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Coherent Cu-rich nanoprecipitates: Achieving both high strength and superior magnetic properties in non-oriented silicon steels

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Journal of Materials Science and technology 2025年 233卷 319-333页

作者： Cheng, Zhaoyang Wen, Qiuyue Zhong, Bolin Liang, Yongfeng Zhang, Xiaobin Liu, Jing The State Key Laboratory of Refractories and Metallurgy Wuhan University of Science and Technology Wuhan430081 China State Key Laboratory for Advanced Metals and Materials University of Science and Technology Beijing Beijing 100083 China Guangdong Provincial Key Laboratory of New Energy Materials Service Safety College of Material Science and Engineering Shenzhen University Shenzhen518060 China Hubei Engineering Technology Research Center of Marine Materials and Service Safety Wuhan University of Science and Technology Wuhan430081 China

Non-oriented silicon steels with both excellent magnetic properties and high strength are essential for the drive motors of new energy vehicles. However, achieving a balance between strength and magnetic properties is a challenging task. This study successfully developed non-oriented silicon steel that met these demanding requirements by utilizing the coherent nano-Cu-rich phases precipitated during aging. In the current investigation, the evolution of precipitation during the aging process of Cu-alloyed non-oriented silicon steel is revealed as: BCC Cu-rich cluster (Fe:Cu > 1) → B2 FeCu cluster (Fe:Cu approaches 1) → BCC Cu cluster (Fe:Cu 1.0/400 of 16.3–18.3 W kg−1, and B5000 of 1.641–1.656 T. © 2025

关键词： Silicon steel

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Highly electrically conductive MOF/conducting polymer nanocomposites toward tunable electromagnetic wave absorption

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材料科学技术（英文版） 2025年第2期205卷 258-269页

作者： Xin Wu Peiyuan Kang Yinghan Zhang Haocheng Guo Shuoying Yang Qi Zheng Lianjun Wang Wan Jiang State Key Laboratory for Modification of Chemical Fibers and Polymer Materials & College of Materials Science and Engineering Donghua UniversityShanghai 201620China State Key Laboratory for Modification of Chemical Fibers and Polymer Materials & College of Materials Science and Engineering Donghua UniversityShanghai 201620China Engineering Research Center of Advanced Glasses Manufacturing Technology Ministry of EducationDonghua UniversityShanghai 201620China State Key Laboratory for Modification of Chemical Fibers and Polymer Materials & College of Materials Science and Engineering Donghua UniversityShanghai 201620China Institute of Functional Materials Donghua UniversityShanghai 201620China

Metal-organic frameworks(MOFs)have attracted significant interest as self-templates and precursors for the synthesis of carbon-based composites aimed at electromagnetic wave(EMW)***,the utilization of high-temperature treatments has introduced uncertainties regarding the compositions and microstructures of resulting ***,complete carbonization has led to diminished yields of the produced carbon composites,significantly limiting their practical ***,the exploration of pristine MOF-based EMW absorbers presents an intriguing yet challenging endeavor,primarily due to inherently low electrical *** this study,we showcase the utilization of struc-turally robust Zr-MOFs as scaffolds to build highly conductive Zr-MOF/PPy composites via an inner-outer dual-modification approach,which involves the production of conducting polypyrrole(PPy)both within the confined nanoporous channels and the external surface of Zr-MOFs via post-synthetic *** interconnection of confined PPy and surface-lined PPy together leads to a consecutive and extensive conducting network to the maximum *** therefore entails outstanding conductivity up to～14.3 S cm-1 in Zr-MOF/PPy composites,which is approximately 1-2 orders of magnitude higher than that for conductive MOF nanocomposites constructed from either inner or outer *** from the strong and tunable conduction loss,as well as the induced dielectric polarization originated from the porous structures and MOF-polymer interfaces,Zr-MOF/PPy exhibits excellent microwave attenuation capabilities and a tunable absorption frequency ***,with only 15 wt.％loading,the mini-mum reflection loss(RLmin)can reach up to-67.4 dB,accompanied by an effective absorption bandwidth(EAB)extending to 6.74 ***,the microwave absorption characteristics can be tailored from the C-band to the Ku-band by adjusting the loading of *** work provide

关键词： Conductive mof nanocomposites electromagnetic wave absorption MOF/conducting polymer Electrical conductivity Zr-MOF/PPy

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Incommensurate modulated structure and its influence on the martensitic transformation temperature span of single phase multielement Ni-Cu-Co-Mn-Ga two-way shape memory single crystals

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材料科学技术（英文版） 2025年第5期208卷 230-240页

