Electrochemical CO_(2)reduction is a sustainable approach in green chemistry that enables the production of valuable chemicals and fuels while mitigating the environmental impact associated with CO_(2)*** its several ...
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Electrochemical CO_(2)reduction is a sustainable approach in green chemistry that enables the production of valuable chemicals and fuels while mitigating the environmental impact associated with CO_(2)*** its several advantages,this technology suffers from an intrinsically low CO_(2)solubility in aqueous solutions,resulting in a lower local CO_(2)concentration near the electrode,which yields lower current densities and restricts product *** diffusion electrodes(GDEs),particularly those with tubular architectures,can solve these issues by increasing the local CO_(2)concentration and triple-phase interface,providing abundant electroactive sites to achieve superior reaction *** this study,robust and self-supported Cu flow-through gas diffusion electrodes(FTGDEs)were synthesized for efficient formate production via electrochemical CO_(2)*** were further compared with traditional Cu electrodes,and it was found that higher local CO_(2)concentration due to improved mass transfer,the abundant surface area available for the generation of the triple-phase interface,and the porous structure of Cu FTGDEs enabled high formate Faradaic efficiency(76%)and current density(265 mA¸cm^(−2))at–0.9 V *** hydrogen electrode(RHE)in 0.5 mol·L^(−1)*** combined phase inversion and calcination process of the Cu FTGDEs helped maintain a stable operation for several *** catalytic performance of the Cu FTGDEs was further investigated in a non-gas diffusion configuration to demonstrate the impact of local gas concentration on the activity and performance of electrochemical CO_(2)*** study demonstrates the potential of flow-through gas-diffusion electrodes to enhance reaction kinetics for the highly efficient and selective reduction of CO_(2),offering promising applications in sustainable electrochemical processes.
Most optimization problems of practical significance are typically solved by highly configurable parameterized *** achieve the best performance on a problem instance,a trial-and-error configuration process is required...
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Most optimization problems of practical significance are typically solved by highly configurable parameterized *** achieve the best performance on a problem instance,a trial-and-error configuration process is required,which is very costly and even prohibitive for problems that are already computationally intensive,*** problems associated with machine learning *** the past decades,many studies have been conducted to accelerate the tedious configuration process by learning from a set of training *** article refers to these studies as learn to optimize and reviews the progress achieved.
Multiarmed bandit(MAB) models are widely used for sequential decision-making in uncertain environments, such as resource allocation in computer communication systems.A critical challenge in interactive multiagent syst...
Multiarmed bandit(MAB) models are widely used for sequential decision-making in uncertain environments, such as resource allocation in computer communication systems.A critical challenge in interactive multiagent systems with bandit feedback is to explore and understand the equilibrium state to ensure stable and tractable system performance.
In the fields of intelligent transportation and multi-task cooperation, many practical problems can be modeled by colored traveling salesman problem(CTSP). When solving large-scale CTSP with a scale of more than 1000d...
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In the fields of intelligent transportation and multi-task cooperation, many practical problems can be modeled by colored traveling salesman problem(CTSP). When solving large-scale CTSP with a scale of more than 1000dimensions, their convergence speed and the quality of their solutions are limited. This paper proposes a new hybrid IT?(HIT?) algorithm, which integrates two new strategies, crossover operator and mutation strategy, into the standard IT?. In the iteration process of HIT?, the feasible solution of CTSP is represented by the double chromosome coding, and the random drift and wave operators are used to explore and develop new unknown regions. In this process, the drift operator is executed by the improved crossover operator, and the wave operator is performed by the optimized mutation strategy. Experiments show that HIT? is superior to the known comparison algorithms in terms of the quality solution.
Despite the promising potential of NaTi2（PO4）3as desalination battery electrode,its mediocre seawater desalination capacity and durability fail to meet the requirements of practical ***,the substitution of Ti by Fe ...
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Despite the promising potential of NaTi2（PO4）3as desalination battery electrode,its mediocre seawater desalination capacity and durability fail to meet the requirements of practical ***,the substitution of Ti by Fe in NaTi2（PO4）3(NT2-xFxP),which possesses a stronger electronegativity relative to Ti,can regulate the electronic structure,thus facilitating charge transfer and ion diffusion during the desalination *** kinetic and thermodynamic facilitation of NT2-xFxP is clarified by the electrochemical analyses and DFT ***,the additional redox center and solid-solution reaction mechanism induced by Fe-dopant further contribute to a superior desalination performance of NT2-xFxP in different seawater *** from the multifunctional effect of Fe-dopant,the optimal NT1.7F0.3P delivers a large salt removal capacity(173.6 mg g-1) with an ultrahigh salt removal rate(8.48 mg g-1min-1),and maintains 96.6%of desalination capacity after 500 cycles in natural ***,the assembled NT1.7F0.3P||NaFeHCF rocking-chair desalination battery（RCDB） demonstrates a higher desalination performance than that of reported RCDB systems,and can desalinate natural seawater to freshwater standards under continuous desalination mode for the first time in RCDB *** work provides a facile but effective strategy to modulate the electronic structure of NaTi2（PO4）3for RCDB,and exploits a new perspective for developing scalable RCDB devices for continuous desalinating real seawater to freshwater.
Electronic 3D printing possesses a remarkable molding ability and convenience in integrated circuits,flex-ible wearables,and individual automobile ***,traditional 3D printing technology still struggles to meet the dem...
