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Recent development of chemically complex metallic glasses: from accelerated compositional design, additive manufacturing to novel applications

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Materials Futures 2022年第1期1卷 9-31页

作者： J Y Zhang Z Q Zhou Z B Zhang M H Park Q Yu Z Li J Ma A D Wang H G Huang M Song B S Guo Q Wang Y Yang Department of Mechanical Engineering College of EngineeringCity University of Hong KongKowloon TongKowloonHong KongPeople’s Republic of China Shenzhen Key Laboratory of High Performance Nontraditional Manufacturing College of Mechatronics and Control EngineeringShenzhen UniversityShenzhenGuangdong 518060People’s Republic of China School of Materials Science and Engineering Dongguan University of TechnologyDongguanGuangdong 523808People’s Republic of China Institute of Materials China Academy of Engineering PhysicsJiangyouSichuan 621907People’s Republic of China State Key Laboratory of Powder Metallurgy Central South UniversityChangshaHunan 410083People’s Republic of China Institute of Advanced Wear&Corrosion Resistant and Functional Materials Jinan UniversityGuangzhouGuangdong 510632People’s Republic of China Institute of Materials Laboratory for MicrostructuresShanghai UniversityShanghai 200444People’s Republic of China Department of Materials Science and Engineering College of EngineeringCity University of Hong KongKowloon TongKowloonHong KongPeople’s Republic of China Department of Advanced Design and System Engineering College of EngineeringCity University of Hong KongKowloon TongKowloonHong KongPeople’s Republic of China

Metallic glasses(MGs)or amorphous alloys are an important engineering material that has a history of research of about 80–90 *** different fast cooling methods were developed for multi-component MGs between 1960s and 1980s,1990s witnessed a surge of research interest in the development of bulk metallic glasses(BGMs).Since then,one central theme of research in the metallic-glass community has been compositional design that aims to search for MGs with a better glass forming ability,a larger size and/or more interesting properties,which can hence meet the demands from more important *** this review article,we focus on the recent development of chemically complex MGs,such as high entropy MGs,with new tools that were not available or mature yet until recently,such as the state-of-the-art additive manufacturing technologies,high throughput materials design techniques and the methods for big data analyses(*** learning and artificial intelligence).We also discuss the recent use of MGs in a variety of novel and important applications,from personal healthcare,electric energy transfer to nuclear energy that plays a pivotal role in the battle against global warming.

关键词： metallic glasses amorphous alloys alloy design additive manufacturing machine learning high throughput materials design

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Printable organic light-emitting diodes for next-generation visible light communications:a review

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advanced Photonics Nexus 2023年第4期2卷 1-14页

作者： Kunping Guo Zhe Tang Xingxing Chou Saihu Pan Chunchen Wan Tao Xue Liping Ding Xiao Wang Jin Huang Fanghui Zhang Bin Wei Shaanxi University of Science and Technology School of Electronic Information and Artificial IntelligenceXi’anChina University College London Department Physics and Astronomy and London Centre for NanotechnologyLondonUnited Kingdom Shaanxi University of Science and Technology School of Electrical and Control EngineeringXi’anChina Changzhou University School of Microelectronics and Control EngineeringChangzhouChina Shanghai University Ministry of EducationKey Laboratory of Advanced Display and System ApplicationsShanghaiChina

Visible light communication(VLC)is an emerging technology employing light-emitting diodes(LEDs)to provide illumination and wireless data transmission *** cost-efficient printable organic LEDs(OLEDs)as environmentally friendly transmitters in VLC systems is extremely attractive for future applications in spectroscopy,the internet of things,sensing,and optical ranging in ***,we summarize the latest research progress on emerging semiconductor materials for LED sources in VLC,and highlight that OLEDs based on nontoxic and cost-efficient organic semiconductors have great opportunities for optical *** further examine efforts to achieve high-performance white OLEDs for general lighting,and,in particular,focus on the research status and opportunities for OLED-based *** solution-processable fabrication and printing strategies to develop high-performance OLEDs are also ***,an outlook on future challenges and potential prospects of the next-generation organic VLC is provided.

