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Current progress in developing metal oxide nanoarrays-based photoanodes for photoelectrochemical water splitting

Science Bulletin 2019年第18期64卷 1348-1380页

作者： Yongcai Qiu Zhenghui Pan Haining Chen Daiqi Ye Lin Guo Zhiyong Fan Shihe Yang Guangdong Provincial Key Laboratory of Atmospheric Environment and Pollution Control School of Environment and EnergySouth China University of TechnologyGuangzhou 510006China State Key Laboratory of Luminescent Materials and Devices South China University of TechnologyGuangzhou 510640China Department of Materials Science and Engineering National University of SingaporeSingapore 117574Singapore School of Materials Science and Engineering Beihang UniversityBeijing 100191China School of Chemistry and Environment Beihang UniversityBeijing 100191China Department of Electronic and Computer Engineering The Hong Kong University of Science and TechnologyHong KongChina Department of Chemistry The Hong Kong University of Science and TechnologyHong KongChina Guangdong Key Lab of Nano-Micro Material Research School of Chemical Biology and Biotechnology Shenzhen Graduate SchoolPeking UniversityShenzhen 518055China

Solar energy driven photoelectrochemical(PEC) water splitting is a clean and powerful approach for renewable hydrogen production. The design and construction of metal oxide based nanoarray photoanodes is one of the promising strategies to make the continuous breakthroughs in solar to hydrogen conversion efficiency of PEC cells owing to their owned several advantages including enhanced reactive surface at the electrode/electrolyte interface, improved light absorption capability, increased charge separation efficiency and direct electron transport pathways. In this Review, we first introduce the structure,work principle and their relevant efficiency calculations of a PEC cell. We then give a summary of the state-of the-art research in the preparation strategies and growth mechanism for the metal oxide based nanoarrays, and some details about the performances of metal oxide based nanoarray photoanodes for PEC water splitting. Finally, we discuss key aspects which should be addressed in continued work on realizing high-efficiency metal oxide based nanoarray photoanodes for PEC solar water splitting systems.

关键词： Photoelectrochemical water splitting Metal oxide based nanoarray photoanodes Preparation strategies and growth mechanism

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Substituent-dependent circularly polarized luminescence in supramolecular gels based on phenylalanine derivatives

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Surfaces and Interfaces 2025年

作者： Guanghui Cao Enquan Tian Qiuya Yang Junjie Xu Qiuju Zhou Xingxing Yue Zhaocun Shen Kunyan Sui Jiaxing Sun College of Materials Science and Engineering Key Laboratory of Marine Bio-based Fibers of Shandong Province Key Laboratory of Shandong Provincial Universities for Advanced Fibers and Composites Qingdao Application Technology Innovation Center of Advanced Fibers and Composites Qingdao University Qingdao 266071 P. R. China College of Chemistry and Chemical Engineering Xinyang Normal University Xinyang 464000 P. R. China Department of Respiratory and Critical Care Medicine The Affiliated Hospital of Qingdao University Qingdao 266001 P. R. China

Circularly polarized luminescence (CPL) materials, owing to their distinctive chiroptical properties, have demonstrated substantial potential in improving display technologies, advancing sensor systems, and functioning as effective biological probes. Recent interest in developing CPL materials based on organic molecules underscores the need to understand how the molecular structure affects CPL signals, thereby enhancing CPL performance. In this study, we demonstrate successful control over the handedness of CPL signals in supramolecular gels by introducing different substituents into the gelators. Specifically, we synthesize four benzene-1,3,5-tricarboxamide derivatives substituted with L - or D -phenylalanine ethyl ester and L - or D -phenylalanine benzyl ester, which are found to form supramolecular gels through hydrogen bonding and π−π stacking in organic solvents. The supramolecular gels comprised of nanofibers exhibit supramolecular chirality and emit CPL with high dissymmetry factors. Intriguingly, the handedness of CPL signals depends on the substituents (ethyl or benzyl groups) of the gelators. This study provides new insights into the relationship between the molecular structure and CPL performance in supramolecular gels.

