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arXiv 2024年

作者： Zhou, Jianbin Wang, Shen Wu, Chaoshan Qi, Ji Wan, Hongli Lai, Shen Feng, Shijie Ko, Tsz Wai Liang, Zhaohui Zhou, Ke Harpak, Nimrod Solan, Nick Liu, Mengchen Hui, Zeyu Ai, Paulina J. Griffith, Kent Wang, Chunsheng Ong, Shyue Ping Yao, Yan Liu, Ping Department of Nanoengineering University of California San Diego La Jolla CA United States Materials Science and Engineering Program Texas Center for Superconductivity The University of Houston University of Houston HoustonTX United States Department of Chemical and Biomolecular Engineering University of Maryland College ParkMD United States Department of Chemistry and Biochemistry University of California San Diego La Jolla CA92093 United States The Bishop's School La Jolla CA92037 United States

Unlike Li-ion transport in the bulk of carbonaceous materials, little is known about Li-ion diffusion on their surface. In this study, we have discovered an ultra-fast Li-ion transport phenomenon on the surface of carbonaceous materials, particularly when they have limited Li insertion capacity along with a high surface area. This is exemplified by a carbon black, Ketjen Black (KB). An ionic conductivity of 18.1 mS cm-1 at room temperature is observed, far exceeding most solid-state ion conductors. Theoretical calculations reveal a low diffusion barrier for the surface Li species. The species is also identified as Li*, which features a partial positive charge. As a result, lithiated KB functions effectively as an interlayer between Li and solid-state electrolytes (SSE) to mitigate dendrite growth and cell shorting. This function is found to be electrolyte agnostic, effective for both sulfide and halide SSEs. Further, lithiated KB can act as a high-performance mixed ion/electron conductor that is thermodynamically stable at potentials near Li metal. A graphite anode mixed with KB instead of a solid electrolyte demonstrates full utilization with a capacity retention of ~85% over 300 cycles. The discovery of this surface-mediated ultra-fast Li-ion transport mechanism provides new directions for the design of solid-state ion conductors and solid-state batteries. Copyright © 2024, The Authors. All rights reserved.

关键词： Solid electrolytes

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Efficient thermo-optic micro-ring phase shifter made of PECVD silicon-rich amorphous silicon carbide

arXiv

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arXiv 2022年

作者： Chang, Li-Yang Sunny Pappert, Steve Yu, Paul K.L. Materials Science and Engineering Program The Department of Mechanical and Aerospace Engineering University of California San Diego 9500 Gilman Drive La Jolla CA92093 United States Department of Electrical & Computer Engineering University of California San Diego 9500 Gilman Drive La Jolla CA92093 United States

In this work, the thermo-optic coefficient (TOC) of the silicon-rich amorphous silicon carbide (a-SiC) thin film deposited by plasma-enhanced chemical vapor deposition is characterized. We found that the TOC of the film increases as its silicon content increases. A more than three-fold improvement in the TOC is measured, reaching a TOC as high as 1.88 × 10−4 ℃−1, which is comparable to that of crystalline silicon. An efficient thermo-optic phase shifter has also been demonstrated by integrating the silicon-rich a-SiC micro-ring structure with a NiCr heater. Its tuning efficiency Pπ as low as 4.4 mW has been measured at an optical wavelength of 1550 nm. These findings make silicon-rich a-SiC a good material candidate for thermo-optic applications in photonic integrated circuits. Copyright © 2022, The Authors. All rights reserved.

关键词： Silicon carbide

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Preprocessing Techniques for Enhancing Vision-Based Detection System for Tire Sidewall Extraction

Preprocessing Techniques for Enhancing Vision-Based Detectio...