作者： Qijjia Yu Yang Liu Chen Si Wenjia Wang Jiaxi Meng Jingmin Wang Jinghua Liu Chengbao Jiang Key Laboratory of Advanced Aerospace Materials and Performance(Ministry of Education) School of Materials Science and EngineeringBeihang UniversityBeijing 100191PR China Center of Microstructure Science Frontier Institute of Science and TechnologyState Key Laboratory for Mechanical Behavior of MaterialsXi'an Jiaotong UniversityXi'an 710049PR China

Significant two-way shape memory effect(TWSME)was achieved in single crystals of single-phase mul-tielement Ni42-xCu8CoxMn37Ga13(8 ≤ x ≤ 12)alloys by performing thermomechanical ***,anomalous dependence of the martensitic transformation temperature span on Co content was *** training,quite a narrow temperature span of the martensitic transformation,nearly independent of the Co content,was observed in all single *** training the temperature span was still narrow for 8 ≤ x ≤ 10.9 but was obviously expanded for 10.9＜x ≤ ***-resolution transmission electron microscopy revealed that at the atomic scale,there exists incommensurate modulated structure in the single phase single crystals,as evidenced by nonperiodic satellite spots in the selected area electronic diffraction ***,the modulated wave vector of the satellite spots was increased by higher Co *** first principal calculations it was considered that the incommensurate modulated structure originates from the formation of Co-Co *** training arrays of ordered dislocations with the same Burgers vector were introduced for 8 ≤ x ≤ 10.9 but the network of dislocations was formed for 10.9＜x ≤ *** on analysis of transmission electron microscopy,geometric phase,thermody-namics,and Landau theory,it was considered that the austenite/martensite phase interface was pinned by the network of dislocations,expanding the temperature span of the martensitic *** work supplies new insights for understanding the microstructure and martensitic transformation of Ni-Mn-Ga-based alloys.

关键词： Martensitic transformation Incommensurate modulated structure Temperature span Dislocation Two-way shape memory effect

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Fatigue failure analysis and heat treatment strategy optimization of torsion bar spring for automobile suspension system used in light vehicles

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Journal of Iron and Steel Research International 2025年第3期32卷 799-811页

作者： Jia-xing Liu Yong-jin Wu Chao-lei Zhang Wan-li Sun Wen-bin Ding Shuai-jun Dong Institute for Carbon Neutrality School of Materials Science and EngineeringUniversity of Science and Technology BeijingBeijing100083China State Key Laboratory for Advanced Metals and Materials University of Science and Technology BeijingBeijing100083China Institute of Steel Sustainable Technology Liaoning Academy of MaterialsShenyang110167LiaoningChina

The failure analysis was conducted on unqualified torsion bar spring in automobile suspension system used for light vehicles during engine *** effects of through hardening,surface induction hardening,quenching and tempering,and tempering temperature on the microstructure and fatigue life of 45CrNiMoVA steel torsion bars were also *** showed that only the torsion bar spring after through quenching and tempering is subjected to surface induction quenching and tempering to achieve the fatigue life of the qualified torsion *** fatigue life of torsion bar spring reaches 3×10^(5) cycles more than the required 2×10^(5) *** is because the distribution of gradient microstructure was helpful to relieve the applied stress during the fatigue *** microstructure of the non-hardened region,which consists of tempered sorbite regardless of whether it is tempered at 330 or 430℃,contributes to minimizing the impact of temper brittleness on the fatigue life of the torsion ***,the fatigue life of the torsion bar is relatively unaffected by temper brittleness due to the presence of tempered sorbite in its non-hardened *** the reason for the unqualified fatigue life was that the depth and hardness of the hardened region did not meet the standard requirements of 5–7 mm and 47–52 HRC,respectively.

关键词： Fatigue life Torsion bar Tempering temperature 45CrNiMoVA steel Fracture

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NaTiOx-modified high-nickel layered oxide cathode for stable sodium-ion batteries

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Carbon Energy 2025年第1期7卷 283-291页

作者： Yingcong Liu Xing Zhou Dongwei He Xiaowei Liu Chao Yang Dawei Xu Meilong Wang Ruitao Sun Bin Zhang Jingjing Xie Jin Han Wen Chen Ya You State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China Yibin Libode New Materials Co.Ltd SichuanChina International School of Materials Science and Engineering School of Materials Science and MicroelectronicsWuhan University of TechnologyWuhan 430070China

The O3-type layered cathode with high Ni content has attracted much attention because of its high capacity and simple synthesis ***,surface side reaction and O3-P3 phase transitions would occur during Na+insertion/extraction,resulting in unsatisfying electrochemical ***,O3-Na[Ni_(0.6)Co_(0.2)Mn_(0.2)]O_(2)(NNCM622)cathode is modified by a NaTiOx coating layer in a wet chemistry method,which reduces the parasitic reaction and facilitates Na+***,the partially doped Ti improves structural stability by restraining the irreversible multiple-phase *** a result,the modified NNCM622 cathode obtains a high specific capacity of 143.4 mAh g^(−1)and an improved capacity retention of 69%after 300 *** work offers new prospects for stabilizing the NNCM622 cathode with a feasible coating strategy.