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Electronic 3D printing possesses a remarkable molding ability and convenience in integrated circuits,flex-ible wearables,and individual automobile ***,traditional 3D printing technology still struggles to meet the demands of high precision and high efficiency in the process of fabricating a curved surface circuit,particularly achieving precise silver circuit molding on irregular ***,a high-precision and muti-scaled conformal manufacturing method for silver circuits is presented through the digital light processing(DLP)of ultraviolet-curable silver paste(UV-SP)with adjustable photocuring prop-erties,enabling the successful preparation of micro-scaled conductive structure on the sharply skewed hook *** minimum modeling depth and width of the cured silver paste can be well controlled to 10 and 88 pm,*** with traditional printing technology,the printing efficiency of com-plex patterns has increased by over 70％.The printed silver circuit demonstrates an exceptionally high electrical conductivity,reaching as high as 1.16 × 107 S/***,the UV-SP exhibits significant manufacturing efficiency and superior molding resolution compared to conventional direct ink writing and inkjet printing techniques,thereby contributing to the attainment of high precision and efficiency of conformal and micro-molding manufacturing in sensors,communication antennas,and other electronic devices based on curved substrates.
1 Introduction Recently,multiple synthetic and real-world datasets have been built to facilitate the training of deep single-image reflection removal(SIRR)***,diverse testing sets are also provided with different type...
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1 Introduction Recently,multiple synthetic and real-world datasets have been built to facilitate the training of deep single-image reflection removal(SIRR)***,diverse testing sets are also provided with different types of reflections and ***,the non-negligible domain gaps between training and testing sets make it difficult to learn deep models generalizing well to testing *** diversity of reflections and scenes further makes it a mission impossible to learn a single model being effective for all testing sets and real-world *** this paper,we tackle these issues by learning SIRR models from a domain generalization perspective.
High thermal conductivity and high strength Mg-1.5Mn-2.5Ce alloy with a tensile yield strength of 387.0 MPa,ultimate tensile strength of 395.8 MPa,and thermal conductivity of 142.1 W/(m·K)was successfully fabrica...
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High thermal conductivity and high strength Mg-1.5Mn-2.5Ce alloy with a tensile yield strength of 387.0 MPa,ultimate tensile strength of 395.8 MPa,and thermal conductivity of 142.1 W/(m·K)was successfully fabricated via hot *** effects of La and Ce additions on the microstructure,thermal conductivity,and mechanical properties of the Mg-1.5Mn alloy were *** results indicated that both the as-extruded Mg-1.5Mn-2.5La and Mg-1.5Mn-2.5Ce alloys exhibited a bimodal grain structure,with dynamically precipitated nano-scaleα-Mn *** comparison with La,the addition of Ce enhanced the dynamic precipitation more effectively during hot extrusion,while its influence on promoting the dynamic recrystallization was relatively *** high tensile strength obtained in the as-extruded Mg-1.5Mn-2.5RE alloys can be attributed to the combined influence of the bimodal grain structure(with fine dynamic recrystallized(DRXed)grain size and high proportion of un-dynamic recrystallized(unDRXed)grains),dense nano-scale precipitates,and broken Mg12RE phases,while the remarkable thermal conductivity was due to the precipitation of Mn-rich phases from the Mg matrix.
Achieving high strength in Mg alloys is usually accompanied by ductility ***,a novel Mg97Y1Zn1Ho1 at.%alloy with a yield strength of 403 MPa and an elongation of 10%is *** strength-ductility synergy is obtained by a c...
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Achieving high strength in Mg alloys is usually accompanied by ductility ***,a novel Mg97Y1Zn1Ho1 at.%alloy with a yield strength of 403 MPa and an elongation of 10%is *** strength-ductility synergy is obtained by a comprehensive strategy,including a lamella bimodal microstructure design and the introduction of nano-spaced solute-segregated 14H long-period stacking-ordered phase(14H LPSO phase)through rare-earth Ho *** lamella bimodal microstructure consists of elongated un-recrystallized(un-DRXed)coarse grains and fine dynamically-recrystallized grains(DRXed regions).The nano-spaced solute-segregated 14H LPSO phase is distributed in DRXed *** outstanding yield strength is mainly contributed by grain-boundary strengthening,18R LPSO strengthening,and fiberlike reinforcement strengthening from the nano-spaced 14H LPSO *** high elongation is due primarily to the combined effects of the bimodal and lamellar microstructures through enhancing the work-hardening capability.
Two new low-alloyed Mg-2RE-0.8Mn-0.6Ca-0.5Zn(wt%,RE=Sm or Y)alloys are developed,which can be produced on an in-dustrial scale via relatively high-speed *** two alloys are not only comparable to commercial AZ31 alloy ...
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Two new low-alloyed Mg-2RE-0.8Mn-0.6Ca-0.5Zn(wt%,RE=Sm or Y)alloys are developed,which can be produced on an in-dustrial scale via relatively high-speed *** two alloys are not only comparable to commercial AZ31 alloy in extrudability,but also have superior mechanical properties,especially in terms of yield strength(YS).The excellent extrudability is related to less coarse second-phase particles and high initial melting point of the two as-cast *** high strength-ductility mainly comes from the formation of fine grains,nano-spaced submicron/nano precipitates,and weak ***,it is worth noting that the YS of the two alloys can maintain above 160 MPa at elevated temperature of 250°C,significantly higher than that of AZ31 alloy(YS:45 MPa).The Zn/Ca solute segregation at grain boundaries,the improved heat resistance of matrix due to addition of RE,and the high melting points of strengthening particles(Mn,MgZn_(2),and Mg-Zn-RE/Mg-Zn-RE-Ca)are mainly responsible for the excellent high-temperature strength.
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