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International Seminar on Research of Information Technology and Intelligent Systems (ISRITI)

作者： Jia Hao Loo Veronica Lestari Jauw Chin Seong Lim Khairul-Rijal Sarmin Nunung Nurul Qomariyah Ahmad Nurul Fajar Department of Mechanical Materials and Manufacturing Engineering University of Nottingham Malaysia Malaysia Continental Tyre Technology Centre Malaysia Petaling Jaya Malaysia Computer Science Department School of Computing and Creative Arts Bina Nusantara University Jakarta Indonesia Information System Management Department BINUS Graduate Program-Master Information Systems Bina Nusantara University Jakarta Indonesia

ISBN: (数字)9798331519643

ISBN: (纸本)9798331519650

This study aims to develop a system for extracting crucial information from tire sidewalls using Optical Character Recognition (OCR). Initially, images of tire were captured manually by smartphone cameras, including Redmi 9T, iPhone 11, and Galaxy S23 Ultra. The captured images are then transferred to a computer for storage. Subsequently, these images were cropped according to the boundaries identified by Hough Circle Transform (HCT). The cropped images were then further pre-processed. During the pre-processing phase, geometrical transformation and image sharpening techniques are applied to enhance the clarity and readability of the text images. The text is then extracted using Google Vision, with the extracted text categorized by size, DOT, brand and pattern. The results indicated that the effectiveness of image pre-processing was constrained by the accuracy of circle detection, which reached a maximum rate of 87.1%. This causes parts of the text to be cut out inaccurately, leading to a suboptimal extraction accuracy of 55.65%. It is also observed that the Redmi 9T camera produced inconsistent results compared to other devices. Specifically, the iPhone 11 and Samsung Galaxy S23 Ultra demonstrated superior extraction accuracies of 69.71% and 66.37%, respectively, whereas the Redmi 9T achieved a lower extraction accuracy of 37.76%.

关键词： Accuracy Optical character recognition Text categorization Lighting Transforms US department of Transportation Cameras Tires Internet Data mining

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Medium-entropy engineering of magnetism in layered antiferromagnet CuxNi2(1-x)CrxP2S6

arXiv

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arXiv 2024年

作者： Upreti, Dinesh Basnet, Rabindra Sharma, M.M. Chhetri, Santosh Karki Acharya, Gokul Nabi, Md Rafique Un Sakon, Josh Mortazavi, Mansour Hu, Jin Department of Physics University of Arkansas FayettevilleAR72701 United States Department of Chemistry & Physics University of Arkansas at Pine Bluff Pine BluffAR71603 United States MonArk NSF Quantum Foundry University of Arkansas FayettevilleAR72701 United States Department of Chemistry & Biochemistry University of Arkansas FayettevilleAR72701 United States Materials Science and Engineering Program Institute for Nanoscience and Engineering University of Arkansas FayettevilleAR72701 United States

engineering magnetism in layered magnets could result in novel phenomena related to two-dimensional (2D) magnetism, which can be useful for fundamental research and practical applications. Extensive doping efforts such as substitution and intercalation have been adopted to tune antiferromagnetic (AFM) properties in M2P2X6 compounds. The substitutional doping in this material family has mainly focused on bimetallic substitution. Recently, the metal substitution can also be extended to more than two metal elements, leading to medium and high-entropy alloys (MEAs and HEAs), which are fairly underexplored in layered magnetic systems including M2P2X6. In this work, we explored the magnetic properties of the previously unreported Cu- and Cr-substituted Ni2P2S6 i.e., CuxNi2(1-x)CrxP2S6. Our study reveals a relatively systematic evolution of AFM phases with substitution than that observed in traditional bimetallic substitution in M2P2X6. Furthermore, the Cu and Cr substitutions in Ni2P2S6 are found to enhance the ferromagnetic (FM) correlation, which is also accompanied by a possible weak FM phase at low temperatures for the intermediate compositions 0.32≤x≤0.80. Our work provides a strategy to establish ferromagnetism in AFM M2P2X6 that can also be used for property tuning in other layered magnets. © 2024, CC BY-NC-SA.