关键词： cathode high-nickel layered oxides sodium-ion battery surface modification

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Editorial for Special Issue on Contact Electrification

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Friction 2025年第2期13卷 1-2页

作者： Shiquan Lin Chi Zhang Tianmin Shao School of Mechanical Engineering Beijing Institute of TechnologyBeijing 100081China Beijing Institute of Nanoenergy and Nanosystems Chinese Academy of SciencesBeijing 100083China State Key Laboratory of Tribology in Advanced Equipment Tsinghua UniversityBeijing 100084China

Contact electrification is a pervasive and complex phenomenon that has been known for more than 2,600 years,and its mechanisms have been debated for decades but remain ***,contact electrification has long been considered an unpredictable effect,which has hindered its *** recent years,the study of contact electrification is in full swing,its mechanism has been analyzed in great depth,and its role in tribology,chemistry,biology,etc.,has been increasingly *** on the phenomenon of contact electrification,various sensing and energy harvesting devices have been *** the past decade,research on the mechanism and application of contact electrification has made great progress,and this phenomenon has become a hot spot in the tribological research community.

关键词： mechanism harvesting contact

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Kinetic investigation of the energy storage process in graphene fiber supercapacitors:Unraveling mechanisms,fabrications,property manipulation,and wearable applications

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Carbon Energy 2025年第1期7卷 133-173页

作者： Juan Zhang Wenwen Liu Minzhi Du Qingli Xu Minren Hung Ruifang Xiang Meng Liao Xinhou Wang Bingjie Wang Aiping Yu Kun Zhang Key Laboratory of Textile Science and Technology(Donghua University) Ministry of EducationCollege of TextilesDonghua UniversityShanghaiChina Department of Chemical Engineering Waterloo Institute for NanotechnologyUniversity of WaterlooWaterlooONCanada Laboratory of Advanced Materials State Key Laboratory of Molecular Engineering of PolymersDepartment of Macromolecular ScienceFudan University2205 Songhu RdShanghai 200438China College of Mechanical Engineering Donghua UniversityShanghai 201620China

Graphene fiber supercapacitors(GFSCs)have garnered significant attention due to their exceptional features,including high power density,rapid charge/discharge rates,prolonged cycling durability,and versatile weaving ***,inherent challenges in graphene fibers(GFs),particularly the restricted ion-accessible specific surface area(SSA)and sluggish ion transport kinetics,hinder the achievement of optimal capacitance and rate *** existing reviews on GFSCs,a notable gap exists in thoroughly exploring the kinetics governing the energy storage process in *** review aims to address this gap by thoroughly analyzing the energy storage mechanism,fabrication methodologies,property manipulation,and wearable applications of *** theoretical analysis of the energy storage process,specific parameters in advanced GF fabrication methodologies are carefully summarized,which can be used to modulate nano/micro-structures,thereby enhancing energy storage *** particular,enhanced ion storage is realized by creating more ion-accessible SSA and introducing extra-capacitive components,while accelerated ion transport is achieved by shortening the transport channel length and improving the accessibility of electrolyte *** on the established structure-property relationship,several critical strategies for constructing optimal surface and structure profiles of GF electrodes are *** on the exceptional flexibility and wearability of GFSCs,the review further underscores their potential as foundational elements for constructing multifunctional e-textiles using conventional textile *** conclusion,this review provides insights into current challenges and suggests potential research directions for GFSCs.

