co-solvents for equivalent *** conditions for LDME extraction were identified as 30℃ with a solvent-to-sample ratio of 10 mL/g and an extraction time of 10 *** extracted with LDME and hexane displayed similar fatty acid compositions and no adverse effects on RB protein and carbohydrate structures after LDME extraction were *** study demon-strates LDME as a promising alternative to replace hexane for RBO extraction to further valorize this abundant low-cost RB residue into bio-oil and its𝛾γ-oryzanol and de-oil RB co-products.

关键词： Rice bran oil γ-oryzanol Liquefied dimethyl ether Hansen solubility sphere Fourier transform infrared

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Removal enhancement of persistent basic fuchsin dye from wastewater using an eco-friendly, cost-effective Fenton process with sodium percarbonate and waste iron catalyst

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Environmental Science and Pollution research 2024年第31期31卷 43673-43686页

作者： Aouni, Saoussen Imene Ghodbane, Houria Merouani, Slimane Lakikza, Imane Boublia, Abir Yadav, Krishna Kumar Djelloul, Chawki Albakri, Ghadah Shukri Elboughdiri, Noureddine Benguerba, Yacine Laboratory of Physics for Matter and Radiation Mohamed Cherif Messadia-Souk Ahras University P.O. Box 1553 Souk Ahras41000 Algeria Laboratory of Environmental Process Engineering Department of Chemical Engineering Faculty of Process Engineering University Salah Boubnider-Constantine 3 P.O. Box 72 Constantine25000 Algeria Département de Génie des Procédés Faculté de Technologie Université Ferhat ABBAS Sétif-1 Sétif19000 Algeria Faculty of Science and Technology Madhyanchal Professional University Ratibad Bhopal462044 India Environmental and Atmospheric Sciences Research Group Scientific Research Center Al-Ayen University Thi-Qar Nasiriyah64001 Iraq Laboratory of Reaction Engineering Faculty of Mechanical Engineering and Process Engineering USTHB Algiers Algeria Department of Teaching and Learning College of Education and Human Development Princess Nourah bint Abdulrahman University P.O. Box 84428 Riyadh11671 Saudi Arabia Chemical Engineering Department College of Engineering University of Ha’il Ha’il81441 Saudi Arabia Chemical Engineering Process Department National School of Engineers Gabes University of Gabes Gabes6029 Tunisia Ferhat Abbas Setif 1 University Setif Algeria

Abstract: In this comprehensive investigation, we evaluate the efficacy of the Fenton process in degrading basic fuchsin (BF), a resistant dye. Our primary focus is on the utilization of readily available, environmentally benign, and cost-effective reagents for the degradation process. Furthermore, we delve into various operational parameters, including the quantity of sodium percarbonate (SPC), pH levels, and the dimensions of waste iron bars, to optimize the treatment efficiency. In the course of our research, we employed an initial SPC concentration of 0.5 mM, a pH level of 3, a waste iron bar measuring 3.5 cm in length and 0.4 cm in diameter, and a processing time of 10 min. Our findings reveal the successful elimination of the BF dye, even when subjected to treatment with diverse salts and surfactants under elevated temperatures and acidic conditions (pH below 3). This underscores the robustness of the Fenton process in purifying wastewater contaminated with dye compounds. The outcomes of our study not only demonstrate the efficiency of the Fenton process but highlight its adaptability to address dye contamination challenges across various industries. Critically, this research pioneers the application of waste iron bars as a source of iron in the Fenton reaction, introducing a novel, sustainable approach that enhances the environmental and economic viability of the process. This innovative use of recycled materials as catalysts represents a significant advancement in sustainable chemical engineering practices. Graphical abstract: (Figure presented.). © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2024.

关键词： Iron

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Adsorption characteristics of sulfate reducing bacteria Clostridium sp. on lignite surface

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Environmental Science and Pollution research 2025年第17期32卷 11052-11062页

作者： He, Huan Zhou, Zi Yang Zhan, Di Zhang, Yong Xia, Wen Cheng Fu, Bo Lan, Feng Juan Tao, Xiu Xiang Huang, Zai Xing Key Laboratory of Coal Processing and Efficient Utilization of Ministry of Education School of Chemical Engineering and Technology China University of Mining and Technology Xuzhou221116 China School of Environmental and Civil Engineering Jiang Nan University Wuxi214122 China Key Laboratory of Coal Bed Methane Resource & Reserving Process of the Ministry of Education School of Resources and Geosciences China University of Mining and Technology Xuzhou221008 China Center for Biogenic Natural Gas Research Department of Civil and Architectural Engineering University of Wyoming LaramieWY82071 United States Department of Chemical and Petroleum Engineering University of Wyoming LaramieWY82071 United States