关键词： Ferromagnetism

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Fate of multipolar physics in 5d2 double perovskites

arXiv

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arXiv 2023年

作者： Rayyan, Ahmed Liu, Xiaoyu Kee, Hae-Young Department of Physics University of Toronto TorontoONM5S 1A7 Canada Department of Materials Science and Engineering University of Washington SeattleWA98195 United States CIFAR Program in Quantum Materials Canadian Institute for Advanced Research TorontoONM5G 1M1 Canada

In a cubic environment, the ground state of spin-orbit coupled 5d2 ions is a non-Kramers Eg doublet, which hosts quadrupole and octupole moments. A series of 5d2 osmium double perovskites Ba2MOsO6 (M = Mg, Ca, Zn, Cd) have recently been proposed to exhibit multipolar orders. We investigate the structural properties of these materials using ab-initio calculations and find that the cubic structure is unstable for the Cd compound while the Mg, Ca, and Zn materials retain Fm3¯m symmetry. We show that Ba2CdOsO6 favours a rhombohedral R3¯ structure characterized by a−a−a− octahedral tiltings as indicated by unstable T1g phonon modes. Trigonal distortions split the excited T2g triplet into an Eg′ doublet and an Ag singlet, which may cross energy levels with the Eg doublet and suppress the multipolar physics. We find a window where Eg remains the lowest energy state under trigonal distortion, enabling the emergence of multipole phases in non-cubic crystal environments. © 2023, CC BY.

关键词： Barium compounds

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Oxidation of Eutectic Gallium-Indium Nanoparticles

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Microscopy and Microanalysis 2024年第SUPPLEMENT_1期30卷

作者： Ye, Shuonan Chen, Xiaobo Sun, Xianhu Singler, Timothy Zhang, Pu Zhou, Guangwen Materials Science and Engineering Program & Department of Mechanical Engineering State University of New York at Binghamton Binghamton New York United States

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Computational design of anisotropic stealthy hyperuniform composites with engineered directional scattering properties

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Physical Review E 2023年第4期108卷 045306-045306页

作者： Wenlong Shi David Keeney Duyu Chen Yang Jiao Salvatore Torquato Materials Science and Engineering Arizona State University Tempe Arizona 85287 USA Materials Research Laboratory University of California Santa Barbara California 93106 USA Department of Physics Arizona State University Tempe Arizona 85287 USA Department of Chemistry Princeton University Princeton New Jersey 08544 USA Department of Physics Princeton University Princeton New Jersey 08544 USA Princeton Institute of Materials Princeton University Princeton New Jersey 08544 USA Program in Applied and Computational Mathematics Princeton University Princeton New Jersey 08544 USA

Disordered hyperuniform materials are an emerging class of exotic amorphous states of matter that endow them with singular physical properties, including large isotropic photonic band gaps, superior resistance to fracture, and nearly optimal electrical and thermal transport properties, to name but a few. Here we generalize the Fourier-space-based numerical construction procedure for designing and generating digital realizations of isotropic disordered hyperuniform two-phase heterogeneous materials (i.e., composites) developed by Chen and Torquato [Acta Mater. 142, 152 (2018)] to anisotropic microstructures with targeted spectral densities. Our generalized construction procedure explicitly incorporates the vector-dependent spectral density function χ̃V(k) of arbitrary form that is realizable. We demonstrate the utility of the procedure by generating a wide spectrum of anisotropic stealthy hyperuniform microstructures with χ̃V(k)=0 for k∈Ω, i.e., complete suppression of scattering in an “exclusion” region Ω around the origin in Fourier space. We show how different exclusion-region shapes with various discrete symmetries, including circular-disk, elliptical-disk, square, rectangular, butterfly-shaped, and lemniscate-shaped regions of varying size, affect the resulting statistically anisotropic microstructures as a function of the phase volume fraction. The latter two cases of Ω lead to directionally hyperuniform composites, which are stealthy hyperuniform only along certain directions and are nonhyperuniform along others. We find that while the circular-disk exclusion regions give rise to isotropic hyperuniform composite microstructures, the directional hyperuniform behaviors imposed by the shape asymmetry (or anisotropy) of certain exclusion regions give rise to distinct anisotropic structures and degree of uniformity in the distribution of the phases on intermediate and large length scales along different directions. Moreover, while the anisotropic exclusion regions

关键词： Amorphous materials Complex materials Simulated annealing

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Flow Electrification of a Corona-Charged Polyethylene Terephthalate Film (vol 36, pg 9571, 2020)

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LANGMUIR 2020年第43期36卷 13124-13124页