关键词： fiber-shaped supercapacitor graphene ion storage ion transport wearable application

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The analysis and assessment of DC-Link voltage control loop dynamics on the transient synchronization stability of grid-following converters

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Electric Power Systems Research 2025年 247卷

作者： Xie, Chenyang Lin, Xinchun Sun, Huiqiang Wei, Juntian Zhang, Jiayan State Key Laboratory of Advanced Electromagnetic Engineering and Technology Huazhong University of Science and Technology Wuhan China

The transient synchronization stability of grid-following voltage source converters has been extensively investigated, but most of the previous literature has only studied the transient dynamics of the phase-locked loop (PLL) while ignoring the dynamics of the DC-link voltage control (DVC) loop. When the bandwidths of the PLL and DVC are relatively close to each other, erroneous conclusions will be derived if neglecting the transient influence of the DVC loop. This paper first takes into account the transient dynamics of the DVC loop while applying the improved equal-area criterion (EAC) analysis, which reveals how the DVC loop affects the transient synchronization stability. Then, a fourth-order model considering the DVC dynamics is obtained to quantitatively determine a reasonable range of bandwidth and damping ratio for the DVC loop. Moreover, the extent of the influence of DVC on transient synchronization stability with variation of grid strength is analyzed. © 2025

关键词： Transient analysis

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Large-scale high uniform optoelectronic synapses array for artificial visual neural network

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Microsystems & Nanoengineering 2025年第1期11卷 247-256页

作者： Fanqing Zhang Chunyang Li Zhicheng Chen Haiqiu Tan Zhongyi Li Chengzhai Lv Shuai Xiao Lining Wu Jing Zhao State Key Laboratory of Explosion Science and Safety Protection Beijing Institute of TechnologyMinistry of Education100081 BeijingChina School of Mechatronical Engineering Beijing Institute of Technology100081 BeijingChina Beijing Advanced Innovation Center for Intelligent Robots and Systems Beijing Institute of Technology100081 BeijingChina Laser Micro/Nano Fabrication Laboratory School of Mechanical EngineeringBeijing Institute of Technology100081 BeijingChina School of Mechanical Engineering Beijing Institute of Technology100081 BeijingChina

Recently,the biologically inspired intelligent artificial visual neural system has aroused enormous ***,there are still significant obstacles in pursuing large-scale parallel and efficient visual memory and *** this study,we demonstrate a 28×28 synaptic devices array for the artificial visual neuromorphic system,within the size of 0.7×0.7 cm 2,which integrates sensing,memory,and processing *** highly uniform floating-gate synaptic transistors array were constructed by the wafer-scale grown monolayer molybdenum disulfide with Au nanoparticles(NPs)acting as the electrons capture *** synaptic plasticity behaviors have been achieved owing to the switchable electronic storage *** excellent optical/electrical coordination capabilities were implemented by paralleled processing both the optical and electrical signals the synaptic array of 784 devices,enabling to realize the badges and letters writing and erasing ***,the established artificial visual convolutional neural network(CNN)through optical/electrical signal modulation can reach the high digit recognition accuracy of 96.5%.Therefore,our results provide a feasible route for future large-scale integrated artificial visual neuromorphic system.

关键词： optoelectronic synapses monolayer molybdenum disulfide artificial visual neural system convolutional neural network artificial visual neuromorphic systemwithin artificial visual neural network floating gate transistors synaptic plasticity

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Visible-light-induced controllable transformations of cumulative aryldienes through an energy transfer process

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Science china Chemistry 2025年第3期68卷 987-1001页

作者： Ling Qian Ziqi Yu Jiaxin Liu Yin Wei Min Shi Key Laboratory for Advanced Materials and Institute of Fine Chemicals Key Laboratory for Advanced Materials and Feringa Nobel Prize Scientist Joint Research CenterSchool of Chemistry&Molecular EngineeringEast China University of Science and TechnologyShanghai 200237China State Key Laboratory of Organometallic Chemistry Center for Excellence in Molecular SynthesisUniversity of Chinese Academy of SciencesShanghai Institute of Organic ChemistryChinese Academy of SciencesShanghai 200032China Key Laboratory of Fluorine and Nitrogen Chemistry and Advanced Materials Shanghai Institute of Organic ChemistryUniversity of Chinese Academy of SciencesChinese Academy of SciencesShanghai 200032China

In this work,we report a visible light-induced energy transfer process related photochemical protocol of cumulative diene containing compounds for the construction of benzocyclohexene skeletons or the corresponding aromatized structures through an energy transfer process,1,5-hydrogen atom transfer and a 6πelectrocyclization or demethoxylation in the presence of different photocatalysts such as[Ir(dF(Me)ppy)_(2)(dtbbpy)]PF_(6) or *** newly developed photochemical strategy is characterized by mild conditions,broad substrate applicability,good functional group tolerance and good *** mechanistic paradigm was clarified by deuterium labeling,kinetic,photophysical and electrochemical analyses,control experiments and density functional theory(DFT)*** transformation of the obtained product to the drug-like molecules such as Sertraline and the luminescent conjugated aromatic compounds has also been disclosed.

关键词： visible-light photocatalysis EnT process 1,5-HAT remote C(sp^(3))-H bond activation

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