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Study of heat and mass transfer control inside channel partially filled with a porous medium using nanofluids

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Thermal Science 2019年 23卷 1-16页

作者： Ben Hamida, Mohamed Bechir Massoudi, Mohamed Dhia Marzouki, Riadh Kolsi, Lioua Almeshaal, Mohammed A. Hussein, Ahmed Kadhim College of Engineering Chemical Engineering Department Hail University Hail City Saudi Arabia Physics Department University of Sousse 4011 Lamine Abassi street Tunisia University of Monastir 5019 Kairouan street Tunisia Chemistry Department College of Science King Khalid University Abha61413 Saudi Arabia Laboratory of Materials Crystal Chemistry and Applied Thermodynamics LR15ES01 Faculty of Sciences of Tunis University of Tunis El Manar 2092 Tunisia Chemistry Department Faculty of Sciences University of Sfax Tunisia College of Engineering Mechanical Engineering Department Hail University Hail City Saudi Arabia Laboratory of Metrology and Energy systems University of Monastir Monastir Tunisia Department of Mechanical Engineering College of Engineering Al Imam Mohammad Ibn Saud Islamic University Riyadh Saudi Arabia College of Engineering Mechanical Engineering Department Babylon University Babylon City Hilla Iraq

The steady mixed convection of heat and mass transfer inside and outside a porous vertical wall is numerically studied. The porous wall, placed in a vertical channel, contains a solid phase, a nanofluid phase (Water-Al2O3 or Water-Cu) and gas phase. The effect of several physical quantities such as nanoparticle volume fraction, ambient temperature and initial nanofluid saturation on heat and mass transfer were investigated. Results reveal that the temperature of porous medium is decreased considerably with nanoparticle volume fraction. It has been also found that the heat and mass transfer are dramatically reduced using Water-Alumina nanofluid when compared with pure water. © Serbian Society of Heat Transfer Engineers.

关键词： Porous materials

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Wide-angle giant photonic spin Hall effect

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Physical Review B 2022年第7期106卷 075409-075409页

作者： Zhihao Chen Yu Chen Yaodong Wu Xinxing Zhou Handong Sun Tony Low Hongsheng Chen Xiao Lin Key Laboratory of Low-Dimensional Quantum Structures and Quantum Control of Ministry of Education Synergetic Innovation Center for Quantum Effects and Applications School of Physics and Electronics Hunan Normal University Changsha 410081 China International Collaborative Laboratory of 2D Materials for Optoelectronics Science and Technology Engineering Technology Research Center for 2D Material Information Function Devices and Systems of Guangdong Province Institute of Microscale Optoelectronics Shenzhen University Shenzhen 518060 China Division of Physics and Applied Physics School of Physical and Mathematical Sciences Nanyang Technological University Singapore 637371 Singapore Centre for Disruptive Photonic Technologies (CDPT) School of Physical and Mathematical Sciences Nanyang Technological University Singapore 637371 Singapore Department of Electrical and Computer Engineering University of Minnesota Minneapolis Minnesota 55455 USA Interdisciplinary Center for Quantum Information State Key Laboratory of Modern Optical Instrumentation ZJU-Hangzhou Global Scientific and Technological Innovation Center College of Information Science and Electronic Engineering Zhejiang University Hangzhou 310027 China International Joint Innovation Center ZJU-UIUC Institute The Electromagnetics Academy at Zhejiang University Zhejiang University Haining 314400 China

The photonic spin Hall effect is a manifestation of the spin-orbit interaction of light and can be measured by a transverse shift δ of photons with opposite spins. The precise measurement of transverse shifts can enable many spin-related applications, such as precise metrology and optical sensing. However, this transverse shift is generally small (i.e., δ/λ<10−1, where λ is the wavelength), which impedes its precise measurement. To date, proposals to generate a giant spin Hall effect (namely, with δ/λ>102) have severe limitations, particularly its occurrence only over a narrow angular cone (with a width of Δθ<1∘). Here we propose a universal scheme to realize the wide-angle giant photonic spin Hall effect with Δθ>70∘ by exploiting the interface between free space and uniaxial epsilon-near-zero media. The underlying mechanism is ascribed to the almost-perfect polarization splitting between s and p polarized waves at the designed interface. Remarkably, this almost-perfect polarization splitting does not resort to the interference effect and is insensitive to the incident angle, which then gives rise to the wide-angle giant photonic spin Hall effect.

