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Tetris-Style Stacking Process to Tailor the Orientation of Carbon Fiber Scaffolds for Efficient Heat Dissipation

Nano-Micro Letters 2023年第9期15卷 310-324页

作者： Shida Han Yuan Ji Qi Zhang Hong Wu Shaoyun Guo Jianhui Qiu Fengshun Zhang The State Key Laboratory of Polymer Materials Engineering Sichuan Provincial Engineering Laboratory of Plastic/Rubber Complex Processing TechnologyPolymer Research Institute of Sichuan UniversityChengdu 610065People’s Republic of China Department of Mechanical Engineering Faculty of Systems Science and TechnologyAkita Prefectural University015-0055AkitaJapan Institute of Chemical Materials China Academy of Engineering PhysicsMianyang 621900People’s Republic of China

As the miniaturization of electronic devices and complication of electronic packaging,there are growing demands for thermal interfacial materials with enhanced thermal conductivity and the capability to direct the heat toward heat sink for highly efficient heat ***-based carbon fiber(CF)with ultrahigh axial thermal conductivity and aspect ratios exhibits great potential for developing thermally conductive composites as ***,it is still hard to fabricate composites with aligned carbon fiber in a general approach to fully utilize its excellent axial thermal conductivity in specific ***,three types of CF scaffolds with different oriented structure were developed via magnetic field-assisted Tetris-style stacking and carbonization *** regulating the magnetic field direction and initial stacking density,the self-supporting CF scaffolds with horizontally aligned(HCS),diagonally aligned and vertically aligned(VCS)fibers were *** embedding the polydimethylsiloxane(PDMS),the three composites exhibited unique heat transfer properties,and the HCS/PDMS and VCS/PDMS composites presented a high thermal conductivity of 42.18 and 45.01 W m^(−1)K^(−1)in fiber alignment direction,respectively,which were about 209 and 224 times higher than that of *** excellent thermal conductivity is mainly ascribed that the oriented CF scaffolds construct effective phonon transport pathway in the *** addition,fishbone-shaped CF scaffold was also produced by multiple stacking and carbonization process,and the prepared composites exhibited a controlled heat transfer path,which can allow more versatility in the design of thermal management system.

关键词： Carbon fiber Magnetic field Thermal management Thermally conductive composites

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Interface engineering and Anion engineering of Mo-Based Heterogeneous Electrocatalysts for Hydrogen Evolution Reaction

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Energy & Environmental Materials 2023年第1期6卷 87-104页

作者： Zehao Yin Xuan Liu Siru Chen Tingli Ma Yanqiang Li State Key Laboratory of Fine Chemicals School of Chemical EngineeringDalian University of TechnologyPanjin CampusPanjin 124221China School of Material and Chemical Engineering Centre for Advanced Materials ResearchZhongyuan University of TechnologyZhengzhou 450007China Department of Materials Science and Engineering China Jiliang UniversityHangzhou 310018China Graduate School of Life Science and Systems Engineering Kyushu Institute of TechnologyKitakyushu Fukuoka 808-0196Japan

Development and utilization of hydrogen energy is an effective way to achieve carbon neutrality,only hydrogen production through electrolytic water splitting meets the goal of zero carbon *** facilitate the large-scale commercialization of water splitting devices,the development of highly efficient and low-cost catalysts to reduce the energy consumption is ***_(2)has been regarded as a promising electrocatalyst to replace platinum in hydrogen evolution reaction due to its low price and unique 2D layered ***,the poor conductivity and inert basal planes of MoS_(2)limited its wide-spread ***,researches have demonstrated that the conductivity and active sites of MoS_(2)can be improved by heteroatoms doping or constructing of heterogeneous *** this review,the recent progress of Mo-based catalysts are summarized centered on MoS_(2)based on interface engineering and anion engineering,including MoS_(2)–MoO_(2),MoS_(2)–Mo_(2)C,MoS_(2)–MoN_(x),MoS_(2)–MoP,and MoS_(2)–MoSe_(2).The preparation method,structure,and performance of the catalysts are introduced and the possible mechanism behind the improved catalytic activity are revealed to give readers an overall comprehension on the progress of the Mo-based electrocatalysts for hydrogen evolution *** addition,an outlook on future opportunities and development directions of Mo-based catalysts are proposed to facilitate the development of Mo-based catalysts for hydrogen production.

