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Magneto-optical Kerr spectra of gold induced by spin accumulation

Physical Review B 2022年第1期106卷 014410-014410页

作者： Víctor H. Ortiz Sinisa Coh Richard B. Wilson Department of Mechanical Engineering and Materials Science and Engineering Program University of California Riverside 92521 CA United States

We report the magneto-optic Kerr effect (MOKE) angle of Au magnetically excited by spin accumulation. We perform time-resolved polar MOKE measurements on Au/Co heterostructures. In our experiment, the ultrafast optical excitation of the Co drives spin accumulation into an adjacent Au layer. The spin accumulation, together with spin-orbit coupling, leads to nonzero terms in the off-diagonal conductivity tensor of Au, which we measure by recording the polarization and ellipticity of light reflected from the Au surface for photon energies between 1.3 and 3.1 eV. In a narrow energy range near the interband transition threshold of Au, the sensitivity to magnetization measured exceeds 1μradperA/m. In the photon energy interval of 0.6–4.4 eV, the maximum value for transition ferromagnetic metals like Ni are <10nradperA/m, while predicted values for heavy metals like Pt or W are <13nradperA/m. The exceptional sensitivity of the optical properties of Au to spin magnetic moments make Au an exceptionally sensitive optical magnetometer, with potential applications in the development of optospintronic technologies.

关键词： Density of states Magneto-optical Kerr effect Spin accumulation Ultrafast magnetic effects

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Evolution of hierarchical petal-like 3D SnS2 as high-performance electrode materials for supercapacitor applications

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materials Today: Proceedings 2022年 67卷 1039-1042页

作者： Kumar, Niraj Bhusan Sahoo, Bibhuti Chandra Sahu, Krushna Kumar Sahoo, Naresh Naik, Brundabana Soam, Ankur Kumar, Rahul Tripathi, Abhishek Kumar Sahoo, Prasanta Maharashtra Pune 411025 India Department of Mechanical Engineering Siksha ‘O’ Anusandhan Deemed to be University Odisha Bhubaneswar 751030 India Department of Chemistry Environmental Science and Technology Program Siksha ‘O’ Anusandhan Deemed to be University Odisha Bhubaneswar 751030 India Department of Energy Science and Engineering IIT Delhi New Delhi 110016 India Department of Metallurgical and Materials Engineering Malaviya National Institute of Technology Jaipur Jaipur 302017 India

A simple one-step solvothermal approach has been adopted for the synthesis of SnS2. SEM shows hierarchically SnS2 with petal-like 3-dimensional layer structures because of this process. In this investigation, the as-prepared electrode material have an excellent specific capacitance of 721F g−1 at 1 mVs−1, indicating extraordinary performance. The improved electrochemical performance is because to unique ultrathin petal discrete structure, which provides increased electrolyte/electrode interface, high active sites, rapid ion/electron transfer, and short diffusion distances. A manufactured symmetric solid-state supercapacitor (SSC) device also has a large capacity to operate commercial LEDs, which allows for the assessment of its practical applicability in device-level application. According to the findings of this work, suitably layered 3D SnS2 electrode materials could be a promising route for the development of environmentally friendly energy storage applications. © 2022

关键词： Supercapacitor

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Correlating the Ambient Conditions and Performance Indicators of the LoRaWAN via Surrogate Gaussian Process-Based Bidirectional LSTM Stacked Autoencoder

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IEEE Transactions on Network and Service Management 2023年第3期20卷 3413-3427页

作者： Bhat, Showkat Ahmad Huang, Nen-Fu Hussain, Imtiyaz Sajjad, Uzair National Tsing Hua University College of Electrical and Computer Science Hsinchu1300044 Taiwan National Tsing Hua University Department of Computer Science Hsinchu1300044 Taiwan National Taipei University of Technology Graduate Program in Energy and Opto-Electronic Materials Taipei10608 Taiwan National Taipei University of Technology Department of Energy and Refrigerating Airconditioning Engineering Taipei10608 Taiwan

