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92nd Annual Meeting of the International Association of applied Mathematics and mechanics, GAMM 2021

作者： Makvandi, Resam Abali, Bilen Emek Eisenträger, Sascha Juhre, Daniel Otto von Guericke University Magdeburg Institute of Mechanics Universitätsplatz 2 Magdeburg39106 Germany Uppsala University Department of Materials Science and Engineering Applied Mechanics UppsalaSE-751 05 Sweden The University of New South Wales School of Civil and Environmental Engineering SydneyNSW2052 Australia

Phase-field modelling has been shown to be a powerful tool for simulating fracture processes and predicting the crack path under complex loading conditions. Note that the total energy of fracture in the classical phase-field formulations includes the strain energy density from the linear elasticity theory resulting in singular stresses at the crack tip. Recently, we have demonstrated that integrating the strain gradient elasticity into the conventional phase-field fracture formulations may improve the final results by alleviating the effects of a singular stress field around the crack tip [1]. The current contribution focuses on a more general formulation of strain gradient elasticity. © 2021 The Authors. Proceedings in applied Mathematics & mechanics published by Wiley-VCH GmbH.

关键词： Crack tips

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Bifurcation of nanoscale thermolubric friction behavior for sliding on MoS2

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Physical Review materials 2021年第8期5卷 083607-083607页

作者： Kathryn R. Hasz Mohammad R. Vazirisereshk Ashlie Martini Robert W. Carpick Department of Materials Science and Engineering University of Pennsylvania Philadelphia Pennsylvania 19104 USA Department of Mechanical Engineering University of California Merced California 95343 USA Department of Mechanical Engineering and Applied Mechanics University of Pennsylvania Philadelphia Pennsylvania 19104 USA

We present atomic force microscopy experiments of wearless sliding between nanoscale tips and both bulk and monolayer MoS2 in ultrahigh vacuum across a wide range of temperatures (150–450 K) and scanning speeds (5 nm/s to 500 μm/s). Atomic lattice stick-slip behavior is consistently resolved. However, a bifurcation of behavior is seen, with some measurements showing a strong decrease in friction with increasing temperature and others showing athermal and low friction under nominally identical conditions. The difference between thermal and athermal behavior is attributed to a change in the corrugation of the potential energy surface, possibly due to trace amounts of adsorbed contaminants. While the speed dependence at a given temperature is consistent with the thermal Prandtl-Tomlinson model for atomic-scale friction, that is not the case for the temperature dependence (when it is present), nor can the temperature dependence be described by other existing models. We discuss the limitations of these models considering the measured results.

关键词： Friction Temperature Tribology Transition metal dichalcogenides Atomic force microscopy

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Designing the pressure-dependent shear modulus using tessellated granular metamaterials

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Physical Review E 2023年第3期108卷 034901-034901页

作者： Jerry Zhang Dong Wang Weiwei Jin Annie Xia Nidhi Pashine Rebecca Kramer-Bottiglio Mark D. Shattuck Corey S. O'Hern Department of Mechanical Engineering & Materials Science Yale University New Haven Connecticut 06520 USA Benjamin Levich Institute and Physics Department The City College of New York New York New York 10031 USA Department of Physics Yale University New Haven Connecticut 06520 USA Department of Applied Physics Yale University New Haven Connecticut 06520 USA Integrated Graduate Program in Physical and Engineering Biology Yale University New Haven Connecticut 06520 USA

Jammed packings of granular materials display complex mechanical response. For example, the ensemble-averaged shear modulus 〈G〉 increases as a power law in pressure p for static packings of soft spherical particles that can rearrange during compression. We seek to design granular materials with shear moduli that can either increase or decrease with pressure without particle rearrangements even in the large-system limit. To do this, we construct tessellated granular metamaterials by joining multiple particle-filled cells together. We focus on cells that contain a small number of bidisperse disks in two dimensions. We first study the mechanical properties of individual disk-filled cells with three types of boundaries: periodic boundary conditions (PBC), fixed-length walls (FXW), and flexible walls (FLW). Hypostatic jammed packings are found for cells with FLW, but not in cells with PBC and FXW, and they are stabilized by quartic modes of the dynamical matrix. The shear modulus of a single cell depends linearly on p. We find that the slope of the shear modulus with pressure λc<0 for all packings in single cells with PBC where the number of particles per cell N≥6. In contrast, single cells with FXW and FLW can possess λc>0, as well as λc<0, for N≤16. We show that we can force the mechanical properties of multicell granular metamaterials to possess those of single cells by constraining the end points of the outer walls and enforcing an affine shear response. These studies demonstrate that tessellated granular metamaterials provide a platform for the design of soft materials with specified mechanical properties.