关键词： electrocatalysis heterostructure hydrogen evolution reaction Mo-based catalysts

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A Joint Estimation Method of SOC and SOH for Lithium-ion Battery Considering Cyber-Attacks Based on GA-BP

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Computers, Materials & Continua 2024年第9期80卷 4497-4512页

作者： Tianqing Yuan Na Li Hao Sun Sen Tan Key Laboratory of Modern Power System Simulation and Control&Renewable Energy Technology Ministry of EducationNortheast Electric Power UniversityJilin132012China Department of Electrical Engineering Northeast Electric Power UniversityJilin132012China College of Information and Control Engineering Jilin Institute of Chemical TechnologyJilin132022China Center for Research on Microgrids Department of EnergyAalborg UniversityAalborg9220Denmark

To improve the estimation accuracy of state of charge(SOC)and state of health(SOH)for lithium-ion batteries,in this paper,a joint estimation method of SOC and SOH at charging cut-off voltage based on genetic algorithm(GA)combined with back propagation(BP)neural network is proposed,the research addresses the issue of data manipulation resulting ***,anomalous data stemming fromcyber-attacks are identified and eliminated using the isolated forest algorithm,followed by data ***,the incremental capacity(IC)curve is derived fromthe restored data using theKalman filtering algorithm,with the peak of the ICcurve(ICP)and its corresponding voltage serving as the health factor(HF).Thirdly,the GA-BP neural network is applied to map the relationship between HF,constant current charging time,and SOH,facilitating the estimation of SOH based on ***,SOC estimation at the charging cut-off voltage is calculated by inputting the SOH estimation value into the trained model to determine the constant current charging time,and by updating the maximum available *** show that the root mean squared error of the joint estimation results does not exceed 1%,which proves that the proposed method can estimate the SOC and SOH accurately and stably even in the presence of false data injection attacks.

关键词： Lithium-ion batteries state of charge state of health cyber-attacks genetic algorithm back propagation neural network

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Sigma-Mixed Unscented Kalman Filter-Based Fault Detection for Traction systems in High-Speed Trains

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Chinese Journal of Electronics 2023年第5期32卷 982-991页

作者： CHENG Chao WANG Weijun MENG Xiangxi SHAO Haidong CHEN Hongtian Department of Computer Science and Technology Changchun University of Technology Department of Mathematics and Statistics Changchun University of Technology Institute of System Research China Industrial Control Systems Cyber Emergency Response Team Department of Mechanical and Vehicle Engineering Hunan University Department of Chemical and Materials Engineering University of Alberta

Fault detection(FD) for traction systems is one of the active topics in the railway and academia because it is the initial step for the running reliability and safety of high-speed trains. Heterogeneity of data and complexity of systems have brought new challenges to the traditional FD methods. For addressing these challenges, this paper designs an FD algorithm based on the improved unscented Kalman filter(UKF) with consideration of performance degradation. It is derived by incorporating a degradation process into the state-space *** network topology of traction systems is taken into consideration for improving the performance of state estimation. We first obtain the mixture distribution by the mixture of sigma points in UKF. Then, the Lévy process with jump points is introduced to construct the degradation model. Finally, the moving average interstate standard deviation(MAISD) is designed for detecting *** the proposed methods via a traction systems in a certain type of trains obtains satisfactory results.