关键词： organic light-emitting diode visible light communication printable vehicular applications internet of things

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Bridging the structure gap between pellets in artificial dissolution media and in gastro-intestinal tract in rats

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Acta Pharmaceutica Sinica B 2022年第1期12卷 326-338页

作者： Hongyu Sun Siyu He Li Wu Zeying Cao Xian Sun Mingwei Xu Shan Lu Mingdi Xu Baoming Ning Huimin Sun Tiqiao Xiao Peter York Xu Xu Xianzhen Yin Jiwen Zhang School of Chemical and Environmental Engineering Shanghai Institute of TechnologyShanghai 201418China Center for Drug Delivery System Shanghai Institute of Materia MedicaChinese Academy of SciencesShanghai 201210China University of Chinese Academy of Sciences Beijing 100049China School of Materials Science and Engineering Center for Supramolecular Chemistry and CatalysisDepartment of ChemistryShanghai UniversityShanghai 200444China NMPA Key Laboratory for Quality Research and Evaluation of Pharmaceutical Excipients National Institutes for Food and Drug ControlBeijing 100050China National Institutes for Food and Drug Control Beijing 100050China Shanghai Synchrotron Radiation Facility/Zhangjiang Lab Shanghai Advanced Research InstituteChinese Academy of SciencesShanghai 201204China Center for MOST and Image Fusion Analysis Shanghai Institute of Materia MedicaChinese Academy of SciencesShanghai 201210China

Changes in structure of oral solid dosage forms(OSDF) elementally determine the drug release and its therapeutic *** this research,synchrotron radiation X-ray micro-computed tomography was utilized to visualize the 3 D structure of enteric coated pellets recovered from the gastrointestinal tract of *** structures of pellets in solid state and in vitro compendium media were *** in vivo underwent morphological and structural changes which differed significantly from those in vitro compendium ***,optimizations of the dissolution media were performed to mimic the appropriate in vivo conditions by introducing pepsin and glass microspheres in *** sphericity,pellet volume,pore volume and porosity of the in vivo esomeprazole magnesium pellets in stomach for2 h were recorded 0.47,1.55 × 10^(8)μm^(3),0.44 × 10^(8)μm^(3)and 27.6%,*** adding pepsin and glass microspheres,the above parameters in vitro reached to 0.44,1.64 × 10^(8)μm^(3)0.38 × 10^(8)μm^(3)and 23.0%,*** magnesium pellets behaved *** structural features of pellets between in vitro media and in vivo condition were bridged successfully in terms of 3 D structures to ensure better design,characterization and quality control of advanced OSDF.

关键词： Internal 3D structure 3D reconstruction Structural parameter Enteric coated pellets Synchrotron radiation X-ray micro computed tomography In vivo and in vitro structure correlation Esomeprazole magnesium Omeprazole magnesium

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Error-state Kalman Filtering with Linearized State Constraints

TechRxiv

引用

TechRxiv 2023年

作者： Do, Hoang Viet Jung, Jae Hyung Park, Chan Gook Song, Jin Woo The Intelligent Navigation and Control Systems Laboratory Department of Convergence Engineering for Intelligent Drone School of Intelligent Mechatronics Engineering Sejong University Seoul05006 Korea Republic of The Department of Aerospace Engineering Automation and Systems Research Institute Seoul National University Seoul08826 Korea Republic of The Navigation and Electronic System Laboratory Department of Aerospace Engineering Institute of Advanced Aerospace Technology Seoul National University Seoul08826 Korea Republic of