LoRa's biggest advantage is its flexibility, which is the ability to increase or decrease data rate and range while decreasing or increasing sensitivity. Whenever propagation conditions change frequently, this function allows the spreading factor to be modified accordingly. Despite their efficiency and scalability, adaptive data rate algorithms ignore and fail to factor in the complex correlation between ambient weather parameters influencing the communication channel design. In this research, a Bayesian surrogate Gaussian process-based bidirectional LSTM stacked autoencoder model (BSGP-BLSTM-SAE) is proposed to estimate the channel performance indicators such as received signal strength indicator (RSSI) and signal-to-noise ratio (SNR) and to determine the correlation between the ambient weather conditions and performance indicators for the LoRaWAN network. Bayesian optimization algorithm has been used to optimize the hyper-parameters of the developed model. A LoRaWAN experimental multivariate time series dataset has been used for the evaluation of the developed model, which upon testing and validation produces high accuracy in predicting the channel performance indicators and ambient conditions of the experimental LoRaWAN network. The mean absolute error of the developed model was around 0.45. Thus, the proposed model can predict the link performance indicators and thereby assist in real-time optimization of the transmission parameters to enhance the network performance in LoRaWAN-based systems at different ambient conditions. © 2004-2012 IEEE.

关键词： Internet of things

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engineering of dendritic dopant-free hole transport molecules:enabling ultrahigh fill factor in perovskite solar cells with optimized dendron construction

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science China Chemistry 2021年第1期64卷 41-51页

作者： Wei Chen Yang Wang Bin Liu Yajun Gao Ziang Wu Yongqiang Shi Yumin Tang Kun Yang Yujie Zhang Weipeng Sun Xiyuan Feng Frédéric Laquai Han Young Woo Aleksandra B.Djurisic Xugang Guo Zhubing He Department of Materials Science and Engineering Southern University of Science and TechnologyShenzhen 518055China Department of Physics The University of Hong KongPokfulamHong KongChina King Abdullah University of Science and Technology KAUST Solar CenterPhysical Sciences and Engineering DivisionMaterial Science and Engineering ProgramThuwal 23955-6900Kingdom of Saudi Arabia Department of Chemistry Korea UniversitySeoul 02841South Korea

Developing dopant-free hole-transporting materials(HTMs)for high-performance perovskite solar cells(PVSCs)has been a very active research topic in recent years since HTMs play a critical role in optimizing interfacial charge carrier kinetics and in turn determining device ***,a novel dendritic engineering strategy is first utilized to design HTMs with a D-A type molecular framework,and diphenylamine and/or carbazole is selected as the building block for constructing *** HTMs show good thermal stability and excellent film morphology,and the key optoelectronic properties could be fine-tuned by varying the dendron *** them,MPA-Cz-BTI and MCz-Cz-BTI exhibit an improved interfacial contact with the perovskite active layer,and non-radiative recombination loss and charge transport loss can be effectively ***,high power conversion efficiencies(PCEs)of 20.8%and 21.35%are achieved for MPA-Cz-BTI and MCz-Cz-BTI based devices,respectively,accompanied by excellent long-term storage *** encouragingly,ultrahigh fill factors of 85.2%and 83.5%are recorded for both devices,which are among the highest values reported to *** work demonstrates the great potential of dendritic materials as a new type of dopant-free HTMs for high-performance PVSCs with excellent FF.

关键词： dendritic molecules hole-transporting materials dopant-free ultrahigh fill factor perovskite solar cells

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Sequence-Defined Nanotubes Assembled from IR780-Conjugated Peptoids for Chemophototherapy of Malignant Glioma

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Research 2021年第1期2021卷 1379-1390页

作者： Xiaoli Cai Mingming Wang Peng Mu Tengyue Jian Dong Liu Shichao Ding Yanan Luo Dan Du Yang Song Chun-Long Chen Yuehe Lin School of Mechanical and Materials Engineering Washington State UniversityPO Box 642920 PullmanWashington 99164USA Physical Sciences Division Pacific Northwest National LaboratoryRichlandWA 99352USA Department of Mechanical Engineering and Materials Science and Engineering Program State University of New YorkBinghamtonNew York 13902USA

Near-infrared(NIR)laser-induced phototherapy through NIR agents has demonstrated the great potential for cancer ***,insufficient tumor killing due to the nonuniform heat or cytotoxic singlet oxygen(1 O2)distribution over tumors from phototherapy results in tumor recurrence and inferior *** achieve high tumor killing efficacy,one of the solutions is to employ the combinational treatment of phototherapy with other modalities,especially with chemotherapeutic *** this paper,a simple and effective multimodal therapeutic system was designed via combining chemotherapy,photothermal therapy(PTT),and photodynamic therapy(PDT)to achieve the polytherapy of malignant glioma which is one of the most aggressive tumors in the ***-780(IR780)dye-labeled tube-forming peptoids(PepIR)were synthesized and self-assembled into crystalline nanotubes(PepIR nanotubes).These PepIR nanotubes showed an excellent efficacy for PDT/PTT because the IR780 photosensitizers were effectively packed and separated from each other within crystalline nanotubes by tuning IR780 density;thus,a self-quenching of these IR780 molecules was significantly ***,the efficient DOX loading achieved due to the nanotube large surface area contributed to an efficient and synergistic chemotherapy against glioma *** the unique properties of peptoids and peptoid nanotubes,we believe that the developed multimodal DOX-loaded PepIR nanotubes in this work offer great promises for future glioma therapy in clinic.