关键词： Degradation Network topology Fault detection Rail transportation State-space methods Safety Kalman filters

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DNA-based supramolecular hydrogels:From construction strategies to biomedical applications

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Chinese chemical Letters 2023年第12期34卷 76-86页

作者： Ping Chen Chenhong Yu Jie Chen Lijin Xu Huajie Liu jiangsu Engineering Laboratory for Environmental Functional Materials Jiangsu Key Lab for Chemistry of Low-Dimensional MaterialsSchool of Chemistry and Chemical EngineeringHuaiyin Normal UniversityHuaian 223300China School of Chemical Science and Engineering Shanghai Research Institute for Intelligent Autonomous SystemsKey Laboratory of Advanced Civil Engineering Materials of Ministry of EducationTongji UniversityShanghai 200092China Department of Chemistry Renmin University of ChinaBeijing 100872China

DNA-based supramolecular hydrogels are important and promising biomaterials for various applications due to their inherent biocompatibility and tunable physicochemical *** three-dimensional supramolecular matrix of DNA formed by non-covalently dynamic cross-linking provides exceptional adaptability,self-healing,injectable and responsive properties for *** addition,DNA hydrogels are also ideal bio-scaffold materials owing to their tissue-like mechanics and intrinsic biological ***,DNA can assemble into supramolecular networks by pure complementary base pairing;it can also be combined with other building blocks to construct hybrid *** review focuses on the development and construction strategies of DNA *** and synthesis methods,diverse responsiveness and biomedical applications are ***,the challenges and prospects of DNA-based supramolecular hydrogels are discussed.

关键词： DNA hydrogels Supramolecular hydrogels Self-assembly DNA nanotechnology Biomedical applications

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Graphitic carbon nitride-based photocatalysts in the applications of environmental catalysis

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Journal of Environmental Sciences 2023年第2期124卷 570-590页

作者： Hongxia Lin JinmoWu Fan Zhou Xiaolong Zhao Pengfei Lu Guanghui Sun Yuhan Song Yayun Li Xiaoyong Liu Hongxing Dai Hefei Institute for Public Safety Research Tsinghua UniversityHefei 230601China Anhui Province Key Laboratory of Human Safety Hefei 230601China Beijing Key Laboratory for Green Catalysis and Separation Key Laboratory of Beijing on Regional Air Pollution ControlKey Laboratory of Advanced Functional MaterialsEducation Ministry of ChinaLaboratory of Catalysis Chemistry and NanoscienceDepartment of Environmental Chemical EngineeringSchool of Environmental and Chemical EngineeringFaculty of Environment and Life ScienceBeijing University of TechnologyBeijing 100124China

Semiconductor photocatalytic technology has shown great prospects in converting solar energy into chemical energy to mitigate energy crisis and solve environmental pollution *** key issue is the development of high-efficiency *** strategies in the state-of-the-art advancements,such as heterostructure construction,heteroatom doping,metal/single atom loading,and defect engineering,have been presented for the graphitic carbon nitride(g-C3N4)-based nanocomposite catalysts to design their surface chemical environments and internal electronic structures to make them more suitable for different photocatalytic *** this review,nanoarchitecture design,synthesis methods,photochemical properties,potential photocatalytic applications,and related reaction mechanisms of the modified high-efficiency carbon nitride-based photocatalysts were briefly *** superior photocatalytic performance was identified to be associated with the enhanced visible-light response,fast photoinduced electron-hole separation,efficient charge migration,and increased unsaturated active ***,the further advance of the visible-light harvesting and solar-to-energy conversions are proposed.

关键词： Graphitic carbon nitride-based photocatalyst Photocatalytic reduction Photocatalytic degradation chemical modification Heterostructure construction Metal doping

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Enhancing photocatalytic CO_(2)reduction with TiO_(2)-based materials:Strategies,mechanisms,challenges,and perspectives

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Environmental Science and Ecotechnology 2024年第4期20卷 18-33页

