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Multifunctional dual-anion compensation of amphoteric glycine hydrochloride enabled highly stable perovskite solar cells with prolonged carrier lifetime

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Nano Research 2024年第6期17卷 5131-5137页

作者： Lina Qin Mengfei Zhu Yuren Xia Xingkai Ma Daocheng Hong Yuxi Tian Zuoxiu Tie Zhong Jin State Key Laboratory of Coordination Chemistry MOE Key Laboratory of Mesoscopic ChemistryMOE Key Laboratory of High Performance Polymer Materials and TechnologyJiangsu Key Laboratory of Advanced Organic MaterialsSchool of Chemistry and Chemical EngineeringNanjing UniversityNanjing 210023China Nanjing Tieming Energy Technology Co.Ltd. Nanjing 210093China Suzhou Tierui New Energy Technology Co.Ltd. Suzhou 215228China

Throughout years,the two-step spin-coating process is the most common method to prepare organic lead halide perovskite ***,the short reaction time of dropping the solution at the second step means that PbI2 cannot be completely transformed into perovskite *** solve this problem,we report the introduction of glycine hydrochloride(GlyHCl)into the second step of the two-step spin-coating process to prepare a FA_(0.9)MA_(0.1)PbI_(3-x)%-GlyHCl perovskite material(namely FAMA-x%-GlyHCl,where FA=formamidinium,MA=methylammonium,and x%stands for the molar ratio of GlyHCl added in FA iodide/MA iodide(FAI/MAI)precursor solution).The Cl−ion in GlyHCl assists the formation ofα-phase perovskite,and the-COO−group coordinates with Pb2+cation in a bridging way,making up for the anion vacancy in perovskite lattice and resulting in high absorption *** perovskite solar cells(PSCs)based on FAMA-9%-GlyHCl achieve a long carrier lifetime(527.0 ns),a photoelectric conversion efficiency(PCE)of 19.40%and good thermal stability,maintaining 85.8%of the initial PCE after being continuously heated at 60℃for 500 *** study helps to solve the problem of incomplete reaction in the two-step spin-coating process and puts forward a new solution for preparing high coverage perovskite films with large grain size.

关键词： dual-anion compensation glycine hydrochloride perovskite solar cells carrier lifetime thermal and moisture stability

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Towards optimized tensor code generation for deep learning on sunway many-core processor

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Frontiers of Computer Science 2024年第2期18卷 1-15页

作者： Mingzhen LI Changxi LIU Jianjin LIAO Xuegui ZHENG Hailong YANG Rujun SUN Jun XU Lin GAN Guangwen YANG Zhongzhi LUAN Depei QIAN State Key Laboratory of Software Development Environment Beijing 100191China School of Computer Science and Engineering Beihang UniversityBeijing 100191China National University of Singapore Singapore 119077Singapore State Key Laboratory of Mathematical Engineering and Advanced Computing Wuxi 214000China Science and Technology on Special System Simulation Laboratory Beijing Simulation Center Beijing 100854China Department of Computer Science and Technology Tsinghua UniversityBeijing 100084China

The flourish of deep learning frameworks and hardware platforms has been demanding an efficient compiler that can shield the diversity in both software and hardware in order to provide application *** the existing deep learning compilers,TVM is well known for its efficiency in code generation and optimization across diverse hardware *** the meanwhile,the Sunway many-core processor renders itself as a competitive candidate for its attractive computational power in both scientific computing and deep learning *** paper combines the trends in these two ***,we propose swTVM that extends the original TVM to support ahead-of-time compilation for architecture requiring cross-compilation such as *** addition,we leverage the architecture features during the compilation such as core group for massive parallelism,DMA for high bandwidth memory transfer and local device memory for data locality,in order to generate efficient codes for deep learning workloads on *** experiment results show that the codes generated by swTVM achieve 1.79x improvement of inference latency on average compared to the state-of-the-art deep learning framework on Sunway,across eight representative *** work is the first attempt from the compiler perspective to bridge the gap of deep learning and Sunway processor particularly with productivity and efficiency in *** believe this work will encourage more people to embrace the power of deep learning and Sunwaymany-coreprocessor.