Biogenic coal bed methane has attracted great attention in recent years. During the process of biogas production, the interaction between microorganisms and coal is a crucial step. Sulfate-reducing bacteria (SRB) play an important role in biogas production. However, the interaction between SRB and coal has always remained an open problem. In the present work, the SRB strain Clostridium sp. and lignite were used to investigate the adsorption process with the extended DLVO (XDLVO) theory, calorimetry, and scanning electron microscopy (SEM). The results showed that the adsorption rate has a positive correlation with pH when it went from 3 to 8. XDLVO theoretical analysis was in good agreement with the adsorption experimental result. Acid–base potential energy is a more critical factor driving the adsorption comparing with electrostatic potential energy and Lifshitz-van Der Waals potential energy. The adsorption process of Clostridium sp. cells on lignite surface can be divided into three main stages: the direct adsorption, or reversible adsorption;desorption process;and irreversible adsorption. From the SEM results, the intercellular cohesion is also a very important adsorption form. The morphology and roughness of coal surface may also have a key effect on adsorption. Overall, our results provide some insights into the surface energy changes of Clostridium sp. adsorbed on coal and their interactions from the perspective of adsorption kinetics. © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2025.

关键词： Lignite

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Evaluation of biohydrogen production from rice straw hydrolysate via Clostridium sp. YM1: In-lab fermentation and techno-economic study

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International Journal of Hydrogen Energy 2024年 138卷 1228-1238页

作者： Mahmod, Safa Senan Krisna, Rohindran Shukor, Hafiza Abdul, Peer Mohamed AL-Rajabi, Maha Mohammad Atabani, A.E. Luthfi, Abdullah Amru Indera Gunny, Ahmad Anas Nagoor Faculty of Chemical Engineering & Technology Universiti Malaysia Perlis UniMAP Perlis Arau02600 Malaysia Centre of Excellence for Biomass Utilization Universiti Malaysia Perlis UniMAP Perlis Arau02600 Malaysia Micron Memory Malaysia Sdn Bhd Bandar Cassia Penang 14110 Malaysia Department of Chemical and Process Engineering Faculty of Engineering and Built Environment Universiti Kebangsaan Malaysia UKM Selangor Bangi43600 Malaysia Faculty of Engineering and Built Environment Universiti Kebangsaan Malaysia Selangor Bangi43600 Malaysia Green Technology Research Center Yuan Ze University Taiwan

This study investigates the potential of rice straw (RS) to be used as a feedstock for the production of biohydrogen (BioH2). To simplify the structure of the RS, thermochemical treatment is applied using HNO3 and NaOH at different concentrations. At a concentration of 1% (v/v) nitric acid (HNO3), the highest sugar concentration achieved was 27.73 g/L. This condition was utilized in dark fermentation with Clostridium sp. YM1 at 30 °C in an anaerobic environment, resulting in a biohydrogen production that surpasses the yield of the control sample by 27%. Furthermore, supplementation of 20 mg of ferrous and magnesium ions enhanced the biohydrogen yield (HY), which achieved 1.12 molH₂/molsugar and 1.19 molH₂/molsugar, respectively. This study demonstrated that butyric acid fermentation was the main pathway for Clostridium sp. YM1 to produce BioH2 from HNO3-treated RS. The findings were further evaluated for their economic profitability using SuperPro designer in batch production mode to treat 100 kgRS/batch that demonstrated the feasibility of the project with payback period (PBP), and net present value (NPV) of 3.78 years and USD 4,722,929, respectively. The study herein provides valuable insights and recommendations aimed at enhancing the feasibility of the conversion of RS into BioH2, thereby advancing the potential for sustainable bioenergy production. © 2024

关键词： Metal ions

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Higher N_(2)O production in sequencing batch reactors compared to continuous stirred tank reactors:effect of feast-famine cycles

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Frontiers of Environmental Science & engineering 2023年第4期17卷 143-154页

作者： Xinjie Yan Xunyu Shen Jipeng Wang Jinlong Zhuang Yu Wang Jinchi Yao Hong Liu Yongdi Liu James P.Shapleigh Wei Li National Engineering Research Center of Industrial Wastewater Detoxication and Resource Recovery East China University of Science and TechnologyShanghai 200237China State Environmental Protection Key Laboratory of Environmental Risk Assessment and Control on Chemical Process School of Resources and Environmental EngineeringEast China University of Science and TechnologyShanghai 200237China School of Environmental and Safety Engineering Changzhou UniversityChangzhou 213164China Shanghai Huayi Group Co.Ltd. Shanghai 201108China Shanghai Institute of Pollution Control and Ecological Security Shanghai 200237China Department of Microbiology Cornell UniversityIthacaNY 14850USA