作者： Kou, Rui Zhong, Ying Qiao, Yu Department of Structural Engineering University of California—San Diego La Jolla California 92093-0085 United States Department of Structural Engineering University of California—San Diego La Jolla California 92093-0085 United States Department of Mechanical Engineering University of South Florida Tampa Florida 33620 United States Department of Structural Engineering University of California—San Diego La Jolla California 92093-0085 United States Program of Materials Science and Engineering University of California—San Diego La Jolla California 92093 United States

Corona charging of a free-standing polymer film can produce a quasi-permanent potential difference across the film thickness, while the absolute amplitude of the surface voltage may be highly sensitive to the free charges. To precisely control the voltage distribution, we investigated the flow electrification technology by exposing corona-charged polyethylene terephthalate films to sodium salt solutions. The surface voltage and the free-charge density were adjusted by the salt concentration, the anion size, and the flow rate. The dipolar component of electric potential remained unchanged. This result has significant scientific interest and technological importance to surface treatment, filtration, energy harvesting, among others.

关键词： Anions Liquids Positron emission tomography Electrical properties Electrodes

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Visualizing Field-free Deterministic Magnetic Switching of all–van der Waals Spin-Orbit Torque System Using Spin Ensembles in Hexagonal Boron Nitride

arXiv

引用

arXiv 2025年

作者： Zhang, Xi Zhou, Jingcheng Hu, Chaowei Deng, Kuangyin Wang, Chuangtang Agarwal, Nishkarsh Jin, Hanshang Al-Matouq, Faris A. Xu, Stelo Trivedi, Roshan S. Li, Senlei Rathi, Sumedh Lu, Hanyi Jiang, Zhigang Taufour, Valentin Hovden, Robert Zhao, Liuyan Cheng, Ran Xu, Xiaodong Chu, Jiun-Haw Du, Chunhui Rita Wang, Hailong School of Physics Georgia Institute of Technology AtlantaGA30332 United States Department of Physics University of Washington SeattleWA98105 United States Department of Electrical and Computer Engineering University of California RiversideCA92521 United States Department of Physics University of Michigan Ann ArborMI48109 United States Department of Materials Science and Engineering University of Michigan Ann ArborMI48109 United States Department of Physics and Astronomy University of California DavisCA95616 United States Department of Physics University of California San Diego La Jolla CA92093 United States Applied Physics Program University of Michigan Ann ArborMI48109 United States Department of Physics and Astronomy University of California RiversideCA92521 United States Department of Materials Science and Engineering University of Washington SeattleWA98105 United States

Recently, optically active spin defects embedded in van der Waals (vdW) crystals have emerged as a transformative quantum sensing platform to explore cutting-edge materials science and quantum physics. Taking advantage of excellent solid-state integrability, this new class of spin defects can be arranged in controllable nanoscale proximity of target materials in vdW heterostructures, showing great promise for improving spatial resolution and field sensitivity of current sensing technologies. Building on this state-of-the-art measurement platform, here we report hexagonal boron nitride-based quantum imaging of field-free deterministic magnetic switching of room-temperature two-dimensional magnet Fe3GaTe2 in an all-vdW spin-orbit torque (SOT) system. By visualizing SOT-driven variations of nanoscale Fe3GaTe2 magnetic stray field profile under different conditions, we have revealed how the observed magnetic switching evolves from deterministic to indeterministic behavior due to the interplay between out-of-plane spins, in-plane spins and Joule heating. This understanding, which is otherwise difficult to access by conventional transport measurements, offers valuable insights on material design, testing, and evaluation of next-generation vdW spintronic devices. Copyright © 2025, The Authors. All rights reserved.

关键词： Van der Waals forces

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Thin curved optics and the Twyman effect

Thin curved optics and the Twyman effect

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Optical Fabrication and Testing, OFT 2021 - Part of OSA Optical Design and Fabrication 2021

作者： Lakshmanan, Sanjay N. Lambropoulos, John C. Department of Mechanical Engineering University of Rochester RochesterNY14627 United States Materials Science Program University of Rochester RochesterNY14627 United States Laboratory for Laser Energetics University of Rochester RochesterNY14627 United States

We use numerical simulations and analytical techniques to assess the role of local thickness nonuniformity and curvature in the Twyman effect. A flat optic of similar thickness is used as a convenient metric for compa...

ISBN: (纸本)9781557528209

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