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Autonomous Electron Tomography Reconstruction Using Bayesian Optimization

Microscopy and microanalysis : the official journal of Microscopy Society of America, Microbeam Analysis Society, Microscopical Society of Canada 2023年第1期29卷 1915-1916页

作者： Millsaps, William Schwartz, Jonathan Di, Zichao Wendy Jiang, Yi Hovden, Robert Department of Nuclear Engineering Radiological Sciences University of Michigan Ann Arbor MI United States Department of Materials Science and Engineering University of Michigan Ann Arbor MI United States Mathematics and Computer Science Division Argonne National Laboratory Lemont IL United States Advanced Photon Source Facility Argonne National Laboratory Lemont IL United States Applied Physics Program University of Michigan Ann Arbor MI United States

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Nucleation effects of coccoliths in portland cement

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Matter 2025年

作者： Beatty, Danielle N. Srubar, Wil V. Materials Science and Engineering Program University of Colorado Boulder 4001 Discovery Drive UCB 027 BoulderCO80303 United States Department of Civil Environmental and Architectural Engineering University of Colorado Boulder 1111 Engineering Drive ECOT 441 UCB 428 BoulderCO80309 United States

This work explores the use of photosynthesized coccoliths (intricate CaCO3 particles) as a nucleation agent or cement replacement in portland cement paste. First, coccoliths were produced and harvested from the marine microalgae Emiliania huxleyi and the particle size, morphology, and mineralogy were characterized. Then, the nucleation effects of E. huxleyi coccoliths as seeding agent (0.5, 1, 3, or 5 wt % additions) and limestone filler (5 and 15 wt % cement replacements) were studied using isothermal conduction calorimetry and compressive strength testing. The results were compared with five commercially available CaCO3 sources used as nucleation agents and fillers. While the high surface area of coccoliths (12.22 m2/g) enhanced water demand, it also enhanced nucleation during cement hydration without accelerating hydration, leading to enhanced early-age strength without detriments to 28-day strength. Results highlight a potential carbon reduction strategy, namely employing photosynthesis as a method of mineral admixture production, for the cement and concrete industry. © 2025 Elsevier Inc.

关键词： Portland cement

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Optoelectric Raman Nanosensors: Overcoming Intrinsic Limit in Nano-biosensing

Research Square

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Research Square 2024年

作者： Lian, Bin Li, Huaizhi Guo, Jianhe Fan, Donglei Emma Materials Science and Engineering Program Texas Materials Institute The University of Texas AustinTX78712 United States Walker Department of Mechanical Engineering Texas Materials Institute The University of Texas at Austin AustinTX78712 United States Chandra Family Department of Electrical and Computer Engineering The University of Texas at Austin AustinTX78712 United States

It is intrinsically difficult to detect low-concentration biomolecules with both ultra-sensitivity and high speed for early-stage disease diagnosis. The challenge originates from the small size of nanosensors, which enables ultra-sensitivity biosensing, while also substantially increases the detection time of dilute molecules. in this work, we report an original optoelectric sensing scheme, along with an innovative device design and a strategic fabrication approach to overcome such a challenge in biosensing. The proposed scheme exploits the profound optoelectric effect of semiconductor silicon nanowires, which can readily enrich trace-amounts of biomolecules at the point of laser and simultaneously detect Raman signals of focused molecules. The device design includes large arrays of silicon nanorods with electrodes integrated at their roots, and surface-distributed dense plasmonic silver nanoparticles for surface-enhanced Raman spectroscopy (SERS) detection. Operating at only -0.8 V in an electrochemical cell, these optoelectric nanosensors readily achieve a 150-fold signal enhancement, improving the detection limit of probing molecules, adenine, by five orders of magnitude, to 0.6 fM. The enhancement effect is robust, observed across concentrations from 1 μM to 1 fM. The working mechanism is general, not only for detecting small molecules, such as adenine, but also for large charged molecules, such as Vertebrate DNA. The underlying novel mechanism is unraveled by multiscale numerical simulations and calculations. This research, addressing an arduous bottleneck issues in nanobiosensing, is expected to inspire a new class of biochemical sensors, important for the practical detection of trace-amount biochemicals in solution, important for clinic relevant early-stage disease diagnostics. © 2024, CC BY.

