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The 2^(nd)Asian Conference on Porphyrins,Phthalocyanines and Related materials

Chinese chemical Letters 2024年第7期35卷 1-3页

作者： Gaojie Zhu Zhen Yang Shijun Li Weihua Zhu Rui Cao Junlong Zhang Jianzhang Zhao Jonathan L.Sessler Xunjin Zhu Jianxin Song Yongshu Xie Jianzhuang Jiang Key Laboratory for Advanced Materials and Institute of Fine Chemicals School of Chemistry and Molecular EngineeringEast China University of Science&TechnologyShanghai 200237China College of Material Chemistry and Chemical EngineeringKey Laboratory of Organosilicon Chemistry and Material Technology of Ministry of EducationHangzhou Normal UniversityHangzhou 311121China School of Chemistry and Chemical Engineering Jiangsu UniversityZhenjiang 212013China Key Laboratory of Applied Surface and Colloid Chemistry Ministry of EducationSchool of Chemistry and Chemical EngineeringShaanxi Normal UniversityXi'an 710119China Beijing National Laboratory for Molecular Sciences State Key Laboratory of Rare Earth Materials Chemistry and ApplicationsCollege of Chemistry and Molecular EngineeringPeking UniversityBeijing 100871China State Key Laboratory of Fine Chemicals Frontier Science Center for Smart MaterialsSchool of Chemical EngineeringDalian University of TechnologyDalian 116024China Department of Chemistry The University of TexasAustinTexas 78712-1224United States Department of Chemistry and Institute of Advanced Materials Hong Kong Baptist UniversityHong Kong 999077China Key Laboratory of Chemical Biology and Traditional Chinese Medicine(Ministry of Educational of China) Key Laboratory of the Assembly and Application of Organic Functional Molecules of Hunan ProvinceCollege of Chemistry and Chemical EngineeringHunan Normal UniversityChangsha 410081China Beijing Advanced Innovation Center for Materials Genome Engineering Beijing Key Laboratory for Science and Application of Functional Molecular and Crystalline MaterialsDepartment of Chemistry and Chemical EngineeringSchool of Chemistry and Biological EngineeringUniversity of Science and Technology BeijingBeijing 100083China

In the past decades,porphyrins,phthalocyanines and related materials have attracted significant attention due to their diverse and brilliant structures[1,2],as well as their unique electronic structures and photophysi... 详细信息

关键词： cyanine phthalocyanine Porphyrin

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Recent progress and challenges in interdigital microbatteries:Fabrication, functionalization and integration

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Journal of Energy Chemistry 2023年第3期78卷 294-314,I0009页

作者： Li Song Xuting Jin Chunlong Dai Yuyang Han Jiatao Zhang Yang Zhao Zhipan Zhang Liangti Qu Key Laboratory of Cluster Science Ministry of Education of ChinaKey Laboratory of Photoelectronic/Electrophotonic Conversion MaterialsSchool of Chemistry and Chemical EngineeringBeijing Institute of TechnologyBeijing 100081China Engineering Research Center of Advanced Functional Material Manufacturing of Ministry of Education School of Chemical EngineeringZhengzhou UniversityZhengzhou 450001Henan China School of Materials Science and Engineering Beijing Institute of TechnologyBeijing 100081China Key Lab of Organic Optoelectronics and Molecular Engineering of Ministry of Education Department of ChemistryTsinghua UniversityBeijing 100084China

Currently,the increasing demands for portable,implantable,and wearable electronics have triggered the interest in miniaturized energy storage *** from conventional energy storage devices,interdigital microbatteries(IMBs) are free of separators and prepared on a single substrate,potentially achieving a short ionic diffusion path and better ***,they can be easily fabricated and integrated into on-chip miniaturized electronics,holding the promise to provide long-lasting power for advanced microelectronic *** date,while many seminal works have been reviewed the topic of microbatteries,there is no work that systematically summarizes the development of IMBs of high energy density and stable voltage platforms from fabrication,functionalization to *** current review focuses on the most recent progress in IMBs,discussing advanced micromachining techniques with compatible features to construct high-performance IMBs with smart functions and intelligent integrated *** future opportunities and challenges of IMBs are also highlighted,calling for more efforts in this dynamic and fast-growing research field.