关键词： sunway processor deep learning compiler code generation performance optimization

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Grid Forming Converters in Renewable Energy Sources Dominated Power Grid:Control Strategy,Stability,Application,and Challenges

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Journal of Modern Power Systems and Clean Energy 2021年第6期9卷 1239-1256页

作者： Haobo Zhang Wang Xiang Weixing Lin Jinyu Wen State Key Laboratory of Advanced Electromagnetic Engineering and Technology Huazhong University of Science and Technology TBEA Sunoasis Company Ltd. the State Key Laboratory of Advanced Electromagnetic Engineering and Technology Huazhong University of Science and Technology

The renewable energy sources(RESs)dominated power grid is an envisaged infrastructure of the future power system,where the commonly used grid following(GFL)control for grid-tied converters suffers from lacking grid support capability,low stability,***,emerging grid forming(GFM)control methods have been proposed to improve the dynamic performance and stability of grid-tied *** paper reviews existing GFM control methods for the grid-tied converters and compares them in terms of control structure,grid support capability,fault current limiting,and *** the impact of fault current limiting strategies,a comprehensive transient stability analysis is *** addition,this paper explores the typical applications of GFM converters,such as AC microgrid and offshore wind farm high-voltage direct current(OWF-HVDC)integration ***,the challenges to the GFM converters in future applications are discussed.

关键词： Grid following(GFL)control grid forming(GFM)control high-voltage direct current(HVDC) microgrid renewable energy small-signal stability transient stability

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Design of a new low power protection method for pumped storage synchronous motor 9

Design of a new low power protection method for pumped stora...

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9th International Conference on Energy Materials and Electrical engineering, ICEMEE 2023

作者： Qiao, Jian He, Rufei Yin, Xianggen Ma, Yiming Lu, Qinghui Peng, Yumin Wang, Wenhui Zhang, Hao State Key Laboratory of Advanced Electromagnetic Engineering and Technology Huazhong University of Science and Technology Wuhan430074 China CSG PGC Power Storage Research Institute Guangzhou510950 China

ISBN: (纸本)9781510672765

In this paper, the characteristics of power oscillation of pumped storage synchronous motor under pumped condition are studied, and the causes of misoperation of conventional low power protection are analyzed. Based on digital simulation and actual data analysis, a multi-stage low power protection is proposed. The power setting value of each section matches the delay setting value, which can adapt to the characteristics of motor power oscillation and effectively solve the misoperation problem of conventional low power protection. The simulation results show that its performance is stable and reliable, and the problem of misoperation of conventional low power protection is solved. © COPYRIGHT SPIE. Downloading of the abstract is permitted for personal use only.

关键词： Failure analysis engineering Silver Analytical research Design and modelling Reliability Frequency modulation Phase modulation Safety Power grids

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Relay C(sp^(3))-H bond trifluoromethylthiolation and amidation by visible light photoredox catalysis

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Science china Chemistry 2024年第11期67卷 3844-3850页

作者： Junheng Liu Suqi Yang Shunruo Yao Chengjian Zhu Yong Liu Weipeng Li Jin Xie State Key Laboratory of Coordination Chemistry Jiangsu Key Laboratory of Advanced Organic MaterialsChemistry and Biomedicine Innovation Center(ChemBIC)School of Chemistry and Chemical EngineeringNanjing UniversityNanjing 210023China Green Catalysis Center College of ChemistryZhengzhou UniversityZhengzhou 450001China State Key Laboratory of Organometallic Chemistry Shanghai Institute of Organic ChemistryShanghai 200032China Nanjing Bready Advanced Materials Technology Co. Ltd.Nanjing 221100China State Key Laboratory of Natural Medicines China Pharmaceutical UniversityNanjing 211198China

Selective functionalization of C(sp^(3))–H bonds is a straightforward and practical method to construct complex molecule skeletons. In this field, direct transformation of unactivated C(sp^(3))–H bonds into C(sp^(3))–SCF_(3) architectures is still a great *** report a highly selective trifluoromethylthiolation of unactivated aliphatic C(sp^(3))–H bonds by combination of proton-coupled electron transfer(PCET) and hydrogen atom transfer(HAT) strategy. A wide range of structurally diverse alkyl trifluoromethyl sulfides are obtained. Furthermore, the use of two different photocatalysts can realize an unprecedented trifluoromethylthiolation and amidation cascade of different C(sp^(3))–H bonds. It can afford a good access to bifunctionalized molecules in synthetically useful yields.