作者： Zhimin Yuan Xianglin Zhu Xianqiang Gao Changhua An Zheng Wang Cheng Zuo Dionysios D.Dionysiou Hong He Zaiyong Jiang School of Chemistry&Chemical Engineering and Environmental Engineering Weifang UniversityWeifang261061PR China State Key Joint Laboratory of Environment Simulation and Pollution Control Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing100085PR China Institute for Energy Research School of Chemistry and Chemical EngineeringJiangsu UniversityZhenjiang212013PR China Tianjin Key Laboratory of Organic Solar Cells and Photochemical Conversion School of Chemistry and Chemical EngineeringTianjin University of TechnologyTianjin300384PR China Environmental Engineering and Science Program Department of Chemical and Environmental Engineering(DChEE)University of CincinnatiCincinnatiOH45221-0012USA College of Forestry Shandong Agricultural UniversityTaian271018PR China

The concentration of atmospheric CO_(2)has exceeded 400 ppm,surpassing its natural variability and raising concerns about uncontrollable shifts in the carbon cycle,leading to significant climate and environmental impacts.A promising method to balance carbon levels and mitigate atmospheric CO_(2)rise is through photocatalytic CO_(2)*** dioxide(TiO_(2)),renowned for its affordability,stability,availability,and eco-friendliness,stands out as an exemplary catalyst in photocatalytic CO_(2)*** strategies have been proposed to modify TiO_(2)for photocatalytic CO_(2)reduction and improve catalytic activity and product ***,few studies have systematically summarized these strategies and analyzed their advantages,disadvantages,and current ***,we comprehensively review recent advancements in TiO_(2)engineering,focusing on crystal engineering,interface design,and reactive site construction to enhance photocatalytic efficiency and product *** discuss how modifications in TiO_(2)'s optical characteristics,carrier migration,and active site design have led to varied and selective CO_(2)reduction *** enhancements are thoroughly analyzed through experimental data and theoretical ***,we identify current challenges and suggest future research directions,emphasizing the role of TiO_(2)-based materials in understanding photocatalytic CO_(2)reduction mechanisms and in designing effective *** review is expected to contribute to the global pursuit of carbon neutrality by providing foundational insights into the mechanisms of photocatalytic CO_(2)reduction with TiO_(2)-based materials and guiding the development of efficient photocatalysts.

关键词： summarized dioxide neutral

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An in-situ biochar-enhanced anaerobic membrane bioreactor for swine wastewater treatment under various organic loading rates

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Journal of Environmental Sciences 2024年第12期146卷 304-317页

作者： Nianwen Chen Xinbo Zhang Qing Du Huizhong Wang Zhiwen Wang Junzhi Ren Hongxia Li Wenshan Guo Huu Hao Ngo Joint Research Centre for Protective Infrastructure Technology and Environmental Green Bioprocess School of Environmental and Municipal EngineeringTianjin Chengjian UniversityTianjin 300384China Tianjin Key Laboratory of Aquatic Science and Technology Tianjin Chengjian UniversityTianjin 300384China Frontier Science Center for Synthetic Biology and Key Laboratory of Systems Bioengineering(Ministry of Education) SynBio Research PlatformCollaborative Innovation Center of Chemical Science and Engineering(Tianjin)Department of Biochemical EngineeringSchool of Chemical Engineering and TechnologyTianjin UniversityTianjin 300072China Tianjin Caring Technology Development Co. Ltd.Tianjin 300381China Centre for Technology in Water and Wastewater School of Civil and Environmental EngineeringUniversity of Technology SydneySydneyNSW 2007Australia

A biochar-assisted anaerobic membrane bioreactor(BC-AnMBR)was conducted to evaluate the performance in treating swine wastewater with different organic loading rates(OLR)ranging from 0.38 to 1.13 kg-COD/(m3.d).Results indicated that adding spent coffee grounds biochar(SCG-BC)improved the organic removal efficiency compared to the conventional AnMBR,with an overall COD removal rate of>95.01%.Meanwhile,methane production of up to 0.22 LCH4/gCOD with an improvement of 45.45%was achieved under a high OLR of 1.13 kg-COD/(m3.d).Furthermore,the transmembrane pressure(TMP)in the BC-AnMBR system was stable at 4.5 kPa,and no irreversible membrane fouling occurred within 125 *** community analysis revealed that the addition of SCG-BC increased the relative abundance of autotrophic methanogenic archaea,particularly Methanosarcina(from 0.11%to 11.16%)and Methanothrix(from 16.34%to 24.05%).More importantly,Desulfobacterota and Firmicutes phylum with direct interspecific electron transfer(DIET)capabilities were also enriched with autotrophic *** of the electron transfer pathway showed that the concentration of c-type cytochromes increased by 38.60%in the presence of SCGBC,and thus facilitated the establishment of DIET and maintained high activity of the elec-tron transfer system even at high *** short,the BC-AnMBR system performs well under various OLR conditions and is stable in the recovery energy system for swine wastewater.