关键词： Interdigital microbatteries Fabrication Functionalization

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Phthalocyanine self-assembled nanoparticles for type I photodynamic antibacterial therapy

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Chinese chemical Letters 2024年第12期35卷 511-516页

作者： Wei Su Xiaoyan Luo Peiyuan Li Ying Zhang Chenxiang Lin Kang Wang Jianzhuang Jiang Guangxi Key Laboratory of Natural Polymer Chemistry and Physics Nanning Normal UniversityNanning 530000China College of Pharmacy Guangxi University of Chinese MedicineNanning 530000China Beijing Advanced Innovation Center for Materials Genome Engineering Beijing Key Laboratory for Science and Application of Functional Molecular and Crystalline MaterialsDepartment of Chemistry and Chemical EngineeringSchool of Chemistry and Biological EngineeringUniversity of Science and Technology BeijingBeijing 100083China

Most photodynamic therapies(PDT)rely on reactive oxygen species(ROS)produced by type II mecha ***,since the production of type I ROS is not limited by oxygen content,making it more favorable for antimicrobial phototherapy in complex ***,we report a substituen cationization design strategy that not only improves the hydrophilicity of the prepared phthalocyanine molecule,but also promotes the electron transfer process in the photosensitizer,resulting in the strong type I photodynamic effect of the phthalocyanine self-assembled photosensitizer to efficiently generate O_(2)^(·-)under both normal and hypoxic *** in combination with its excellent bacteria recogni tion capability derived from the cationic part on its surface and intrinsic photothermal therapy effect o the phthalocyanine macrocycle endows the phthalocyanine self-assembled photosensitizer with excellen phototherapeutic antimicrobial properties in preclinical models,effectively promoting the wound healing *** work provides a promising strategy for designing efficient multi-mode photosensitizers.

关键词： Phthalocyanine Nanoparticles Photodynamic therapy Type I reactive oxygen species Antibacterial therapy

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Non-destructive buffer enabling near-infrared-transparent inverted inorganic perovskite solar cells toward 1400 h light-soaking stable perovskite/Cu(In,Ga)Se_(2) tandem solar cells

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Journal of Energy Chemistry 2024年第10期97卷 622-629,I0013页

作者： Yu Zhang Zhaoheng Tang Zhongyang Zhang Jiahong Tang Minghua Li Siyuan Zhu Wenyan Tan Xi Jin Tongsheng Chen Jinsong Hu Chao Zhou Chunlei Yang Qijie Liang Xugang Guo Weimin Li Weiqiang Chen Yan Jiang MOE Key Laboratory of Laser Life Science&Guangdong Provincial Key Laboratory of Laser Life Science Guangzhou Key Laboratory of Spectral Analysis and Functional ProbesCollege of BiophotonicsSouth China Normal UniversityGuangzhou 510631GuangdongChina school of Materials Science and Engineering Beijing Institute of TechnologyBeijing 100081China Songshan Lake Materials Laboratory Dongguan 523429GuangdongChina Department of Materials Science and Engineering Guangdong Provincial Key Laboratory of Functional Oxide Materials and DevicesSouthern University of Science and TechnologyShenzhen 518055GuangdongChina Beijing Advanced Innovation Center for Soft Matter Science and Engineering College of Chemical EngineeringCollege of Materials Science and EngineeringBeijing University of Chemical TechnologyBeijing 100029China Department of Physics Liaoning UniversityShenyang 110036LiaoningChina Beijing National Laboratory for Molecular Sciences(BNLMS) Institute of ChemistryChinese Academy of SciencesBeijing 100190China School of Physics and Materials Science Guangzhou UniversityGuangzhou 510006GuangdongChina Shenzhen Institute of Advanced Technology Chinese Academy of SciencesShenzhen 18055GuangdongChina