关键词： Light-matter interaction Photonics Spin Hall effect Spin-orbit coupling

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Preparation and application of teamed boronate affinity magnetic protein imprinted polymer: Pollutants removal, filter resistance improvement and synergistic glycoprotein recovery under physiological pH in sequencing batch reactors

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chemical engineering Journal 2025年 518卷

作者： Qiming Zhang Jiajun Hu Chen Yang Wenshan Guo Jiaxiang Liu Nan Liu Liang Wang Huu Hao Ngo Jixiang Li Shanghai Advanced Research Institute Chinese Academy of Sciences Shanghai 200120 China University of Chinese Academy of Sciences Beijing 100049 China Shanghai Key Laboratory of Bio-Energy Crops School of Life Sciences Shanghai University Shanghai 200444 China School of Civil and Environmental Engineering University of Technology Sydney Sydney NWS 2007 Australia Collaborative Innovation Center of Environmental Pollution Control and Ecological Restoration of Henan Province Department of Material and Chemical Engineering Zhengzhou University of Light Industry Zhengzhou 450001 China State Key Laboratory of Separation Membrane and Membrane Process School of Environmental Science and Engineering Tiangong University Tianjin 300387 China

In this study, a teamed boronate affinity (TBA) strategy was employed to prepare a novel low p K a glycoprotein magnetic molecularly imprinted polymer (MMIP-TBA) with 3-Aminophenylboronic acid and 1,6-hexanediamine as precursors for improving the performance of sequencing batch reactors (SBRs) under physiological conditions (pH = 7.4). The effects of MMIP-TBA on pollutants removal, filter resistance improvement and synergistic glycoprotein recovery were comprehensively investigated in SBRs, and the mechanisms were further explained by density functional theory (DFT) and microbial community analysis. The adsorption tests indicated that the MMIP-TBA retained high adsorption capacity (201 mg·g −1 ), excellent specificity (imprinting factor, IF = 5.74) on ovalbumin, and showed the desired selectivity (selectivity factor, SF BSA = 4.52, SF Lyz = 2.44, SF BHb = 1.86) on competing proteins. Also, the MMIP-TBA showed a remarkable recovery ability (75 mg·g −1 ) of glycoprotein-type substances in soluble microbial products (SMPs) derived from SBRs. Moreover, the adsorption process is a monolayer chemical adsorption and is thermodynamically spontaneous (△G Θ = -13.58 kJ·mol −1 ). DFT calculations elucidated that the B N bond was responsible for specific adsorption of TBA with 1.2-cis diol. The microbial community analysis suggested that the MMIP-TBA inhibited the colonization of biofouling bacteria thereby reducing the SMP production. Consequently, the specific filtration resistance was reduced by 30.6 % with slight improvement on pollutants removal. Also, the glycoprotein could be synergistically recovered. The improvement of SBRs performance by MMIP-TBA may be aroused by the specific adsorption and microbial regulation in SBRs. These findings provided that the MMIP-TBA had great potential in improving performance for biological systems under physiological conditions.

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Energy and Co2 Emission Analysis of a bio-Energy with Ccs System: biomass Gasification-Solid Oxide Fuel Cell-Mini Gas Turbine-Co2 Capture

SSRN

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SSRN 2022年

作者： Zhang, Yuxin Wu, Shiliang Cui, Dongxu Yoon, Sang-Jun Bae, Youn-Sang Park, Bugae Wu, Yinlong Xiao, Rui Key Laboratory of Energy Thermal Conversion and Control of Ministry of Education School of Energy and Environment Southeast University Nanjing210018 China 152 Gajeongro Yuseong-gu Daejeon34129 Korea Republic of Department of Chemical and Biomolecular Engineering Yonsei University 50 Yonsei-ro Seodaemun-gu Seoul03722 Korea Republic of Sun Brand Industrial Inc. 52 5 road Nano industrial Nam-myeon Jangseong-gun Jeollanam-do Korea Republic of Hefei Debo Bio-Energy Technology Co. Ltd Hefei230088 China