Nitrous oxide(N_(2)O)is a potent greenhouse gas that can be emitted during the biological treatment of *** this study,a comparison of the long-term performance characteristics and N_(2)O production of sequencing batch reactors(SBR)and continuous stirred tank reactors(CSTR)during nitrite-based denitrification was *** was found that both reactors had NO_(2)^(-)-N removal efficiencies over 99.9%,but the N_(2)O-N emissions from the SBR reached~2.3%of the removal nitrite-N load,while in the CSTR it never exceeded 0.1%.High frequency sampling during one operation cycle of the SBR demonstrated that the N_(2)O accumulation ratio was~0.1%during the feast period,increased to~1.9%in the first five hours of the famine period,and then gradually reached~2.3%at the end of *** experiments showed that limiting extracellular electron donor is required for N_(2)O accumulation in cells from the SBR-famine period and that cells from the CSTR do not accumulate N_(2)O when either nitrite or carbon is *** notable difference in the two reactor communities was the high level of accumulation of intracellular granules,most likely polyhydroxybutyrate(PHB),in cells during the feast period in the *** assembly and binning found that one genome(PRO1),which is a Thauera,accounted for over half the metagenomic reads in both *** shifts in gene regulation nor community composition explained the observed differences in reactor performance suggesting some post-transcriptional regulation obligatorily linked to antecedent conditions underly increased N_(2)O production in the SBR.

关键词： Denitrifying N_(2)O mitigation SBR CSTR Meta-omics PHB

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Synergistically S/N self-doped biochar as a green bifunctional cathode catalyst in electrochemical degradation of organic pollutant

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Green Energy & Environment 2025年第1期10卷 214-230页

作者： Xuechun Wang Huizhong Wu Jiana Jing Ge Song Xuyang Zhang Minghua Zhou Raf Dewil Key Laboratory of Pollution Process and Environmental Criteria Ministry of EducationCollege of Environmental Science and EngineeringNankai UniversityTianjin300350China Tianjin Key Laboratory of Environmental Technology for Complex Trans-Media Pollution Nankai UniversityTianjin300350China Tianjin Advanced Water Treatment Technology International Joint Research Center College of Environmental Science and EngineeringNankai UniversityTianjin300350China Department of Chemical Engineering KU LeuvenJ.De Nayerlaan 5Sint-Katelijne-Waver B2860Belgium

Biomass-derived heteroatom self-doped cathode catalysts has attracted considerable interest for electrochemical advanced oxidation processes(EAOPs)due to its high performance and sustainable ***,we illustrated the morphological fates of waste leaf-derived graphitic carbon(WLGC)produced from waste ginkgo leaves via pyrolysis temperature regulation and used as bifunctional cathode catalyst for simultaneous H_(2)O_(2) electrochemical generation and organic pollutant degradation,discovering S/N-self-doping shown to facilitate a synergistic effect on reactive oxygen species(ROS)*** the optimum temperature of 800℃,the WLGC exhibited a H_(2)O_(2) selectivity of 94.2%and tetracycline removal of 99.3%within 60 *** functional theory calculations and in-situ Fourier transformed infrared spectroscopy verified that graphitic N was the critical site for H_(2)O_(2) *** pyridinic N and thiophene S were the main active sites responsible for OH generation,N vacancies were the active sites to produce ^(1)O_(2) from O_(2).The performance of the novel cathode for tetracycline degradation remains well under a wide pH range(3–11),maintaining excellent stability in 10 *** is also industrially applicable,achieving satisfactory performance treating in real water *** system facilitates both radical and non-radical degradation,offering valuable advances in the preparation of cost-effective and sustainable electrocatalysts and hold strong potentials in metal-free EAOPs for organic pollutant degradation.

关键词： Biochar S and N self-doping H_(2)O_(2)production In-situ FTIR Metal-free electrochemical advanced oxidation processes

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Design,synthesis,and biological evaluation of 1,2,4-triazole derivatives as potent antitubercular agents

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Chinese chemical Letters 2024年第3期35卷 326-331页

作者： Yu Wen Shichun Lun Yuxue Jiao Wei Zhang Tianyu Hu Ting Liu Fan Yang Jie Tang Bing Zhang William R.Bishai Li-Fang Yu Shanghai Engineering Research Center of Molecular Therapeutics and New Drug Development School of Chemistry and Molecular EngineeringEast China Normal UniversityShanghai 200062China Center for Tuberculosis Research Department of MedicineDivision of Infectious DiseaseJohns Hopkins School of MedicineBaltimoreMD21231-1044United States Shanghai Institute for Advanced Immunochemical Studies and School of Life Science and Technology ShanghaiTech UniversityShanghai 201210China Shanghai Key Laboratory of Green Chemistry and Chemical Process School of Chemistry and Molecular EngineeringEast China Normal UniversityShanghai 200062China