Near-infrared(NIR)transparent inverted all-inorganic perovskite solar cells(PSCs)are excellent top cell candidates in tandem *** essential challenge is the replacement of metal contacts with transparent conductive oxide(TCO)electrodes,which requires the introduction of a buffer layer to prevent sputtering *** this study,we show that the conventional buffers(i.e.,small organic molecules and atomic layer deposited metal oxides)used for organic-inorganic hybrid perovskites are not applicable to all-inorganic perovskites,due to non-uniform coverage of the vulnerable layers underneath,deterioration upon ion bombardment and moisture induced perovskite phase transition,A thin film of metal oxide nanoparticles by the spin-coating method serves as a non-destructive buffer layer for inorganic ***-inorganic inverted near-infrared-transparent PSCs deliver a PCE of 17.46%and an average transmittance of 73.7%between 780 and 1200 *** combination with an 18.56%Cu(In,Ga)Se_(2) bottom cell,we further demonstrate the first all-inorganic perovskite/CIGS 4-T tandem solar cell with a PCE of 24.75%,which exhibits excellent illumination stability by maintaining 86.7%of its initial efficiency after 1400 *** non-destructive buffer lays the foundation for efficient and stable NIR-transparent inverted inorganic perovskite solar cells and perovskite-based tandems.

关键词： CsPbI_(3)perovskite Inverted perovskite solar cells Tandem solar cells Buffer layer Stability

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Simultaneously enhanced interfacial shear strength and tensile strength of heterocyclic aramid fiber by graphene oxide

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Nano Research 2023年第10期16卷 12286-12293页

作者： Ziyi Zhang Xiangzheng Jia Chun Li Lanying Li Yeye Wen Zhenfei Gao Jiangwei Zhang Enlai Gao Kun Jiao Jin Zhang College of Science China University of Petroleum(Beijing)Beijing 102249China Beijing National Laboratory for Molecular Sciences School of Materials Science and EngineeringCollege of Chemistry and Molecular EngineeringBeijing Science and Engineering Center for NanocarbonsPeking UniversityBeijing 100871China Beijing Graphene Institute(BGI) Beijing 100095China Department of Engineering Mechanics School of Civil EngineeringWuhan UniversityWuhan 430072China China Bluestar Chengrand Chemical Co. Ltd.Chengdu 610041China Science Center of Energy Material and Chemistry College of Chemistry and Chemical EngineeringInner Mongolia UniversityHohhot 010021China

Heterocyclic aramid fibers,a typical kind of high-performance fibers,have been widely used in aerospace and protection fields because of their excellent mechanical ***,the application of heterocyclic aramid fibers as a reinforcement is hindered by the weak interfacial combination with matrix materials,especially *** strategies enhancing the interfacial shear strength(IFSS)usually decrease the tensile ***,simultaneous enhancement of both mechanical properties remains a ***,we report a novel heterocyclic aramid fiber with high interfacial shear strength(49.3 MPa)and tensile strength(6.27 GPa),in which 4,4′-diamino-2′-chlorobenzanilide(DABA-Cl)and a small amount of graphene oxide(GO)are introduced through in-situ *** bonds andπ–πinteraction between GO and polymer chains trigger the enhancement in crystallinity,orientation,and lateral interaction of the fibers,thus improving the tensile strength and interfacial shear strength of the ***,the interfacial interaction between fiber and epoxy is enhanced due to the improvement of the surface polarity of the fibers caused by ***,a method to improve both tensile strength and interfacial shear strength of heterocyclic aramid fibers was found by introducing GO and DABA-Cl,which may provide guidance for the design and preparation of other high-performance fibers.

关键词： heterocyclic aramid fibers graphene oxide(GO) 4 4′-diamino-2′-chlorobenzanilide(DABA-Cl) interfacial shear strength tensile strength

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Electrochemical Reduction of Benzo[b]thiophene 1,1-Dioxides with HFIP as Hydrogen Donor

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Chinese Journal of Chemistry 2024年第6期42卷 585-591页

作者： Ming-Zhong Guo Mei-Jin Mou Zhuo Chen Shao-Fei Ni Ming Li Li-Rong Wen Lin-Bao Zhang State Key Laboratory Base of Eco-Chemical Engineering College of Chemistry and Molecular EngineeringQingdao University of Science & TechnologyQingdaoShandong266042 China Department of Chemistry and Key Laboratory for Preparation and Application of Ordered Structural Materials of Guangdong Province Shantou UniversityShantouGuangdong515063 China

A straightforward electrochemical reduction of benzo[b]thiophene 1,1-dioxides with HFIP as the hydrogen donor has been reported in an undivided cell under metal-free ***,the tolerance of various functional groups and ... 详细信息