关键词： Nanorods

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A Comprehensive Review on plant and animal fiber reinforced composites: Experimental and theoretical approaches to interfacial strength optimization and potential applications

Hybrid Advances

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Hybrid Advances 2025年 10卷

作者： Olanrewaju, Olajesu Oladele, Isiaka Oluwole Adelani, Samson Oluwagbenga Department of Materials Science and Engineering Iowa State University Ames IA United States Department of Metallurgical and Materials Engineering Federal University of Technology PMB Akure 704 Nigeria Centre for Nanomechanics and Tribocorrosion School of Metallurgy Chemical and Mining Engineering University of Johannesburg Johannesburg South Africa Materials Science and Engineering Program University of Colorado Boulder 80303 CO United States

Natural fiber-reinforced composites (NFRCs) have become vital in various engineering applications due to their exceptional properties and ease of manufacturing. Properties such as lightweight, sustainability, design flexibility, microstructure, durability, and advanced fabrication techniques have expanded their use across industries. Also, NFRCs are preferred because the extensive reliance on synthetic fibers presents significant challenges in recycling and waste management. Despite their excellent properties, NFRCs have three main challenges: fiber degradation, water degradation, and weak interfacial strength (incompatibility of fibers with the matrix). Consequently, research efforts have been directed at combating these challenges using different surface treatment techniques. However, research has been skewed towards experimental approaches for improving the interfacial strength in plant fiber polymer matrix composites (PMCs). Hence, there exists a dearth of information on the computational approaches for optimizing the interfacial properties of NFRCs. Hence, this review provides experimental and computational approaches (machine learning) for comprehensive optimizing strategies for different natural fibers (plant, animal, and microorganism) and matrices (polymers, metals, and ceramics). This review also highlights the importance of theoretical approaches and numerical modeling in analyzing and optimizing NFRCs. Finally, the review highlights recent advancements in NFRCs, their mechanical properties, potential applications, and future directions. © 2025 The Authors

关键词： Animal fiber Interfacial shear strength Machine-learning Natural fiber-reinforced composites Plant fiber

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Piezoelectricity of strain-induced overall water splitting of Ni(OH)2/MoS2 heterostructure

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Journal of materials Chemistry A 2023年第7期11卷 3481-3492页

作者： Le, Kim Tuyen Pham, Nguyet N. T. Liao, Yin-Song Ranjan, Ashok Lin, Hsun-Yen Chen, Po-Han Nguyen, Hoang Lu, Ming Yen Lee, Seung Geol Wu, Jyh Ming Department of Materials Science and Engineering National Tsing Hua University 101 Section 2 Kuang Fu Road Hsinchu300 Taiwan Department of Chemistry University of Science Vietnam National University Ho Chi Minh City Viet Nam School of Chemical Engineering Pusan National University 2 Busandaehak-ro 63 beon-gil Geumjeong-gu Busan46241 Korea Republic of Department of Organic Material Science and Engineering Pusan National University 2 Busandaehak-ro 63 beon-gil Geumjeong-gu Busan46241 Korea Republic of PhD Program in Prospective Functional Materials Industry National Tsing Hua University 101 Section 2 Kuang Fu Road Hsinchu300 Taiwan High Entropy Materials Center National Tsing Hua University 101 Section 2 Kuang Fu Road Hsinchu300 Taiwan Vietnam National University Ho Chi Minh City Linh Trung Ward Thu Duc City Ho Chi Minh City700000 Viet Nam

In this study, we synthesized several active sites of molybdenum disulfide (MoS2) nanoflowers (NFs) decorated with Ni(OH)2 nanoparticles (NPs) to form heterostructures. Our results revealed that Ni(OH)2/MoS2 NF heterostructures caused the splitting of water into hydrogen (H2) and oxygen (O2) gas. The Ni(OH)2/MoS2 NF interface exhibited strain-induced piezoelectric potential (piezopotential) that promoted charge separation, reducing the kinetic barrier in the water splitting process and promoting the hydrogen evolution reaction (HER) and the oxygen evolution reaction (OER). In high-resolution transmission microscopy images, the measured lattice fringe d spacing was approximately 0.67 nm, which was higher than the reported value. The calculated tensile strain of Ni(OH)2/MoS2 NF heterostructures was approximately 3.5%. The findings based on density-functional theory and using the finite element method indicated that the interfacial piezopotential generated between Ni(OH)2 and MoS2 NFs enhanced charge transfer and electrochemical reactions. To obtain a current density up to 10 mA cm−2, we set the overpotential and Tafel slope of Ni(OH)2/MoS2 NF heterostructures at 155 mV and 62.1 mV dec−1 for the HER and 328 mV and 69.3 mV dec−1 for the OER, respectively. Moreover, a high Faraday efficiency (84.1%) was observed over 48 h, with no significant decline in the HER and OER. © 2023 The Royal Society of Chemistry.

