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Z-Laminating Assembly of Graphene Nanoflakes for Super-Strong Membranes and Functional Coatings

ACS Applied Nano materials 2024年第13期7卷 14957-14963页

作者： Santos, Ian Daniell Tjarks, Patrick Muthu, Jeyavelan Lin, You-Chen Yen, Zhi-Long Chand, Pradyumna Kumar Raman, Radha Nguyen, Dinh Tuan Rouhani, Mehdi Jeng, Yeau-Ren Hsieh, Ya-Ping Hofmann, Mario Department of Physics National Taiwan University Taipei 106 Taiwan Nano Science and Technology Program Taiwan International Graduate Program Academia Sinica and National Taiwan University Taipei 106 Taiwan J. Heyrovsky Institute of Physical Chemistry of the Czech Academy of Sciences Prague 18200 Czech Republic Institute of Atomic and Molecular Sciences Academia Sinica Taipei 106 Taiwan Department of Chemistry National Taiwan University Taipei 106 Taiwan Department of Physics National Central University Taoyuan 320 Taiwan Molecular Science and Technology Program Taiwan International Graduate Program Academia Sinica and National Central University Taipei 106 Taiwan Department of Biomedical Engineering National Cheng Kung University 1 University Road Tainan 70101 Taiwan Department of Materials Science and Engineering National Cheng Kung University Tainan 70101 Taiwan Academy of Innovative Semiconductor and Sustainable Manufacturing National Cheng-Kung University (NCKU) Tainan 70101 Taiwan

We demonstrate the strengthening of graphene, an atomically thin carbon allotrope, by out-of-plane folding. Through lateral confinement of graphene at the water-air interface, nanoscale buckling was induced in suspended flakes, leading to an unexpected folding transition beyond a critical surface pressure. The emergence of folding was confirmed by in situ Brewster angle reflectivity and ex situ microscopy, showing a unique “z-laminated” nanostructure. Molecular dynamics simulations indicate that z-lamination yields an enhanced adhesion between neighboring flakes compared to lateral sliding, which was confirmed by a surface pressure hysteresis during the folding process. Mechanical testing reveals superior Young’s modulus and yield strength when compared to conventional graphene assemblies and even compared to composites. We demonstrate the potential of the z-lamination approach for applications in graphene-based structural materials, tribological layers, and functional electrochemical coatings. Finally, the complete recyclability of z-laminated graphene opens up new routes toward sustainable nanostructured materials. © 2024 The Authors. Published by American Chemical Society

关键词： 2D materials composites laminated graphene membranes recyclable

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Effect of Parasitic Leakage Currents Associated with the Regrown Aperture of AlGaN/GaN Current Aperture Vertical Electron Transistors (CAVETs)

Effect of Parasitic Leakage Currents Associated with the Reg...

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IEEE Electron Devices Technology and Manufacturing Conference (EDTM)

作者： Sara Pouladi Jae Hyun Ryou Department of Mechanical Engineering Texas Center for Superconductivity at UH Advanced Manufacturing Institute University of Houston USA Department of Electrical and Computer Engineering Materials Science and Engineering Program University of Houston USA

We present a numerical simulation on the effect of leakage paths in the regrown GaN layer in the aperture and above the current blocking layer (CBL) of current aperture vertical electron transistor (CAVET) devices. Here, a 2D TCAD modeling is employed to simulate a CAVET device structure considering two main origins of parasitic leakage current from CBL/regrown-GaN interface and gate/regrown-GaN bulk and their degree of detrimental effect on the characteristics of AlGaN/GaN CAVETs.

关键词： Performance evaluation Apertures Logic gates Numerical simulation Wide band gap semiconductors Numerical models Leakage currents

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Moderate-Refractive-Index Mie Resonators for Versatile Modulation of Two-Dimensional Excitons

Moderate-Refractive-Index Mie Resonators for Versatile Modul...

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Conference on Lasers and Electro-Optics (CLEO)

作者： Jie Fang Yuebing Zheng Materials Science & Engineering Program and Texas Materials Institute The University of Texas at Austin Austin TX USA Walker Department of Mechanical Engineering The University of Texas at Austin Austin TX USA

By coupling well-designed moderate-refractive-index Mie resonators to monolayer semiconductors, we have demonstrated efficient modulation of two-dimensional excitons in multiple dimensions: far-field excitonic radiati... 详细信息

ISBN: (纸本)9781957171258

关键词： Excitons Mie resonances Mie theory Optical resonators Refractive index Semiconductors

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Optothermal multimodal manipulation of micro/nanoparticles

Optothermal multimodal manipulation of micro/nanoparticles

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Conference on Lasers and Electro-Optics (CLEO)

作者： Hongru Ding Pavana Siddhartha Kollipara Kan Yao Yuebing Zheng Walker Department of Mechanical Engineering The University of Texas at Austin Austin TX USA Materials Science & Engineering Program and Texas Materials Institute The University of Texas at Austin Austin TX USA

We report a new optical platform to achieve on-demand multimodal manipulation of micro/nanoparticles by a synergy of optical and thermal forces.