In recent years, the error-state Kalman filter (ErKF) has been extensively employed across various applications, including but not limited to robotics, aerospace, and localization. However, incorporating constraints into the ErKF framework when state constraint is necessary has remained a challenging task due to its intrinsic properties. This paper explores all possible ways to achieve this goal in the context of the estimate projection method. In particular, the constraint can be enforced before or after the ErKF’s correction step. We approach the problem from a mathematical perspective by deriving analytical solutions and discussing their statistical properties. We prove that the two mentioned methods are statistically identical for a linear system with linear constraints. Conversely, the filter’s behavior remains uncertain in the presence of linearized constraints. However, we provide a special case of the nonlinear constraint, wherein the results of the linear case remain valid. To support our theorem and verify the filter’s performance when the assumptions are invalidated, we present two Monte Carlo simulations under the increasing initialization error and the constraint’s incompleteness. The simulation results clearly confirm our insights and lead to the conclusion that constraining the error-state after the correction may offer superior outcomes compared to its competitor. © 2023, CC BY.

关键词： Linearization

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3D Scene Flow Estimation on Pseudo-LiDAR: Bridging the Gap on Estimating Point Motion

arXiv

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arXiv 2022年

作者： Jiang, Chaokang Wang, Guangming Miao, Yanzi Wang, Hesheng Engineering Research Center of Intelligent Control for Underground Space Ministry of Education School of Information and Control Engineering Advanced Robotics Research Center China University of Mining and Technology Xuzhou221116 China Department of Automation Key Laboratory of System Control and Information Processing Ministry of Education Key Laboratory of Marine Intelligent Equipment and System of Ministry of Education Shanghai Engineering Research Center of Intelligent Control and Management Shanghai Jiao Tong University Shanghai200240 China

3D scene flow characterizes how the points at the current time flow to the next time in the 3D Euclidean space, which possesses the capacity to infer autonomously the non-rigid motion of all objects in the scene. The previous methods for estimating scene flow from images have limitations, which split the holistic nature of 3D scene flow by estimating optical flow and disparity separately. Learning 3D scene flow from point clouds also faces the difficulties of the gap between synthesized and real data and the sparsity of LiDAR point clouds. In this paper, the generated dense depth map is utilized to obtain explicit 3D coordinates, which achieves direct learning of 3D scene flow from 2D images. The stability of the predicted scene flow is improved by introducing the dense nature of 2D pixels into the 3D space. Outliers in the generated 3D point cloud are removed by statistical methods to weaken the impact of noisy points on the 3D scene flow estimation task. Disparity consistency loss is proposed to achieve more effective unsupervised learning of 3D scene flow. The proposed method of self-supervised learning of 3D scene flow on real-world images is compared with a variety of methods for learning on the synthesized dataset and learning on LiDAR point clouds. The comparisons of multiple scene flow metrics are shown to demonstrate the effectiveness and superiority of introducing pseudo-LiDAR point cloud to scene flow estimation. © 2022, CC BY.

关键词： Three dimensional computer graphics

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Unsupervised Learning of 3D Scene Flow with 3D Odometry Assistance

arXiv

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arXiv 2022年

作者： Wang, Guangming Feng, Zhiheng Jiang, Chaokang Wang, Hesheng Department of Automation Key Laboratory of System Control and Information Processing of Ministry of Education Key Laboratory of Marine Intelligent Equipment and System of Ministry of Education Shanghai Engineering Research Center of Intelligent Control and Management Shanghai Jiao Tong University Shanghai200240 China Engineering Research Center of Intelligent Control for Underground Space Ministry of Education School of Information and Control Engineering Advanced Robotics Research Center China University of Mining and Technology Xuzhou221116 China