关键词： Molybdenum disulfide

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Understanding ADC variation by fat content effect using a dual-function MRI phantom

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European Radiology Experimental 2024年第1期8卷 19页

作者： Liu, Yi-Jui Tsai, Tung-Sheng Li, Ya-Hui Peng, Jo-Hua Chang, Hing-Chiu Peng, Hsu-Hsia Lee, Ying-Chieh Lee, Tung-Yang Liou, Chang-Hsien Lin, Tz-Feng Chew, Fatt-Yang Chou, Ruey-Hwang Juan, Chun-Jung Department of Automatic Control Engineering Feng Chia University Taichung Taiwan Ph.D. Program in Electrical and Communication Engineering Feng Chia University Taichung Taiwan Department of Medical Imaging China Medical University Hsinchu Hospital 199 Sec. 1 Xinglong Rd. Hsinchu County Zhubei City 302 Taiwan Department of Biomedical Engineering and Environmental Sciences National Tsing Hua University Hsinchu Taiwan Department of Biomedical Engineering Chinese University of Hong Kong Hong Kong Master’s Program of Biomedical Informatics and Biomedical Engineering Feng Chia University Taichung Taiwan Cheng Ching Hospital Taichung Taiwan Institute of Nuclear Engineering and Science National Tsing Hua University Hsinchu Taiwan Department of Fiber and Composite Materials Feng Chia University Taichung Taiwan Department of Medical Imaging China Medical University Hospital Taichung Taiwan Department of Radiology School of Medicine China Medical University Taichung Taiwan Graduate Institute of Biomedical Sciences China Medical University Taichung 406 Taiwan Center for Molecular Medicine China Medical University Hospital Taichung Taiwan Department of Medical Laboratory and Biotechnology Asia University Taichung Taiwan

Background: A dual-function phantom designed to quantify the apparent diffusion coefficient (ADC) in different fat contents (FCs) and glass bead densities (GBDs) to simulate the human tissues has not been documented yet. We propose a dual-function phantom to quantify the FC and to measure the ADC at different FCs and different GBDs. Methods: A fat-containing diffusion phantom comprised by 30 glass-bead-containing fat-water emulsions consisting of six different FCs (0, 10, 20, 30, 40, and 50%) multiplied by five different GBDs (0, 0.1, 0.25, 0.5, and 1.0 g/50 mL). The FC and ADC were measured by the “iterative decomposition of water and fat with echo asymmetry and least squares estimation-IQ,” IDEAL-IQ, and single-shot echo-planar diffusion-weighted imaging, SS-EP-DWI, sequences, respectively. Linear regression analysis was used to evaluate the relationship among the fat fraction (FF) measured by IDEAL-IQ, GBD, and ADC. Results: The ADC was significantly, negatively, and linearly associated with the FF (the linear slope ranged from -0.005 to -0.017, R² = 0.925 to 0.986, all p < 0.001). The slope of the linear relationship between the ADC and the FF, however, varied among different GBDs (the higher the GBD, the lower the slope). ADCs among emulsions across different GBDs and FFs were overlapped. Emulsions with low GBDs plus high FFs shared a same lower ADC range with those with median or high GBDs plus median or lower FFs. Conclusions: A novel dual-function phantom simulating the human tissues allowed to quantify the influence of FC and GBD on ADC. Relevance statement: The study developed an innovative dual-function MRI phantom to explore the impact of FC on ADC variation that can affect clinical results. The results revealed the superimposed effect on FF and GBD density on ADC measurements. Key points: • A dual-function phantom made of glass bead density (GBD) and fat fraction (FF) emulsion has been developed. • Apparent diffusion coefficient (ADC) values

关键词： Adipose tissue Diffusion magnetic resonance imaging Phantoms (imaging) Quality assurance (healthcare) Quality control

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Recent advances in natural fiber reinforced metal/ceramic/polymer composites: An overview of the structure-property relationship for engineering applications