ISBN: (纸本)9781957171258

We report a new optical platform to achieve on-demand multimodal manipulation of micro/nanoparticles by a synergy of optical and thermal forces.

关键词： Laser beams Nanoparticles Optical force Optical manipulation Optical tweezers Spatial resolution

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Carbon nitride- and graphene-based materials for the photocatalytic degradation of emerging water pollutants

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materials Advances 2024年第7期5卷 2668-2688页

作者： Indra Jaya Budiarso Valentinus Alphano Dabur Riska Rachmantyo Hermawan Judawisastra Chechia Hu Arie Wibowo Master Program in Materials Science and Engineering Faculty of Mechanical and Aerospace Engineering Institut Teknologi Bandung Ganesha 10 Bandung 40132 West Java Indonesia Doctoral Program in Materials Science and Engineering Faculty of Mechanical and Aerospace Engineering Institut Teknologi Bandung Ganesha 10 Bandung 40132 West Java Indonesia Materials Science and Engineering Faculty of Mechanical and Aerospace Engineering Institut Teknologi Bandung Ganesha 10 Bandung 40132 West Java Indonesia ariewibowo@itb.ac.id Department of Chemical Engineering National Taiwan University of Science and Technology Taipei 106 Taiwan R&D Center for Membrane Technology Chung Yuan Christian University Taoyuan 320 Taiwan Research Center for Nanoscience and Nanotechnology Institut Teknolgi Bandung Ganesha 10 Bandung 40132 West Java Indonesia

Photocatalytic degradation is a promising way to treat emerging pollutants in wastewater. Recently, metal-free photocatalysts such as carbon nitride- and graphene-based materials have attracted much interest in the photocatalytic degradation of emerging water pollutants owing to their visible light activity and unique electrical properties, respectively. Graphitic carbon nitride (GCN) is considered a superior visible light–active photocatalyst because of its suitable bandgap (2.7 eV). Moreover, the facile synthesis process and the high chemical and thermal stability of GCN make it one of the research hotspots in photocatalytic wastewater treatment. Besides GCN, graphene and its derivatives are utilized to support main photocatalysts by enhancing their light absorption, pollutant adsorption, and photogenerated charge separation. Furthermore, the vast modification of these materials has promoted various outstanding performances in carbon nitride- and graphene-based photocatalysts in the application of pollutant degradation. In this review, we highlight recent developments in carbon nitride- and graphene-based photocatalysts (2018–2023), focusing on the strategies to improve the activity of GCN as a visible light–active photocatalyst and the role of graphene and its derivatives as supporting materials in wastewater pollutant remediation applications.

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Surface Characterization of Sodium Cholate Treated CVD Graphene

Surface Characterization of Sodium Cholate Treated CVD Graph...

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IEEE Conference on Nanotechnology

作者： Evans Addo-Mensah Janet Obaemo Katie Welch Yang Tian Shiva Dolatabadi Hugh Churchill Uchechukwu Wejinya Materials Science and Engineering Graduate Program University of Arkansas Microelectronics and Photonics Program University of Arkansas Department of Physics University of Arkansas Fayetteville Arkansas Department of Mechanical Engineering University of Arkansas Fayetteville Arkansas

The advancement of graphene has created a need in exploring its properties for different applications. One way to explore its properties is by reducing its hydrophobicity. To overcome hydrophobicity of graphene, surfactants have been used in functionalization, hence improving the surface properties of the graphene monolayer. Therefore, investigating surfactant treatment for CVD graphene becomes useful in understanding the surface property effects on graphene. This study utilizes CVD graphene on silicon substrates. Its treatment was done with varying concentrations of Sodium Cholate (SC) for different treatment times. These samples were then characterized using Atomic Force Microscopy (AFM) to investigate the surface properties of the samples before and after treatment. To be optimized, the graphene must remain attached to the silicon substrate. The result shows that the integrity of the graphene, which is basically the Sp2 structure, is preserved as there was no delamination from the substrate even after treatment for as long as 2 hours in 1% weight/volume concentration of the SC solution.

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An ultra thin,bright,and sensitive interactive tactile display based on organic mechanoluminescence for dual-mode handwriting identification