关键词： Electrochemistry Reduction Benzo[b]thiophene 1,1-dioxides Deuterium Hydrogen source

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A dynamically stable self-healable wire based on mechanical-electrical coupling

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国家科学评论（英文版） 2024年第3期11卷 244-252页

作者： Shuo Wang Zhaofeng Ouyang Shitao Geng Yan Wang Xiaoju Zhao Bin Yuan Xiao Zhang Qiuchen Xu Chengqiang Tang Shanshan Tang Han Miao Huisheng Peng Hao Sun Frontiers Science Center for Transformative Molecules School of Chemistry and Chemical EngineeringZhangjiang Institute for Advanced Studyand Key Laboratory of Green and High-End Utilization of Salt Lake Resources(Chinese Academy of Sciences)Shanghai Jiao Tong UniversityShanghai 200240China State Key Laboratory of Molecular Engineering of Polymers Department of Macromolecular ScienceInstitute of Fiber Materials and Devicesand Laboratory of Advanced MaterialsFudan UniversityShanghai 200438China School of Materials Science and Engineering East China University of Science and TechnologyShanghai 200433China

The rise in wearable electronics has witnessed the advancement of self-healable wires,which are capable of recovering mechanical and electrical properties upon structural ***,their highly fluctuating electrical resistances in the range of hundreds to thousands of ohms under dynamic conditions such as bending,pressing,stretching and tremoring may seriously degrade the precision and continuity of the resulting electronic devices,thus severely hindering their wearable ***,we report a new family of self-healable wires with high strengths and stable electrical conductivities under dynamic conditions,inspired by mechanical-electrical coupling of the myelinated axon in *** self-healable wire based on mechanical-electrical coupling between the structural and conductive components has significantly improved the electrical stability under dynamic scenarios,enabling precise monitoring of human health status and daily activities,even in the case of limb tremors from simulated Parkinson's *** mechanical-electrical coupling strategy opens a new avenue for the development of dynamically stable electrodes and devices toward real-world wearable applications.

关键词： self-healable wire interfacial chemistry polymer materials mechanical–electrical coupling fiber device

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Unassisted photoelectrochemical CO_(2)reduction by employingⅢ-Ⅴphotoelectrode with 15%solar-to-fuel efficiency

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Carbon Energy 2025年第3期7卷 1-10页

作者： Karthik Peramaiah Purushothaman Varadhan Vinoth Ramalingam Bilawal Khan Pradip Kumar Das Hao Huang Hui-Chun Fu Xiulin Yang Vincent Tung Kuo-Wei Huang Jr-Hau He Chemistry Program Center for Renewable Energy and Storage Technologies(CREST)and Division of Physical Science and EngineeringKing Abdullah University of Science and Technology(KAUST)ThuwalSaudi Arabia Institute of Sustainability for Chemicals Energyand Environment(ISCE2)Agency for ScienceTechnologyand Research(A*STAR)Singapore School of Computing Engineering and TechnologyRobert Gordon UniversityAberdeenUK Department of Materials Science and Engineering City University of Hong KongKowloonSARHong KongChina Guangxi Key Laboratory of Low Carbon Energy Materials School of Chemistry and Pharmaceutical SciencesGuangxi Normal UniversityGuilinChina Department of Chemical System and Engineering University of TokyoTokyoJapan

Solar-driven carbon dioxide reduction reaction(CO_(2)RR)provides an oppor tunity to produce value-added chemical feedstocks and ***,achieving efficient and stable photoelectrochemical(PEC)CO_(2)RR into selec tive products is challenging owing to the difficulties associated with the optical and the electrical configuration of PEC devices and electrocatalyst ***,we construct an efficient,concentrated sunlight-driven CO_(2)RR setup consisting of InGaP/GaAs/Ge triple-junction cell as a photoanode and oxide-derived Au(Ox-Au)as a cathode to perform the unassisted PEC CO_(2)*** one-sun illumination,a maximum operating current density of 11.5 mA cm^(-2) with an impressive Faradaic efficiency(FE)of~98%is achieved for carbon monoxide(CO)production,leading to a solar-to-fuel conversion efficiency of~15%.Under concentrated intensity of 10 sun,the photoanode records a maximum current density of~124 mAcm^(-2) and maintains~60%of FE for CO *** results demonstrate crucial advancements in usingⅢ-Ⅴbased photoanodes for concentrated PEC CO_(2)RR.