The global goal of carbon neutrality calls for the development of carbon-negative technologies. And one of the large-scale technology that can offset CO2 from the atmosphere and generate power is bioenergy with CCS, also known as BECCS. A BECCS system combined biomass gasification (BG), solid oxide fuel cell (SOFC), mini gas turbine (MGT), heat recovery (HR), and CO2 capture and storage (CCS) was proposed in this study. The energy and CO2 emission analysis and the parameter sensitivity analysis of the proposed systems with and without CCS were carried out to evaluate its technical and environmental feasibility as a provider of carbon-negative electricity. For the system without CCS (BG-SOFC-MGT), the electrical efficiency and the combined heat and power (CHP) efficiency are 46.2% and 73.6%, and the CO2 emission is 0.220 kg/kWh. In the system with CCS (BG-SOFC-MGT-CCS), the electrical efficiency and CHP efficiency decreased by 11.7%, and 34.6%, respectively, and CO2 emissions decreased to -0.516 kg/kWh. Due to the energy consumption of CCS, the electrical efficiency and CHP efficiency decrease to varying degrees. Nevertheless, the CO2 emission of the system has changed from positive to negative, and the system has great potential for development under the goal of global carbon neutrality. © 2022, The Authors. All rights reserved.

关键词： Solid oxide fuel cells (SOFC)

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Author Correction: Sub-femtonewton force sensing in solution by super-resolved photonic force microscopy

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Nature Photonics 2024年 998页

作者： Xuchen Shan Dajing Wang Jinlong Shi Hongyan Zhu Xiaolan Zhong Baolei Liu Weichang Hao Fan Wang Lei Ding Qian Peter Su Shihui Wen Dayong Jin Lei Jiang Chaohao Chen Yang Wang Zhaocun Huang Lingqian Chang Shen S. J. Wang Peter John Reece Wei Ren Xunyu Lu Jie Lu Lingdong Sun School of Physics Beihang University Beijing People’s Republic of China Science and Technology Center for Quantum Biology National Institute of Extremely-Weak Magnetic Field Infrastructure Hangzhou People’s Republic of China School of Biomedical Engineering Faculty of Engineering and Information Technology University of Technology Sydney Sydney New South Wales Australia Centre for Atomaterials and Nanomanufacturing School of Science RMIT University Melbourne Victoria Australia Institute for Biomedical Materials and Devices (IBMD) School of Mathematical and Physical Sciences Faculty of Science University of Technology Sydney Sydney New South Wales Australia Eastern Institute for Advanced Study Eastern Institute of Technology Ningbo People’s Republic of China Key Laboratory of Bio-Inspired Materials and Interfaces Sciences Technical Institute of Physics and Chemistry Chinese Academy of Sciences Beijing People’s Republic of China Australian Research Council Centre of Excellence for Transformative Meta-Optical Systems Department of Electronic Materials Engineering Research School of Physics The Australian National University Canberra Australian Capital Territory Australia Key Laboratory of Biomechanics and Mechanobiology (Ministry of Education) Beijing Advanced Innovation Center for Biomedical Engineering School of Biological Science and Medical Engineering Beihang University Beijing People’s Republic of China Computing and Information Systems Department Melbourne School of Engineering University of Melbourne Melbourne Victoria Australia School of Physics The University of New South Wales Sydney New South Wales Australia School of Chemistry & Chemical Engineering Shaanxi Normal University Xi’an People’s Republic of China Particles and Catalysis Research Laboratory School of Chemical Engineering The University of New South Wales Sydney New South Wales Australia Australian Artificial Intelligence Institute Faculty of Engineering and IT University of Technology

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Ionized jet deposition of antimicrobial and stem cell friendly silver-substituted tricalcium phosphate nanocoatings on titanium alloy

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bioactive materials 2021年第8期6卷 2629-2642页