关键词： chemotherapy IR780 modal

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Squeezing out and characterization of silicon from sand by mg-thermite reduction process

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Micro and Nanosystems 2021年第1期13卷 55-60页

作者： Islam, Md. Shoriful Sattar, M.A. Halim, M.A. Hoque, Md. Asadul Quader, Abdul Ga-Fur, M.A. Hakim, M.A. Department of Materials Science and Engineering University of Rajshahi Rajshahi6205 Bangladesh Department of physics University of Toledo OH United States Bangladesh Council of Scientific and Industrial Research Dhaka1205 Bangladesh Department of Glass and Ceramic Engineering BUET Dhaka1000 Bangladesh

Background: Sand is one of the efficient sources of Silicon. We get quite easily the plethora of sand from the river side, Bangladesh. Utilization of the superfluous sand can be assisted to enhance our economy. Methods: In this work, silicon is extracted from sand by metal–thermite reduction process and the sample of sand is collected from padma river Rajshahi, Bangladesh. The process is environmentally benign and low cost. The reduction of the sand was performed with Mg powder, and purification was done by leaching out with HCl and HF. We have studied the structural properties, chemical nature and physical morphology. Results and conclusion: X-ray Diffraction (XRD) confirmed that the presence of elemental Si in the samples produced by Mg-thermite reduction process and the particle size was found 25.72±1.3 nm in an average. Surface morphology has been studied using Scanning Electron Microscopy (SEM) and the particle size seemed around 30 to 40 nm which was comparable to the obtained particle size from XRD. Fourier transform infrared spectroscopy (FTIR) showed the presence of Si-Si bonding in the investigating materials. The chemical nature of the sand has been studied by X-ray Fluorescence (XRF) analysis. Silicon content of sand was found about maximum 80%. © 2021 Bentham science Publishers.

关键词： Structural properties

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Specular Inverse Faraday Effect in Transition Metals

arXiv

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arXiv 2023年

作者： Ortiz, Victor H. Mishra, Shashi B. Vuong, Luat Coh, Sinisa Wilson, Richard B. Department of Mechanical Engineering and Materials Science and Engineering Program University of California RiversideCA92521 United States

The inverse Faraday effect is an opto-magnetic phenomenon that describes the ability of circularly polarized light to induce magnetism in solids. The capability of light to control magnetic order in solid state materials and devices is of interest for a variety of applications, such as magnetic recording, quantum computation and spintronic technologies. However, significant gaps in understanding about the effect persist, such as what material properties govern the magnitude of the effect in metals. In this work, we report time-resolved measurements of the specular inverse Faraday effect in non-magnetic metals, i.e., the magneto-optic Kerr effect induced by circularly polarized light. We measure this specular inverse Faraday effect in Cu, Pd, Pt, W, Ta, and Au at a laser wavelength of 783 nm. For Ta and W, we investigate both α and β phases. We observe that excitation of these metals with circularly polarized light induces significant circular dichroism. This nonlinear magneto-optical response to circularly polarized light is an order of magnitude larger in α-W than other metals, e.g., Pt, Au, and is greater than nearly all other reported values for the inverse Faraday effect in other materials. Our results benchmark the range of the inverse Faraday effect that can be observed in non-magnetic metals and provide insight into what material properties govern the inverse Faraday effect in metals. © 2023, CC BY.