关键词： Jamming Granular solids Mechanical metamaterials

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Reducing Effective System Dimensionality with Long-Range Collective Dipole-Dipole Interactions

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Physical Review Letters 2024年第17期132卷 173803-173803页

作者： Ashwin K. Boddeti Yi Wang Xitlali G. Juarez Alexandra Boltasseva Teri W. Odom Vladimir Shalaev Hadiseh Alaeian Zubin Jacob Elmore Family School of Electrical and Computer Engineering Purdue University West Lafayette Indiana 47907 USA Birck Nanotechnology Center Purdue University West Lafayette Indiana 47907 USA Graduate Program in Applied Physics Northwestern University Evanston Illinois 60208 USA Department of Materials Science and Engineering Northwestern University Evanston Illinois 60208 USA Department of Chemistry Northwestern University Evanston Illinois 60208 USA School of Physics and Astronomy Purdue University West Lafayette Indiana 47907 USA

Dimensionality plays a crucial role in long-range dipole-dipole interactions (DDIs). We demonstrate that a resonant nanophotonic structure modifies the apparent dimensionality in an interacting ensemble of emitters, as revealed by population decay dynamics. Our measurements on a dense ensemble of interacting quantum emitters in a resonant nanophotonic structure with long-range DDIs reveal an effective dimensionality reduction to d¯=2.20(12), despite the emitters being distributed in 3D. This contrasts with the homogeneous environment, where the apparent dimension is d¯=3.00. Our work presents a promising avenue to manipulate dimensionality in an ensemble of interacting emitters.

关键词： Light-matter interaction Long-range interactions Metamaterials Optics & lasers Photonics Plasmonics Quantum optics

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Field-Dependent Magnetic Domain Behavior in van der Waals Fe3GeTe2

arXiv

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arXiv 2022年

作者： Li, Yue Basnet, Rabindra Pandey, Krishna Hu, Jin Wang, Wei Ma, Xuedan McCray, Arthur R.C. Petford-Long, Amanda K. Phatak, Charudatta Materials Science Division Argonne National Laboratory LemontIL60439 United States Department of Physics University of Arkansas FayettevilleAR72701 United States Materials Science and Engineering Program University of Arkansas FayettevilleAR72701 United States Center for Nanoscale Materials Argonne National Laboratory LemontIL60439 United States Applied Physics Program Northwestern University EvanstonIL60208 United States Department of Materials Science and Engineering Northwestern University EvanstonIL60208 United States

Two-dimensional magnetic van der Waals (vdW) materials can show a variety of topological nontrivial spin textures, such as Bloch- or Néel-type stripe, skyrmion or bubble domains under certain external stimuli. It is critical to understand the magnetic domain behavior in vdW materials in order to control their size, and density in response to external stimuli such as electric and magnetic fields. Here we examine the magnetic field dependence of topologically non-trivial magnetization spin textures in vdW Fe3GeTe2. Néel-type stripe domains and skyrmions are formed depending on the magnetic field-cooling protocol used during in-situ Lorentz transmission electron microscopy (LTEM) experiments. Use of quantitative reconstruction of magnetic induction maps, and micromagnetic simulations, allow for understanding the LTEM results of Néel-type stripe domains as well as skyrmions. In addition, the deformation of skyrmion contrast is observed as a result of the introduction of an in-plane magnetic field. We demonstrate the stability of the stripe domains and skyrmions in response to externally applied magnetic field due to energy barrier for domain wall annihilation. Our results establish an understanding of the energy landscape that governs the behavior of the topologically non-trivial spin textures in vdW materials which can be harnessed for spintronic applications. Copyright © 2022, The Authors. All rights reserved.