作者： Gabriela Graziani Katia Barbaro Inna V.Fadeeva Daniele Ghezzi Marco Fosca Enrico Sassoni Gianluca Vadalà Martina Cappelletti Francesco Valle Nicola Baldini Julietta V.Rau IRCSS Istituto Ortopedico Rizzoli Laboratory of NanoBiotechnologyvia di Barbiano 1/1040136BolognaItaly Istituto Zooprofilattico Sperimentale Lazio e Toscana“M.Aleandri” Via Appia Nuova 1411-00178RomeItaly A.A.Baikov Institute of Metallurgy and Materials Science Russian Academy of SciencesLeninsky prospect 49119334MoscowRussia Istituto di Struttura della Materia Consiglio Nazionale delle Ricerche(ISM-CNR)Via del Fosso del Cavaliere100-00133RomeItaly University of Bologna Department of CivilChemicalEnvironmental and Materials Engineeringvia Terracini 2840131BolognaItaly UniversitàCampus Bio-Medico di Roma Research Unit of Orthopaedic SurgeryFaculty of Medicine and SurgeryVia Alvaro del Portillo 2100128RomeItaly University of Bologna Department of Pharmacy and Biotechnologyvia Irnerio 4240126BolognaItaly Institute of Nanostructured Materials National Research Council(ISMN-CNR)Via Piero Gobetti10140129BolognaItaly IRCSS Istituto Ortopedico Rizzoli BST Biomedical Science and Technologies Labvia di Barbiano 1/1040136BolognaItaly University of Bologna Department of Biomedical and Neuromotor SciencesVia Massarenti940128BolognaItaly Sechenov First Moscow State Medical University Institute of PharmacyDepartment of AnalyticalPhysical and Colloid ChemistryTrubetskaya 8build.2119991MoscowRussia

Orthopedic infections pose severe societal and economic burden and interfere with the capability of the implanted devices to integrate in the host bone,thus significantly increasing implants failure *** address infection and promote integration,here nanostructured antibacterial and bioactive thin films are proposed,obtained,for the first time,by Ionized Jet Deposition(IJD)of silver-substituted tricalcium phosphate(Ag-TCP)targets on *** morphology,composition and mechanical properties are characterized and proof-of-concept of biocompatibility is *** efficacy is investigated against four Gram positive and Gram negative bacterial strains and against *** fungus,by investigating the modifications in planktonic bacterial growth in the absence and presence of ***,for all bacterial strains,the capability of the film to inhibit bacterial adhesion is also *** indicate that IJD permits a fine control over films composition and morphology and deposition of films with suitable mechanical *** studies show a good efficacy against Escherichia coli,Staphylococcus aureus,Pseudomonas aeruginosa,Enterococcus faecalis and against fungus Candida albicans,with evidences of efficacy against planktonic growth and significant reduction of bacterial cell *** cytotoxic effects are evidenced for equine adipose tissue derived mesenchymal stem cells(ADMSCs),as no reductions are caused to cells viability and no interference is assessed in cells differentiation towards osteogenic lineage,in the presence of ***,thanks to nanostructuration and biomimetic composition,tricalcium phosphate(TCP)coatings favor cells viability,also when *** findings show that silver-substituted nanostructured coatings are promising for orthopedic implant applications.

关键词： Tricalcium phosphate Silver Nanostructured coatings Antibacterial coatings Orthopedics Antibacterial ceramics

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Insight into the effect of pyrolysis temperature on photoreactivity of biochar-derived dissolved organic matter: Impacts of aromaticity and carbonyl groups

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The Science of the total environment 2023年 871卷 162048页

作者： Hanzhuo Luo Eydhah Almatrafi Wenjun Wang Yang Yang Danlian Huang Weiping Xiong Min Cheng Chengyun Zhou Yin Zhou Qing Lin Guoge Fang Guangming Zeng Chen Zhang College of Environmental Science and Engineering Hunan University and Key Laboratory of Environmental Biology and Pollution Control Hunan University Ministry of Education Changsha Hunan 410082 PR China Center of Research Excellence in Renewable Energy and Power Systems Center of Excellence in Desalination Technology Department of Mechanical Engineering Faculty of Engineering-Rabigh King Abdulaziz University Jeddah 21589 Saudi Arabia. School of Resources and Environment Hunan University of Technology and Business Changsha 410205 China. Department of Chemical and Materials Engineering University of Alberta Edmonton Alberta T6G 1H9 Canada. College of Environmental Science and Engineering Hunan University and Key Laboratory of Environmental Biology and Pollution Control Hunan University Ministry of Education Changsha Hunan 410082 PR China. Center of Research Excellence in Renewable Energy and Power Systems Center of Excellence in Desalination Technology Department of Mechanical Engineering Faculty of Engineering-Rabigh King Abdulaziz University Jeddah 21589 Saudi Arabia. Electronic address: zgming@***. College of Environmental Science and Engineering Hunan University and Key Laboratory of Environmental Biology and Pollution Control Hunan University Ministry of Education Changsha Hunan 410082 PR China. Electronic address: zhangchen@***.