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InfoMat 2024年第6期6卷 76-87页

作者： Tingting Hou Wenlang Li Haoyu Wang Yuantian Zheng Chaojie Chen Haoran Zhang Kai Chen Huilin Xie Xin Li Shaoshuai He Siwei Zhang Dengfeng Peng Cheng Yang Jacky W.Y.Lam Ben Zhong Tang Yunlong Zi Department of Mechanical and Automation Engineering The Chinese University of Hong KongHong Kongthe People's Republic of China Department of Chemistry Hong Kong Branch of Chinese National Engineering Research Center for Tissue Restoration and Reconstruction and Institute for Advanced StudyThe Hong Kong University of Science and TechnologyHong Kongthe People's Republic of China Key Laboratory of Optoelectronic Devices and Systems of Ministry of Education and Guangdong Province College of Physics and Optoelectronic EngineeringShenzhen UniversityShenzhenthe People's Republic of China Thrust of Sustainable Energy and Environment The Hong Kong University of Science and Technology(Guangzhou)Guangzhouthe People's Republic of China The Hong Kong University of Science and Technology Interdisciplinary Program Office Hong Kong SARthe People's Republic of China Institute of Materials Research Tsinghua Shenzhen International Graduate SchoolTsinghua UniversityShenzhenthe People's Republic of China School of Science and Engineering Shenzhen Institute of Aggregate Science and TechnologyThe Chinese University of Hong KongShenzhenthe People's Republic of China HKUST Shenzhen-Hong Kong Collaborative Innovation Research Institute Shenzhenthe People's Republic of China Guangzhou HKUST Fok Ying Tung Research Institute Guangzhouthe People's Republic of China

Visible light-based human–machine interactive media is capable of transmitting electrical readouts to machines and providing intuitive feedback to users ***,many inorganic mechanoluminescent(ML)materials-based interactive media,typically ZnS-loaded phosphors(ZLPs),have been successfully ***,organic ML materials-based solutions were rarely exploited despite their huge merits of strong structural modification,abundant luminescence property,low cost,easy preparation,and so ***,we propose a novel interactive tactile display(ITD)based on organic ML materials(Cz-A6-dye)and triboelectric nanogenerator,with ultra-brightness(130%enhancement)and ultra-low threshold pressure(57%reduction)as compared to *** proposed ITD achieves the conversion of weak mechanical stimuli into visible light and electrical signals simultaneously,without extra power ***,the relationship between the luminous performance of organic ML materials and mechanical force is quantified,benefiting from the uniform ML layer *** by convolutional neural networks,the high-accuracy recognition(97.1%)for handwriting and identity of users is realized at the same ***,the ITD has great potential for intelligent wearable electronics and classified military applications.

关键词： interactive media organic mechanoluminescence triboelectric nanogenerators

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Optothermal Manipulation at Fluid Interfaces

Optothermal Manipulation at Fluid Interfaces

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Conference on Lasers and Electro-Optics (CLEO)

作者： Youngsun Kim Carolina Ponce Zhihan Chen Yuebing Zheng Materials Science & Engineering Program Texas Materials Institute The University of Texas at Austin Austin TX USA Walker Department of Mechanical Engineering The University of Texas at Austin Austin TX USA

Optothermal manipulation of particles at fluid interfaces was studied with a film of gold nanoparticles assembled at aqueous/oil interfaces. The unique optothermal behaviors of particles and fluid interfaces under opt... 详细信息

ISBN: (纸本)9781957171258

关键词： Gold Laser beams Laser irradiation Light scattering Optical force Optical tweezers

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Vortex Formation of Active Particles within a Confined Geometry by Velocity Alignment

Vortex Formation of Active Particles within a Confined Geome...

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Conference on Lasers and Electro-Optics (CLEO)

作者： Zhihan Chen Hongru Ding Yuebing Zheng Materials Science & Engineering Program and Texas Materials Institute The University of Texas at Austin Austin TX USA Walker Department of Mechanical Engineering The University of Texas at Austin Austin TX USA

we have developed an optical feedback control system with synchronous control of active particles to study collective motion in nature. Fish-like vortex is observed within a circular confined geometry based on the par... 详细信息

ISBN: (纸本)9781957171258

关键词： Coherence Light fields Optical feedback Polarization Rubidium Spatial light modulators

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Quantifying Electrochemical Processes in Batteries and Beyond

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Energy & Environmental materials 2022年第4期5卷 1001-1004页

作者： Emma N.Antonio Michael F.Toney Materials Science and Engineering Program University of Colorado BoulderBoulderColorado 80309USA Joint Center for Energy Storage Research(JCESR) University of Colorado BoulderBoulderColorado 80309USA Department of Chemical and Biological Engineering University of Colorado BoulderBoulderColorado 80309USA Renewable and Sustainable Energy Institute University of Colorado BoulderBoulderColorado 80309USA

The correlation of electrochemical measurements with materials characterization has advanced our understanding of operation and degradation mechanisms in electrochemical energy storage and many other ***,often these correlations are qualitative,preventing the unambiguous identification of both operational principles and the root causes of performance *** we suggest quantitative approaches to define competing mechanisms and determine their relative *** illustrate the importance of quantitative methodologies over a range of electrochemical systems and highlight the need to consider the effect of the experimental design and measurement *** approaches will reveal the most detrimental degradation mechanisms and enable the development of strategies to suppress,stabilize or eliminate them,leading to materials and devices with longer lifetimes,reduced environmental impact,and improved performance.

关键词： electrochemistry in situ and operando characterization batteries quantification materials science

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