关键词： Van der Waals forces

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Energy based methods applied in mechanics by using the extended Noether's formalism

arXiv

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arXiv 2021年

作者： Abali, Bilen Emek Uppsala University Division of Applied Mechanics Department of Materials Science and Engineering Box 534 UppsalaSE-751 21 Sweden

Physical systems are modeled by field equations, these are coupled, partial differential equations in space and time. Field equations are often given by balance equations and constitutive equations, where the former is axiomatically given and the latter is thermodynamically derived. This method has difficulties in damage mechanics in generalized continua. An alternative method to derive governing equations is based on a variational framework known as the extended Noether's formalism. Its formal introduction relies on mathematical concepts limiting its use in applied mechanics as a field theory. In this work, we demonstrate the power of extended Noether's formalism by using tensor algebra and usual continuum mechanics nomenclature in order to make use of it in generalized mechanics. Copyright © 2021, The Authors. All rights reserved.

关键词： Continuum mechanics

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Thermal Hysteresis Behavior of Skyrmion Lattices in the van der Waals Ferromagnet Fe3GeTe2

arXiv

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arXiv 2022年

作者： McCray, Arthur R.C. Li, Yue Basnet, Rabindra Pandey, Krishna Hu, Jin Phelan, Daniel Ma, Xuedan Petford-Long, Amanda K. Phatak, Charudatta Materials Science Division Argonne National Laboratory LemontIL60439 United States Applied Physics Program Northwestern University EvanstonIL60208 United States Department of Physics University of Arkansas FayettevilleAR72701 United States Materials Science and Engineering Program University of Arkansas FayettevilleAR72701 United States Center for Nanoscale Materials Argonne National Laboratory LemontIL60439 United States Department of Materials Science and Engineering Northwestern University EvanstonIL60208 United States

Understanding the physics of phase transitions in two-dimensional (2D) systems underpins the research in diverse fields including statistical mechanics, quantum systems, nanomagnetism, and soft condensed matter. However, many fundamental aspects of 2D phase transitions are still not well understood, including the effects of interparticle potential, polydispersity, and particle shape. Magnetic skyrmions, which are non-trivial chiral spin structures, can be considered as quasi-particles that form two-dimensional lattices. Here we show, by real-space imaging using in situ cryo-Lorentz transmission electron microscopy coupled with machine learning, the ordering behavior of Néel skyrmion lattices in van der Waals Fe3GeTe2. We demonstrate a distinct change in the skyrmion size distribution during field-cooling, which leads to a loss of lattice order and an evolution of the skyrmion liquid phase. Remarkably, the lattice order is restored during field heating and demonstrates a thermal hysteresis. Our quantitative analysis explains this behavior based on the energy landscape of skyrmions and demonstrates the potential to control the lattice order in 2D phase transitions. Copyright © 2022, The Authors. All rights reserved.

关键词： Van der Waals forces

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Facile Li-Ion Transport via LLTO Scaffold with Crosslinked Polyethylene Glycol Composite Electrolyte for Solid-State Batteries

SSRN

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SSRN 2025年

作者： Lee, Jungkuk Counihan, Michael J. Barai, Pallab Burns, Meghan E. Singh, Vibhu V. Jamnuch, Sasawat Pascal, Tod A. Shrinivasan, Venkat Tepavcevic, Sanja Zhang, Yuepeng Applied Materials Division Argonne National Laboratory LemontIL60439 United States Materials Science Division Argonne National Laboratory LemontIL60439 United States Department of Chemistry University of Illinois Chicago ChicagoIL60607 United States ATLAS Materials Physics Lab Aiiso Yufeng Li Family Department of Chemical and Nano Engineering University of California San Diego La Jolla CA92093 United States Microscopy and Microanalysis Research Group Materials Measurement Science Division National Institute of Standards and Technology GaithersburgMD20899 United States Material Science and Engineering Program University of California San Diego La Jolla CA92093 United States Chemical Sciences and Engineering Division Argonne National Laboratory LemontIL60439 United States

Composite polymer electrolytes (CPEs) hold significant promise for solid-state batteries due to their ability to combine the benefits of inorganic fillers and polymer matrices. However, agglomeration of inorganic fillers can disrupt the formation of a percolation pathway, hindering lithium-ion transport. Here, we developed a stable, porous, and interconnected 3-dimentional LLTO (Li0.33La0.557TiO3) nanofiber scaffold and fabricate CPEs using in-situ crosslinked polyethylene glycol (xPEG). The resulting self-standing LLTOxPEG-65 achieved an ionic conductivity of 5.0 × 10−4 S/cm at 30 °C and a critical current density of 0.5 mA/cm2. A significantly lower activation energy (~0.2 eV) was observed in LLTOxPEG-65 compared to pristine xPEG (0.44 eV), indicating a transition of lithium-ion transport pathways from xPEG to the LLTO scaffold. However, increasing the xPEG content led to a decrease in ionic conductivity and a rise in activation energy, approaching that of pristine xPEG. DFT calculations revealed that Li+ transport in the [010] and [001] planes of LLTO predominantly takes place within the bulk rather than along the surface, while a concerted diffusion mechanism was observed in the [100] plane. Additionally, mesoscale-level computational analysis indicated that the high LLTO scaffold fraction (90 wt %) can ensure transport through the bulk of the fibers even with larger interfacial charge transfer resistance, around 1 Ω·cm2 between LLTO and xPEG. Presence of the highly percolated LLTO scaffold helps to promote efficient Li+ transport through the bulk of LLTO. © 2025, The Authors. All rights reserved.