Inhibition of mycobacterial membrane protein large 3(MmpL3)thereby affecting the mycolic acid biosynthetic pathway has been proven to be an effective strategy for developing antitubercular *** on the X-ray crystal structure of MmpL3 inhibitor complexes,a series of novel 1,2,4-triazole derivatives were designed,synthesized and evaluated antitubercular activity against Mtb strain *** structure–activity relationship exploration resulted in the identification of compounds 21 and 28,which possess potent antitubercular activity against Mtb strain H37Rv[minimum inhibitory concentration(MIC)=0.03–0.13μg/mL]and the clinical isolates of multidrug resistance(MDR)and extensive drug resistance(XDR)tuberculosis(MIC=0.06–1.0μg/mL).Moreover,compounds 21 and 28 showed neglectable cytotoxicity(IC_(50)≥32μg/mL)to the mammalian Vero cells and favorable physicochemical and pharmacokinetic properties according to the in silico absorption,distribution,metabolism and excretion(ADME)***,the potential target of representative 1,2,4-triazole 28 was identified to be MmpL3 using a microscale thermophoresis(MST)assay.

关键词： Tuberculosis MDR and XDR-TB MmpL3 inhibitor 1 2 4-Triazole Structure-based drug design

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Development of CAE and CAD Sy1stem for Six-Axis Manipulator control System 6

Development of CAE and CAD Sy1stem for Six-Axis Manipulator ...

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6th IEEE Eurasian Conference on Educational Innovation, ECEI 2023

作者： Jhang, Hao-Jyun Chen, Chih-Cheng Zheng, Wun-Jie Chen, Chiu-Hung Yang, Cheng-Fu Yu, Wen-Yuan Department of Automatic Control Engineering Feng Chia University Taichung Taiwan School of Ocean Information Engineering Jimei University Xiamen China Department of Chemical and Materials Engineering Feng Chia University Taichung Taiwan Department of Chemical and Materials Engineering National University of Kaohsiung Kaohsiung Taiwan Research Center National Tsing Hua University Hsinchu Taiwan

ISBN: (纸本)9798350334289

Automated mechanical equipment is adjusted as the production line changes with the manipulator. Through real-time equipment monitoring and management, it is ensured that the equipment runs and adjust at any time. Modern equipment monitoring and control are used to accurately judge equipment usage status with the help of sensors, big data, the Internet, and artificial intelligence. The computer-aided design (CAD) is used to establish a six-axis manipulator including the dimensions of each axis, the speed, and acceleration of the motor, and kinematics. All the data is collected in one archive to create a 3D model and simulate and analyze its performance with the computer-aided engineering (CAE) method. © 2023 IEEE.

关键词： Computer aided design

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Continuous generation of lattice oxygen via redox engineering for boosting toluene degradation performances

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Chinese Journal of chemical engineering 2021年第6期34卷 258-266页

作者： Shiya He Zhimin You Xin Jin Yi Wu Cheng Chen He Zhao Jian Shen Department of Environment and Resources Xiangtan UniversityXiangtan 411105China State Key Laboratory of Heavy Oil Processing College of Chemical EngineeringChina University of PetroleumQingdao 266580China Beijing Engineering Research Center of Process Pollution Control Division of Environment Technology and EngineeringKey Laboratory of Green Process and EngineeringInstitute of Process EngineeringChinese Academy of SciencesBeijing 100190China

Excellent performances promoted by lattice oxygen have attracted wide attention for catalytic degradation of volatile organic compounds(VOCs).However,how to control the continuous regeneration of lattice oxygen from the support is seldom *** this study,we selected sepiolite supported manganese-cobalt oxides(Co_(x)Mn_(100-x)O_(y))as model catalysts by tuning Co/(Co+Mn)mass ratio(x=3%,10%,15%,and 20%)to enhance toluene degradation efficiency,owing to lattice oxygen regeneration by redox cycle existing at the interface and Mn species with high valence state,initiated by cobalt catalytic performance under the role of crystal field stability *** results of activity test show that the sepiolite-Co_(15)Mn_(85)O_(y)catalyst exhibit outperformances at 193℃with 10,000 h^(-1)*** addition,the catalyst existed at the bottom of the"volcano"curve correlated T_(50)or T_(90)with Co/(Co+Mn)weight ratio is sepiolite-Co_(15)Mn_(85)O_(y),conforming its *** characterized by investigating active sites structural and electronic properties,the essential of superior catalytic activity is attributed to the grands of lattice oxygen continuous formation resulted from redox engineering based on the high atomic ratio of surface lattice oxygen with continuous refilled from the support and that of Mn^(4+)/Mn^(3+)cycle initiated by cobalt catalytic *** in all,redox engineering,not only promotes grands of active species reversible regeneration,but supplies an alternative catalyst design strategy towards the terrific efficiency-to-cost ratio performance.

关键词： Redox engineering Crystal field stability phase Lattice oxygen Toluene degradation

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