Scene flow represents the 3D motion of each point in the scene, which explicitly describes the distance and the direction of each point’s movement. Scene flow estimation is used in various applications such as autonomous driving fields, activity recognition, and virtual reality fields. As it is challenging to annotate scene flow with ground truth for real-world data, this leaves no real-world dataset available to provide a large amount of data with ground truth for scene flow estimation. Therefore, many works use synthesized data to pre-train their network and real-world LiDAR data to finetune. Unlike the previous unsupervised learning of scene flow in point clouds, we propose to use odometry information to assist the unsupervised learning of scene flow and use real-world LiDAR data to train our network. Supervised odometry provides more accurate shared cost volume for scene flow. In addition, the proposed network has mask-weighted warp layers to get a more accurate predicted point cloud. The warp operation means applying an estimated pose transformation or scene flow to a source point cloud to obtain a predicted point cloud and is the key to refining scene flow from coarse to fine. When performing warp operations, the points in different states use different weights for the pose transformation and scene flow transformation. We classify the states of points as static, dynamic, and occluded, where the static masks are used to divide static and dynamic points, and the occlusion masks are used to divide occluded points. The mask-weighted warp layer indicates that static masks and occlusion masks are used as weights when performing warp operations. Our designs are proved to be effective in ablation experiments. The experiment results show the promising prospect of an odometry-assisted unsupervised learning method for 3D scene flow in real-world data. Copyright © 2022, The Authors. All rights reserved.

关键词： Deep learning

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Numerical Investigation on Thermal Characteristics and Energy Efficiency of Lithium-Ion Battery Under Different Charging Stresses

SSRN

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SSRN 2024年

作者： Xie, Wenlong Gao, Xinlei Zhang, Zhengjie Tianjin Key Laboratory for Advanced Mechatronic System Design and Intelligent Control School of Mechanical Engineering Tianjin University of Technology Tianjin300384 China National Demonstration Center for Experimental Mechanical and Electrical Engineering Education Tianjin University of Technology China Department of Mechanical Engineering Imperial College London LondonSW7 2AZ United Kingdom School of Transportation Science and engineering Beihang University Beijing100191 China

The thermal characteristics of lithium-ion batteries during the charging process significantly impact their electrochemical performance and safety, particularly under high-rate or extreme temperature conditions. In this study, an electrochemical-thermal coupling model for a 2.5 Ah LiNi0.8Co0.1Mn0.1O2 18650 lithium-ion battery is proposed and experimentally validated. The heat generation and variation patterns of the electrodes at different charging rates and temperatures are evaluated, and the influence mechanisms of various electrode design parameters on charging energy efficiency are elucidated. The results reveal that high-rate charging increases the proportion of irreversible heat in the total heat generation, primarily due to the increase in ohmic heating at the positive electrode. Ambient temperature is less sensitive to heat generation than the C-rate, but low temperatures can also increase irreversible heat and are associated with an increase in positive polarization heat. Analyzing thermal characteristics at the electrode level can contribute to the optimization of battery design and the improvement of thermal safety. Electrode architectures, including electrode thickness, active material porosity, particle radius and negative/positive electrode capacity (N/P) ratio, are determined to analyze their effects on the heat generation of various components within the battery. Thick electrodes or active materials with high porosity induce significant ohmic heating and increase irreversible heat, with a slight effect on reversible heat, which is detrimental to energy efficiency. Large particle radii primarily increase reaction heat and polarization heat, and a high N/P ratio reduces the battery heat generation and is related to the reduction of negative reaction heat. Notably, variations in both two parameters have limited impact on to energy efficiency. Therefore, implementing appropriate thermal management across various charging scenarios is crucial for achievin

关键词： Lithium-ion batteries

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FFPA-Net: Efficient Feature Fusion with Projection Awareness for 3D Object Detection

arXiv

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arXiv 2022年

作者： Jiang, Chaokang Wang, Guangming Wu, Jinxing Miao, Yanzi Wang, Hesheng Engineering Research Center of Intelligent Control for Underground Space Ministry of Education School of Information and Control Engineering Advanced Robotics Research Center China University of Mining and Technology Xuzhou221116 China Department of Automation Key Laboratory of System Control and Information Processing of Ministry of Education Key Laboratory of Marine Intelligent Equipment and System of Ministry of Education Shanghai Engineering Research Center of Intelligent Control and Management Shanghai Jiao Tong University Shanghai200240 China The Department of Engineering Mechanics Shanghai Jiao Tong University Shanghai200240 China