Hybrid Advances

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Hybrid Advances 2025年 8卷

Advances in the material science world drive the birth of a new generation of sustainable materials. Natural fiber (NFs) biocomposites are emerging as valuable alternatives to conventional materials for engineering applications such as construction, automobiles, and aerospace due to their exceptional mechanical properties, lightweight, low carbon footprint, energy efficiency, and cost-effectiveness. These outstanding properties have made them more desirable for engineering applications. However, the focus has been on lignocellulosic fibers, neglecting other sources, such as keratinous, fibrinous, and microorganism fibers. Only a few reviews have considered the structure-property relationship of all classes of natural fibers, such as lignocellulosic (plant), keratinous and fibrinous (animal), and microorganism (mycelium) fibers. Although NFs have outstanding potential from an economic, technical, environmental, and green credentials perspective, they have limitations, such as fiber-matrix incompatibility and moisture damage. These limitations make using NFs as reinforcement for different material systems challenging. Surface alterations are usually necessary to improve the adherence between fiber and matrix. With the upgrade, NFs have the potential as sustainable replacement for conventional materials for engineering applications. Future research should aim at reconciling the mechanical properties of NFs to improve composite quality and fiber-matrix adherence and performance. © 2025 The Authors

关键词： Biocomposites Fibrinous Keratinous Lignocellulosic Microorganism Natural fiber

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Micro-Helical Ni3fe Chain Encapsulated in Ultralight Mxene/C Aerogel to Realize Multi-Functionality: Radar Stealth, Thermal Insulation, Fire Resistance, and Mechanical Properties

SSRN

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SSRN 2024年

作者： Lin, Sen Lin, Jing Xiong, Zhiqiang He, Xue Li, Xin Liu, Chongbo Wang, Chengying Zeng, Xiaojun Nie, Xuliang Che, Renchao Key Laboratory of Jiangxi Province for Persistent Pollutants Control and Resources Recycle School of Environmental and Chemical Engineering Nanchang Hangkong University Nanchang330063 China School of Materials Science and Engineering Nanchang Hangkong University Nanchang330063 China School of Materials Science and Engineering Jingdezhen Ceramic University Jingdezhen333403 China College of Chemistry and Materials Jiangxi Agricultural University Nanchang330045 China Laboratory of Advanced Materials Department of Materials Science Collaborative Innovation Center of Chemistry for Energy Materials and Collaborative Innovation Center of Chemistry for Energy Materials Fudan University Shanghai200438 China

Owing to their high porosity, ultralow density, and excellent impedance matching, magnetic carbon aerogels are considered to be a promising microwave absorption (MA) material. However, the inevitable agglomeration of traditional magnetic microspheres in carbon materials makes it difficult to realize perfect electromagnetic synergy. In this study, Ni3Fe alloy particles are first assembled into a micro-helical Ni3Fe chain under ethylene glycol polymerization, which are further wrapped by MXene. Then, carbonyl-amine condensation reaction is used for the in-situ growth of poly-Schiff-base aerogels on the independent caterpillar-like Ni3Fe/MXene. Finally, ultralight TiO2/Ni3Fe/MXene/C (NFMC) aerogels are synthesized through calcination treatment. Benefiting from the electromagnetic synergistic effect of multi-dimensional and multi-component materials, the NFMC-7 aerogel exhibits excellent MA performance with a minimum reflection loss of -61.6 dB at 3.0-mm thickness and an effective absorption bandwidth of 8.16 GHz at 2.77-mm thickness under a low filler loading of 7.6 wt.%. Commercial computer simulation technology is used to verify the strong magnetic and dielectric loss characteristics of Ni3Fe chains. Meanwhile, the radar cross-section (RCS) simulation of NFMC-7 aerogels reveals their excellent radar stealth performance with a maximum RCS reduction value of 20.1 dB·m2 at 0° as well as thermal insulation property with a thermal conductivity of 0.046 W/m·K. Notably, the NFMC-7 aerogel is fire-resistant and can withstand nearly 750 times its own weight without damage, which verifies its practical applicability. Overall, this work establishes an effective strategy to fabricate multi-functional magnetic aerogels, which can serve as lightweight, thin, and strong microwave absorbers with broad absorption bandwidth. © 2024, The Authors. All rights reserved.