关键词： Biochar Microbial community Anaerobic membrane bioreactor Organic loading rates Methane production

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Multilayer core–shell structured FeNi_(3)@C with enhanced interfacial polarization for microwave absorbers

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Nano research 2025年第2期18卷 833-842页

作者： Shaohan Guo Junying Zhang Chengyou Lin Jin Ge Song Bi Zhi-Ling Hou College of Mathematics and Physics Beijing University of Chemical TechnologyBeijing 100029China School of Physics and Optoelectronic Engineering Beijing University of TechnologyBeijing 100124China National Key Laboratory of Electromagnetic Information Control and Effects Shenyang Aircraft Design and Research InstituteShenyang 110035China 501 Department Xi’an Research Institute of High-TechXi’an 710025China

Magnetoelectric composites can achieve magneto-electric synergy to optimize impedance ***,it is challenging to enhance the broadband absorption performance for thin thickness ***,FeNi_(3)@C composite with magnetic alloy core and N-doped macroporous multilevel layered carbon shell was constructed by hierarchical interface *** uniform multilevel layered carbon shell could induce interfacial polarization and multiple scattering,and further endows enhanced electromagnetic attenuation and optimized impedance *** ultra-thin broadband absorber with an effective absorption bandwidth of 7.4 GHz is achieved at a thickness of only 1.6 ***,full-band absorption from 2 to 18 GHz at a thickness of 9.8 mm is realized through metastructure *** work provides an alternative strategy to prepare coreshell structured magnetoelectric composites for ultra-thin and broadband absorbers.

关键词： covalent organic frameworks(COFs) FeNi_(3)@C core-shell structure interfacial polarization impedance matching

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An Improved Machine Learning Model for Pure Component Property Estimation

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engineering 2024年第8期39卷 61-73页

作者： Xinyu Cao Ming Gong Anjan Tula Xi Chen Rafiqul Gani Venkat Venkatasubramanian State Key Laboratory of Industrial Control Technology College of Control Science and EngineeringZhejiang UniversityHangzhou 310027China Department of Physics Bard College at Simon’s RockGreat BarringtonMA 01230USA PSE for SPEED Company Charlottenlund DK-2920Denmark Sustainable Energy and Environment Thrust The Hong Kong University of Science and Technology(Guangzhou)Guangzhou 510000China Department of Applied Sustainability Széchenyi István UniversityGyör 9026Hungary Complex Resilient Intelligent Systems Laboratory Department of Chemical EngineeringColumbia UniversityNew YorkNJ 10027USA

Information on the physicochemical properties of chemical species is an important prerequisite when performing tasks such as process design and product ***,the lack of extensive data and high experimental costs hinder the development of prediction techniques for these ***,accuracy and predictive capabilities still limit the scope and applicability of most property estimation *** paper proposes a new Gaussian process-based modeling framework that aims to manage a discrete and high-dimensional input space related to molecular structure representation with the group-contribution approach.A warping function is used to map discrete input into a continuous domain in order to adjust the correlation between different *** selection techniques,including prior elicitation and prior predictive checking,are also applied during the building procedure to provide the model with more information from previous research *** framework is assessed using datasets of varying sizes for 20 pure component *** 18 out of the 20 pure component properties,the new models are found to give improved accuracy and predictive power in comparison with other published models,with and without machine learning.

关键词： Group contribution Gaussian process Warping function Prior predictive checking

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