关键词： 3J photoanode CO_(2)reduction high STF unassisted PEC

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High Fluorescence Porous Organic Cage for Sensing Divalent Palladium Ion and Encapsulating Fine Palladium Nanoparticles

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Chinese Journal of Chemistry 2022年第3期40卷 385-391页

作者： Huimin Ren Chao Liu Xu Ding Xianzhang Fu Hailong Wang Jianzhuang Jiang Beijing Advanced Innovation Center for Materials Genome Engineering Beijing Key Laboratory for Science and Application of Functional Molecular and Crystalline MaterialsDepartment of Chemistry and Chemical EngineeringSchool of Chemistry and Biological EngineeringUniversity of Science and Technology BeijingBeijing 100083China

Porous organic cages(POCs)as an innovative type of porous molecular materials enable multifunctional ***,a fluorescence POC(denoted as 1)has been constructed by means of 5/5'-((2/5-dimethoxy-l/4-phenylene)bis(ethyne-2/1-diyl))diiso-phthalaldehyde condensing with cyclohexanediamine enantiomer with the aid of trifluoroacetic acid.1 exhibits the permanent void and prominent fluorescence with relative quantum yield of 73%confirmed by gas sorption and emission experiments,***,this organic cage is capable of sensing diavalent Pd2+according to the fluorescence response to the addition of various metal *** dispersion of 1 in methanol containing palladium acetate was stirred at 25℃and then 80℃to reduce Pd2+ions into nanoparticles(NPs),leading to the composite(Pd@l)composed of fine Pd NPs with the size of co.1.8 *** catalytic nature of Pd@l over NaBH4 promoted the degeneration of nitrobenzene and congo *** work introduces one new case of POCs with versatile properties and functions,including ion fluorescence recognition,fine Pd NPs stabilizer,and gas adsorption,enriching the family of POC-based materials.

关键词： Catalysis Fluorescence recognition Nanoparticles Cage compounds Palladium

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An amorphous manganese iron oxide hollow nanocube cathode for aqueous zinc ion batteries

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Journal of Energy Chemistry 2023年第12期87卷 314-321,I0008页

作者： Fengyang Jing Chade Lv Liangliang Xu Yaru Shang Jian Pei Pin Song Yuanheng Wang Gang Chen Chunshuang Yan MIIT Key Laboratory of Critical Materials Technology for New Energy Conversion and Storage School of Chemistry and Chemical EngineeringHarbin Institute of TechnologyHarbin 150001HelongjiangChina Department of Chemical and Biomolecular Engineering Korea Advanced Institute of Science and Technology(KAIST)Daejeon 34141Republic of Korea Key Laboratory of Functional Molecular Solids Ministry of EducationAnhui Engineering Research Center of Carbon NeutralityCollege of Chemistry and Materials ScienceAnhui Normal UniversityWuhu 241000AnhuiChina

Aqueous zinc ion batteries(ZIBs) are attracting considerable attentions for practical energy storage because of their low cost and high ***,the traditional manganese oxide cathode materials suffer from the low intrinsic electronic conductivity,sluggish ions diffusion kinetics,and structural collapse,hindering their large-scale ***,we successfully developed a latent amorphous Mn_(1.8)Fe_(1.2)O_(4) hollow nanocube(a-H-MnFeO) cathode material derived from Prussian blue analogue *** amorphous nature endows the cathode with lower diffusion barrier and narrower band gap compared with crystalline counterpart,resulting in the superior Zn^(2+) ions and electrons transport *** structure can furnish abundant surface sites and suppress the structural collapse during the repeated charge/discharge *** virtue of the multiple advantageous features,the a-H-MnFeO cathode exhibits exceptional electrochemical performance,in terms of high capacity,excellent rate capability,and prolonged cycle *** strategy will pave the way for the structural design of emerging cathode materials.

关键词： Aqueous zinc-ion batteries Manganese iron oxide cathode Amorphous structure Hollow nanostructure lons transport kinetics

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