Practical application of biochar may result in more biochar-derived dissolved organic matter (denoted as BDOM) inevitably release into surface waters by infiltration and surface runoff. The photochemical reaction of BDOM has gained intense attention, which played a key role in the fate of organic contaminants. However, the relationships between specific characteristics of BDOM and its photoreactivity are still uncertain. In this study, the characteristics of BDOM pyrolyzed from rice husk derived biochar at different temperature (from 400 °C to 700 °C) and their effect on the photodegradation of oxytetracycline (OTC) were carefully investigated. The C NMR and EEM results indicated the dominated component of BDOM was gradually turned from humic acid like substances with low aromaticity to high aromaticity with abundant oxygen-containing functional groups as pyrolytic temperature increases. Experimental results showed that the apparent rate constants (k) of BDOM700 (4.53 × 10 min) for OTC photodegradation was approximately one order of magnitude higher than BDOM400 (4.52 × 10 min), which was closely correlated with their aromaticity (R = 0.944). It was found that BDOM* rather than O played the major role in BDOM mediated photodegradation of OTC (80.13 % vs 14.34 %), and the carbonyl-containing group was identified as the main BDOM* precursor by NaBH reduction experiment. This work highlighted both aromaticity and carbonyl group contents were critical indicators for assessing the potential to generate BDOM* and corresponding photoreactivity.

关键词： Dissolved organic matter Electron transfer Photochemistry Pyrolysis temperature Triplet state

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bioinspired supramolecular fibrillization enables stretchable and biodegradable piezoelectric bioelectronics

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Science Advances 2025年第25期11卷

作者： Haoran Wu Hao Lyu Hongbo Jiang Yancheng Wang Rusen Yang Syed A. M. Tofail Hai Xu Chengchen Guo Deqing Mei Ehud Gazit Kai Tao State Key Laboratory of Fluid Power and Mechatronic Systems School of Mechanical Engineering Zhejiang University Hangzhou 310058 China. Future Science Research Institute Hangzhou Global Scientific and Technological Innovation Centre Hangzhou 311200 China. Key Laboratory of Advanced Manufacturing Technology of Zhejiang Province School of Mechanical Engineering Zhejiang University Hangzhou 310058 China. Zhejiang-Israel Joint Laboratory of Self-Assembling Functional Materials Hangzhou 311200 China. Zhejiang-Ireland Joint Laboratory of Bio-Organic Dielectric Materials and Devices Hangzhou 310058 China. Department of Materials Science and Engineering Westlake University Hangzhou 310030 China. School of Advanced Materials and Nanotechnology Xidian University Xi’an 710126 China. Department of Physics Bernal Institute University of Limerick Limerick V94 T9PX Ireland. State Key Laboratory of Heavy Oil Processing and Centre for Bioengineering and Biotechnology China University of Petroleum (East China) Qingdao 266580 China. The Shmunis School of Biomedicine and Cancer Research George S. Wise Faculty of Life Sciences Tel Aviv University Tel Aviv 6997801 Israel. Department of Materials Science and Engineering Iby and Aladar Fleischman Tel Aviv University Tel Aviv 6997801 Israel.

bioinspired piezoelectricity is extensively explored for diverse bio-machine interface and biomedical engineering applications. Nevertheless, state-of-the-art bio-piezoelectricity mainly focuses on crystallization. Yet, crystalized structures exhibit several shortcomings, including limited biocompatibility or biodegradability along with intrinsic non-stretchability. Herein, peptides fibrillization is reported to present inherent bio-piezoelectricity. Upon forming double-network framework with silk fibroin, fibrous peptide piezogels of innate biocompatibility and biodegradability are achieved, showing a programmable piezoelectricity. In particular, the bioinspired supramolecular piezogel can linearly respond to external compression and stretching in large force regions, extensively expanding the application potential bio-piezoelectricity. Upon designing a “W”-shaped structural conformation, a peptide fibrous piezogel–based piezoelectric sensor is shown to be used for detection of limb movements and subcutaneous implantation of the bioinspired piezoelectric electronics, realizing in situ and real-time monitoring of stimuli responses. The findings suggest the promising potential of peptide fibrillization–based bio-piezoelectricity for diverse bio-machine interface and biomedical engineering applications.

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