关键词： Activation energy

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Effect of storage conditions on the dietary and pharmaceutical values of ginger oil, and modeling its dielectric properties

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Grasas y Aceites 2024年第4期75卷

作者： Abushal, S.A. Uguru, H. Akpomedaye, O. Kuzmin, A. Sami, R. Helal, M. Alsanei, W.A. Almehmadi, A.M. ALmasoudi, A.G. Program of Food Sciences and Nutrition Turabah University College Taif University Saudi Arabia Department of Agricultural Engineering Delta State University of Science and Technology Ozoro Nigeria Department of Electrical Engineering Delta State University of Science and Technology Ozoro Nigeria Department of Mechanization of Agricultural Products Processing National Research Mordovia State University Saransk Russia Scientific Laboratory of Advanced Composite Materials and Technologies Plekhanov Russian University of Economics Moscow Russia Department of Food Science and Nutrition College of Sciences Taif University Saudi Arabia Department of Mechanical Engineering Faculty of Engineering Taif University Saudi Arabia Department of Food and Nutrition Faculty of Human Sciences and Design King Abdulaziz University Jeddah Saudi Arabia Department of Clinical Nutrition Faculty of Applied Medical Sciences Umm Al-Qura University Makkah Saudi Arabia Program of Food Sciences and Nutrition Biology Department Branch of the College at Turbah Taif University Taif Saudi Arabia

This research was conducted to evaluate the impact of the storage conditions of ginger rhizomes on the nutritional and therapeutic properties of the ginger oil (GO). The physicochemical and phytochemical properties, fatty acid contents and dielectric constant (Ε′) of the GO were analyzed in accordance with standard guidelines. The findings revealed that the storage temperature significantly impacted the quality of GO (p ©2024 CSIC.

关键词： Polyunsaturated fatty acids

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A Mesoscopic Model for Competitive Adsorption of Albumin and Fibrinogen Based on Dissipative Particle Dynamics

SSRN

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SSRN 2022年

作者： Wu, Xiao Wang, Chenyang Hao, Pengfei He, Feng Yao, Zhaohui Wei, Zon-Han Zhang, Xiwen School of Mechanics and Safety Engineering Zhengzhou University Henan Zhengzhou450001 China Applied Mechanics Laboratory Department of Engineering Mechanics Tsinghua University Beijing100084 China AVIC Aerodynamics Research Institute Joint Research Center for Advanced Materials and Anti Icing School of Materials Science and Engineering Tsinghua University Beijing100084 China University of Chinese Academy of Sciences Beijing101408 China

The protein layer generated by the competitive adsorption of body proteins on the surface dominates the biological response of the material. Further understanding of competitive adsorption of body proteins is vital to the development of biomaterial. Meanwhile, such competitive adsorption is a mesoscopic process at physiological protein concentration, and neither macroscopic experiment nor microscopic MD (molecular dynamics) simulation is suitable to clarify it. Here, we proposed a mesoscopic DPD (dissipative particle dynamics) model to illustrate the competitive process of albumin and fibrinogen with its parameters deduced from our previous MD simulation, and proved the model well retained the diffusion and adsorption properties of proteins in the competitive adsorption on the plane surface. We then applied the model to the competitive adsorption on the surfaces with different nanostructures, and found that nanostructures provide greater surface area and adsorption sites, which usually promotes the competitive advantage of the albumin. Meanwhile, when the structure size is much larger than that of protein, the increase in surface area is the main effect of nanostructures. When the structure size is close to that of protein, the coordination of the nanostructure and the shape of protein has a significant effect on competitive adsorption. © 2022, The Authors. All rights reserved.

关键词： Proteins

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