Ontology matching plays a crucial role in the realm of ontology engineering, specifically in ontology development and integration. It serves the purpose of resolving the issue of heterogeneous semantics between ontolo...
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Electrocatalytic oxygen evolution reaction(OER)has been recognized as the bottleneck of overall water splitting,which is a promising approach for sustainable production of H_(2).Transition metal(TM)hydroxides are the ...
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Electrocatalytic oxygen evolution reaction(OER)has been recognized as the bottleneck of overall water splitting,which is a promising approach for sustainable production of H_(2).Transition metal(TM)hydroxides are the most conventional and classical non-noble metal-based electrocatalysts for OER,while TM basic salts[M^(2+)(OH)_(2-x)(A_(m^(-))_(x/m),A=CO_(3)^(2−),NO_(3)^(−),F^(−),Cl^(−)]consisting of OH−and another anion have drawn extensive research interest due to its higher catalytic activity in the past *** this review,we summarize the recent advances of TM basic salts and their application in OER and further overall water *** categorize TM basic salt-based OER pre-catalysts into four types(CO_(3)^(2−),NO_(3)^(−),F^(−),Cl^(−)according to the anion,which is a key factor for their outstanding performance towards *** highlight experimental and theoretical methods for understanding the structure evolution during OER and the effect of anion on catalytic *** develop bifunctional TM basic salts as catalyst for the practical electrolysis application,we also review the present strategies for enhancing its hydrogen evolution reaction activity and thereby improving its overall water splitting ***,we conclude this review with a summary and perspective about the remaining challenges and future opportunities of TM basic salts as catalysts for water electrolysis.
Link prediction is used to complete the knowledge graph. Convolutional neural network models are commonly used for link prediction tasks, but they only consider the direct relations between entity pairs, ignoring the ...
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Medical reports play an important role in diagnosing a patient’s illness. However, writing medical reports is time-consuming and labor-intensive, and writing high-quality medical reports often requires extensive clin...
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Li metal is widely recognized as the desired anode for next-generation energy storage,Li metal batteries,due to its highest theoretical capacity and lowest ***,it suffers from unstable elec-trochemical behaviors like ...
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Li metal is widely recognized as the desired anode for next-generation energy storage,Li metal batteries,due to its highest theoretical capacity and lowest ***,it suffers from unstable elec-trochemical behaviors like dendrite growth and side reactions in practical ***,we report a highly stable anode with collector,Li5Mg@Cu,realized by the melting-rolling *** Li5Mg@Cu anode delivers ultrahigh cycle stability for 2000 and 1000 h at the current densities of 1 and 2 mA cm-2,respectively in symmetric ***,the Li5Mg@Cu|LFP cell exhibits a high-capacity retention of 91.8%for 1000 cycles and 78.8%for 2000 cycles at 1 ***,we investigate the suppression effects of Mg on the dendrite growth by studying the performance of LixMg@Cu electrodes with different Mg contents(2.0-16.7 at%).The exchange current density,surface energy,Li+diffusion coefficient,and chem-ical stability of LixMg@Cu concretely reveal this improving suppression effect when Mg content becomes *** addition,a Mg-rich phase with"hollow brick"morphology forming in the high Mg content LixMg@Cu guides the uniform deposition of *** study reveals the suppression effects of Mg on Li dendrites growth and offers a perspective for finding the optimal component of Li-Mg alloys.
Optical-flow-based and kernel-based approaches have been extensively explored for temporal compensation in satellite Video Super-Resolution (VSR). However, these techniques are less generalized in large-scale or compl...
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Photon tunneling effects give rise to surface waves,amplifying radiative heat transfer in the near-field *** research has highlighted that the introduction of nanopores into materials creates additional pathways for h...
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Photon tunneling effects give rise to surface waves,amplifying radiative heat transfer in the near-field *** research has highlighted that the introduction of nanopores into materials creates additional pathways for heat transfer,leading to a substantial enhancement of near-field radiative heat transfer(NFRHT).Being a direct bandgap semiconductor,GaN has high thermal conductivity and stable resistance at high temperatures,and holds significant potential for applications in optoelectronic ***,study of NFRHT between nanoporous GaN films is currently lacking,hence the physical mechanism for adding nanopores to GaN films remains to be discussed in the field of *** this work,we delve into the NFRHT of GaN nanoporous films in terms of gap distance,GaN film thickness and the vacuum filling *** results demonstrate a 27.2%increase in heat flux for a 10 nm gap when the nanoporous filling ratio is ***,the spectral heat flux exhibits redshift with increase in the vacuum filling *** be more precise,the peak of spectral heat flux moves fromω=1.31×10^(14)rad·s^(-1)toω=1.23×10^(14)rad·s^(-1)when the vacuum filling ratio changes from f=0.1 to f=0.5;this can be attributed to the excitation of surface phonon *** introduction of graphene into these configurations can highly enhance the NFRHT,and the spectral heat flux exhibits a blueshift with increase in the vacuum filling ratio,which can be explained by the excitation of surface plasmon *** findings offer theoretical insights that can guide the extensive utilization of porous structures in thermal control,management and thermal modulation.
Transformer-based method has demonstrated promising performance in image super-resolution tasks, due to its long-range and global aggregation capability. However, the existing Transformer brings two critical challenge...
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Biomass carbon and small redox biomolecules are attractive materials for green,sustainable energy storage devices owing to their environmentally friendly,low-cost,scalable,and novel ***,most devices manufactured using...
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Biomass carbon and small redox biomolecules are attractive materials for green,sustainable energy storage devices owing to their environmentally friendly,low-cost,scalable,and novel ***,most devices manufactured using these materials have low specific capacitance,poor cycle stability,short lifetime,complexity,and low precision of device ***,we report the directed self-assembly of mononuclear anthraquinone(MAQ)derivatives and porous lignin-based graphene oxide(PLGO)into a renewable colloidal gel through noncovalent *** self-assembled gel electrode materials exhibited high capacitance(484.8 F g^(−1) at a current density of 1 A g^(−1))and could be further printed as flexible micro-supercapacitors(FMSCs)with arbitrary patterns and a relatively high resolution on specific *** FMSCs exhibited excellent areal capacitance(43.6 mF cm^(−2)),energy and power densities(6.1μWh cm^(−2) and 50μW cm^(−2),respectively),and cycle stability(>10,000 cycles).Furthermore,the printed FMSCs and integrated FMSC arrays exhibited remarkable flexibility while maintaining a stable *** proposed approach can be applied to other quinone biomolecules and biomass-based carbon *** study provides a basis for fabricating green and sustainable energy storage device architectures with high capacitance,long-term cycling,high scalability,and high precision.
Hyperspectral imaging has transformed remote sensing by offering detailed spectral data for monitoring environmental changes, like urban development and terrestrial cover variations. However, existing change detection...
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