Promising complementarity exists between the texture features of color images and the geometric information of LiDAR point clouds. However, there still present many challenges for efficient and robust feature fusion in the field of 3D object detection. In this paper, first, unstructured 3D point clouds are filled in the 2D plane and 3D point cloud features are extracted faster using projection-aware convolution layers. Further, the corresponding indexes between different sensor signals are established in advance in the data preprocessing, which enables faster cross-modal feature fusion. To address LiDAR points and image pixels misalignment problems, two new plug- and-play fusion modules, LiCamFuse and BiLiCamFuse, are proposed. In LiCamFuse, soft query weights with perceiving the Euclidean distance of bimodal features are proposed. In BiLiCamFuse, the fusion module with dual attention is proposed to deeply correlate the geometric and textural features of the scene. The quantitative results on the KITTI dataset demonstrate that the proposed method achieves better feature-level fusion. In addition, the proposed network shows a shorter running time compared to existing methods. Copyright © 2022, The Authors. All rights reserved.

关键词： Object detection

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Understanding the Limitations of Thick Electrodes on the Rate Capability of High-Energy Density Lithium-Ion Batteries

SSRN

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SSRN 2024年

作者： Xie, Wenlong Zhang, Zhengjie Gao, Xinlei Tianjin Key Laboratory for Advanced Mechatronic System Design and Intelligent Control School of Mechanical Engineering Tianjin University of Technology Tianjin300384 China National Demonstration Center for Experimental Mechanical and Electrical Engineering Education Tianjin University of Technology China School of Transportation Science and engineering Beihang University Beijing100191 China Department of Mechanical Engineering Imperial College London LondonSW7 2AZ United Kingdom

As a core component of transportation electrification, lithium-ion batteries need to address two critical challenges: achieving high energy density and enabling fast charging. However, changes in electrode thickness could result in a trade-off between these two characteristics. Herein, the impact of electrode thickness on the electrochemical performance, thermal behavior, as well as energy and power density of LiNi0.8Co0.1Mn0.1O2(NCM)/graphite batteries are investigated through mathematical modeling. Underutilization of active materials of the thick electrode is identified as the primary limitation on rate capability, which can be attributed to the slow solid-state diffusion and poor electrolyte transport within the electrode, especially the enlarged concentration gradients in the solid phase and the lithium depletion in the electrolyte phase during high-rate charging. Evolutions of local current density and heat generation rate along the electrode thickness are compared, identifying the underlying mechanism of inducing uneven reaction kinetics inside the battery. The trade-off between the energy and power density as a function of electrode thickness is investigated based on the limitations of charge transfer and mass transport. Furthermore, the rate-limiting factors under various application requirements are elucidated. This study will provide guidance for the electrode design of high-energy-density batteries with fast-charging capabilities. © 2024, The Authors. All rights reserved.

关键词： Lithium-ion batteries

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Basic reason for the accumulation of charge on the surface of polymer dielectrics

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Science China Materials 2022年第10期65卷 2884-2888页

作者： Tianyu Wang Xiaofen Li Boya Zhang Dayu Li Jianbo Liu Guixin Zhang State Key Laboratory of Control and Simulation of Power System and Generation Equipment Department of Electrical EngineeringTsinghua UniversityBeijing 100084China Key Laboratory of Advanced Materials(MOE) School of Materials Science and EngineeringTsinghua UniversityBeijing 100084China State Key Laboratory of Electrical Insulation and Power Equipment Xi’an Jiaotong UniversityShaanxi 710049China

Due to their outstanding electrical insulation performance,low energy loss and high reliability,polymer dielectrics are widely used in flexible electronics,capacitors and large-scale power transmission equipment[1–5].However,polymer dielectrics accumulate large amounts of charge on their surface during use,which causes local electric field distortion and induces flashover,explosion,and equipment damage[6–9].Although researchers have attempted to develop methods to reduce the accumulation of surface charge through material modification,such as plasma treatment[10],direct fluorination[11],and coating[7,9,12],each of these methods has drawbacks;thus,the bottleneck has yet to be overcome.

关键词：电荷量第一性原理计算聚合物表面电介质电场畸变深能级缺陷电荷测量电荷特性

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