关键词： photoredox catalysis C–H activation trifluoromethylthiolation amidation PCET

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Interface catalytic reduction of alumina by nickle for the aluminum nanowire growth: Dynamics observed by in situ TEM

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Nano Research 2024年第3期17卷 1225-1231页

作者： Zichun Wang Dan Wang Ang Li Lizhuo Wang Xiaodong Han Yijiao Jiang Jianfeng Chen Jun Huang Beijing Advanced Innovation Center for Soft Matter Science and Engineering State Key Laboratory of Organic–Inorganic CompositesBeijing University of Chemical TechnologyBeijing 100029China Laboratory for Catalysis Engineering School of Chemical and Biomolecular EngineeringThe University of SydneyNew South Wales 2006Australia Beijing Key Laboratory of Microstructure and Property of Advanced Materials Beijing University of TechnologyBeijing 100024China Department of Engineering Macquarie UniversitySydneyNew South Wales 2109Australia

Metal nanowires show promise in a broad range of applications and can be fabricated via a number of methods,such as vapor–liquid–solid process and template-based ***,the synthesis of Al nanowires(NWs)is still challenging from the stable alumina *** this work,the Ni-catalyzed fabrication of Al NWs has been realized using various Al_(2)O_(3) *** growth dynamics of Al NWs on Ni/Al_(2)O_(3) was studied using in situ transmission electron microscopy(TEM).The effect of alumina structures,compositions,and growth temperature were *** growth of Al NWs correlates with the Na addition to the alumina *** no eutectic mixture of nickel aluminide was formed,a mechanism of Ni-catalyzed reduction of Al_(2)O_(3) for Al NWs growth has been proposed instead of the vapor–liquid–solid *** key insights reported here are not restricted to Ni-catalyzed Al NWs growth but can be extended to understanding the dynamic change and catalytic performance of Ni/Al_(2)O_(3) under working conditions.

关键词： in situ transmission electron microscopy(TEM) Al nanowires alumina reduction nanowire growth

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Characteristics Evaluation of SiC MOSFET in DC Circuit Breaker

Characteristics Evaluation of SiC MOSFET in DC Circuit Break...

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2024 CPSS and IEEE International Symposium on Energy Storage and Conversion, CPSS and ISESC 2024

作者： Guo, Zhongqi Liang, Lin Wan, Xiangyu Qing, Zhengheng Zhang, Ziyang Yan, Xiaoxue School of Electrical and Electronic Engineering Engineering Research Center of Power Safety and Efficiency Ministry of Education of China Huazhong University of Science and Technology State Key Laboratory of Advanced Electromagnetic Technology Wuhan China

ISBN: (纸本)9798350380514

In order to evaluate the characteristics of SiC MOSFET under the mission profile of DC Circuit Breaker (DCCB), a complete DCCB test platform considering the RCD transfer loop and the MOV absorption loop is set up. Based on this platform, single and repetitive short-circuit interrupting experiments are carried out. Through these tests, the characteristics evaluation of 1200V/66A SiC MOSFET under DCCB is tested and analyzed. The aging test results are given. DCCB has its unique mission profile (interruption of large short-circuit current, fast current transfer, etc.), and the characteristics evaluation of SiC MOSFET in DCCB is necessary. For the single tests, the maximum interrupted current is 2.02 times the rated current. For the repetitive tests, the number of interruptions exceeds 2000 times and the interruption boundary is 2004 times under 1.85 times rated current. The failure causes of the devices in two cases are drain thermal failure and gate-source short circuit respectively. After 2000 experiments, the interruption time of DCCB increased significantly, and the Idss, Vgs(th), and Rds(on) of the device increased by about 53.36%, 4.29%, and 16.94% respectively. © 2024 IEEE.

关键词： MOSFET devices

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Inverse Design of electromagnetic Induced Transparency Metamaterials Based on Generative Adversarial Network 4

Inverse Design of Electromagnetic Induced Transparency Metam...