关键词： Aerogels

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Review Integration of smartphone technology and artificial intelligence for advanced ophthalmic care:A systematic review

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Advances in Ophthalmology Practice and Research 2024年第3期4卷 120-127页

作者： Kai Jin Yingyu Li Hongkang Wu Yih Chung Tham Victor Koh Yitian Zhao Ryo Kawasaki Andrzej Grzybowski Juan Ye Eye Center The Second Affiliated Hospital of Zhejiang University School of MedicineZhejiang Provincial Key Laboratory of OphthalmologyZhejiang Provincial Clinical Research Center for Eye DiseasesZhejiang Provincial Engineering Institute on Eye DiseasesHangzhouChina Centre for Innovation and Precision Eye Health National University of SingaporeSingapore Department of Ophthalmology National University of SingaporeSingapore Singapore Eye Research Institute Singapore National Eye CentreSingapore Ophthalmology and Visual Science Academic Clinical Program Duke-NUS Medical SchoolSingapore Cixi Institute of Biomedical Engineering Ningbo Institute of Materials Technology and EngineeringChinese Academy of SciencesNingboChina Ningbo Eye Hospital NingboChina Zhejiang International Scientific and Technological Cooperative Base of Biomedical Materials and Technology Ningbo Institute of Materials Technology and EngineeringChinese Academy of SciencesNingboChina Zhejiang Engineering Research Center for Biomedical Materials Ningbo Institute of Materials Technology and EngineeringChinese Academy of SciencesNingboChina Division of Public Health Department of Social MedicineGraduate School of MedicineOsaka UniversityOsakaJapan Artificial Intelligence Center for Medical Research and Application Osaka University HospitalOsakaJapan Institute for Research in Ophthalmology Foundation for Ophthalmology DevelopmentPoznanPoland

Background:The convergence of smartphone technology and artificial intelligence(AI)has revolutionized the landscape of ophthalmic care,offering unprecedented opportunities for diagnosis,monitoring,and management of ocular ***,there is a lack of systematic studies on discussing the integration of smart-phone and AI in this *** text:This review includes 52 studies,and explores the integration of smartphones and AI in ophthalmology,delineating its collective impact on screening methodologies,disease detection,telemedicine initiatives,and patient *** collective findings from the curated studies indicate promising performance of the smartphone-based AI screening for various ocular diseases which encompass major retinal diseases,glaucoma,cataract,visual impairment in children and ocular surface ***,the utilization of smartphone-based imaging modalities,coupled with AI algorithms,is able to provide timely,efficient and cost-effective screening for ocular *** modality can also facilitate patient self-monitoring,remote patient monitoring and enhancing accessibility to eye care services,particularly in underserved *** involving data pri-vacy,algorithm validation,regulatory frameworks and issues of trust are still need to be ***,evaluation on real-world implementation is imperative as well,and real-world prospective studies are currently ***:Smartphone ocular imaging merged with AI enables earlier,precise diagnoses,personalized treat-ments,and enhanced service accessibility in eye *** is crucial to navigate ethical and data security challenges while responsibly leveraging these innovations,promising a potential revolution in care access and global eye health equity.

关键词： Artificial intelligence Smartphone imaging Ophthalmology Telemedicine Ocular disease management

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Porous FeAl alloys via powder sintering:Phase transformation,microstructure and aqueous corrosion behavior

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Journal of materials science & Technology 2021年第27期86卷 64-69页

作者： Gang Chen Klaus-Dieter Liss Chao Chen Yuehui He Xuanhui Qu Peng Cao Beijing Advanced Innovation Center for Materials Genome Engineering Institute for Advanced Materials and TechnologyUniversity of Science and Technology BeijingBeijing100083PR China Materials and Engineering Science Program Guangdong Technion-Israel Institute of TechnologyShantouGuangdong515063PR China Technion-Israel Institute of Technology Haifa32000Israel School of Mechanical MaterialsMechatronic and Biomedical EngineeringFaculty of Engineering&Information SciencesUniversity of WollongongWollongongNSW2522Australia State Key Laboratory for Powder Metallurgy Central South UniversityChangsha410083PR China Department of Chemical and Materials Engineering The University of AucklandPrivate Bag 92019Auckland1142New Zealand MacDiarmid Institute of Advanced Materials and Nanotechnology Victoria University of WellingtonPO Box 600Wellington6140New Zealand

This study investigates the phase transformation and microstructure of porous Fe Al parts sintered from elemental powder mixtures using in-situ neutron diffraction and in-situ thermal dilatometry.A single B2 structured Fe Al phase was determined in the sintered Fe Al *** combined effects of the Kirkendall porosity,transient liquid phase,and phase transformations associated with powder sintering all contribute to the swelling phenomenon of the final sintered *** aqueous corrosion test indicates that the corrosion products include iron oxides in the porous Fe Al *** accumulation of corrosion products blocks the pore channel and decreases pore size and permeability over the soaking time.

关键词： Powder sintering Intermetallic Porous Corrosion Neutron diffraction

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