关键词： Light polarization

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Effect of exposure to a light-emitting diode (LED) on the physicochemical characteristics of natural latex biomembranes used to treat diabetic ulcers

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Research on Biomedical engineering 2022年第3期38卷 901-911页

作者： Santana, Thamis Fernandes Oliveira, Rebeca Hannah de Melo dos Santos, Ludmila Evangelista Lima, Eunice Paloma Nascimento Faria, Sylvia de Sousa Fonseca, Marcos Augusto Moutinho da Silva, Jaqueline Rodrigues Tatmatsu-Rocha, José Carlos Gomes, Marília Miranda Forte Fleury Rosa, Mário Fabrício Fleury Rosa, Suélia de Siqueira Rodrigues Carneiro, Marcella Lemos Brettas Postgraduate Program in Biomedical Engineering University of Brasilia Federal District Brasilia Brazil Postgraduate Program in Materials Science and Engineering Federal University of Campina Grande Paraiba Campina Grande Brazil Department of Electrical Engineering University of Brasilia Federal District Brasilia Brazil Postgraduate Program in Biology Animal University of Brasilia Federal District Brasilia Brazil Medicine Faculty Physical Therapy Department Federal University of Ceara Ceara Fortaleza Brazil Postgraduate Technology and Health Program University of Brasília Federal District Brasília Brazil

Purpose: Natural latex biomembrane has shown high therapeutic potential for the treatment of diabetic ulcers when associated with phototherapy. In this study, physical and chemical alterations in the latex biomembranes were evaluated after exposure to light-emitting diode (LED) irradiation and after contact with NaCl solution. Methods: There were three experimental groups: natural latex biomembranes (1) in natura;(2) after 35 min of LED light irradiation;and (3) after immersion in NaCl 0.9 g% solution. The samples were analyzed by tensile strength test, thermogravimetry, contact angle wettability, and Fourier-transform infrared spectroscopy. Results: The biomembranes that were submitted to contact with NaCl aqueous solution or exposure to LED did not undergo impairment of mechanical resistance. The thermogravimetry analysis indicated that increasing temperature led to mass loss in all samples, referring to their decomposition temperatures. In the wettability test, biomembranes exposed to LED showed a significant reduction in the contact angle between 0 and 10 min, indicating an increase in hydrophilicity, suggesting water storage capacity. The Fourier-transform infrared spectrometry assay showed that there was a more significant reduction in vibration intensity after immersion in NaCl solution compared to untreated biomembranes. An increase in the intensity of the entire spectrum of biomembranes exposed to LED was observed in comparison with the other samples, which may be related to photodegradation caused by LED light irradiation. Conclusion: The biomembranes underwent significant changes in its chemical structure after being subjected to different types of exposure and maintained its elasticity and tensile strength properties, in addition to showing good water retention capacity after exposure to LED. Thus, it maintains many of its properties for application as a tissue-regenerating biomaterial, even when subjected to LED irradiation and a humid environment. © 20

关键词： Tissue regeneration

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Correction to: Emergence of melt and glass states of halide perovskite semiconductors (Nature Reviews materials, (2025), 10.1038/s41578-024-00759-x)

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Nature Reviews materials 2025年

作者： Singh, Akash Mitzi, David B. Department of Mechanical Engineering and Materials Science Duke University DurhamNC United States University Program in Materials Science and Engineering Duke University DurhamNC United States Department of Chemistry Duke University DurhamNC United States

Correction to: Nature Reviews materialshttps://***/10.1038/s41578-024-00759-x, published online 9 January 2025 In the version of the article initially published, the Acknowledgements section was missing and has now been added to read "This work is supported by the National science Foundation under grant no. DMR-2114117" in the HTML and PDF versions of the article. © Springer Nature Limited 2025.

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Cascaded multiparameter quantum metrology

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Physical Review A 2025年第1期111卷 012618-012618页

作者： Gregory Krueper Lior Cohen Juliet T. Gopinath Department of Physics University of Colorado Boulder Boulder Colorado 80309 USA Department of Electrical Computer and Energy Engineering University of Colorado Boulder Boulder Colorado 80309 USA Materials Science and Engineering Program University of Colorado Boulder Boulder Colorado 80309 USA

We present an innovative, platform-independent concept for multiparameter sensing where the measurable parameters are in series, or cascaded, enabling measurements as a function of position. With temporally resolved detection, we show that squeezing can give a quantum enhancement in sensitivity over that of classical states by a factor of e2r, where r≈1 is the squeezing parameter. As an example, we have modeled an interferometer that senses multiple phase shifts along the same path, demonstrating a maximal quantum advantage by combining a coherent state with squeezed vacuum. Further classical modeling with up to 100 phases shows linear scaling potential for adding nodes to the sensor. The approach can be applied to remote sensing, geophysical surveying, and infrastructure monitoring.

关键词： Interferometers

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