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4th IEEE china International Youth Conference on Electrical engineering, CIYCEE 2023

作者： Zhou, Xingyu Tian, Peishuai Hu, Yanqi Sun, Qitai Xiong, Yongqian Huazhong University of Science and Technology State Key Laboratory of Advanced Electromagnetic Technology School of Electrical and Electronic Engineering Wuhan430074 China

ISBN: (纸本)9798350305562

The unique properties of electromagnetic induced transparency (EIT) metamaterials have caused a lot of concern in the field of terahertz wave regulation, but the traditional design methods of metamaterials have the problems of long design cycle and high trial and error cost. Applying deep learning method to the inverse design process of terahertz metamaterials can greatly reduce the design complexity, so that the EIT metamaterial structure can be quickly designed according to the requirements. In this paper, a generative adversarial network (GAN) model for EIT metamaterial structure design is constructed, which realizes the mapping relationship between target spectrum and metamaterial structure parameters. The proposed GAN model can accurately predict structure parameters of the EIT metamaterial according to the target spectrum, and the error between the generated and the real parameters is less than 1μm. Moreover, by introducing the fuzzy processing, the proposed GAN model can accurately generate multiple sets of metamaterial structure according to the same target spectrum, which provides more options for designers. This model offers a novel and efficient design method for EIT metamaterials. © 2023 IEEE.

关键词： Metamaterials

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Reduction of Rotor Loss in High-Speed Electrical Machines With a Novel Composite Sleeve 26

Reduction of Rotor Loss in High-Speed Electrical Machines Wi...

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26th International Conference on Electrical Machines and Systems, ICEMS 2023

作者： Ding, Minyue Fang, Haiyang Qu, Ronghai Huazhong University of Science and Technology State Key Laboratory of Advanced Electromagnetic Engineering and Technology School of Electrical and Electronic Enginnering Wuhan China

ISBN: (纸本)9798350317589

The rotor eddy-current loss caused by high frequency current and magnetic field changes is very high in high-speed permanent magnet machines (HSPMM). This is one of the important factors contributing to the overheat of the PMs. Since the sleeve loss is the main component of the overall rotor loss, it is widely concerned in HSPMM. In this paper, a novel composite sleeve is proposed to reduce the rotor loss. The proposed sleeve is applied to a 90kW, 16000r/min PM machine, the total rotor loss and temperature rise are respectively decreased by 44.5% and 18.7% (25.2°C) compared with a conventional carbon fiber sleeve. Furthermore, the rotor maximum stress is obtained and validated to be within the safe range. © 2023 IEEE.

关键词： Carbon fibers

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Hierarchical hollow microspheres assembled from carbon nanosheets integrated with molybdenum carbide nanoparticles for boosting microwave absorption properties

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Nano Research 2025年第1期18卷 10-20页

作者： Zongsheng Chen Yahui Wang Yi Liu Zhigang Li Xiangyin Lv Liping Liu Yajing Chang Jiaming Shi Xiao Zhang State Key Laboratory of Pulsed Power Laser Technology School of Electronic EngineeringNational University of Defense TechnologyHefei 230037China Anhui Provincial Laboratory of Advanced Laser Technology School of Electronic EngineeringNational University of Defense TechnologyHefei 230037China Centre for Environmental and Energy Nanomaterials Anhui Key Laboratory of Nanomaterials and NanotechnologyCAS Centre for Excellence in NanoscienceInstitute of Solid State PhysicsHefei Institutes of Physical ScienceChinese Academy of SciencesHefei 230031China

Hierarchical hollow structure has demonstrated potential for enhancing electromagnetic(EM)attenuation and improving impedance matching,garnering significant attention for ***,we have successfully implemented compositional and structural engineering to fabricate hollow Mo2C/C microspheres with controllable composition by coupling interaction between dopamine hydrochloride and ammonium *** the synergistic effect of composition and hollow structure,the strongest reflection loss intensity and broadest effective absorption of the optimized sample reach-70.2 dB and 6.2 GHz,*** formation of hollow heterogeneous structures not only favors impedance matching feature,but also generates considerable contribution to EM attenuation ***,radar cross-section simulation data indicate that hollow Mo2C/C microspheres with compositional optimization and heterogeneous structures have broad prospects for practical applications.

关键词： electromagnetic absorption Mo2C/C microwave absorption hollow structure

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